arXiv subjects

Shailesh Kumar

Publications and source records attributed to Shailesh Kumar.

53 records · Page 3Linked to original sources

arXiv2018

Band Gap tunability in One-dimensional system

The ability to tune the gaps of direct bandgap materials has tremendous potential for applications in the fields of LEDs and solar cells. However, lack of reproducibility of bandgaps due to quantum confinement observed in experiments on reduced dimensional materials, severely affects tunability of their bandgaps. In this letter, we report broad theoretical investigations of direct bandgap one-dimensional functionalized isomeric system using their periodic potential profile, where bandgap tunability is demonstrated simply by modifying the potential profile by changing the position of the functional group in a periodic supercell. It is verified for known synthetic, as well as natural polymers (biological and organic), and also for other one-dimensional direct bandgap systems. This insight would greatly help experimentalists in designing new isomeric systems of various bandgap values for polymers and one-dimensional inorganic systems for LEDs applications, and for effectively harvesting energy in solar cells.

cond-mat.mtrl-sci↗

arXiv2018

Effect of edge defects on band structure of zigzag graphene nanoribbons

In this article, we report band structure studies of zigzag graphene nanoribbons (ZGNRs) on introducing defects (sp_3 hybridized carbon atoms) in different concentrations at edges by varying the ratio of sp_3 to sp_2 hybridized carbon atoms. On the basis of theoretical analyses, band gap values of ZGNRs are found to be strongly dependent on relative arrangement of sp3 to sp2 hybridized carbon atoms at the edges for a defect concentration; so the findings would greatly help in understanding band gap of nanoribbons for their electronic applications.

cond-mat.mes-hall↗

arXiv2018

On-chip excitation of single germanium-vacancies in nanodiamonds embedded in plasmonic waveguides

Monolithic integration of quantum emitters in nanoscale plasmonic circuitry requires low-loss plasmonic configurations capable of confining light well below the diffraction limit. We demonstrate on-chip remote excitation of nanodiamond-embedded single quantum emitters by plasmonic modes of dielectric ridges atop colloidal silver crystals. The nanodiamonds are produced to incorporate single germanium-vacancy (GeV) centers, providing bright, spectrally narrow and stable single-photon sources suitable for highly integrated circuits. Using electron-beam lithography with hydrogen silsesquioxane (HSQ) resist, dielectric-loaded surface plasmon polariton waveguides (DLSPPWs) are fabricated on single crystalline silver plates so as to contain those of spin-casted nanodiamonds that are found to feature appropriate single GeV centers. The low-loss plasmonic configuration enabled the 532 nm pump laser light to propagate on-chip in the DLSPPW and reach to an embedded nanodiamond where a single GeV center is incorporated. The remote GeV emitter is thereby excited and coupled to spatially confined DLSPPW modes with an outstanding figure-of-merit of 180 due to a ~6-fold Purcell enhancement, ~56% coupling efficiency and ~33 μm transmission length, revealing the potential of our approach for on-chip realization of nanoscale functional quantum devices.

cond-mat.mes-hall↗

arXiv2017

Chip-integrated plasmonic cavity-enhanced single nitrogen-vacancy center emission

High temporal stability and spin dynamics of individual nitrogen-vacancy (NV) centers in diamond crystals make them one of the most promising quantum emitters operating at room temperature. We demonstrate a chip-integrated cavity-coupled emission into propagating surface plasmon polariton (SPP) modes narrowing NV center's broad emission bandwidth with enhanced coupling efficiency. The cavity resonator consists of two distributed Bragg mirrors that are built at opposite sides of the coupled NV emitter and are integrated with a dielectric-loaded SPP waveguide (DLSPPW), using electron-beam lithography of hydrogen silsesquioxane resist deposited on silver-coated silicon substrates. A quality factor of ~ 70 for the cavity (full width at half maximum ~ 10 nm) with full tunability of the resonance wavelength is demonstrated. An up to 42-fold decay rate enhancement of the spontaneous emission at the cavity resonance is achieved, indicating high DLSPPW mode confinement.

cond-mat.mes-hall↗

arXiv2017

Nanofabrication of Plasmonic Circuits Containing Single Photon Sources

Nanofabrication of photonic components based on dielectric-loaded surface plasmon-polariton waveguides (DLSPPWs) excited by single nitrogen vacancy (NV) centers in nanodiamonds is demonstrated. DLSPPW circuits are built around NV containing nanodiamonds, which are certified to be single-photon emitters, using electron-beam lithography of hydrogen silsesquioxane (HSQ) resist on silver-coated silicon substrates. A propagation length of ~20 μm for the NV single-photon emission is measured with DLSPPWs. A 5-fold enhancement in the total decay rate and up to 63% coupling efficiency to the DLSPPW mode is achieved, indicating significant mode confinement. Finally, we demonstrate routing of single plasmons with DLSPPW-based directional cou-plers, revealing the potential of our approach for on-chip realization of quantum-optical networks.

physics.optics↗

arXiv2017

Ultrabright Linearly Polarized Photon Generation from a Nitrogen Vacancy Center in a Nanocube Dimer Antenna

We demonstrate an exceptionally bright photon source based on a single nitrogen- vacancy center (NV-center) in a nanodiamond (ND), placed in the nanoscale gap between two monocrystalline silver cubes in a dimer configuration. The system is operated near saturation at a stable photon rate of 850 kcps, while we further achieve strongly polarized emission and high single photon purity, evident by the measured auto-correlation with a g(2)(0)-value of 0.08. These photon source features are key parameters for quantum technological applications, such as secure communication based on quantum key distribution. The cube antenna is assembled with an atomic force microscope, which allows us to predetermine the dipole orientation of the NV-center and optimize cube positioning accordingly, while also tracking the evolution of emission parameters from isolated ND to the 1 and 2 cube configuration. The experiment is well described by finite element modelling, assuming an instrinsic quantum efficiency of 0.35. We attribute the large photon rate of the assembled photon source, to increased quantum efficiency of the NV-center and high antenna efficiency.

physics.optics↗

arXiv2017

Excitation of nanowire surface plasmons by silicon vacancy centers in nanodiamonds

Silicon vacancy (SiV) centers in diamonds have emerged as a very promising candidate for quantum emitter due to their narrow emission line resulting in their indistinguishability. While many different quantum emitters have already been used for excitation of various propagating plasmonic modes, the corresponding exploitation of SiV centers remained so far uncharted territory. Here, we report on excitation of surface plasmon modes supported by silver nanowires using SiV centers in nanodiamonds. The coupling of SiV center fluorescence to surface plasmons is observed, when a nanodiamond situated close to a nanowire is illuminated by the pump, as radiated emission from the distal nanowire end. The effect of coupling is also seen as a change in the SiV center lifetime. Finally, we discuss possible avenues for strengthening the SiV center coupling to surface plasmon modes.

physics.optics↗

arXiv2016

Origin of multiple band gap values in single width nanoribbons

Deterministic band gap in quasi-one-dimensional nanoribbons is prerequisite for their integrated functionalities in high-performance molecular-electronics based devices. However, multiple band gap values commonly observed in the same width of graphene nanoribbons fabricated in same slot of the experiments remains unresolved, and raise a critical concern over scalable production of pristine and/or hetero-structure nanoribbons with deterministic properties and functionalities for plethora of applications. Here, we show that a modification in the depth of potential wells in the periodic direction of a supercell on relative shifting of passivating atoms at the edges is the origin of multiple band gap values for the same width of nanoribbons in a crystallographic orientation, although they carry practically the same ground state energy. The results are similar when calculations are extended from planar graphene to buckled silicene nanoribbons. Thus, the findings facilitate tuning of the electronic properties of quasi-one-dimensional materials such as bio-molecular chains, organic and inorganic nanoribbons by performing edge engineering.

cond-mat.mtrl-sci↗

arXiv2016

Excitation of surface plasmon polariton modes with multiple nitrogen vacancy centers in single nanodiamonds

Nitrogen-vacancy (NV) centers in diamonds are interesting due to their remarkable characteristics that are well suited to applications in quantum-information processing and magnetic field sensing, as well as representing stable fluorescent sources. Multiple NV centers in nanodiamonds (NDs) are especially useful as biological fluorophores due to their chemical neutrality, brightness and room-temperature photostability. Furthermore, NDs containing multiple NV centers also have potential in high-precision magnetic field and temperature sensing. Coupling NV centers to propagating surface plasmon polariton (SPP) modes gives a base for lab-on-a-chip sensing devices, allows enhanced fluorescence emission and collection which can further enhance the precision of NV-based sensors. Here, we investigate coupling of multiple NV centers in individual NDs to the SPP modes supported by silver surfaces protected by thin dielectric layers and by gold V-grooves (VGs) produced via the self-terminated silicon etching. In the first case, we concentrate on monitoring differences in fluorescence spectra obtained from a source ND, which is illuminated by a pump laser, and from a scattering ND illuminated only by the fluorescence-excited SPP radiation. In the second case, we observe changes in the average NV lifetime when the same ND is characterized outside and inside a VG. Fluorescence emission from the VG terminations is also observed, which confirms the NV coupling to the VG-supported SPP modes.

cond-mat.mes-hall↗

arXiv2016

Local excitation of surface plasmon polaritons using nitrogen-vacancy centers

Surface plasmon polaritons (SPPs) are locally excited at silver surfaces using (~100) nm-sized nanodiamonds (NDs) with multiple nitrogen-vacancy (NV) centers (~400). The fluorescence from an externally illuminated (at 532 nm) ND and from nearby NDs, which are not illuminated but produce out-of-plane scattering of SPPs excited by the illuminated ND, exhibit distinctly different wavelength spectra, showing short-wavelength filtering due to the SPP propagation loss. The results indicate that NDs with multiple NV centers can be used as efficient sub-wavelength SPP sources in planar integrated plasmonics for various applications.

cond-mat.mes-hall↗

arXiv2015

Class Vectors: Embedding representation of Document Classes

Distributed representations of words and paragraphs as semantic embeddings in high dimensional data are used across a number of Natural Language Understanding tasks such as retrieval, translation, and classification. In this work, we propose "Class Vectors" - a framework for learning a vector per class in the same embedding space as the word and paragraph embeddings. Similarity between these class vectors and word vectors are used as features to classify a document to a class. In experiment on several sentiment analysis tasks such as Yelp reviews and Amazon electronic product reviews, class vectors have shown better or comparable results in classification while learning very meaningful class embeddings.

cs.CL↗

arXiv2014

Increasing the photon collection rate from a single NV center with a silver mirror

In the pursuit of realizing quantum optical networks, a large variety of different approaches have been studied to achieve a single photon source on-demand. The common goal for these approaches is to harvest all the emission from a quantum emitter into a single spatial optical mode while maintaining a high signal-to-noise ratio. In this work, we use a single nitrogen vacancy center in diamond as a quantum emitter operating at ambient conditions and we demonstrate an increased photon count rate up to a factor of 1.76 by placing a silver mirror fabricated on the end facet of an optical fiber near the emitter.

quant-ph↗

arXiv2013

Coupling of single quantum emitters to plasmons propagating on mechanically etched wires

We demonstrate the coupling of a single nitrogen vacancy center in a nanodiamond to propagating plasmonic modes of mechanically etched silver nanowires. The mechanical etch is performed on single crystalline silver nanoplates by the tip of an atomic force microscope cantilever to produce wires with pre-designed lengths. We show that single plasmon propgation can be obtained in these wires, thus making these structures a platform for quantum information processing.

cond-mat.mes-hall↗

arXiv2013

Propagation of plasmons in designed single crystalline silver nanostructures

We demonstrate propagation of plasmons in single crystalline silver nanostructures fabricated using a combination of a bottom-up and a top-down approach. Silver nanoplates of thickness around 65 nm and a surface area of about 100 μm^2 are made using a wet chemical method. Silver nanotips and nanowires are then sculptured by focused ion beam milling. The plasmons are excited by using the fluorescence from the redeposited silver clusters during the milling process. Propagation of plasmons in the nanowires is observed in the visible spectral region. We also observe a cavity effect by measuring the emission spectrum from the distal wire end.

cond-mat.mes-hall↗

arXiv2013

Coupling of a Single Quantum Emitter to End-to-end Aligned Silver Nanowires

We report on the observation of coupling a single nitrogen vacancy (NV) center in a nanodiamond crystal to a propagating plasmonic mode of silver nanowires. The nanocrystal is placed either near to the apex of a single silver nanowire or in the gap between two end-to-end aligned silver nanowires. We observe an enhancement of the NV-centers' decay rate in both cases as a result of the coupling to the plasmons. The devices are nano-assembled with a scanning probe technique. Through simulations, we show that end-to-end aligned silver nanowires can be used as a controllable splitter for emission from a dipole emitter.

quant-ph↗

arXiv2010

Controlled coupling of a single nitrogen-vacancy center to a silver nanowire

We report on the controlled coupling of a single nitrogen-vacancy (NV) center to a surface plasmon mode propagating along a chemically grown silver nanowire. We locate and optically characterize a single NV-center in a uniform dielectric environment before we controllably position this emitter in the close proximity of the nanowire. We are thus able to control the coupling of this particular emitter to the nanowire and directly compare the photon emission properties before and after the coupling. The excitation of single plasmonic modes is witnessed and a total rate enhancement by a factor of up to 4.6 is demonstrated.

quant-ph↗

arXiv2010

Failover in cellular automata

A cellular automata (CA) configuration is constructed that exhibits emergent failover. The configuration is based on standard Game of Life rules. Gliders and glider-guns form the core messaging structure in the configuration. The blinker is represented as the basic computational unit, and it is shown how it can be recreated in case of a failure. Stateless failover using primary-backup mechanism is demonstrated. The details of the CA components used in the configuration and its working are described, and a simulation of the complete configuration is also presented.

cs.AI↗