arXiv subjects

Shahal Ilani

Publications and source records attributed to Shahal Ilani.

At least 19 recordsLinked to original sources

arXiv2024

Imaging the Sub-Moiré Potential Landscape using an Atomic Single Electron Transistor

Electrons in solids owe their properties to the periodic potential landscapes they experience. The advent of moiré lattices has revolutionized our ability to engineer such landscapes on nanometer scales, leading to numerous groundbreaking discoveries. Despite this progress, direct imaging of these electrostatic potential landscapes remains elusive. In this work, we introduce the Atomic Single Electron Transistor (SET), a novel scanning probe utilizing a single atomic defect in a van der Waals (vdW) material, which serves as an ultrasensitive, high-resolution potential imaging sensor. Built upon the quantum twisting microscope (QTM) platform, this probe leverages the QTM's distinctive capability to form a pristine, scannable 2D interface between vdW heterostructures. Using the Atomic SET, we present the first direct images of the electrostatic potential in one of the most canonical moiré interfaces: graphene aligned to hexagonal boron nitride. Our results reveal that this potential exhibits an approximate C6 symmetry, has minimal dependence on the carrier density, and has a substantial magnitude of ~60 mV even in the absence of carriers. Theoretically, the observed symmetry can only be explained by a delicate interplay of physical mechanisms with competing symmetries. Intriguingly, the magnitude of the measured potential significantly exceeds theoretical predictions, suggesting that current understanding may be incomplete. With a spatial resolution of 1 nm and a sensitivity to detect the potential of even a few millionths of an electron charge, the Atomic SET opens the door for ultrasensitive imaging of charge order and thermodynamic properties for a range of quantum phenomena, including various symmetry-broken phases, quantum crystals, vortex charges, and fractionalized quasiparticles.

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arXiv2024

Measuring Phonon Dispersion and Electron-Phason Coupling in Twisted Bilayer Graphene with a Cryogenic Quantum Twisting Microscope

The coupling between electrons and phonons is one of the fundamental interactions in solids, underpinning a wide range of phenomena such as resistivity, heat conductivity, and superconductivity. However, direct measurements of this coupling for individual phonon modes remains a significant challenge. In this work, we introduce a novel technique for mapping phonon dispersions and electron phonon coupling (EPC) in van der Waals materials. By generalizing the quantum twisting microscope to cryogenic temperatures, we demonstrate its capability to map not only electronic dispersions via elastic momentum-conserving tunnelling, but also phononic dispersions through inelastic momentum-conserving tunnelling. Crucially, the inelastic tunnelling strength provides a direct and quantitative measure of the momentum and mode resolved EPC. We use this technique to measure the phonon spectrum and EPC of twisted bilayer graphene (TBG). Surprisingly, we find that unlike standard acoustic phonons, whose coupling to electrons diminishes as their momentum goes to zero, TBG exhibits a low energy mode whose coupling increases with decreasing twist angle. We show that this unusual coupling arises from the modulation of the inter-layer tunnelling by a layer-antisymmetric 'phason' mode of the moiré system. The technique demonstrated here opens the way for probing a large variety of other neutral collective modes that couple to electronic tunnelling, including plasmons, magnons and spinons in quantum materials.

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arXiv2024

Theory of phonon spectroscopy with the quantum twisting microscope

We develop a theory of probing phonon modes of van-der-Waals materials using the quantum twisting microscope. While elastic tunneling dominates the tunneling current at small twist angles, the momentum mismatch between the K-points of tip and sample at large twist angles can only be bridged by inelastic scattering. This allows for probing phonon dispersions along certain lines in reciprocal space by measuring the tunneling current as a function of twist angle and bias voltage. We illustrate this modality of the quantum twisting microscope by developing a systematic theory for graphene-graphene junctions. We show that beyond phonon dispersions, the tunneling current also encodes the strength of electron-phonon couplings. Extracting the coupling strengths for individual phonon modes requires careful consideration of various inelastic tunneling processes. These processes are associated with the intralayer and interlayer electron-phonon couplings and appear at different orders in a perturbative calculation of the tunneling current. We find that the dominant process depends on the particular phonon mode under consideration. Our results inform the quest to understand the origin of superconductivity in twisted bilayer graphene and provide a case study for quantum-twisting-microscope investigations of collective modes.

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arXiv2024

Collective tunneling of a Wigner necklace in carbon nanotubes

The collective tunneling of a Wigner necklace - a crystal-like state of a small number of strongly interacting electrons confined to a suspended nanotube and subject to a double well potential - is theoretically analyzed and compared with experiments in [Shapir \emph{et al.}, Science {\bf 364}, 870 (2019)]. Density Matrix Renormalization Group computations, exact diagonalization, and instanton theory provide a consistent description of this very strongly interacting system, and show good agreement with experiments. Experimentally extracted and theoretically computed tunneling amplitudes exhibit a scaling collapse. Collective quantum fluctuations renormalize the tunneling, and substantially enhance it as the number of electrons increases.

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arXiv2024

Probing quantum spin liquids with a quantum twisting microscope

The experimental characterization of quantum spin liquids poses significant challenges due to the absence of long-range magnetic order, even at absolute zero temperature. The identification of these states of matter often relies on the analysis of their excitations. In this paper, we propose a method for detecting the signatures of the fractionalized excitations in quantum spin liquids using a tunneling spectroscopy setup. Inspired by the recent development of the quantum twisting microscope, we consider a planar tunneling junction, in which a candidate quantum spin liquid material is placed between two graphene layers. By tuning the relative twist angle and voltage bias between the leads, we can extract the dynamical spin structure factor of the tunneling barrier with momentum and energy resolution. Our proposal presents a promising tool for experimentally characterizing quantum spin liquids in two-dimensional materials.

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arXiv2022

Spread and erase -- How electron hydrodynamics can eliminate the Landauer-Sharvin resistance

It has long been realized that even a perfectly clean electronic system harbors a Landauer-Sharvin resistance, inversely proportional to the number of its conduction channels. This resistance is usually associated with voltage drops on the system's contacts to an external circuit. Recent theories have shown that hydrodynamic effects can reduce this resistance, raising the question of the lower bound of resistance of hydrodynamic electrons. Here we show that by a proper choice of device geometry, it is possible to spread the Landauer-Sharvin resistance throughout the bulk of the system, allowing its complete elimination by electron hydrodynamics. We trace the effect to the dynamics of electrons flowing in channels that terminate within the sample. For ballistic systems this termination leads to back-reflection of the electrons and creates resistance. Hydrodynamically, the scattering of these electrons off other electrons allows them to transfer to transmitted channels and avoid the resistance. Counter-intuitively, we find that in contrast to the ohmic regime, for hydrodynamic electrons the resistance of a device with a given width can decrease with its length, suggesting that a long enough device may have an arbitrarily small total resistance.

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arXiv2022

The Quantum Twisting Microscope

The invention of scanning probe microscopy has revolutionized the way electronic phenomena are visualized. While present-day probes can access a variety of electronic properties at a single location in space, a scanning microscope that can directly probe the quantum mechanical existence of an electron at multiple locations would provide direct access to key quantum properties of electronic systems, so far unreachable. Here, we demonstrate a conceptually new type of scanning probe microscope - the Quantum Twisting Microscope (QTM) - capable of performing local interference experiments at its tip. The QTM is based on a unique van-der-Waals tip, allowing the creation of pristine 2D junctions, which provide a multitude of coherently-interfering paths for an electron to tunnel into a sample. With the addition of a continuously scanned twist angle between the tip and sample, this microscope probes electrons in momentum space similar to the way a scanning tunneling microscope probes electrons in real space. Through a series of experiments, we demonstrate room temperature quantum coherence at the tip, study the twist angle evolution of twisted bilayer graphene, directly image the energy bands of monolayer and twisted bilayer graphene, and finally, apply large local pressures while visualizing the evolution of the flat energy bands of the latter. The QTM opens the way for novel classes of experiments on quantum materials.

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arXiv2021

Imaging Hydrodynamic Electrons Flowing Without Landauer-Sharvin Resistance

Electrical resistance usually originates from lattice imperfections. However, even a perfect lattice has a fundamental resistance limit, given by the Landauer conductance caused by a finite number of propagating electron modes. This resistance, shown by Sharvin to appear at the contacts of electronic devices, sets the ultimate conductance limit of non-interacting electrons. Recent years have seen growing evidence of hydrodynamic electronic phenomena, prompting recent theories to ask whether an electronic fluid can radically break the fundamental Landauer-Sharvin limit. Here, we use single-electron transistor imaging of electronic flow in high-mobility graphene Corbino disk devices to answer this question. First, by imaging ballistic flows at liquid-helium temperatures, we observe a Landauer-Sharvin resistance that does not appear at the contacts but is instead distributed throughout the bulk. This underpins the phase-space origin of this resistance - as emerging from spatial gradients in the number of conduction modes. At elevated temperatures, by identifying and accounting for electron-phonon scattering, we reveal the details of the purely hydrodynamic flow. Strikingly, we find that electron hydrodynamics eliminates the bulk Landuer-Sharvin resistance. Finally, by imaging spiraling magneto-hydrodynamic Corbino flows, we reveal the key emergent length scale predicted by hydrodynamic theories - the Gurzhi length. These observations demonstrate that electronic fluids can dramatically transcend the fundamental limitations of ballistic electrons, with important implications for fundamental science and future technologies

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arXiv2020

Entropic evidence for a Pomeranchuk effect in magic angle graphene

In the 1950's, Pomeranchuk predicted that, counterintuitively, liquid 3He may solidify upon heating, due to a high excess spin entropy in the solid phase. Here, using both local and global electronic entropy and compressibility measurements, we show that an analogous effect occurs in magic angle twisted bilayer graphene. Near a filling of one electron per moir'e unit cell, we observe a dramatic increase in the electronic entropy to about 1kB per unit cell. This large excess entropy is quenched by an in-plane magnetic field, pointing to its magnetic origin. A sharp drop in the compressibility as a function of the electron density, associated with a reset of the Fermi level back to the vicinity of the Dirac point, marks a clear boundary between two phases. We map this jump as a function of electron density, temperature, and magnetic field. This reveals a phase diagram that is consistent with a Pomeranchuk-like temperature- and field-driven transition from a low-entropy electronic liquid to a high-entropy correlated state with nearly-free magnetic moments. The correlated state features an unusual combination of seemingly contradictory properties, some associated with itinerant electrons, such as the absence of a thermodynamic gap, metallicity, and a Dirac-like compressibility, and others associated with localized moments, such as a large entropy and its disappearance with magnetic field. Moreover, the energy scales characterizing these two sets of properties are very different: whereas the compressibility jump onsets at T~30K, the bandwidth of magnetic excitations is ~3K or smaller. The hybrid nature of the new correlated state and the large separation of energy scales have key implications for the physics of correlated states in twisted bilayer graphene.

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arXiv2020

Ballistic and hydrodynamic magnetotransport in narrow channels

An increasing number of low carrier density materials exhibit a surprisingly large transport mean free path due to inefficient momentum relaxation. Consequently, charge transport in these systems is markedly non-ohmic but rather ballistic or hydrodynamic, features which can be explored by driving current through narrow channels. Using a kinetic equation approach we theoretically investigate how a non-quantizing magnetic field discerns ballistic and hydrodynamic transport, in particular in the spatial dependence of the transverse electric field, $E_y$: We find that $E_y$ is locally enhanced when the flow exhibits a sharp directional anisotropy in the non-equilibrium density. As a consequence, at weak magnetic fields, the curvature of $E_y$ has opposite signs in the ballistic and hydrodynamic regimes. Moreover, we find a robust signature of the onset of non-local correlations in the form of distinctive peaks of the transverse field, which are accessible by local measurements. Our results demonstrate that a purely hydrodynamic approach is insufficient in the Gurzhi regime once a magnetic field is introduced.

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arXiv2019

Cascade of Phase Transitions and Dirac Revivals in Magic Angle Graphene

Twisted bilayer graphene near the magic angle exhibits remarkably rich electron correlation physics, displaying insulating, magnetic, and superconducting phases. Here, using measurements of the local electronic compressibility, we reveal that these phases originate from a high-energy state with an unusual sequence of band populations. As carriers are added to the system, rather than filling all the four spin and valley flavors equally, we find that the population occurs through a sequence of sharp phase transitions, which appear as strong asymmetric jumps of the electronic compressibility near integer fillings of the moire lattice. At each transition, a single spin/valley flavor takes all the carriers from its partially filled peers, "resetting" them back to the vicinity of the charge neutrality point. As a result, the Dirac-like character observed near the charge neutrality reappears after each integer filling. Measurement of the in-plane magnetic field dependence of the chemical potential near filling factor one reveals a large spontaneous magnetization, further substantiating this picture of a cascade of symmetry breakings. The sequence of phase transitions and Dirac revivals is observed at temperatures well above the onset of the superconducting and correlated insulating states. This indicates that the state we reveal here, with its strongly broken electronic flavor symmetry and revived Dirac-like electronic character, is a key player in the physics of magic angle graphene, forming the parent state out of which the more fragile superconducting and correlated insulating ground states emerge.

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arXiv2019

Electric and Magnetic Field Nano-Sensing Using a New, Atomic-like Qubit in a Carbon Nanotube

Quantum sensing techniques have been successful in pushing the sensitivity limits in numerous fields, and hold great promise for scanning probes that study nano-scale devices and novel materials. However, forming a nano-scale qubit that is simple and robust enough to be placed on a scanning tip, and sensitive enough to detect various physical observables, is still a great challenge. Here we demonstrate a conceptually new qubit implementation in a carbon nanotube that achieves these requirements. In contrast to the prevailing semiconducting qubits that use electronic states in double quantum dots, our qubit utilizes the natural electronic wavefunctions in a single quantum dot. Using an ultraclean nanotube we construct a qubit from two wavefunctions with significantly different magnetic moments and spatial charge distributions, making it sensitive to both magnetic and electric fields. We use an array of gates to directly image these wavefunctions and demonstrate their localized moments. Owing to their different spatial structure, these wavefunctions also show radically different transport properties, giving us a simple transport-based qubit readout mechanism. Due to its narrow coherence-limited transition, the qubit demonstrates significantly better electric field detection sensitivity than a single electron transistor. Moreover, with the same qubit we demonstrate simultaneous probing of magnetic fields with DC sensitivity comparable to that of NV centers. Our technique has minimal requirements for device complexity, which can be implemented using a number of straightforward fabrication methods. These features make this atomic-like qubit a powerful new tool that enables a variety of new nanoscale imaging experiments.

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arXiv2019

Visualizing Poiseuille flow of hydrodynamic electrons

Hydrodynamics is a general description for the flow of a fluid, and is expected to hold even for fundamental particles such as electrons when inter-particle interactions dominate. While various aspects of electron hydrodynamics were revealed in recent experiments, the fundamental spatial structure of hydrodynamic electrons, the Poiseuille flow profile, has remained elusive. In this work, we provide the first real-space imaging of Poiseuille flow of an electronic fluid, as well as visualization of its evolution from ballistic flow. Utilizing a scanning nanotube single electron transistor, we image the Hall voltage of electronic flow through channels of high-mobility graphene. We find that the profile of the Hall field across the channel is a key physical quantity for distinguishing ballistic from hydrodynamic flow. We image the transition from flat, ballistic field profiles at low temperature into parabolic field profiles at elevated temperatures, which is the hallmark of Poiseuille flow. The curvature of the imaged profiles is qualitatively reproduced by Boltzmann calculations, which allow us to create a 'phase diagram' that characterizes the electron flow regimes. Our results provide long-sought, direct confirmation of Poiseuille flow in the solid state, and enable a new approach for exploring the rich physics of interacting electrons in real space.

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arXiv2018

Simultaneous imaging of voltage and current density of flowing electrons in two dimensions

Electron transport in nanoscale devices can often result in nontrivial spatial patterns of voltage and current that reflect a variety of physical phenomena, particularly in nonlocal transport regimes. While numerous techniques have been devised to image electron flows, the need remains for a nanoscale probe capable of simultaneously imaging current and voltage distributions with high sensitivity and minimal invasiveness, in magnetic field, across a broad range of temperatures, and beneath an insulating surface. Here we present such a technique for spatially mapping electron flows based on a nanotube single-electron transistor, which achieves high sensitivity for both voltage and current imaging. In a series of experiments using high-mobility graphene devices, we demonstrate the ability of our technique to visualize local aspects of intrinsically nonlocal transport, as in ballistic flows, which are not easily resolvable via existing methods. This technique should both aid in understanding the physics of two-dimensional electronic devices, as well as enable new classes of experiments that image electron flow through buried nanostructures in the quantum and interaction-dominated regimes.

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arXiv2018

Imaging the Wigner Crystal of Electrons in One Dimension

The quantum crystal of electrons, predicted more than eighty years ago by Eugene Wigner, is still one of the most elusive states of matter. Here, we present experiments that observe the one-dimensional Wigner crystal directly, by imaging its charge density in real-space. To measure this fragile state without perturbing it, we developed a new scanning probe platform that utilizes a pristine carbon nanotube as a scanning charge perturbation to image, with minimal invasiveness, the many-body electronic density within another nanotube. The obtained images, of few electrons confined in one-dimension, match those of strongly interacting crystals, with electrons ordered like pearls on a necklace. Comparison to theoretical modeling demonstrates the dominance of Coulomb interactions over kinetic energy and the weakness of exchange interactions. Our experiments provide direct evidence for this long-sought electronic state, and open the way for studying other fragile interacting states by imaging their many-body density in real-space.

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arXiv2017

Topological transitions and fractional charges induced by strain and magnetic field in carbon nanotubes

We show that carbon nanotubes (CNT) can be driven through a topological phase transition using either strain or a magnetic field. This can naturally lead to Jackiw-Rebbi soliton states carrying fractionalized charges, similar to those found in a domain wall in the Su-Schrieffer-Heeger model, in a setup with a spatially inhomogeneous strain and an axial field. Two types of fractionalized states can be formed at the interface between regions with different strain: a spin-charge separated state with integer charge and spin zero (or zero charge and spin $\pm \hbar/2$), and a state with charge $\pm e/2$ and spin $\pm \hbar/4$. The latter state requires spin-orbit coupling in the CNT. We show that in our setup, the precise quantization of the fractionalized interface charges is a consequence of the symmetry of the CNT under a combination of a spatial rotation by $π$ and time reversal. Finally, we comment on the effects of many-body interaction on this phenomena.

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arXiv2016

Electron Attraction Mediated by Coulomb Repulsion

One of the defining properties of electrons is their mutual Coulombic repulsion. In solids, however, this basic property may change. A famous example is that of superconductors, where coupling to lattice vibrations make electrons attract each other and leads to the formation of bound pairs. But what if all degrees of freedom are electronic? Is it still possible to make electrons attractive via their repulsion from other electrons? Such a mechanism, termed 'excitonic', was proposed fifty years ago by W. A. Little, aiming to achieve stronger and more exotic superconductivity, yet despite many experimental efforts, direct evidence for such 'excitonic' attraction is still lacking. Here, we demonstrate this unique attraction by constructing, from the bottom up, the fundamental building block of this mechanism. Our experiments are based on quantum devices made from pristine carbon nanotubes, combined with cryogenic precision manipulation. Using this platform we demonstrate that two electrons can be made to attract using an independent electronic system as the binding glue. Owing to its large tunability, our system offers crucial insights into the underlying physics, such as the dependence of the emergent attraction on the underlying repulsion and the origin of the pairing energy. We also demonstrate transport signatures of 'excitonic' pairing. This experimental demonstration of 'excitonic' pairing paves the way for the design of exotic states of matter.

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arXiv2014

Competition Between Kondo Screening and Magnetism at the LaAlO$_3$/SrTiO$_3$ Interface

We present a theory of magnetic and magneto-transport phenomena at LaAlO$_3$/SrTiO$_3$ interfaces, which as a central ingredient includes coupling between the conduction bands and local magnetic moments originating from charge traps at the interface. Tuning the itinerant electron density in the model drives transitions between a heavy Fermi liquid phase with screened moments and various magnetic states. The dependence of the magnetic phenomena on the electron density or gate voltage stems from competing magnetic interactions between the local moments and the different conduction bands. At low densities only the lowest conduction band, composed of the $d_{xy}$ orbitals of Ti, is occupied. Its antiferromagnetic interaction with the local moments leads to screening of the moments at a Kondo scale that increases with density. However, above a critical density, measured in experiments to be $n_c\approx 1.7\times 10^{13} cm^{-2}$, the $d_{xz}$ and $d_{yz}$ bands begin to populate. Their ferromagnetic interaction with the local moments competes with the antiferromagnetic interaction of the $d_{xy}$ band leading to eventual reduction of the Kondo scale with density. We explain the distinct magneto transport regimes seen in experiments as manifestations of the magnetic phase diagram computed from the model. We present new data showing a relation between the anomalous Hall effect and the resistivity in the system. The data strongly suggests that the concentration of local magnetic moments affecting the transport in the system is much lower than the carrier density, in accord with the theoretical model.

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