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Sheng Ran

Publications and source records attributed to Sheng Ran.

At least 19 recordsLinked to original sources

Hexagonal Stacking Maximizes Proton Configurational Entropy among Ice-I Polytypes

Ice I admits cubic, hexagonal, and mixed layer stackings, but rigorous entropy comparisons have focused on the two ideal endmembers. We represent every cyclic uniform-registry stacking by a word in a nonnegative transfer operator K and its transpose. For every such even-length word, applying the Schatten-H\"older inequality proves that alternating hexagonal stacking maximizes the ice-rule count at every common finite cross-section; the configuration constant is therefore maximal among all periodic uniform-registry polytypes. We obtain the lower endpoint by restricting Nagle's positive even-subgraph expansion to exactly enumerated disjoint blocks. Finner's degree-two hypergraph H\"older inequality and rational Collatz-Wielandt certificates for two-replica prism transfer operators give the upper endpoints. These constructions yield $1.503360 \le w \le 1.540196$, with $w(\mathrm{Ic}) \le 1.527699$.

cond-mat.stat-mech

A d-Electron Heavy-Fermion-Like Superconductor with Frustration-Induced Flat Bands

Heavy-fermion superconductors are mostly associated with f-electron materials with Kondo lattices, while known d-electron heavy-fermion-like systems are often linked to orbital-selective local moments, Hund-metal physics, or a charge-density-wave mechanism. Here we report Mo4PtGa17, a noncentrosymmetric itinerant d-electron superconductor with a geometrically frustrated breathing-pyrochlore Mo lattice. Thermodynamic, transport and NMR measurements reveal heavy-fermion-like behavior superconductivity and dominant ferromagnetic spin fluctuations near a ferromagnetic instability. Theoretical calculations identify nearly flat bands, van Hove singularities and Kramers nodal lines near the Fermi energy, derived intrinsically from Mo-4d states and are robust against on-site electronic correlations. These results suggest that the geometrically frustrated lattice in Mo4PtGa17 generates an intriguing electronic structure that enhances the density of states, spin susceptibility and quasiparticle mass. Mo4PtGa17 therefore identifies a unique route to heavy-fermion-like superconductivity in d-electron materials through geometrical frustration, different from the previously reported systems.

cond-mat.str-el

Field-rigid Ising antiferromagnetism with giant spin-flip fields in Van der Waals UOTe

Van der Waals antiferromagnets provide a route to thickness-controlled magnetic order, but few combine high-temperature Ising order with conducting, correlated, and topological electronic structure. Here we show that UOTe realizes this combination. Magnetic susceptibility reveals a strongly anisotropic paramagnetic response, while neutron diffraction establishes c-axis antiferromagnetic order below $T_N \simeq 150$ K with an order-parameter exponent $\beta = 0.14$, close to the two-dimensional Ising value. Torque magnetometry further shows that the ordered state remains well described by a uniaxial antiferromagnet below the high-field transition. Pulsed-field magnetization up to 73 T shows that the ordered state survives to very large fields applied along the c axis before entering a broad metamagnetic regime that begins near 50 T, and remains unsaturated at the highest measured field. Angle-dependent proximity detector oscillator measurements show that the metamagnetic instability is set by the field component along the ordered moment direction, providing direct evidence for Ising-like field rigidity. UOTe therefore establishes a field-rigid Ising antiferromagnet with giant spin-flip fields in a compensated Van der Waals metal, where high-temperature c-axis order, quasi-two-dimensional magnetic criticality, Kondo-associated uranium 5f hybridization, metallic transport, and symmetry-enabled topology coexist in a single material.

cond-mat.str-el

Endogenous Regime Switching Driven by Scalar-Irreducible Learning Dynamics

Achieving endogenous regime switching is crucial for the emergence of autonomous intelligence, yet remains a central challenge for existing machine learning frameworks, where such transitions are typically externally imposed. In this work, we introduce a classification that distinguishes scalar-reducible dynamics, which can be expressed as gradient flows driven by a scalar objective, from scalar-irreducible dynamics that cannot be reduced to such a form. While most existing machine learning systems operate within the scalar-reducible class, we demonstrate that scalar-irreducible dynamics naturally enable internally generated regime switching through feedback between fast dynamical variables and slow structural adaptation. Using a minimal dynamical model, we illustrate how this mechanism produces sustained endogenous regime transitions without external scheduling. Our results suggest a new dynamical paradigm for regime exploration and provide a potential route toward autonomous learning systems whose adaptive behavior is organized internally rather than externally prescribed.

cs.LG

Signature of Unconventional Superconductivity in the High Temperature Normal State Resistivity

Unconventional superconductivity remains one of the central unsolved problems in quantum materials, and revealing its connection to the normal state is widely believed to be key to uncovering the pairing mechanism. Previous efforts have largely focused on the temperature range immediately above the superconducting transition, where specific scattering channels-such as strange-metal transport-have been identified as sharing a possible microscopic origin with superconductivity. Here, using machine learning, we demonstrate a strong correlation between normal-state resistivity and superconductivity in Fe-based superconductors. Remarkably, the predictive information reside in a wide window of 150-300 K, far above $T_c$ of this family. We further show that the signatures of superconductivity are distributed across multiple scattering channels, which requires further theoretical investigation.

cond-mat.supr-con

Scaling Breakdown as a Signature of Spinon-Gauge Interaction in the Quantum Spin Liquid YbZn$_2$GaO$_5$

Scaling behavior in magnetization has been reported in a wide range of quantum spin liquid (QSL) candidates and is often interpreted as evidence for scale-free spin liquid physics. Here we present a comprehensive scaling analysis of high-field magnetization measurements on the QSL material YbZn$_2$GaO$_5$. Between 5 K and 70 K, $M(H)$ displays scale invariance resembling that of a zero-field quantum critical point. Below 3 K, we observe a breakdown of this scale invariance that cannot be recovered by simply changing the critical exponents. This temperature coincides with the onset of enhanced spin correlations observed in $\mu$SR measurements. Moreover, the form of the deviation from scaling is consistent with collective spinon excitations coupled via emergent gauge interactions. These results indicate that the breakdown of scaling reflects the emergence of intrinsic low-energy excitations upon entering the QSL regime. Our work clarifies that magnetic scaling is associated with quantum critical fluctuations rather than with the spin liquid phase itself, and establishes magnetization scaling as a sensitive thermodynamic probe of emergent energy scales in QSL systems.

cond-mat.str-el

Limited coincidence between ultrahigh-field superconductivity and line of metamagnetic endpoints in UTe$_2$

The field-dependent magnetization of UTe$_2$ was measured through the metamagnetic transition at a variety of field angles, tracking how the step in magnetization evolves with fields tilted away from the $b$ axis. For fields oriented within the $ab$ plane, jumps in both $M_a$ and $M_b$ vanish approximately 18{\deg} away from the $b$ axis. From contactless conductivity measurements, we find that the halo-like high-field superconducting region extends to the $ab$ plane, where it exists only within a very narrow ($<$1{\deg}) angular range near the termination of the metamagnetic phase boundary and extends beyond the highest measured field of 73 T. As the field orientation tilts towards the $c$ axis, the superconducting and metamagnetic phase boundaries no longer coincide and exhibit distinct trends.

cond-mat.supr-con

Kondo driven suppression of charge density wave in Van der Waals material UTe$_3$

Competing electronic instabilities lie at the heart of emergent phenomena in quantum materials. In low-dimensional metals, Fermi-surface nesting can drive charge density wave (CDW) formation through a Peierls-like mechanism, while in strongly correlated systems, Kondo hybridization reconstructs the electronic structure by entangling localized moments with itinerant electrons. How these two fundamentally different instabilities interact$-$whether they coexist, compete, or mutually exclude each other$-$remains an open question. Here, we present suppression of charge density wave via the Kondo interaction in van der Waals material UTe$_3$. The angle-resolved photoemission spectroscopy (ARPES) data reveals Fermi surface nesting under similar conditions as seen in RETe$_3$ compounds. Despite that, no CDW is found in UTe$_3$ after an extensive search. We demonstrate that strong hybridization between U 5$f$ electrons and Te $p$ states reconstructs the low-energy electronic structure, removes the instability, and preempts CDW formation. Our results reveal a rare example where Kondo hybridization preempts density wave formation, offering a new route to controlling ordering phenomena in correlated 2D materials.

cond-mat.str-el

Kondo Reshapes Multiple Orders in a $5f$ van der Waals Material

Electron interactions can drive magnetism, superconductivity, and topology. However, the realization of these phases remains limited in van der Waals materials, and the full landscape of strong correlations remains uncharted in any context. While interactions between conduction electrons and localized spins yield a well-known competition between heavy fermions (Kondo hybridization) and magnetic order (RKKY exchange), such spin-driven competition represents only part of the correlated electron phase diagram. Here we demonstrate that a heavy-fermion state can also compete with charge order, such as the charge density wave (CDW) state typical in the van der Waals $4f$ rare-earth tritellurides (RTe$_3$). We exploit the spatially-extended $5f$ orbitals of $\beta$-UTe$_3$ to enhance Kondo hybridization compared to its isostructural RTe$_3$ cousins. Our scanning tunneling spectroscopy on $\beta$-UTe$_3$ shows Fano resonances characteristic of the heavy fermion state, while our quasiparticle interference imaging reveals the disappearance of Fermi-level nesting and the appearance of flat bands. We extend the tritelluride tight-binding model to include Kondo coupling and quantify the Fermi surface reconstruction. Consistent with the destruction of nesting, we observe no CDW in $\beta$-UTe$_3$. Our expansion of the Kondo phase diagram beyond spin-mediated competition opens new possibilities for proximity-induced phase engineering in correlated van der Waals heterostructures.

cond-mat.str-el

Learning Beyond Optimization: Stress-Gated Dynamical Regime Regulation in Autonomous Systems

Despite their apparent diversity, modern machine learning methods can be reduced to a remarkably simple core principle: learning is achieved by continuously optimizing parameters to minimize or maximize a scalar objective function. This paradigm has been extraordinarily successful for well-defined tasks where goals are fixed and evaluation criteria are explicit. However, if artificial systems are to move toward true autonomy-operating over long horizons and across evolving contexts-objectives may become ill-defined, shifting, or entirely absent. In such settings, a fundamental question emerges: in the absence of an explicit objective function, how can a system determine whether its ongoing internal dynamics are productive or pathological? And how should it regulate structural change without external supervision? In this work, we propose a dynamical framework for learning without an explicit objective. Instead of minimizing external error signals, the system evaluates the intrinsic health of its own internal dynamics and regulates structural plasticity accordingly. We introduce a two-timescale architecture that separates fast state evolution from slow structural adaptation, coupled through an internally generated stress variable that accumulates evidence of persistent dynamical dysfunction. Structural modification is then triggered not continuously, but as a state-dependent event. Through a minimal toy model, we demonstrate that this stress-regulated mechanism produces temporally segmented, self-organized learning episodes without reliance on externally defined goals. Our results suggest a possible route toward autonomous learning systems capable of self-assessment and internally regulated structural reorganization.

cs.LG

Layer-dependent antiferromagnetic Chern and axion insulating states in UOTe

Magnetic topological insulators have received significant interest due to their dissipationless edge states, which promise advances in energy-efficient electronic transport. However, the magnetic topological insulator state has typically been found in ferromagnets (FMs) that suffer from low magnetic ordering temperatures and stray fields. Identifying an antiferromagnetic topological insulator that exhibits the quantum anomalous Hall effect (QAHE) with a relatively high N\'eel temperature has been a longstanding challenge. Here, we focus on the recently discovered van der Waals (vdW) antiferromagnet (AFM) UOTe, which not only features a high N\'eel temperature (\(\sim\)150K) but also exhibits intriguing Kondo interaction and topological characteristics. Our systematic analysis of the layer-dependent topological phases based on \textit{ab} initio computations predicts the two-layer UOTe film to be an ideal 2D AFM Chern insulator in which the Hall conductivity is quantized with a fully compensated spin magnetization. By applying an in-plane strain or electric field, we show how the itinerancy of U-5f electrons can be manipulated to trigger a transition between the nontrivial ($C = 1$) and trivial ($C = 0$) phases. Interestingly, the 3-layer UOTe film is found to have zero charge conductance but it hosts a quantized spin Hall conductivity (SHC) with finite magneto-electric coupling, suggesting the presence of an axion insulator-like state. The unique magnetic structure of UOTe supports a layer-tunable topology in which films with an odd number of layers are axion-like insulators, while films with an even number of layers are Chern insulators, and the bulk material is a Dirac semimetal. Our study offers a new intrinsic AFM materials platform for realizing correlated topological phases for next-generation spintronics applications and fundamental science studies.

cond-mat.mtrl-sci

Visualizing the low-energy electronic structure of the triplet superconductor UTe$_2$ through quasiparticle interference

The identification, control and theoretical modelling of spin-triplet superconductors (STC) remain a central theme in quantum materials research. Intrinsic STC are rare but offer rich condensate properties and unique surface properties allowing insights into the nature of the spin-triplet order, and promising applications in quantum technologies. Owing to interactions, the order parameter in STCs can often be intertwined with other symmetry breaking orders like charge/spin density waves (CDW/SDW) or pair density waves (PDW) complicating their phase diagrams. UTe2 stands out as the only known odd-parity, STC that harbors such intertwined orders on the surface and possible topological surface states composed of Majorana fermions. While the (0-11) facet is the most heavily studied, the fermiology of this surface that gives rise to such exotic phenomena is still lacking and continues to be an area of active interest. Here, we employ low-temperature spectroscopic imaging to reveal the Fermi surface of UTe2 through quasiparticle interference. We find scattering originating from the uranium-derived bands that play a major role in the formation of the CDW and the PDW phases. Tunneling spectroscopy further reveals spectral signatures of the CDW gap, corroborating its onset temperature. Suppressing the CDW with a magnetic field, highlights the presence of small, circular Fermi pockets that disperse strongly near the Fermi energy. We discuss the nature of the interference patterns and the origin of the small Fermi pockets in the context of the calculated band structure and the unconventional CDW phase.

cond-mat.supr-con

Enhancement of antiferromagnetic spin fluctuations in UTe$_2$ under pressure revealed by $^{125}$Te NMR

Characterizing magnetic fluctuations is one of the keys to understanding the origin of superconductivity in the spin-triplet superconductor UTe$_2$ which exhibits two superconducting (SC) phases (SC1 and SC2) under pressure: SC1 where a superconducting transition temperature of $T_{\rm c}$ decreases with pressure while $T_{\rm c}$ of SC2 rises with pressure. Previously, D. Ambika et al. [Phys. Rev. B 105, L220403 (2022)] have reported the possible coexistence of ferromagnetic (FM) and antiferromagnetic (AFM) spin fluctuations in UTe$_2$ under pressure from their nuclear magnetic resonance (NMR) measurements. To delve the relationship between the magnetic fluctuations and the two SC phases, we have carried out detailed $^{125}$Te NMR measurements on a single crystal of UTe$_2$ with $T_{\rm c}$ = 1.6 K at various pressures ranging from 0 to 2.05 GPa. By comparing the temperature $T$ dependence of nuclear spin-lattice relaxation rates divided by temperature 1/$T_1T$ with that of the Knight shift $K$ for magnetic fields along the $a$, $b$, and $c$ directions, we evidence the enhancement of AFM spin fluctuations with increasing pressure. Based on the results, we suggest that FM spin fluctuations are more favorable for SC1 and AFM spin fluctuations are crucial for SC2. Our findings will inspire further study on this material to understand the peculiar SC phases in detail.

cond-mat.supr-con

Visualizing Pair-breaking Scattering Interference in Bulk FeSe

Spatially periodic modulations of the superconducting gap have been recently reported in diverse materials and are often attributed to pair density wave order. An alternative mechanism, termed pair-breaking scattering interference (PBSI), was proposed to produce gap modulations without finite-momentum pairing. Here we investigate signatures of PBSI in bulk FeSe using scanning tunneling microscopy with superconductive tips, enabling enhanced energy resolution and Josephson tunneling. Subsurface magnetic scatterers with Yu-Shiba-Rusinov states are identified in FeSe, around which we observe particle-hole symmetric gap modulations accompanied by spatial modulation of the Josephson current. Those modulations have wavevectors consistent with intra-pocket PBSI. We further demonstrate that phase-referenced quasiparticle interference imaging offers an independent and direct probe of PBSI beyond gap mapping. These results establish PBSI as a viable origin of gap modulations in superconductors lacking preexisting charge/spin density wave orders, and motivate further investigation of the intriguing gap modulation phenomenology.

cond-mat.supr-con

Restoring a Missing Meta-Symmetry of Quantum Mechanics

In conventional quantum mechanics, all unitary evolution takes place within the space-time Hilbert space $\mathcal H_{xt}=L^2(\mathcal M_{xt})$, with time as the sole evolution parameter. The momentum-energy representation $\phi(k,E)$ is treated merely as a Fourier re-expression of the same state-kinematically equivalent but dynamically inert. Here we restore the fundamental symmetry between the conjugate pairs $(x,t)$ and $(k,E)$ by extending the quantum theory to an enlarged Hilbert space $\mathcal H_{\text{total}} = \mathcal H_{xt} \oplus \mathcal H_{kE}$, within which the momentum-energy sector $\mathcal H_{kE}=L^2(\mathcal M_{kE})$ carries its own autonomous unitary evolution generated by a self-adjoint operator $\hat{\mathcal T}$. The resulting structure establishes a meta-symmetry: a symmetry between two conjugate dynamical projections of a single global quantum state. It produces a dual-manifold geometry in which each domain is locally complete yet globally open, with divergent limits in one mapping onto extended regions in the other. Remarkably, the dual-manifold symmetry alone reproduces both the uniform dark-energy background and the exponential boundary mapping near black-hole horizons that underlies Hawking radiation. This framework thus opens a quantum-theoretic route to cosmological phenomena that are ordinarily treated within general relativity.

quant-ph

Atomic-scale Frustrated Josephson Coupling and Multi-condensate Visualization in FeSe

In a Josephson junction involving multi-band superconductors, competition between inter-band and inter-junction Josephson coupling gives rise to frustration and spatial disjunction of superfluid densities among superconducting condensates. Such frustrated coupling manifests as quantum interference of Josephson currents from different tunneling channels and becomes tunable if channel transparency can be varied. To explore these unconventional effects in the prototypical $s^\pm$-wave superconductor FeSe, we use atomic resolution scanned Josephson tunneling microscopy SJTM for condensate resolved imaging and junction tuning -- capabilities unattainable in macroscopic Josephson devices with fixed characteristics. We quantitatively demonstrate frustrated Josephson tunneling by examining two tunneling inequalities. The relative transparency of two parallel tunneling pathways is found tunable, revealing a tendency towards a 0-pi transition with decreasing SJTM junction resistance. Simultaneous visualization of both superconducting condensates reveals anti correlated superfluid modulations, highlighting the role of inter-band scattering. Our study establishes SJTM as a powerful tool enabling new research frontiers of multi condensate superconductivity.

cond-mat.supr-con

Observation of a spin-textured nematic Kondo lattice

The Kondo lattice mode, as one of the most fundamental models in condensed matter physics, has been employed to describe a wide range of quantum materials such as heavy fermions, transition metal dichalcogenides and two-dimensional Moire systems. Discovering new phases on Kondo lattice and unveiling their mechanisms are crucial to the understanding of strongly correlated systems. Here, in a layered Kondo magnet USbTe, we observe a spin-textured nematic state and visualize a heavy electronic liquid-crystal phase. Employing scanning tunneling microscopy and spectroscopy (STM/STS), we visualize a tetragonal symmetry breaking of heavy electronic states around the Fermi level. Through systematically investigating the temperature and energy dependence of spectroscopic data, we find that the nematic state coincides with the formation of heavy quasi-particles driven by band hybridization. Remarkably, using spin polarized STM, we demonstrate that the nematic state is spin polarized, which not only suggests its intrinsically electronic nature, but also represents the unique magnetic texture of nematic heavy fermions. Our findings unveil a novel correlation-mediated order whose mechanism is inherently tied to Kondo-lattice physics. The observation of heavy nematic states enriches the phase diagram of correlated systems and provides a rare platform to explore the interplay of Kondo physics, spontaneous symmetry breaking and quantum criticality.

cond-mat.str-el

Odd-Parity Quasiparticle Interference in the Superconductive Surface State of UTe2

Although no known material exhibits intrinsic topological superconductivity, wherein spin-triplet odd-parity electron pairing occurs, UTe2 is now the leading representative of this class. Conventionally, the parity of the superconducting order parameter may be established by using Bogoliubov quasiparticle interference (QPI) imaging. However, odd-parity superconductors should support a topological quasiparticle surface band (QSB) at energies within the maximum superconducting energy gap. QPI would then be dominated by the electronic structure of the QSB and only reveal the characteristics of the bulk order parameter excursively. Here, we visualize quasiparticle interference patterns of UTe2 and find that, at the (0-11) cleave surface, a new band of Bogoliubov quasiparticles appears only in the superconducting state. QPI visualization then allows study of dispersion of states within this QSB, which we demonstrate exists only within the range of Fermi momenta projected onto the (0-11) surface. Finally, we develop a theoretical framework to predict the QPI signatures of such a QSB at the (0-11) surface of UTe2. Its predictions are most consistent with the experimental results if the bulk superconducting gap function exhibits time-reversal conserving, odd-parity, a-axis nodal, B3u symmetry.

cond-mat.supr-con