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Selim Elhadj

Publications and source records attributed to Selim Elhadj.

3 recordsLinked to original sources

An Optically Addressable Transmissive Liquid Crystal Metasurface Spatial Light Modulator

Active wavefront control in high-power laser illumination systems is important for technologies such as additive manufacturing, free-space laser communication, and power transmission. Conventional spatial light modulators (SLMs) and mechanical beam-steering devices are unsuitable for such applications as they rely on metal mirrors and electrical contacts which are damaged under high laser irradiances. Here, we report on the design and realization of an optically addressable metasurface liquid crystal (LC)-based SLM for the modulation of high-power transmitted light. Our device uses a photoactive top contact which is optically addressed with a patterned 435 nm laser, creating a transient electrical contact that selectively switches the underlying LC medium. A TiO$_2$ metasurface, resonant in the 915-985 nm wavelength range, is embedded within a thin (~2 $\mu$m) LC layer and enables large optical tunability. We demonstrate 90$^\circ$ linear polarization rotation in reconfigurable patterns across a 5x5 mm$^2$ active area with an overall transmittance of >60%. Additionally, we develop a multiphysics approach to simulate transmittance modulation in our device by modeling the LC interactions with TiO$_2$ nanopillars under an applied electrostatic field. This model exhibits good agreement with measurements and provides improved understanding of how LCs interact with both transmitted light and nanoscale metastructures in active devices. We show that our design and fabrication approach can yield high-efficiency transmissive metasurface SLM devices and lay the groundwork for the design of future LC-based active nanophotonics.

physics.optics

High sub-bandgap response and fast switching enabled by thermal quenching in carbon-doped semi-insulating GaN

Carbon-doped GaN is a promising material for sub-bandgap triggered optical switches. When incorporated in GaN, carbon introduces deep compensating centers that enable defect-mediated extrinsic photoconductivity. Here, we investigate the optical responsivity and switching kinetics of semi-insulating carbon-doped GaN actuated by sub-bandgap blue illumination. A high ON/OFF ratio exceeding $\mathrm{10^7}$ is achieved under low-irradiance 405-nm excitation. Temperature-dependent transient measurements reveal that the photocurrent decay is thermally quenched above a crossover temperature of ~300 K. This behavior is attributed to hole-emission-assisted recombination. The extracted activation energies vary across samples; a commonly observed value of ~0.83 eV is attributed to the $\mathrm{C_N}$ defect. Notably, when heating above the crossover temperature, thermal quenching accelerates the photocurrent decay by up to a factor of five, enabling significantly faster switching.

cond-mat.mtrl-sci

Quantized grain boundary states promote nanoparticle alignment during imperfect oriented attachment

Oriented attachment (OA) has become a well-recognized mechanism for the growth of metal, ceramic, and biomineral crystals. While many computational and experimental studies of OA have shown that particles can attach with some misorientation then rotate to remove adjoining grain boundaries, the underlying atomistic pathways for this "Imperfect OA" process remain the subject of debate. In this study, molecular dynamics and in situ TEM were used to probe the crystallographic evolution of up to 30 gold and copper nanoparticles during aggregation. It was found that Imperfect OA occurs because (1) grain boundaries become quantized when their size is comparable to the separation between constituent dislocations and (2) kinetic barriers associated with the glide of grain boundary dislocations are small. In support of these findings, TEM experiments show the formation of a single crystal aggregate after annealing 9 initially misoriented, agglomerated particles with evidence of dislocation slip and twin formation during particle/grain alignment. These observations motivate future work on assembled nanocrystals with tailored defects and call for a revision of Read-Shockley models for grain boundary energies in nanocrystalline materials.

cond-mat.mtrl-sci