SearcharxivSearch

arXiv subjects

Sergio Caprara

Publications and source records attributed to Sergio Caprara.

At least 19 recordsLinked to original sources

Superconducting dome due to the Fano-Feshbach shape resonance in artificial high-Tc superlattices

In this work we provide compelling experimental validation of the Bianconi Perali Valletta (BPV) theory predicting a superconducting dome based on a quantum material design of Artificial High TC Superlattices (AHTS) made with a selected nanoscale heterostructure geometry. These AHTS are SNSN superlattices of quantum wells of period d, composed of first units, superconducting doped Mott insulator layers with Rashba spin orbit coupling (S) of thickness L, intercalated by second units, normal metal spacers (N). In these superlattices, grown by molecular beam epitaxy (MBE), the experimental superconducting dome is obtained by material quantum design changing the chemical potential via the quantum geometrical factor L/d which tunes the Fano-Feshbach shape resonance in the pair transfer between superconducting gaps in the BCS regime and different gaps in the BEC-BCS crossover. Here we present a systematic magneto-transport study of AHTS artificial superlattices across the full doping range of the superconducting dome, from the deeply underdoped to the overdoped regime, using pulsed magnetic fields up to 72 T. By varying the L/d ratio, we tune the effective hole concentration delta=0.45(1-L/d) and map the evolution of the resistive transitions, the upper critical magnetic field and the Ginzburg-Landau coherence length

cond-mat.supr-con

The charge density fluctuations and the Shrinking Fermi Liquid scenario for strange metallicity in cuprates

We interpret the strange metal (SM) properties of slightly overdoped cuprates in terms of the recently proposed Shrinking Fermi Liquid theory. This is based on the pervading presence in the cuprate phase diagram of charge density fluctuations (CDF), which have been identified and characterized in RIXS. These fluctuations are abundant and have a low energy due to the proximity of the charge density wave quantum critical point hidden under the superconducting dome of cuprates, but have a short range and non-critical character with a finite energy M/\gamma ~10 meV as measured above Tc. Here M~ \xi^-2 is determined by the short correlation length \xi, while \gamma encodes the Landau damping ruling the lifetime of the charge fluctuations. Besides these low energy CDF, cuprates also display phonons and a broad continuum of particle-hole excitations, mostly due to spin paramagnons arising from their strongly correlated character. With these experimentally characterized ingredients we show that above Tc the SM properties in transport are well described in terms of fermionic Landau quasiparticles scattering with CDF and phonons. The optical properties can instead be interpreted by the combined effect of low energy CDF determining the temperature dependence, and of the paramagnon continuum determining a linear in frequency scattering rate. Remarkably, the combined effect of these simple ingredients also induces \omega/T scaling properties for frequencies larger than M/\gamma. When superconductivity is suppressed by strong magnetic fields the SM properties extend down to a few Kelvin. By assuming that the CDF dissipation parameter \gamma grows logarithmically by lowering T, we account for all anomalous transport and thermodynamic properties of cuprates (specific heat, Seebeck, heat transport, resistivity, and magnetoresistance) thereby providing a consistent scenario for the SM phase of cuprates.

cond-mat.str-el

Unveiling the Interplay of Charge and Magnetic Excitations in HgBa$_2$Ca$_2$Cu$_3$O$_{8+\delta}$

Unraveling the mechanism that binds electrons into Cooper pairs in cuprate high-temperature superconductors remains one of the most fundamental challenges in condensed-matter physics. While both magnetic interactions and lattice vibrations are known to govern key electronic properties, their possible cooperation has never been directly observed. We investigate HgBa$_2$Ca$_2$Cu$_3$O$_{8+\delta}$ (Hg1223) - the cuprate with the highest $T_{\mathrm{c}}$ at ambient pressure - as a magnifying glass to probe the possible entwining of the excitations at the core of the pairing. Using resonant inelastic X-ray scattering, we find that the charge response is dominated by dynamic charge density fluctuations (CDF) extending up to several hundred meV, where magnetic excitations reside. At the same momentum where CDF are most intense, the paramagnon energy exhibits a pronounced softening, revealing a strong interplay among charge, lattice, and spin excitations. Our results point to a cooperative mechanism in which dynamic charge fluctuations mediate the coupling between lattice, charge and spin degrees of freedom-shedding new light on the fundamental origin of high-$T_{\mathrm{c}}$ superconductivity.

cond-mat.supr-con

Majorana fermions at self-generated interfaces

The Kitaev model describing a one-dimensional topological superconducting chain is known to support two Majorana fermions localized at the systems endpoints when the parameters are tuned to the topological phase. In this work, we investigate the possibility that Majorana fermions may also emerge away from the physical boundaries of the chain. To this purpose, we generalize the Kitaev model by incorporating a local coupling between the electronic density and a classical elastic (lattice) field. This electron-lattice interaction can induce phase separation between superconducting regions characterized by distinct topological invariants, thereby generating internal interfaces that host Majorana bound states. Under these conditions, a dilute gas of Majorana fermions can be realized in the bulk of the system.

cond-mat.supr-con

Electron-phonon coupling revealed by charge density fluctuations in cuprate superconductors

Electron-phonon coupling (EPC) governs lattice dynamics, charge transport, and collective electronic phases in quantum materials. In several families of unconventional superconductors, including transition-metal dichalcogenides and kagome metals, growing evidence points to a cooperative role of EPC and dynamic charge-density fluctuations (CDF) in stabilizing superconductivity. However, how the EPC strength evolves across phase diagrams and relates to superconducting properties in strongly correlated systems remains an open question. Here we investigate the interplay between phonons and the CDF recently identified in cuprate superconductors. Using resonant inelastic x-ray scattering, we track the dispersion and intensity of bond-stretching phonons in YBa$_2$Cu$_3$O$_{7-\delta}$ over wide ranges of doping, temperature, and momentum. We find that both the phonon softening at the CDF wave vector and the EPC strength, extracted from a pronounced phonon intensity anomaly, are maximized near $p = 0.19$, where superconducting properties are optimal and CDF intensity is strongest. These results identify dynamic charge-density fluctuations, rather than quasi-static charge density waves, as the dominant source of phonon renormalization in cuprates, and establish a direct correlation between EPC strength and the superconducting dome. More broadly, our measurements highlight EPC as a doping-dependent property of correlated materials, shaped by the electronic environment in which lattice vibrations are embedded.

cond-mat.supr-con

Superconductivity with repulsion: a variational approach

We revisit the stability of the superconducting state within mean-field theory in the presence of repulsive pairing interactions, focusing on multiband systems where such channels naturally arise. We show that, when repulsion is present, the self-consistent BCS solution appears as a saddle point of the conventional mean-field free energy, casting doubt on its physical stability. We show that this pathology is an artifact of using a non-variational functional. Recasting the problem with Bogoliubov's variational principle restores a free energy that is bounded from below and places the BCS solution at a genuine minimum. Using a two-band toy model relevant to iron-based superconductors, we demonstrate the stability of the s$_\pm$ state and clarify how projection schemes that rely only on the interaction matrix can misidentify the attractive eigenmode that drives pairing. Our results clarify the instability issue highlighted by Aase et al. and provide a consistent foundation for analyzing fluctuations in the presence of repulsive interactions.

cond-mat.supr-con

Kondo versus Fano in superconducting artificial high-Tc heterostructures

Recently, the quest for high-Tc superconductivity has evolved from the trial-and-error methodology to the growth of nanostructured artificial high-Tc superlattices (AHTS) with tailor-made superconducting functional properties by quantum design. Superlattices are composed of nanoscale superconducting units of modulation doped Mott insulator La2CuO4 with thickness L intercalated by metallic overdoped La1.55Sr0.45CuO4 and period d. Quantum design based on the multi-gap Bogoliubov theory including spin-orbit coupling (SOC). has been employed for prediction of the amplification of the critical temperature as a function of the conformational parameter L/d. At the top of the superconducting dome, at the magic ratio L/d=2/3, the heterostructures are tuned at the Fano-Feshbach resonance and the normal phase exhibits the Planckian T-linear resistivity. Here, we report experimental evidence that the Kondo proximity effect competes with the Fano-Feshbach resonance suppressing Tc on both sides of the superconducting dome. The Kondo proximity effect is expected in electrical resistance of AHTS nanoscale heterostructures following a Kondo universal scaling obtained by numerical renormalization group theory. We show the vanishing Kondo temperature TK and Kondo scattering amplitude R0K at L/d=2/3, while TK and R0K increase on the underdoped (L/d>2/3) and overdoped (L/d<2/3) side of the superconducting dome.

cond-mat.supr-con

Berezinskii-Kosterlitz-Thouless to BCS-like superconducting transition crossover driven by weak magnetic fields in ultra-thin NbN films

The Berezinskii-Kosterlitz-Thouless (BKT) transition in ultra-thin NbN films is investigated in the presence of weak perpendicular magnetic fields. A jump in the phase stiffness at the BKT transition is detected up to 5 G, while the BKT features are smeared between 5 G and 50 G, disappearing altogether at 100 G, where conventional current-voltage behaviour is observed. Our findings demonstrate that weak magnetic fields, insignificant in bulk systems, deeply affect our ultra-thin system, promoting a crossover from Halperin-Nelson fluctuations to a BCS-like state with Ginzburg-Landau fluctuations, as the field increases. This behavior is related to field-induced free vortices that screen the vortex-antivortex interaction and smear the BKT transition.

cond-mat.supr-con

Thermodynamic phase diagram of the competition between superconductivity and charge order in cuprates

We argue that there is a special doping point in the phase diagram of cuprates, such that the condensation of holes into a charge-ordered and into a superconducting phase are degenerate in energy but with an energy barrier in between. We present a Monte Carlo simulation of this problem without and with quenched disorder. While in the clean case charge order and superconductivity are separated by a first-order line which is nearly independent of temperature, in the presence of quenched disorder, charge order is fragmented into domains separated by superconducting filaments reminiscent of the supersolid behavior in $^4$He. The resulting phase diagram is in good agreement with the experiments.

cond-mat.supr-con

Charge-Density Waves vs. Superconductivity: Some Results and Future Perspectives

Increasing experimental evidence suggests the occurrence of filamentary superconductivity in different (quasi) two-dimensional physical systems. In this piece of work, we discuss the proposal that under certain circumstances, this occurrence may be related to the competition with a phase characterized by charge ordering in the form of charge-density waves. We provide a brief summary of experimental evidence supporting our argument in two paradigmatic classes of materials, namely transition metal dichalcogenides and cuprates superconductors. We present a simple Ginzburg-Landau two-order-parameters model as a starting point to address the study of such competition. We finally discuss the outcomes of a more sophisticated model, already presented in the literature and encoding the presence of impurities, and how it can be further improved in order to really address the interplay between charge-density waves and superconductivity and the possible occurrence of filamentary superconductivity at the domain walls between different charge-ordered regions.

cond-mat.supr-con

Superfluid response of two-dimensional filamentary superconductors

Different classes of low-dimensional superconducting systems exhibit an inhomogeneous filamentary superconducting condensate whose macroscopic coherence still needs to be fully investigated and understood. Here we present a thorough analysis of the superfluid response of a prototypical filamentary superconductor embedded in a {two-dimensional} metallic matrix. By mapping the system into an exactly solvable random impedance network, we show how the dissipative (reactive) response of the system non-trivially depends on both the macroscopic and microscopic characteristics of the metallic (superconducting) fraction. We compare our calculations with resonant-microwave transport measurements performed on LaAlO$_3$/SrTiO$_3$ heterostructures over an extended range of temperatures and carrier densities finding that the filamentary character of superconductivity accounts for unusual peculiar features of the experimental data.

cond-mat.supr-con

Quantum zero point electromagnetic energy difference between the superconducting and the normal phase in a HTc superconducting metal bulk sample

We provide a novel methodological approach to the estimate of the change of the Quantum Vacuum electromagnetic energy density in a High critical Temperature superconducting metal bulk sample, when it undergoes the transition in temperature, from the superconducting to the normal phase. The various contributions to the Casimir energy in the two phases are highlighted and compared. While the TM polarization of the vacuum mode allows for a macroscopic description of the superconducting transition, the changes in the TE vacuum mode induced by the superconductive correlations are introduced within a microscopic model, which does not explicitly take into account the anisotropic structure of the material.

cond-mat.supr-con

Effect of the Anomalous Diffusion of Fluctuating Cooper Pairs in the Density of States of Superconducting NbN Thin Films

Recent scanning tunnelling microscopy experiments in NbN thin disordered superconducting films found an emergent inhomogeneity at the scale of tens of nanometers. This inhomogeneity is mirrored by an apparent dimensional crossover in the paraconductivity measured in transport above the superconducting critical temperature $T_c$. This behavior was interpreted in terms of an anomalous diffusion of fluctuating Cooper pairs, that display a {\em quasi-confinement} (i.e., a slowing down of their diffusive dynamics) on length scales shorter than the inhomogeneity identified by tunnelling experiments. Here we assume this anomalous diffusive behavior of fluctuating Cooper pairs and calculate the effect of these fluctuations on the electron density of states above $T_c$. We find that the density of states is substantially suppressed up to temperatures well above $T_c$. This behavior, which is closely reminiscent of a pseudogap, only arises from the anomalous diffusion of fluctuating Cooper pairs in the absence of stable preformed pairs, setting the stage for an intermediate behavior between the two common paradigms in the superconducting-insulator transition, namely the localisation of Cooper pairs (the so-called bosonic scenario) and the breaking of Cooper pairs into unpaired electrons due to strong disorder (the so-called fermionic scenario).

cond-mat.supr-con

Law without law or "just" limit theorems?

About 35 years ago Wheeler introduced the motto `law without law' to highlight the possibility that (at least a part of) Physics may be understood only following {\em regularity principles} and few relevant facts, rather than relying on a treatment in terms of fundamental theories. Such a proposal can be seen as part of a more general attempt (including the maximum entropy approach) summarized by the slogan `it from bit', which privileges the information as the basic ingredient. Apparently it seems that it is possible to obtain, without the use of physical laws, some important results in an easy way, for instance, the probability distribution of the canonical ensemble. In this paper we will present a general discussion on those ideas of Wheeler's that originated the motto `law without law'. In particular we will show how the claimed simplicity is only apparent and it is rather easy to produce wrong results. We will show that it is possible to obtain some of the results treated by Wheeler in the realm of the statistical mechanics, using precise assumptions and nontrivial results of probability theory, mainly concerning ergodicity and limit theorems.

cond-mat.stat-mech

Theory of charge-spin conversion at oxide interfaces: The inverse spin-galvanic effect

We evaluate the non-equilibrium spin polarization induced by an applied electric field for a tight-binding model of electron states at oxides interfaces in LAO/STO heterostructures. By a combination of analytic and numerical approaches we investigate how the spin texture of the electron eigenstates due to the interplay of spin-orbit coupling and inversion asymmetry determines the sign of the induced spin polarization as a function of the chemical potential or band filling, both in the absence and presence of local disorder. With the latter, we find that the induced spin polarization evolves from a non monotonous behavior at zero temperature to a monotonous one at higher temperature. Our results may provide a sound framework for the interpretation of recent experiments.

cond-mat.mes-hall

Chaos and Stochastic Models in Physics: Ontic and Epistemic Aspects

There is a persistent confusion about determinism and predictability. In spite of the opinions of some eminent philosophers (e.g., Popper), it is possible to understand that the two concepts are completely unrelated. In few words we can say that determinism is ontic and has to do with how Nature behaves, while predictability is epistemic and is related to what the human beings are able to compute. An analysis of the Lyapunov exponents and the Kolmogorov-Sinai entropy shows how deterministic chaos, although with an epistemic character, is non subjective at all. This should clarify the role and content of stochastic models in the description of the physical world.

nlin.CD

Glue function of optimally and overdoped cuprates from inversion of the Raman spectra

We address the issue of identifying the mediators of effective interactions in cuprates superconductors. Specifically, we use inversion theory to analyze Raman spectra of optimally and over-doped La$_{2-x}$Sr$_x$CuO$_4$ samples. This allows us to extract the so-called glue function without making any a priori assumption based on any specific model. We use instead two different techniques, namely the singular value decomposition and a multi-rectangle decomposition. With both techniques we find consistent results showing that: i) two distinct excitations are responsible for the glue function, which have completely different doping dependence. One excitation becomes weak above optimal doping, where on the contrary the other keeps (or even slightly increases) its strength; ii) there is a marked temperature dependence on the weight and spectral distribution of these excitation, which therefore must have a somewhat critical character. It is quite natural to identify and characterize these two distinct excitations as damped antiferromagnetic spin waves and damped charge density waves, respectively. This sets the stage for a scenario in which superconductivity is concomitant and competing with a charge ordering instability.

cond-mat.supr-con

Nematic fluctuations and the magneto-structural phase transition in ${\rm Ba(Fe_{1-x}Co_x)_2As_2}$

An inelastic light (Raman) scattering study of nematicity and critical fluctuations in ${\rm Ba(Fe_{1-x}Co_x)_2As_2}$ ($0\le x \le 0.051$) is presented. It is shown that the response from fluctuations appears only in $B_{1g}$ (${x^2-y^2}$) symmetry. The scattering amplitude increases towards the structural transition at $T_s$ but vanishes only below the magnetic ordering transition at $T_{\rm SDW} < T_s$, suggesting a magnetic origin of the fluctuations. The theoretical analysis explains the selection rules and the temperature dependence of the fluctuation response. These results make magnetism the favorite candidate for driving the series of transitions.%Below $T_{\rm SDW}$ the gap of the magnetically ordered phase opens up.

cond-mat.str-el