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Seong-Joo Lee

Publications and source records attributed to Seong-Joo Lee.

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Floquet analysis of coherence in periodically driven diamond NV ensemble systems

High-density nitrogen-vacancy (NV) ensembles are promising platforms for solid-state quantum sensing, but their performance is limited by dipolar interactions and inhomogeneous dephasing. Periodic decoupling sequences such as Waugh-Huber-Haeberlen (WAHUHA) can extend the observed stroboscopic decay time, but a longer fitted lifetime does not necessarily imply improved magnetic-field sensitivity. Here, we experimentally demonstrate this disconnect experimentally. WAHUHA increases the fitted stroboscopic decay time from $T_{2}^*$ of 0.9 $μ$s to $T_{2,eff}^*$ of 31 $μ$s, while producing little improvement in dc magnetic-field sensitivity. Using detuning-resolved stroboscopic spectroscopy and finite-pulse Floquet analysis, we show that the long-lived signal arises from phase wrapping and quasienergy branch folding of the one-cycle unitary. These effects reshape the stroboscopic spectrum, and the experimentally relevant folded branches exhibit a reduced local detuning-to-phase transduction slope, $dΦ/dΔ$, which governs the dc magnetic-field response. Our results demonstrate that, under periodic driving, an extended effective dephasing time does not necessarily translate into enhanced dc sensitivity and establish finite pulse Floquet analysis as a practical framework for evaluating coherence in spin ensembles.

quant-ph

Frequency limits of sequential readout for sensing AC magnetic fields using nitrogen-vacancy centers in diamond

The nitrogen-vacancy (NV) centers in diamond have ability to sense alternating-current (AC) magnetic fields with high spatial resolution. However, the frequency range of AC sensing protocols based on dynamical decoupling (DD) sequences has not been thoroughly explored experimentally. In this work, we aimed to determine the sensitivity of ac magnetic field as a function of frequency using sequential readout method. The upper limit at high frequency is clearly determined by Rabi frequency, in line with the expected effect of finite DD-pulse width. In contrast, the lower frequency limit is primarily governed by the duration of optical repolarization rather than the decoherence time (T$_2$) of NV spins. This becomes particularly crucial when the repetition (dwell) time of the sequential readout is fixed to maintain the acquisition bandwidth. The equation we provide successfully describes the tendency in the frequency dependence. In addition, at the near-optimal frequency of 1 MHz, we reached a maximum sensitivity of 229 pT/$\sqrt{\mathrm{Hz}}$ by employing the XY4-(4) DD sequence.

quant-ph

Quantum diamond microscopy with optimized magnetic field sensitivity and sub-ms temporal resolution

Quantum diamond magnetometers using lock-in detection have successfully detected weak bio-magnetic fields from neurons, a live mammalian muscle, and a live mouse heart. This opens up the possibility of quantum diamond magnetometers visualizing microscopic distributions of the bio-magnetic fields. Here, we demonstrate a lock-in-based wide-field quantum diamond microscopy, achieving a mean volume-normalized per pixel sensitivity of 43.9 $\mathrm{nTμm^{1.5}/Hz^{0.5}}$. We optimize the sensitivity by implementing a double resonance with hyperfine driving and magnetic field alignment along the $<$001$>$ orientation of the diamond. Additionally, we show that sub-ms temporal resolution ($\sim$ 0.4 ms) can be achieved while keeping the per-pixel sensitivity at a few tens of nanotesla per second using quantum diamond microscopy. This lock-in-based diamond quantum microscopy could be a step forward in mapping functional activity in neuronal networks in micrometer spatial resolution.

quant-ph

Multiplexed sensing of magnetic field and temperature in real time using a nitrogen vacancy spin ensemble in diamond

Nitrogen-Vacancy (NV) spin in diamond is a versatile quantum sensor, being able to measure physical quantities such as magnetic field, electric field, temperature, and pressure. In the present work, we demonstrate a multiplexed sensing of magnetic field and temperature. The dual frequency driving technique we employ here is based on frequency-division multiplexing, which enables sensing both measurables in real time. The pair of NV resonance frequencies for dual frequency driving must be selected to avoid coherent population trapping of NV spin states. With an enhanced optical collection efficiency higher than 50 $\%$ and a type 1b diamond crystal with natural abundance $^{13}$C spins, we achieve sensitivities of about 70 pT/$\sqrt{\mathrm{Hz}}$ and 25 $μ$K/$\sqrt{\mathrm{Hz}}$ simultaneously. A high isolation factor of 34 dB in NV thermometry signal against magnetic field was obtained, and we provide a theoretical description for the isolation factor. This work paves the way for extending the application of NV quantum diamond sensors into more demanding conditions.

quant-ph

Dynamic nuclear polarisation of liquids at one microtesla using circularly polarised RF with application to millimetre resolution MRI

Magnetic resonance imaging in ultra-low fields is often limited by mediocre signal-to-noise ratio hindering a higher resolution. Overhauser dynamic nuclear polarisation (O-DNP) using nitroxide radicals has been an efficient solution for enhancing the thermal nuclear polarisation. However, the concurrence of positive and negative polarisation enhancements arises in ultra-low fields resulting in a significantly reduced net enhancement, making O-DNP far less attractive. Here, we address this issue by applying circularly polarised RF. O-DNP with circularly polarised RF renders a considerably improved enhancement factor of around 150,000 at 1.2 microtesla. A birdcage coil was adopted into a ultra-low field MRI system to generate the circularly polarised RF field homogeneously over a large volume. We acquired an MR image of a nitroxide radical solution with an average in-plane resolution of 1 mm. De-noising through compressive sensing further improved the image quality.

physics.app-ph