SearcharxivSearch

arXiv subjects

Seno Aji

Publications and source records attributed to Seno Aji.

7 recordsLinked to original sources

Collinear ferromagnetism with reduced moment length in kagome magnet Nd3Ru4Al12

We determine the magnetic ground state of the kagome lattice magnet Nd3Ru4Al12 by single-crystal neutron diffraction, supported by experiments with polarized neutrons. We identify this material as a collinear ferromagnet ("hex-FM") with uniform moment length mc = 2.1 {\mu}B/Nd and ordering vector Q = 0, in contrast to a previous, seminal report that proposed unequal moment lengths on two Nd sites, here called the "ortho-FM" state. Our analysis of the flipping ratio in polarized neutron scattering is consistent with the hex-FM state. The results provide a microscopic basis for understanding the large fluctuation-induced Hall and Nernst responses near TC = 41 K, as previously reported for Nd3Ru4Al12.

cond-mat.str-el

Emergent electric fields driven by phonon-coupled skyrmion resonances

We develop a coarse-grained theoretical description of the macroscopic emergent electric field generated by phonon-coupled lattice deformations in the breathing and rotational dynamics of a skyrmion lattice under microwave excitation. The analysis identifies the symmetry and dynamical conditions that yield rectified (dc) and oscillating (ac) electric fields, even in the absence of net translational motion of the skyrmion lattice, particularly in the dilute-lattice limit. Using experimentally measurable skyrmion profile parameters such as the equilibrium radius, domain-wall width, and dynamical resonance frequency of skyrmion lattice, the model further enables identification of harmonic components contributing to the observed macroscopic electrodynamic response in the long-wavelength phonon limit ($q \to 0$) and at finite phonon frequency, providing a unified framework for phonon-driven spin-charge-lattice coupling in topological magnets.

cond-mat.mtrl-sci

Spin current generation driven by skyrmion dynamics under magnetic anisotropy and polarized microwaves

We have investigated the spin-current pumped by the skyrmion-host material with the lack of inversion symmetry through the microwave resonance process. The effects of magnetic anisotropy and polarized microwaves are examined by micromagnetic simulations. Our results reveal two distinct skyrmion phases, designated as SkX type-I and II, which emerge at low ($K_z<0.1$ meV) and high ($K_z>0.1$ meV) magnetic anisotropy constants, respectively, having different characteristics of spin excitations. The SkX type-I exhibits spin dynamics where the resonant frequency of the breathing mode is lying in between the clockwise and counterclockwise gyration modes of Bloch-type skyrmion at a very low anisotropy, and is crossing over the counterclockwise mode at $K_z \sim 0.04$ meV. Meanwhile, the SkX type-II exhibits distinct spin excitations in which the clockwise mode is notably absent, while the counterclockwise modes exist at both low and high resonant frequencies. This suggests that the magnetic anisotropy plays an essential role in the spin dynamics. Furthermore, the resulting spin excitations induce spin currents with exotic features under the polarized microwaves. The spin currents induced, for instance, by low-lying in-plane excitations are strongly enhanced under the left-handed circularly polarized microwaves, but quenched by the right-handed circularly polarized microwaves regardless of the sign of the Dzyaloshinskii-Moriya interaction. These results may pave the way for understanding the non-trivial interplay between magnetic anisotropy and polarized microwaves in the generation of spin currents by a resonant process.

cond-mat.mtrl-sci

Non-coplanar helimagnetism in the layered van-der-Waals metal DyTe$_3$

Magnetic materials with highly anisotropic chemical bonding can be exfoliated to realize ultrathin sheets or interfaces with highly controllable optical or spintronics responses, while also promising novel cross-correlation phenomena between electric polarization and the magnetic texture. The vast majority of these van-der-Waals magnets are collinear ferro-, ferri-, or antiferromagnets, with a particular scarcity of lattice-incommensurate helimagnets of defined left- or right-handed rotation sense, or helicity. Here we use polarized neutron scattering to reveal cycloidal, or conical, magnetic structures in DyTe$_3$, with coupled commensurate and incommensurate order parameters, where covalently bonded double-slabs of dysprosium square nets are separated by highly metallic tellurium layers. Based on this ground state and its evolution in a magnetic field as probed by small-angle neutron scattering (SANS), we establish a one-dimensional spin model with off-diagonal on-site terms, spatially modulated by the unconventional charge order in DyTe$_3$. The CDW-driven term couples to antiferromagnetism, or to the net magnetization in applied magnetic field, and creates a complex magnetic phase diagram indicative of competing interactions in an easily cleavable helimagnet. Our work paves the way for twistronics research, where helimagnetic layers can be combined to form complex spin textures on-demand, using the vast family of rare earth chalcogenides and beyond.

cond-mat.mtrl-sci

Direct observations of spin fluctuations in spin-hedgehog-anti-hedgehog lattice states in MnSi$_{1-x}$Ge$_x$ ($x=0.6$ and $0.8$) at zero magnetic field

The helimagnetic compounds MnSi$_{1-x}$Ge$_{x}$ show the three-dimensional multiple-$q$ order as referred to as spin-hedgehog-anti-hedgehog (SHAH) lattice. Two representative forms of SHAH are cubic-3$q$ lattice with $q \| \langle100\rangle$ and tetrahedral-4$q$ lattice with $q \| \langle111\rangle$, which show up typically for $x=1.0-~0.8$ and for $x=0.6$, respectively. Here, we have investigated the spin fluctuations in the MnSi$_{1-x}$Ge$_{x}$ polycrystalline samples with $x=0.6$ and $0.8$ by using the time-of-flight (TOF) neutron inelastic scattering and MIEZE-type neutron spin echo techniques to elucidate the microscopic origin of the unconventional Hall effect in the SHAH lattice states. This research is motivated by the observation of a sign change in the unconventional Hall resistivity as a function of temperature [Y. Fujishiro et al., Nat. Comm. $\textbf{10}$, 1059 (2019)]. The present results reveal the correspondences between the temperature ranges where the positive Hall resistivity and spin fluctuations are observed. These results agree well with the theoretical model of the conduction electrons scattered by the fluctuating spin clusters with a non-zero average of sign-biased scalar spin chirality as a mechanism of the positive Hall resistivity [H. Ishizuka and N. Nagaosa, Sci. Adv. $\textbf{4}$, eaap9962 (2018)].

cond-mat.str-el

Higher-order modulations in the skyrmion-lattice phase of Cu$_2$OSeO$_3$

Using small angle neutron scattering, we have investigated higher-order peaks in the skyrmion-lattice phase of Cu$_2$OSeO$_3$, in which two different skyrmion lattices, SkX1 and SkX2, are known to form. For each skyrmion-lattice phase, we observed two sets of symmetrically inequivalent peaks at the higher-order-reflection positions with the indices $(110)$ and $(200)$. Under the condition where the SkX1 and SkX2 coexist, we confirmed the absence of the scattering at $\mathbf{Q}$ positions combining reflections from the two phases, indicating a significantly weak double-scattering component. Detailed analysis of the peak profile, as well as the temperature and magnetic-field dependence of the peak intensity, also supports the intrinsic higher-order modulation rather than the parasitic double scattering. The two higher-order modulations show contrasting magnetic-field dependence; the former $(110)$ increases as the field is increased, whereas the latter $(200)$ decreases. This indicates that, in Cu$_2$OSeO$_3$, skyrmions are weakly distorted, and the distortion is field-dependent in a way that the dominant higher-order modulation switches from $(110)$ to $(200)$ under field. Monte Carlo simulations under sweeping external magnetic field qualitatively reproduce the observed magnetic-field dependence, and suggests that the higher-order modulations correspond to the superlattices of weak swirlings appearing in the middle of the original triangular-latticed skyrmions.

cond-mat.str-el

Effect of Ge-substitution on Magnetic Properties in the Itinerant Chiral Magnet MnSi

We have investigated the effect of Ge-substitution to the magnetic ordering in the B20 itinerant chiral magnet MnSi prepared by melting and annealing under ambient pressure. From metallurgical survey, the solubility limit of Ge was found to be $x=0.144(5)$ with annealing temperature $T_\mathrm{an} = 1073$ K. Magnetization measurements on MnSi$_{1-x}$Ge$_x$ samples show that the helical ordering temperature $T_{\mathrm{c}}$ increases rapidly in the low-$x$ range, whereas it becomes saturated at higher concentration $x>~0.1$. The Ge substitution also increases both the saturation magnetization $M_\mathrm{s}$ and the critical field to the fully polarized state $H_\mathrm{c2}$. In contrast to the saturation behavior of $T_\mathrm{c}$, those parameters increase linearly up to the highest Ge concentration investigated. In the temperature-magnetic field phase diagram, we found enlargement of the skyrmion phase region for large $x$ samples. We, furthermore, observed the non-linear behavior of helical modulation vector $k$ as a function of Ge concentration, which can be described qualitatively using the mean field approximation.

cond-mat.mtrl-sci