arXiv subjects

Shanta R. Saha

Publications and source records attributed to Shanta R. Saha.

At least 19 recordsLinked to original sources

arXiv2026

A Strategy Toward Room Temperature Topological Hall Effect via Local Moment Magnetism

Topological spin textures in local moment systems hold great promise for technological applications due to their large magnetic moments, strong spin-orbit coupling (SOC), and high tunability. Finding new spin textures that are stable near room temperature is paramount to maximizing their potential for applications. Here, we provide a strategy for realizing topological spin textures at high temperatures by identifying rare earth ($R$) magnets ordering at or near room temperature. We demonstrate the feasibility of this strategy in one of these magnets, hexagonal Gd$_5$Pb$_3$, which orders at $T_C$ = 285 K. The indication for topological spin textures comes from topological Hall effect (THE), which, in Gd$_5$Pb$_3$, occurs between $T$ = 100 - 200 K, an order of magnitude higher temperature than in other reported $R$-based systems. Our results present an opportunity to explore the role of SOC, anisotropic exchange, geometric frustration, and magnetic interactions in stabilizing topological spin textures, and provide a pathway toward realizing them near room temperature in $R$-based magnets.

cond-mat.mtrl-sci↗

arXiv2026

Evidence of intertwined pair density and charge density wave orders in UTe2

The strongly correlated spin-triplet superconductor UTe2 hosts an unusual landscape of magnetic-field-sensitive charge density wave (CDW) phases, positioning it as a compelling system for studying intertwined electronic orders. A central challenge is determining whether the observed charge modulations arise from a triplet pair density wave (PDW) order and, if so, how the anisotropic magnetic field response of triplet superconductivity is manifested in the CDW response. Here, using a scanning tunneling microscope equipped with a vector magnetic field, we systematically investigate the evolution and interrelation of distinct CDW orders. Complementing the previously identified incommensurate CDW peaks (qi=1,2,3), we resolve an additional set of nondispersive modulations (pi=1,2,3 and h1,2) with distinct temperature and magnetic field dependencies. The pi CDW peaks vanish near Tc, while the qi peaks survive well above Tc but are progressively suppressed by magnetic field in an anisotropic manner. The critical fields of the qi peaks mirror the directional hierarchy of Hc2, which suggests a PDW is present above the bulk Tc. This is consistent with a Landau free-energy picture where PDWs with wavevectors pi form above the bulk Tc, leading to composite CDW orders with wavevector qi. Below Tc, the coupling of PDWs and uniform superconductivity leads to the pi CDWs. Together, these findings establish UTe2 as a rare platform where both the parent PDW and descendant orders are directly resolved, enabling access to both the fundamental and emergent manifestations of PDW physics.

cond-mat.supr-con↗

arXiv2026

Topological surface states revealed by the Zeeman effect in superconducting UTe2

Intrinsic topological superconductors with protected boundary modes obeying non-Abelian statistics constitute a vanishingly small class of quantum materials. A defining spectroscopic signature of such phases is the presence of in-gap topological surface states (TSS). However, despite extensive theoretical proposals, their unambiguous experimental identification has remained elusive. Here we use vector magnetic-field scanning tunnelling microscopy to obtain direct spectroscopic evidence of TSS in the spin-triplet superconductor UTe2. Atomic-scale spectroscopy reveals striking site-dependent superconductivity: Te sites host a large in-gap density of states that nearly fills the superconducting gap, whereas neighboring atomic sites remain gapped. Upon application of a magnetic field, the in-gap states on the Te sites are selectively suppressed, yielding a spatially homogeneous superconducting state with a markedly deeper gap relative to zero field. This site-selective gap evolution is in quantitative agreement with theoretical predictions for TSS in UTe2 that possess dominant Te-orbital character. Spectral-function calculations incorporating the Zeeman coupling reproduce the observed magnetic-field response. Our results provide a spectroscopic fingerprint of the long-sought TSS in superconductors and establish UTe2 as a compelling system for exploring intrinsic topological superconductivity.

cond-mat.supr-con↗

arXiv2026

Anisotropic magnetism at the surface of a non-magnetic bulk insulator

The potential for topological Kondo insulating behavior in d-electron systems has attracted interest in studying the surface states of the correlated insulators FeSb2 and FeSi. While detailed studies and theoretical description of a spin-orbit coupled ferromagnetic surface state have been applied to FeSi, the magnetic properties of the surface states of FeSb2 have not been addressed. Here, we report on the surface magnetic properties of FeSb2, utilizing the surface area dependence of magnetic susceptibility to separate the surface Curie-Weiss temperature dependence from the bulk spin-gap susceptibility. We use these results to further extract the surface magnetic anisotropy of a thin, rough-surfaced single-crystal FeSb2 to compare with the observed magnetotransport anisotropy, and find good agreement between the anisotropy in the surface magnetization and surface magnetotransport. We conclude with evidence of an anomalous Hall contribution to the low-temperature surface transport.

cond-mat.str-el↗

arXiv2026

Magnetic field-tuned magnetic order and metamagnetic criticality in non-stoichiometric CeAuBi$_2$

We present a detailed study of magnetization, resistivity, heat capacity, and X-ray and neutron powder diffraction measurements performed on single crystals of non-stoichiometric CeAuBi$_2$, Au deficiency 18$\%$, a strongly correlated antiferromagnet with Néel temperature T$_N$ = 13.2 K. Field-dependent magnetization measurements reveal a large magnetic anisotropy at low temperatures with an easy axis along the crystallographic c-axis, in which direction a spin-flop transition exhibits strong features in magnetization, specific heat, and resistivity at H$_c$ = 75 kOe. The constructed temperature-field phase diagram connects this transition to the suppression of magnetic order, which evolves from a second-order nature into a first-order transition that bifurcates at the spin-flop into three transitions below 1 K. The smoothed nature of the metamagnetic transitions in non-stoichiometric CeAuBi$_2$ is well described by an Ising model with weak quenched disorder, suggesting that the presence of Au vacancies is sufficient to smear the complex metamagnetic behavior and tune the critical behavior of magnetic order.

cond-mat.str-el↗

arXiv2026

Visualizing the low-energy electronic structure of the triplet superconductor UTe$_2$ through quasiparticle interference

The identification, control and theoretical modelling of spin-triplet superconductors (STC) remain a central theme in quantum materials research. Intrinsic STC are rare but offer rich condensate properties and unique surface properties allowing insights into the nature of the spin-triplet order, and promising applications in quantum technologies. Owing to interactions, the order parameter in STCs can often be intertwined with other symmetry breaking orders like charge/spin density waves (CDW/SDW) or pair density waves (PDW) complicating their phase diagrams. UTe2 stands out as the only known odd-parity, STC that harbors such intertwined orders on the surface and possible topological surface states composed of Majorana fermions. While the (0-11) facet is the most heavily studied, the fermiology of this surface that gives rise to such exotic phenomena is still lacking and continues to be an area of active interest. Here, we employ low-temperature spectroscopic imaging to reveal the Fermi surface of UTe2 through quasiparticle interference. We find scattering originating from the uranium-derived bands that play a major role in the formation of the CDW and the PDW phases. Tunneling spectroscopy further reveals spectral signatures of the CDW gap, corroborating its onset temperature. Suppressing the CDW with a magnetic field, highlights the presence of small, circular Fermi pockets that disperse strongly near the Fermi energy. We discuss the nature of the interference patterns and the origin of the small Fermi pockets in the context of the calculated band structure and the unconventional CDW phase.

cond-mat.supr-con↗

arXiv2025

Field-angle-resolved heat transport in UTe$_2$: determination of nodal positions in the superconducting order parameter

One of the recurring hurdles in studying unconventional superconductivity is the challenge of efficiently and conclusively identifying the symmetry of the superconducting order parameter in a new material. Uranium ditelluride (UTe$_2$) exhibits an unprecedented number of superconducting phases as a function of pressure and magnetic field, each presumably characterized by a different symmetry of the superconducting gap function. None of these phases has had its symmetry conclusively identified so far. In this article, we report results of an extensive study of the thermal conductivity of UTe$_2$ in its low-field, low-temperature superconducting state as a function of the angle of an applied magnetic field rotated in the $b$-$c$ plane. We observe clear and substantial oscillations in the thermal conductivity as a function of field angle, which naturally suggests the existence of point nodes in the gap. Utilizing the experimentally determined Fermi surface, we are able to model this phenomenon for all the potential gap structures in UTe$_2$ and positively identify the location of these nodes as being along the crystallographic $b$-axis, implying that the superconducting order parameter belongs to the $B_{2u}$ irreducible representation of the crystal point group. The clarity of this result will accelerate the identification of other superconducting phases in UTe$_2$, and guide future studies through the use of high resolution field-angle-dependent measurements.

cond-mat.supr-con↗

arXiv2025

Magnetocrystalline Anisotropy and 3D Hopping Conduction at the Surface of FeSb2

Motivated by the recent discovery of metallic surface states in the d-electron Kondo insulator candidates FeSi and FeSb2, along with some recent reports of magnetic correlations in the surface transport properties of FeSi, we have investigated the low temperature surface magnetotransport properties of FeSb2. By using a Corbino disk transport geometry, we were able to isolate the electrical transport properties of a single surface of our samples and study the [110] and [101] naturally forming faces separately. Studying the relationship between the applied magnetic field, current direction and crystal symmetry has allowed us to separate possible contributions to the magnetotransport anisotropy. Unlike previous studies of SmB6 surface states, we find no two-dimensional Drude-like dependence on field orientation relative to current direction, but instead a magnetocrystalline anisotropy that appears to originate from local moment scattering with a well defined easy-axis along the [100] direction. We compare these results with the magnetotransport properties of the conducting surface states on the [111] facet of FeSi. We also find evidence of 3D variable-range hopping conduction below the bulk-to-surface crossover, extending below 1 K, which implies that the electrical transport at the surface of these materials is carried by a thin, but 3D conducting channel, which is inconsistent with the lower dimensional states expected for a strong topological insulator.

cond-mat.str-el↗

arXiv2025

Complex single-site magnetism and magnetotransport in single-crystalline Gd$_{2}$AlSi$_{3}$

We present a detailed investigation of single-crystal samples of the magnetic compound Gd$_{2}$AlSi$_{3}$, which crystallizes in the $α$-ThSi$_2$ type tetragonal structure. We report the temperature and magnetic field dependence of the magnetic susceptibility, magnetization, heat capacity, electrical resistivity, and magnetoresistance for magnetic fields applied along both the tetragonal $c$-axis and in the basal $ab$-plane. X-ray diffraction measurements confirm a centrosymmetric, $I4_{1}/amd$ space group of the crystal structure. Despite single-site occupancy of the Gd position in this tetragonal structure, we identify two successive antiferromagnetic phase transitions at Neél temperatures 32~K and 23~K via magnetic susceptibility, heat capacity and transport measurements, as well as a complex magnetic interaction with a magnetic anisotropy that plays an important role in the direction-dependent transport response. Our identification of multiple magnetic phases in Gd$_{2}$AlSi$_{3}$, where Gd is the only magnetic species, helps to elucidate the field-induced skyrmionic behavior in the Gd-based intermetallic compounds.

cond-mat.str-el↗

arXiv2025

Revealing isotropic abundant low-energy excitations in UTe$_2$ through complex microwave surface impedance

The complex surface impedance is a well-established tool to study the super- and normal-fluid responses of superconductors. Fundamental properties of the superconductor, such as the pairing mechanism, Fermi surface, and topological properties, also influence the surface impedance. We explore the microwave surface impedance of spin-triplet UTe$_2$ single crystals as a function of temperature using resonant cavity perturbation measurements employing a novel multi-modal analysis to gain insight into these properties. We determine a composite surface impedance of the crystal for each mode using resonance data combined with the independently measured normal state dc resistivity tensor. The normal state surface impedance reveals the weighting of current flow directions in the crystal of each resonant mode. For UTe$_2$, we find an isotropic $Δλ(T) \sim T^α$ power-law temperature dependence for the magnetic penetration depth for $T\le T_c/3$ with $α< 2$, which is inconsistent with a single pair of point nodes on the Fermi surface under weak scattering. We also find a similar power-law temperature dependence for the low-temperature surface resistance $R_s(T) \sim T^{α_R}$ with $α_R < 2$. We observe a strong anisotropy of the residual microwave loss across these modes, with some modes showing loss below the universal line-nodal value, to those showing substantially more. We compare to predictions for topological Weyl superconductivity in the context of the observed isotropic power-laws, and anisotropy of the residual loss.

cond-mat.supr-con↗

arXiv2025

Dilute Paramagnetism and Non-Trivial Topology in Quasicrystal Approximant Fe$_4$Al$_{13}$

A very fundamental property of both weakly and strongly interacting materials is the nature of its magnetic response. In this work we detail the growth of crystals of the quasicrystal approximant Fe$_4$Al$_{13}$ with an Al flux solvent method. We characterize our samples using electrical transport and heat capacity, yielding results consistent with a simple non-magnetic metal. However, magnetization measurements portray an extremely unusual response for a dilute paramagnet and do not exhibit the characteristic Curie-Weiss behavior expected for a weakly interacting material at high temperature. Electronic structure calculations confirm metallic behavior, but also indicate that each isolated band near the Fermi energy hosts non-trivial topologies including strong, weak and nodal components, with resultant topological surface states distinguishable from bulk states on the (001) surface. With half-filled flat bands apparent in the calculation but absence of long-range magnetic order, the unusual paramagnetic response suggests the dilute paramagnetic behavior in this quasicrystal approximant is surprising and may serve as a test of the fundamental assumptions that are taken for granted for the magnetic response of weakly interacting systems.

cond-mat.str-el↗

arXiv2025

Nanomolding single-crystalline CoIn3 and RhIn3 nanowires

Intermetallic compounds containing transition metals and group III-V metals tend to possess strong correlations and high catalytic activities, both of which can be enhanced via reduced dimensionality. Nanostructuring is an effective approach to explore this possibility, yet the synthesis of nanostructured intermetallics is challenging due to vast differences in melting points and vapor pressures of the constituent elements. In this work, we demonstrate that this challenge can be overcome with thermomechanical nanomolding (TMNM), exemplified by the synthesis of intermetallic CoIn3 and RhIn3 nanowires. We show that TMNM successfully extrudes single-crystalline nanowires of these compounds down to the 20 nm diameter range, and the nanowires remain metallic with resistivity values higher than calculated bulk resistivity. We discuss possible effects of surface roughness scattering, vacancy-induced scattering, and surface oxidation, on the measured resistivities of the nanowires. For CoIn3 nanowires, the measured resistivity values are the first reported values for this compound.

cond-mat.mtrl-sci↗

arXiv2024

Absence of a bulk charge density wave signature in x-ray measurements of UTe$_2$

The long-sought pair density wave (PDW) is an exotic phase of matter in which charge density wave (CDW) order is intertwined with the amplitude or phase of coexisting, superconducting order \cite{Berg2009,Berg2009b}. Originally predicted to exist in copper-oxides, circumstantial evidence for PDW order now exists in a variety of materials. Recently, scanning tunneling microscopy (STM) studies have reported evidence for a three-component charge density wave (CDW) at the surface of the heavy-fermion superconductor, UTe$_2$, persisting below its superconducting transition temperature. Here, we use hard x-ray diffraction measurements on crystals of UTe$_2$ at $T = 1.9$ K and $12$ K to search for a bulk signature of this CDW. Using STM measurements as a constraint, we calculate the expected locations of CDW superlattice peaks, and sweep a large volume of reciprocal space in search of a signature. We failed to find any evidence for a CDW near any of the expected superlattice positions in many Brillouin zones. We estimate an upper bound on the CDW lattice distortion of $u_{max} \lesssim 4 \times 10^{-3} \mathrmÅ$. Our results suggest that the CDW observed in STM is either purely electronic, somehow lacking a signature in the structural lattice, or is restricted to the material surface.

cond-mat.str-el↗

arXiv2024

Disordered 2D ferromagnetism at the surface of FeSi

FeSi is a curious example of a $d$-electron system that manifests many of the same phenomena associated with $f$-electron Kondo insulators, including conducting surface states with potentially non-trivial topology. Here we investigate the magnetization and magnetotransport of these surface states and how a 2D ferromagnetic state at the surface of FeSi influences the surface conductivity. We confirm the 2D ferromagnetism via a systematic study of magnetization on groups of filtered fragments with increasing surface area-to-volume ratios, identifying characteristic temperatures and magnetic fields associated with the ordered state. The paramagnetic to ferromagnetic transition appears broadened, suggesting disorder, which allows spin fluctuations to manifest up to at least 9 T at 2 K. This highlights the need to understand the relation between the disorder of the 2D ferromagnetism and the surface conductivity in FeSi.

cond-mat.str-el↗

arXiv2024

Probing $p$-wave superconductivity in UTe$_2$ via point-contact junctions

Uranium ditelluride (UTe$_2$) is the strongest contender to date for a $p$-wave superconductor in bulk form. Here we perform a spectroscopic study of the ambient pressure superconducting phase of UTe$_2$, measuring conductance through point-contact junctions formed by metallic contacts on different crystalline facets down to 250 mK and up to 18 T. Fitting a range of qualitatively varying spectra with a Blonder-Tinkham-Klapwijk(BTK) model for $p$-wave pairing, we can extract gap amplitude and interface barrier strength for each junction. We find good agreement with the data for a $p_y$ -wave gap function with amplitude in 0.26 $\pm$ 0.06 meV. Our work provides spectroscopic evidence for a gap structure consistent with the proposed spin-triplet pairing in the superconducting state of UTe$_2$.

cond-mat.supr-con↗

arXiv2024

Pressure-induced exciton formation and superconductivity in platinum-based mineral Sperrylite

We report a comprehensive study of Sperrylite (PtAs2), the main platinum source in natural minerals, as a function of applied pressures up to 150 GPa. While no structural phase transition was detected from pressure-dependent X-ray measurements, the unit cell volume shrinks monotonically with pressure following the third-order Birch-Murnaghan equation of state. The mildly semiconducting behavior found in pure synthesized crystals at ambient pressures becomes more insulating upon increasing applied pressure before metalizing at higher pressures, giving way to the appearance of an abrupt decrease in resistance near 3 K at pressures above 92 GPa consistent with the onset of a superconducing phase. The pressure evolution of the calculated electronic band structure reveals the same physical trend as our transport measurements, with a non-monotonic evolution explained by a hole band that is pushed below the Fermi energy and an electron band that approaches it as a function of pressure, both reaching a touching point suggestive of an excitonic state. A topological Lifshitz transition of the electronic structure and an increase in the density of states may naturally explain the onset of superconductivity in this material

cond-mat.supr-con↗

arXiv2024

Robust nodal behavior in the thermal conductivity of superconducting UTe$_2$

The superconducting state of the heavy-fermion metal UTe$_2$ has attracted considerable interest because of evidence for spin-triplet Cooper pairing and non-trivial topology. Progress on these questions requires identifying the presence or absence of nodes in the superconducting gap function and their dimension. In this article we report a comprehensive study of the influence of disorder on the thermal transport in the superconducting state of UTe$_2$. Through detailed measurements of the magnetic field dependence of the thermal conductivity in the zero-temperature limit, we obtain clear evidence for the presence of point nodes in the superconducting gap for all samples with transition temperatures ranging from 1.6~K to 2.1~K obtained by different synthesis methods, including a refined self-flux method. This robustness implies the presence of symmetry-imposed nodes throughout the range studied, further confirmed via disorder-dependent calculations of the thermal transport in a model with a single pair of nodes. In addition to capturing the temperature dependence of the thermal conductivity up to $T_c$, this model allows us to limit the possible locations of the nodes, suggesting a B$_{1u}$ or B$_{2u}$ symmetry for the superconducting order parameter. Additionally, comparing the new, ultra-high conductivity samples to older samples reveals a crossover between a low-field and a high field regime at a single value of the magnetic field in all samples. In the high field regime, the thermal conductivity at different disorder levels differ from each other by a simple offset, suggesting that some simple principle determines the physics of the mixed state, a fact which may illuminate trends observed in other clean nodal superconductors.

cond-mat.supr-con↗

arXiv2023

Visualizing the melting of the charge density wave in UTe2 by generation of pairs of topological defects with opposite winding

Topological defects are singularities in an ordered phase that can have a profound effect on phase transitions and serve as a window into the order parameter. In this work we use scanning tunneling microscopy to visualize the role of topological defects in the novel magnetic field induced disappearance of an intertwined charge density wave (CDW) in the heavy fermion superconductor, UTe2. By simultaneously imaging the amplitude and phase of the CDW order, we reveal pairs of topological defects with positive and negative phase winding. The pairs are directly correlated with a zero CDW amplitude and increase in number with increasing magnetic field. These observations can be captured by a Ginzburg Landau model of a uniform superconductor coexisting with a pair density wave. A magnetic field generates vortices of the superconducting and pair density wave order which can create topological defects in the CDW and induce the experimentally observed melting of the CDW at the upper critical field. Our work reveals the important role of magnetic field generated topological defects in the melting the CDW order parameter in UTe2 and provides support for the existence of a parent pair density wave order on the surface of UTe2.

cond-mat.supr-con↗