arXiv subjects

Serafim Teknowijoyo

Publications and source records attributed to Serafim Teknowijoyo.

13 recordsLinked to original sources

arXiv2026

Revisiting apparent ideal diamagnetism at ambient conditions in graphene-n-heptane-permalloy systems

We previously reported apparent ideal diamagnetism at ambient conditions in a graphene-n-heptane-permalloy system. At the same time, the experiments revealed inconsistent behavior, including signal freezing and occasional paramagnetic responses. Further measurements performed without graphene produced similar signals, indicating that graphene is not responsible for the observed effects. The results suggest that magnetic field redistribution caused by inhomogeneities in the permalloy foil and experimental geometry can mimic ideal diamagnetism in sub-milligauss measurements. These findings revise the interpretation of our earlier results and emphasize caution in interpreting ultra-low-field magnetic measurements.

cond-mat.supr-con↗

arXiv2026

Glassy magnetic freezing of interacting clusters in LK-99-family materials

We report reproducible magnetization anomalies appearing below room temperature in copper-doped apatite materials belonging to the LK-99 family synthesized via hydrothermal methods. These anomalies are observed consistently across samples prepared under comparable conditions. Although the extracted Mydosh parameter lies within the range often associated with vortex-glass behavior in superconductors, a detailed analysis of DC magnetization, AC susceptibility, field dependence, and magnetic memory effects demonstrates that the observed phenomena are not related to superconductivity. Instead, the data are consistent with glassy magnetic freezing of interacting clusters. Compositional and structural analysis identifies covellite (CuS), an ubiquitous secondary phase in these intrinsically multiphase materials, as the primary origin of the observed behavior. Our results clarify the magnetic origin of LK-99-related anomalies and highlight the importance of phase complexity in interpreting apparent superconducting signatures in this materials family.

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arXiv2026

Diode Effect May Assist Finding Proper Superconductivity Mechanism in Copper Oxides

We present measurements demonstrating that copper-oxide high-temperature superconductors can exhibit broken time-reversal symmetry in the absence of external magnetic fields. Using $Tl_{2}Ba_{2}CaCu_{2}O_{8}$ microbridges, we observe a pronounced superconducting diode effect at 100 K under strictly zero-field conditions. This nonreciprocal response remains unchanged in magnetic fields up to $\pm 100 Oe$. Our results are consistent with recent reports of zero-field diode behavior in $Bi_{2}Sr_{2}CaCu_{2}O_{8+δ }$ and together indicate that time-reversal symmetry breaking may be an intrinsic property of the cuprate superconducting state. These findings significantly constrain theoretical models of high-temperature superconductivity that rely on time-reversal-symmetric mechanisms.

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arXiv2023

Gate-controlled supercurrent effect in dry-etched Dayem bridges of non-centrosymmetric niobium rhenium

The application of a gate voltage to control the superconducting current flowing through a nanoscale superconducting constriction, named as gate-controlled supercurrent (GCS), has raised great interest for fundamental and technological reasons. To gain a deeper understanding of this effect and develop superconducting technologies based on it, the material and physical parameters crucial for GCS must be identified. Top-down fabrication protocols should be also optimized to increase device scalability, although studies suggest that top-down fabricated devices are more resilient to show GCS. Here, we investigate gated superconducting nanobridges made with a top-down fabrication process from thin films of the non-centrosymmetric superconductor NbRe. Unlike other devices previously reported, our NbRe devices systematically exhibit GCS, when made in specific conditions, which paves the way for higher device scalability. Our results also suggest that surface properties of NbRe nanobridges and their modification during fabrication are key for GCS.

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arXiv2023

Superconducting Polycrystalline Rhenium Films Deposited at Room Temperature

We report on magnetron deposition of thin superconducting rhenium films on sapphire substrates. During the deposition, substrates were held at ambient temperature. Critical temperature of the films is Tc~3.6 K. Films have polycrystalline structure, and grazing incidence X-ray diffractometry indicates that crystalline lattice parameters are somewhat larger compared to the bulk ones. Magnetoresistive and AC/DC susceptibilities allowed us to determine $H_{c1}$ and $H_{c2}$ of these films, as well as estimate coherence length $ξ$(0) and magnetic penetration depth $λ_L$(0). We also provide information on surface morphology of these films.

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arXiv2023

Superconductivity in amorphous and crystalline Re-Lu films

We report on magnetron deposition and superconducting properties of a novel superconducting material: rhenium-lutetium films on sapphire substrates. Different compositions of Re$_{x}$Lu binary are explored from $x\approx 3.8$ to close to pure Re stoichiometry. The highest critical temperature, up to $T_{c}\approx $ 6.95 K, is obtained for $x\approx 10.5$. Depending on the deposition conditions, polycrystalline or amorphous films are obtainable, both of which are interesting for practice. Crystalline structure of polycrystalline phase is identified using grazing incidence X-ray diffractometry as a non-centrosymmetric superconductor. Superconducting properties were characterized both resistively and magnetically. Demonstration of superconductivity in this material justifies the point of view that Lu plays a role of group 3 transition metal in period 6 of the Periodic table of elements. In analogy with Re$_{0.82}$Nb$_{0.18}$, Re$_{6}$Ti, Re$_{6}$Hf and Re$_{6}$Zr, one can expect that crystalline Re--Lu is also breaking the time-reversal symmetry (this still waits confirmation). Magnetoresistivity and AC/DC susceptibility measurements allowed us to determine H$_{c1}$ and H$_{c2}$ of these films, as well as estimate coherence length $ξ(0)$ and magnetic penetration depth $λ_{L}(0)$. We also provide information on surface morphology of these films.

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arXiv2023

Unconventional nodal superconductivity in miassite Rh$_{17}$S$_{15}$

Unconventional superconductivity has long been believed to arise from a lab-grown correlated electronic system. Here we report compelling evidence of unconventional nodal superconductivity in a mineral superconductor \rhs. We investigated the temperature-dependent London penetration depth $Δλ(T)$ and disorder evolution of the critical temperature $T_c$ and upper critical field $H_{c2}(T)$ in synthetic miassite \rhs. We found a power-law behavior of $Δλ(T)\sim T^n$ with $n\approx 1.1$ at low temperatures below $0.3T_c$ ($T_c$ = 5.4 K), which is consistent with the presence of lines of the node in the superconducting gap of \rhs. The nodal character of the superconducting state in \rhs~was supported by the observed pairbreaking effect in $T_c$ and $H_{c2}(T)$ in samples with the controlled disorder that was introduced by low-temperature electron irradiation. We propose a nodal sign-changing superconducting gap in the $A_{1g}$ irreducible representation, which preserves the cubic symmetry of the crystal and is in excellent agreement with the superfluid density, $λ^2(0)/λ^2(T)$.

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arXiv2023

High-frequency diode effect in superconducting Nb$_3$Sn micro-bridges

The superconducting diode effect has been recently reported in a variety of systems and different symmetry breaking mechanisms have been examined. However, the frequency range of these potentially important devices still remains obscure. We investigated superconducting micro-bridges of Nb$_{3}$Sn in out-of-plane magnetic fields; optimum magnetic fields of $\sim$10 mT generate $\sim $10% diode efficiency, while higher fields of $\sim$15-20 mT quench the effect. The diode changes its polarity with magnetic field reversal. We documented superconductive diode rectification at frequencies up to 100 kHz, the highest reported as of today. Interestingly, the bridge resistance during diode operation reaches a value that is a factor of two smaller than in its normal state, which is compatible with the vortex-caused mechanism of resistivity. This is confirmed by finite element modeling based on time-dependent Ginzburg-Landau equations. To explain experimental findings, no assumption of lattice thermal inequilibrium was required. Dissimilar edges of the superconductor strip can be responsible for the inversion symmetry breaking by vortex penetration barrier; visual evidence of this opportunity was revealed by scanning electron microscopy. Estimates are in favor of much higher (GHz) range of frequencies for this type of diode.

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arXiv2022

Quadristor: a novel device for superconducting electronics

We designed and experimentally demonstrated a four-terminal superconducting device which can function as a non-latching (reversible) superconducting switch from the diode regime to the resistive state by applying a control current much smaller than the main transport current. The device utilizes a vortex-based superconducting diode mechanism which is switched back and forth via the injection of flux quanta through auxiliary current leads. Various applications in superconducting electronics can be foreseen.

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arXiv2022

Novel results obtained by modeling of dynamic processes in superconductors: phase-slip centers as cooling engines

Based on a time-dependent Ginzburg-Landau system of equations and finite element modeling, we present novel results related with the physics of phase-slippage in superconducting wires surrounded by a non-superconductive environment. These results are obtained within our previously reported approach related to superconducting rings and superconductive gravitational wave detector transducers. It is shown that the phase-slip centers (PSCs) can be effective in originating not only positive but also negative thermal fluxes. With an appropriate design utilizing thermal diodes, PSCs can serve as cryocooling engines. Operating at $T\sim 1$ K cryostat cold-finger, they can achieve sub-Kelvin temperatures without using $^3$He.

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arXiv2020

Terahertz spectroscopy evidence of possible 40 K superconductivity in rhenium-doped strontium ruthenates

Strontium ruthenates have many similarities with copper oxide superconductors and are of particular interest for the investigation of the mechanisms and conditions which lead to high-temperature superconductivity. We report here on multiple experimental indications of superconductivity with onset at 40 K in strontium ruthenate doped by rhenium and selenium with chlorine used as the flux. The main experimental evidence arises from terahertz spectroscopy of this material followed by AC and DC magnetization, as well as measurements of its heat capacity and magnetoresistance. Structural and morphological studies revealed the heterophase nature of this polycrystalline material as well as the changes of lattice parameters relative to the original phases. Experimental data show a higher critical temperature on the surface compared to that of the bulk of the sample.

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arXiv2018

Dependence of the absolute value of the penetration depth in $\mathrm{\mathbf{{(Ba_{1-x}K_x)Fe_2As_2}}}$ on doping

We report magnetic force microscopy (MFM) measurements on the iron-based superconductor $\mathrm{Ba_{1-x}K_xFe_2As_2}$. By measuring locally the Meissner repulsion with the magnetic MFM tip, we determine the absolute value of the in-plane magnetic penetration depth ($λ_{ab}$) in underdoped, optimally-doped, and overdoped samples. The results suggest an abrupt increase of $λ_{ab}$ as doping is increased from $x_\mathrm{opt}$, which is potentially related to the presence of a quantum critical point. The response of superconducting vortices to magnetic forces exerted by the MFM tip for $x=0.19$ and $0.58$ is compatible with previously observed structural symmetries at those doping levels.

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arXiv2018

Nodeless superconductivity in type-II Dirac semimetal PdTe2: low-temperature London penetration depth and symmetry analysis

Superconducting gap structure was probed in type-II Dirac semimetal PdTe$_2$ by measuring the London penetration depth using tunnel diode resonator technique. At low temperatures, the data for two samples are well described by weak coupling exponential fit yielding $λ(T=0)=230$~nm as the only fit parameter at a fixed $Δ(0)/T_c\approx 1.76$, and the calculated superfluid density is consistent with a fully gapped superconducting state characterized by a single gap scale. Electrical resistivity measurements for in-plane and inter-plane current directions find very low and nearly temperature-independent normal- state anisotropy. The temperature dependence of resistivity is typical for conventional phonon scattering in metals. We compare these experimental results with expectations from a detailed theoretical symmetry analysis and reduce the number of possible superconducting pairing states in PdTe$_2$ to only three nodeless candidates: a regular, topologically trivial, $s$-wave pairing, and two distinct odd-parity triplet states that both can be topologically non-trivial depending on the microscopic interactions driving the superconducting instability.

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