arXiv subjects

Shaun C. Burd

Publications and source records attributed to Shaun C. Burd.

6 recordsLinked to original sources

arXiv2026

Microsecond-Scale Coherent Control of a Forbidden Clock Transition with Doppler-Free Multiphoton Excitations

We demonstrate two Doppler-free (DF) excitation schemes for coherent manipulation of the ${}^1\!S_0 - {}^3\!P_0$ clock transition in $^{88}$Sr that achieve microsecond-scale excitation times. The first approach uses three-photon excitation with distinct phase-coherent spectral components to couple the ground and clock states while canceling the first-order Doppler shift. The second approach is a sequential protocol that combines a single-photon excitation with a two-photon Raman excitation, reducing coherent clock transition manipulation times to below a microsecond. With both methods, we perform high-contrast Ramsey spectroscopy on thermal ensembles of $3 \times 10^{6}$ atoms in free space. We observe three orders of magnitude suppression of Doppler dephasing compared to single-photon excitation, relaxing the need for tight confinement or ultra-low temperatures. These broadly applicable techniques enable fast, coherent manipulation of narrow-line transitions, with implications for optical atomic clocks, matter-wave interferometers, quantum-enhanced metrology, and quantum information processing.

physics.atom-ph↗

arXiv2025

Quantum-optimal nonlinear microscopy with classical light

Nonlinear optical processes are used in biological microscopy to surpass the diffraction limit on resolution, image deeper into brain tissues, and identify biomolecules without exogenous labels. These techniques typically require high optical intensities to increase the strength of the nonlinear interactions, which can perturb native biochemistry and damage or kill living samples. Stimulated Raman scattering (SRS) microscopy visualizes the spatial distribution of molecules using a nonlinear interaction between light and chemically specific molecular vibrations. However, the detection of biomolecules at low concentrations is limited by the total photon dose that can be applied before photodamage alters the sample, and photon shot noise sets the minimum achievable noise floor for most microscopes. Here we demonstrate a cavity-enhanced SRS microscope that is more sensitive than an equivalent conventional SRS microscope by up to 8.3(7) dB in spectroscopy and 8.6(1) dB in cell imaging. These results approach quantum limits on sensitivity and demonstrate that quantum states of light are sufficient but not necessary to enhance the sensitivity of microscopy techniques that are limited by photodamage.

physics.optics↗

arXiv2024

Doppler-free three-photon spectroscopy on narrow-line optical transitions

We demonstrate coherent Doppler-free three-photon excitation of the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ optical clock transition and the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ intercombination transition in free-space thermal clouds of $^{88}$Sr atoms. By appropriate orientation of the wavevectors of three lasers incident on the atoms, the first-order Doppler shift can be eliminated for all velocity classes. Three-photon excitation of the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ transition enables high-contrast Ramsey spectroscopy with interrogation times comparable to the 21$μ$s natural lifetime using a single near-resonant laser source. Three-photon spectroscopy on the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ clock transition, using only laser frequencies nearly resonant with the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ and $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ transitions, enables a reduction in Doppler broadening by two orders of magnitude and a corresponding $\sim470$Hz linewidth without a confining potential.

physics.atom-ph↗

arXiv2023

Towards Improved Quantum Simulations and Sensing with Trapped 2D Ion Crystals via Parametric Amplification

Improving coherence is a fundamental challenge in quantum simulation and sensing experiments with trapped ions. Here we discuss, experimentally demonstrate, and estimate the potential impacts of two different protocols that enhance, through motional parametric excitation, the coherent spin-motion coupling of ions obtained with a spin-dependent force. The experiments are performed on 2D crystal arrays of approximately one hundred $^9$Be$^+$ ions confined in a Penning trap. By modulating the trapping potential at close to twice the center-of-mass mode frequency, we squeeze the motional mode and enhance the spin-motion coupling while maintaining spin coherence. With a stroboscopic protocol, we measure $5.4 \pm 0.9$ dB of motional squeezing below the ground-state motion, from which theory predicts a $10$ dB enhancement in the sensitivity for measuring small displacements using a recently demonstrated protocol [Science $\textbf{373}$, 673 (2021)]. With a continuous squeezing protocol, we measure and accurately calibrate the parametric coupling strength. Theory suggests this protocol can be used to improve quantum spin squeezing, limited in our system by off-resonant light scatter. We illustrate numerically the trade-offs between strong parametric amplification and motional dephasing in the form of center-of-mass frequency fluctuations for improving quantum spin squeezing in our set-up.

quant-ph↗

arXiv2019

Quantum-enhanced sensing of a mechanical oscillator

The use of special quantum states to achieve sensitivities below the limits established by classically behaving states has enjoyed immense success since its inception. In bosonic interferometers, squeezed states, number states and cat states have been implemented on various platforms and have demonstrated improved measurement precision over interferometers based on coherent states. Another metrologically useful state is an equal superposition of two eigenstates with maximally different energies; this state ideally reaches the full interferometric sensitivity allowed by quantum mechanics. By leveraging improvements to our apparatus made primarily to reach higher operation fidelities in quantum information processing, we extend a technique to create number states up to $n=100$ and to generate superpositions of a harmonic oscillator ground state and a number state of the form $\textstyle{\frac{1}{\sqrt{2}}}(\lvert 0\rangle+\lvert n\rangle)$ with $n$ up to 18 in the motion of a single trapped ion. While experimental imperfections prevent us from reaching the ideal Heisenberg limit, we observe enhanced sensitivity to changes in the oscillator frequency that initially increases linearly with $n$, with maximal value at $n=12$ where we observe 3.2(2) dB higher sensitivity compared to an ideal measurement on a coherent state with the same average occupation number. The quantum advantage from using number-state superpositions can be leveraged towards precision measurements on any harmonic oscillator system; here it enables us to track the average fractional frequency of oscillation of a single trapped ion to approximately 2.6 $\times$ 10$^{-6}$ in 5 s. Such measurements should provide improved characterization of imperfections and noise on trapping potentials, which can lead to motional decoherence, a leading source of error in quantum information processing with trapped ions.

physics.atom-ph↗

arXiv2016

VECSEL systems for generation and manipulation of trapped magnesium ions

Experiments in atomic, molecular, and optical (AMO) physics rely on lasers at many different wavelengths and with varying requirements on spectral linewidth, power, and intensity stability. Vertical external-cavity surface-emitting lasers (VECSELs), when combined with nonlinear frequency conversion, can potentially replace many of the laser systems currently in use. Here we present and characterize VECSEL systems that can perform all laser-based tasks for quantum information processing experiments with trapped magnesium ions. For photoionization of neutral magnesium, 570.6$\,$nm light is generated with an intracavity frequency-doubled VECSEL containing a lithium triborate (LBO) crystal for second harmonic generation. External frequency doubling produces 285.3$\,$nm light for resonant interaction with the $^{1}S_{0}\leftrightarrow$ $^{1}P_{1}$ transition of neutral Mg. Using an externally frequency-quadrupled VECSEL, we implement Doppler cooling of $^{25}$Mg$^{+}$ on the 279.6$\,$nm $^{2}S_{1/2}\leftrightarrow$ $^{2}P_{3/2}$ cycling transition, repumping on the 280.4$\,$nm $^{2}S_{1/2}\leftrightarrow$ $^{2}P_{1/2}$ transition, coherent state manipulation, and resolved sideband cooling close to the motional ground state. Our systems serve as prototypes for applications in AMO requiring single-frequency, power-scalable laser sources at multiple wavelengths.

physics.atom-ph↗