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Sergei Urazhdin

Publications and source records attributed to Sergei Urazhdin.

At least 19 recordsLinked to original sources

Light-Driven Ultrafast Control of Time-Reversal Symmetry in SrTiO3

Light-driven control of material symmetry enables the engineering of phenomena forbidden in equilibrium. Although electromagnetic fields have been used to break time-reversal symmetry, its dynamic control on ultrafast timescales in nonmagnetic insulating oxides remains virtually unexplored. Here, we demonstrate simultaneous magnetic symmetry lowering and timereversal-symmetry breaking in cubic SrTiO3 driven by an off-resonant, elliptically polarized THz pulse. Second harmonic generation (SHG) polarimetry reveals emergent SHG circular dichroism inconsistent with third-order nonlinear processes under cubic m3m symmetry. The SHG polar patterns exhibit mirror-symmetry breaking, indicating a transient reduction to tetragonal 4/mm'm' magnetic symmetry. Furthermore, the SHG response scales linearly with the angular momentum of THz pulse, providing direct evidence for THz-field-induced timereversal-symmetry breaking. These results establish a direct pathway for ultrafast symmetry control in non-magnetic oxides, enabling dynamic manipulation of emergent phases on ultrafast timescales.

cond-mat.mtrl-sci

Transport-Noise Witnesses of Electronic Multipartite Entanglement

Entanglement among particles is a defining feature of strongly correlated quantum materials, distinguishing them from conventional metals and semiconductors. The ability to certify intrinsic entanglement among interacting electrons in solid-state materials is important not only for classifying quantum states of matter, but also for developing material-based quantum technologies. Here, we introduce a transport-based protocol for witnessing multipartite entangled electronic states, based on the equilibrium noise spectrum as an experimentally accessible observable. The appropriately integrated, symmetrized, and projected current noise obeys an upper bound that can be derived from microscopic model parameters and is invariant with respect to the choice of electronic basis. We benchmark this framework in several paradigmatic systems, including twisted bilayer graphene, twisted bilayer MoTe$_2$, and Hubbard models, certifying entanglement in the fractional Chern insulating state. The method extends recently developed scattering-based entanglement witnesses to ultralow-temperature materials, where conventional spectroscopic probes are inaccessible but candidate entangled states are expected to arise.

cond-mat.str-el

Fluctuation-Driven Enhancement of Spin-Orbit Torque near the Curie Temperature of Ultrathin Ferromagnets

We investigate how magnetic fluctuations influence spin-orbit torque in ultrathin-film magnetic heterostructures whose Curie temperature $T_C$ is suppressed by confinement. Above $T_C$, the damping-like contribution to spin-orbit field is significantly enhanced while the field-like contribution is suppressed, with the two contributions exhibiting opposite field dependencies. We show that these behaviors are consistent with fluctuation driven mixing between the longitudinal and transverse interfacial spin conductances, which enhances absorption of transversely polarized spin current by the ferromagnet. This mechanism can be activated below $T_C$ by engineering the microscopic magnetic state and by harnessing spin current-generated short-wavelength magnons, suggesting a spintronic analog of heat-assisted magnetic recording.

cond-mat.mtrl-sci

Evidence for Bose liquid from anomalous shot noise in nanojunctions of bad metal beta-Ta

We report anomalous shot noise in nanojunctions of beta-tantalum, a ``bad" metal whose electronic properties are inconsistent with the Fermi liquid theory. Fano factors cluster around even multiples of the values expected for Fermi liquids, suggesting that beta-Ta may host a correlated charge liquid of Cooper pair-like electron groups. Further evidence for correlations is provided by the effects of magnetic impurities, as well as reduced density of states near the Fermi level indicated by point contact spectroscopy and first principles calculations. Our results open new avenues for studies and applications of electron correlations.

cond-mat.mtrl-sci

The role of electron interactions in a failed insulator revealed by shot noise

In materials known as failed insulators, electrical resistivity increases as temperature decreases, yet does not diverge - a phenomenon inconsistent with single-particle theories. We investigate the origin of this behavior by measuring shot noise in nanojunctions of nitrogen-doped beta-Ta, a prototypical failed insulator. Junctions as short as 8 nanometers exhibit hot-electron shot noise, indicating strong electron interactions. We show that charge hopping mediated by these interactions explains the anomalous electronic properties. Our findings open new avenues for exploiting electron interactions in spin-orbitronic and superconducting applications of failed insulators.

cond-mat.mes-hall

Symmetries of electron interactions in Hubbard models of unconventional superconductors

We use symmetry arguments to show that the matrix elements of electron-electron interaction on a lattice reach extrema in states composed of wavevectors near high-symmetry points of the Brillouin zone. The mechanism is illustrated by minimal models of cuprates and Fe-based superconductors, where this dependence originates from the wavevector-dependent orbital composition of wavefunctions. We discuss how these dependences can facilitate finite-momentum pairing. Our results provide symmetry-based guidance for the search for new high-temperature superconductors.

cond-mat.supr-con

Atomic and inter-atomic orbital magnetization induced in SrTiO$_3$ by chiral phonons

An unexpectedly large transient magnetization induced by circularly polarized ferroelectric phonons was recently observed in a nonmagnetic insulator SrTiO3 [Nature 628, 534 (2024)]. We use a minimal molecular orbital model to demonstrate two electronic contributions to this effect. An atomic orbital contribution arises from the pumping of orbital angular momentum of Ti by chiral motion of coordinating oxygen atoms. An additional inter-atomic contribution is associated with the transient circulating current around the oxygen atoms, resulting in efficient dressing of phonons by electron dynamics. The insights provided by our model may facilitate the development of ultrafast magnetization control and orbitronic sources.

cond-mat.mtrl-sci

Observation of Rashba Magnetism in Ultrathin Ferromagnet-Heavy Metal Bilayers

Both magnetism and spin-orbit coupling in systems with broken inversion symmetry lift the spin degeneracy of electronic bands, but the consequences of interplay between these mechanisms remain poorly understood. Here, we show that ultrathin transition ferromagnet-heavy metal bilayers exhibit anomalous temperature- and electric bias-dependent behaviors in the vicinity of the Curie temperature, inconsistent with the usual Weiss magnetism. Characterization by several complementary techniques and analysis of the dependence on composition reveal that these effects originate from interfacial spin-orbit interaction, which results in the emergence of a state with distinct magnetic and magnetoelectronic properties that can be described as Rashba magnetism. Our findings open a new route for the characterization and control of spin-orbit phenomena in heterostructures enabling the development of efficient spin-orbitronic devices.

cond-mat.mtrl-sci

Shot noise in a metal close to Mott transition

SrIrO$_3$ is a metallic complex oxide with unusual electronic and magnetic properties believed to originate from electron correlations due to its proximity to Mott metal-insulator transition. However, the nature of its electronic state and the mechanism of metallic conduction remain poorly understood. We demonstrate that shot noise produced by nanoscale SrIrO$_3$ junctions is strongly suppressed, inconsistent with diffusive quasiparticle transport. Analysis of thermal effects and scaling with the junction length reveals that conduction is mediated by collective hopping of electrons almost localized by correlations. Our results provide insight into the non-Fermi liquid state close to Mott transition, and advance shot noise measurements as a powerful technique for the studies of quantum materials.

cond-mat.str-el

Anomalous Zeeman effect in SrTiO3 and its possible all-electric detection

We show that the interplay between spin-orbit coupling and cubic symmetry breaking in SrTiO3 results in a highly anomalous Zeeman effect of conduction electrons substantially different among the three conduction sub-bands and strongly dependent on their splitting. This effect can be measured via electrically-driven spin resonance enabled by the interplay between electron hopping and spin-orbit coupling, and enhanced by the near-degeneracy of the conduction sub-bands. The proposed effects can provide a unique insight into the electronic properties of SrTiO3 and its heterostructures.

cond-mat.mtrl-sci

Electronic properties of the mean-field resonating valence bond model of cuprates

We show that the mean-field resonating valence bond approximation proposed in 1987 by Baskaran, Zou, and Anderson describes gapless charge pair excitations confined to the boundaries of the spinon Brillouin zone. The existence of such pairs accounts for all the essential anomalous electronic properties of cuprates, with superconductivity arising due to the charge drag by the spinon superflow. This mechanism may be relevant to other unconventional superconductors.

cond-mat.str-el

Effects of spin-orbit interaction and electron correlations in strontium titanate

We show that the Bloch states in the conduction band of SrTiO$_3$ arise from the interplay between highly anisotropic hopping in sub-bands derived from the Ti $t_{2g}$ orbitals and spin-orbit coupling that mixes these orbitals. Because of the nearly flat-band characteristics for one of the principal axes, at sufficiently high doping these Bloch states become unstable with respect to electron interactions, resulting in Mott-like singlet correlations. These findings may be relevant to the anomalous electronic properties of SrTiO$_3$, including its unusual superconductivity.

cond-mat.supr-con

Orbital correlations in ultrathin films of late transition metals

We develop a two-orbital Hubbard model of electron correlations in ultrathin (111)-oriented fcc films of late transition metals such as Co and Ni. Our model indicates that the Mott-Hund's interaction results in ferromagnetic nearest-neighbor orbital correlations. Frustration associated with the mismatch between orbital and crystal symmetries prevents orbital ordering, resulting in the orbital liquid state. This state can be manifested in phenomena involving spin-orbit coupling, such as magnetic anisotropy.

cond-mat.str-el

Chiral superconductivity in cuprates mediated by spin-orbit coupling to spinon superfluidity

We utilize the Hubbard model to demonstrate that doping of the antiferromagnetic parent compounds of cuprate superconductors stabilizes a spin liquid state. Superconductivity in such a state emerges due to the spin-orbit coupling between charge current and superfluidity of spinon condensate, resulting in a chiral relation between the order parameter phase gradient and supercurrent. We propose simple experimental tests for the presented mechanism.

cond-mat.supr-con

Orbital entanglement mechanism of superconductivity in cuprates

We utilize a 1d Hubbard model to show that the superconductivity in cuprate superconductors likely arises due to the orbital entanglement between holes in the copper oxide plane mediated by orbitally-selective charge hopping. The main role of doping required to achieve superconductivity in cuprates is to suppress the Mott correlations and orbital ordering. The proposed mechanism explains superconductivity in other unconventional superconductors, and provides guidance in the search for new high-temperature superconductors.

cond-mat.str-el

Ultrafast electron dynamics in platinum and gold thin films driven by optical and terahertz fields

We investigate the ultrafast electron dynamics triggered by terahertz and optical pulses in thin platinum and gold films by probing their transient optical reflectivity. The response of the platinum film to an intense terahertz pulse is similar to the optically-induced dynamics of both films and can be described by a two-temperature model. Surprisingly, gold can exhibit a much smaller terahertz pulse-induced reflectivity change and with opposite sign. For platinum, we estimate a 20% larger electron-phonon coupling for the terahertz-driven dynamics compared to the optically-induced one, which we ascribe to an additional nonthermal electron-phonon coupling contribution. We explain the remarkable response of gold to terahertz radiation with the field emission of electrons due the Fowler-Nordheim tunneling process, in samples with thickness below the structural percolation threshold where near-field enhancement is possible. Our results provide a fundamental insight into the ultrafast processes relevant to modern electro- and magneto-optical applications.

cond-mat.mtrl-sci

Transport and relaxation of current-generated nonequilibrium phonons from nonlocal electronic measurements

We study phonons generated by current in a Pt nanowire, by measuring resistance of another nanowire separated from the first one by an insulating spacer. For thin spacers, the resistance varies almost linearly with current at cryogenic temperatures, while an additional quadratic contribution emerges for thicker spacers. These observations suggest a non-thermal distribution of current-generated phonons that relax via strongly nonlinear dynamical processes rather than few-phonon scattering. Our results provide insight into the nonequilibrium phonon dynamics at nanoscale, which may facilitate efficient heat management in electronic nanodevices.

cond-mat.mes-hall

Exchange bias without directional anisotropy in Permalloy/CoO bilayers

We utilize transverse ac susceptibility measurements to characterize magnetic anisotropy in archetypal exchange-bias bilayers of ferromagnet Permalloy (Py) and antiferromagnet CoO. Unidirectional anisotropy is observed for thin Py, but becomes negligible at larger Py thicknesses, even though the directional asymmetry of the magnetic hysteresis loop remains significant. Additional magnetoelectronic measurements, magneto-optical imaging, as well as micromagnetic simulations show that these surprising behaviors are likely associated with asymmetry of spin flop distribution created in CoO during Py magnetization reversal, which facilitates the rotation of the latter back into its field-cooled direction. Our findings suggest new possibilities for efficient realization of multistable nanomagnetic systems for neuromorphic applications.

cond-mat.mtrl-sci