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Shannon Gould

Publications and source records attributed to Shannon Gould.

5 recordsLinked to original sources

A d-Electron Heavy-Fermion-Like Superconductor with Frustration-Induced Flat Bands

Heavy-fermion superconductors are mostly associated with f-electron materials with Kondo lattices, while known d-electron heavy-fermion-like systems are often linked to orbital-selective local moments, Hund-metal physics, or a charge-density-wave mechanism. Here we report Mo4PtGa17, a noncentrosymmetric itinerant d-electron superconductor with a geometrically frustrated breathing-pyrochlore Mo lattice. Thermodynamic, transport and NMR measurements reveal heavy-fermion-like behavior superconductivity and dominant ferromagnetic spin fluctuations near a ferromagnetic instability. Theoretical calculations identify nearly flat bands, van Hove singularities and Kramers nodal lines near the Fermi energy, derived intrinsically from Mo-4d states and are robust against on-site electronic correlations. These results suggest that the geometrically frustrated lattice in Mo4PtGa17 generates an intriguing electronic structure that enhances the density of states, spin susceptibility and quasiparticle mass. Mo4PtGa17 therefore identifies a unique route to heavy-fermion-like superconductivity in d-electron materials through geometrical frustration, different from the previously reported systems.

cond-mat.str-el

Field-rigid Ising antiferromagnetism with giant spin-flip fields in Van der Waals UOTe

Van der Waals antiferromagnets provide a route to thickness-controlled magnetic order, but few combine high-temperature Ising order with conducting, correlated, and topological electronic structure. Here we show that UOTe realizes this combination. Magnetic susceptibility reveals a strongly anisotropic paramagnetic response, while neutron diffraction establishes c-axis antiferromagnetic order below $T_N \simeq 150$ K with an order-parameter exponent $\beta = 0.14$, close to the two-dimensional Ising value. Torque magnetometry further shows that the ordered state remains well described by a uniaxial antiferromagnet below the high-field transition. Pulsed-field magnetization up to 73 T shows that the ordered state survives to very large fields applied along the c axis before entering a broad metamagnetic regime that begins near 50 T, and remains unsaturated at the highest measured field. Angle-dependent proximity detector oscillator measurements show that the metamagnetic instability is set by the field component along the ordered moment direction, providing direct evidence for Ising-like field rigidity. UOTe therefore establishes a field-rigid Ising antiferromagnet with giant spin-flip fields in a compensated Van der Waals metal, where high-temperature c-axis order, quasi-two-dimensional magnetic criticality, Kondo-associated uranium 5f hybridization, metallic transport, and symmetry-enabled topology coexist in a single material.

cond-mat.str-el

Scaling Breakdown as a Signature of Spinon-Gauge Interaction in the Quantum Spin Liquid YbZn$_2$GaO$_5$

Scaling behavior in magnetization has been reported in a wide range of quantum spin liquid (QSL) candidates and is often interpreted as evidence for scale-free spin liquid physics. Here we present a comprehensive scaling analysis of high-field magnetization measurements on the QSL material YbZn$_2$GaO$_5$. Between 5 K and 70 K, $M(H)$ displays scale invariance resembling that of a zero-field quantum critical point. Below 3 K, we observe a breakdown of this scale invariance that cannot be recovered by simply changing the critical exponents. This temperature coincides with the onset of enhanced spin correlations observed in $\mu$SR measurements. Moreover, the form of the deviation from scaling is consistent with collective spinon excitations coupled via emergent gauge interactions. These results indicate that the breakdown of scaling reflects the emergence of intrinsic low-energy excitations upon entering the QSL regime. Our work clarifies that magnetic scaling is associated with quantum critical fluctuations rather than with the spin liquid phase itself, and establishes magnetization scaling as a sensitive thermodynamic probe of emergent energy scales in QSL systems.

cond-mat.str-el

Tunable Giant Anomalous Hall in a Kondo Lattice Ferromagnet UBiTe

Kondo lattice systems are recognized for potentially hosting a variety of rich topological phases. Several pioneering studies have demonstrated significant anomalous Hall and anomalous Nernst effects in these systems, attributed to the Berry curvature of the hybridization bands. In this study, we investigate UBiTe, a ferromagnetic Kondo lattice system. Our findings reveal that the intrinsic contribution to the anomalous Hall conductivity is closely tied to the Kondo coherence temperature. Moreover, we demonstrate that slight shifts in the Fermi level across three different samples significantly influence this intrinsic contribution, in alignment with the Berry curvature localized within the narrow hybridization bands. This provides a stark contrast to the less pronounced sensitivity observed in weakly correlated Weyl semimetals, underscoring the distinctive electronic properties of Kondo lattice systems. The anomalous Hall conductivity of one samples ranks among the highest reported for topological magnetic materials.

cond-mat.str-el

Observation of vortex stripes in UTe$_2$

Quantum vortices are fundamentally important for properties of superconductors. In conventional type-II superconductor they determine the magnetic response of the system and tend to form regular lattices. UTe$_2$ is a recently discovered heavy fermion superconductor exhibiting many anomalous macroscopic behaviors. However, the question whether it has a multicomponent order parameter remains open. Here, we study magnetic properties of UTe$_2$ by employing scanning superconducting quantum interference device microscopy. We find vortex behavior which is very different from that in ordinary superconductors. We imaged vortices generated by cooling in magnetic field applied along different crystalline directions. While a small out-of-plane magnetic field produces typical isolated vortices, higher field generates vortex stripe patterns which evolve with vortex density. The stripes form at different locations and along different directions in the surface plane when the vortices are crystalized along the crystalline b or c axes. The behavior is reproduced by our simulation based on an anisotropic two-component order parameter. This study shows that UTe$_2$ has a nontrivial disparity of multiple length scales, placing constraints on multicomponent superconductivity. The tendency of vortex stripe formation and their control by external field may be useful in fluxonics applications.

cond-mat.supr-con