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Shengpu Huang

Publications and source records attributed to Shengpu Huang.

6 recordsLinked to original sources

Light-Tunable Giant Anomalous Hall Effect in the Flat-Band Magnetic Weyl Semimetal $\mathrm{AlFe_2O_4}$

Achieving a giant anomalous Hall effect (AHE) and enabling its effective tuning are fundamental goals for topological spintronics. Magnetic Weyl semimetals hosting flat bands offer a promising route to maximize the AHE. However, while theoretical models are well-established, realistic material candidates remain scarce. Since the intrinsic anomalous Hall conductivity (AHC) is topologically dictated by the momentum separation ($\kappa$) between Weyl nodes, actively manipulating remains a key challenge. Here, through comprehensive first-principles calculations, we establish the inverse spinel $\mathrm{AlFe_2O_4}$ as a realistic ferromagnetic half-metallic platform integrating three-dimensional flat bands and Weyl physics. Spin-orbit coupling induces a single pair of Weyl nodes, yielding a giant intrinsic AHC of $398\ \mathrm{S}\cdot\mathrm{cm}^{-1}$. By constructing a symmetry-constrained tight-binding model, we uncover a deterministic relationship between microscopic electronic couplings and the macroscopic AHE. Exploiting this via Floquet engineering with circularly polarized light, we demonstrate that the effective couplings are dynamically suppressed. This optical modulation controllably enlarges $\kappa$, shortens the topological Fermi arcs, and drives a dramatic, quantitative suppression of the AHC, providing a practical blueprint for ultrafast, light-controlled topological transport.

cond-mat.mtrl-sci

Anomalous Hall Conductivity as an Effective Means of Tracking the Floquet Weyl Nodes in Quasi-One-Dimensional $\beta$-Bi$_4$I$_4$

While Floquet engineering offers a powerful paradigm for manipulating topological phases, particularly Floquet Weyl semimetals, establishing an experimentally feasible strategy for tracking the dynamic evolution of such states remains a significant challenge. Here, we propose that the anomalous Hall effect (AHE), as a sensitive, all-electrical probe, can be used to track Floquet Weyl nodes. Using first-principles calculations and symmetry analysis on the quasi-one-dimensional material $\beta$-Bi$_4$I$_4$, we demonstrate that circularly polarized light breaks time-reversal symmetry, driving the system from a trivial insulator into a Floquet Weyl semimetal phase characterized by a nonzero Berry curvature flux. Crucially, by continuously tuning the polarization phase $\varphi$ of the driving field, we show that the trajectory of the induced Weyl nodes is highly controllable, leading to their migration and eventual annihilation at high-symmetry points. We reveal that the anomalous Hall conductivity maps directly onto this topological evolution, serving as a definitive fingerprint for the generation and dynamics of Weyl nodes.

cond-mat.mtrl-sci

Light-induced Odd-parity Magnetism in Conventional Collinear Antiferromagnets

Recent studies have drawn growing attention on non-relativistic odd-parity magnetism in the wake of altermagnets. Nevertheless, odd-parity spin splitting is often believed to appear in non-collinear magnetic configurations. Here, using symmetry arguments and effective model analysis, we show that Floquet engineering offers a universal strategy for achieving odd-parity magnetism in two-dimensional (2D) collinear antiferromagnets under irradiation of periodic driving light fields such as circularly polarized light, elliptically polarized light, and bicircular light. A comprehensive classification of potential candidates for collinear monolayer or bilayer antiferromagnets is established. Strikingly, the light-induced odd-parity spin splitting can be flexibly controlled by adjusting the crystalline symmetry or the polarization state of incident light, enabling the reversal or conversion of spin-splitting. By combining first-principles calculations and Floquet theorem, we present illustrative examples of 2D collinear antiferromagnetic (AFM) materials to verify the light-induced odd-parity magnetism. Our work not only offers a powerful approach for uniquely achieving odd-parity spin-splitting with high tunability, but also expands the potential of Floquet engineering in designing unconventional compensated magnetism.

cond-mat.mtrl-sci

Semiconducting behaviors at epitaxial Ca0.5TaO3 interfaces

Emergent phenomena take place in symmetry-breaking systems, notably the recently discovered two-dimensional electron gas and its tunable superconductivities near the KTaO3 interfaces. Here, we synthesized perovskite Ca0.5TaO3 films along both [001] and [111] orientations. Different from the KTaO3 system, Ca0.5TaO3 films show semiconducting behaviors when capped with LaAlO3 films in both [001] and [111] orientations. By growing films at higher temperatures, more oxygen vacancies can be introduced, and the carrier density can be tuned from ~ 1014 cm-2 to ~ 1016 cm-2. Another difference is that the superconducting transition temperature Tc in KTaO3 (111) increases linearly along with its carrier density, while the Ca0.5TaO3 (111) remains semiconducting when carrier density ranges from ~ 1014 cm-2 to ~ 1016 cm-2. Based on the density function theory calculation, Ca0.5TaO3 and KTaO3 show similar electronic band structures. According to the energy-dispersive X-ray spectroscopy, we found heavy Sr diffusion from the substrate to the Ca0.5TaO3 layer, which may destroy the interfacial conductivity. Our work demonstrates that besides the oxygen vacancies, electronic transport is sensitive to the atomic intermixing near the interface in tantulates.

cond-mat.mtrl-sci

Controllable Weyl Nodes and Fermi Arcs from Floquet Engineering Triple Fermions

Floquet engineering with periodic driving as a powerful tool for designing desirable topological states has been the subject of intense recent studies. Here, we present the application of Floquet engineering to investigate evolution of topological triple fermions under irradiation of circularly polarized light (CPL), a phenomenon that currently remains a mystery. By using first-principles calculations and Floquet theorem, we demonstrate that WC-type TiO and its analogues are promising candidates for Floquet engineering of triple fermions. The symmetry analysis reveals that the electric field of CPL can break the specific symmetries, such as the time-reversal symmetry and its combination of spatial symmetries, inducing a transition to a flexibly controllable Weyl semimetallic phase. The survived spatial symmetry, controlled by light, guarantees that the Weyl nodes are located along the high-symmetry line or in high-symmetry planes in momentum space. Our findings focusing on Floquet engineering in realistic materials featured by triple fermions would facilitate both theoretical and experimental interest.

cond-mat.mtrl-sci

Circularly polarized light irradiated ferromagnetic MnBi$_2$Te$_4$: the long-sought ideal Weyl semimetal

The interaction between light and non-trivial energy band topology allows for the precise manipulation of topological quantum states, which has attracted intensive interest in condensed matter physics. In this work, using first-principles calculations, we studied the topological transition of ferromagnetic (FM) MnBi$_2$Te$_4$ upon irradiation with circularly polarized light (CPL). We revealed that the MnBi$_2$Te$_4$ can be driven from an FM insulator to a Weyl semimetal with a minimum number of Weyl points, i.e., two Weyl points in systems without time-reversal symmetry. More importantly, in FM MnBi$_2$Te$_4$ with out-of-plane easy magnetization axis, we found that the band dispersion of the WP evolves from Type-II to Type-III and finally to Type-I when the light intensity increases. Moreover, we show that the profile of the characteristic Fermi arc of Weyl semimetal phase is sensitive to changes in light intensity, which enables efficient manipulation of the Fermi arc length of FM MnBi$_2$Te$_4$ in experiments. In addition, for FM MnBi$_2$Te$_4$ with in-plane easy magnetization axis, the system becomes a type I Weyl semimetal under CPL irradiation. With controllable band dispersion, length of Fermi arc, and minimum number of WPs, our results indicate that CPL-irradiated FM MnBi$_2$Te$_4$ is an ideal platform to study novel transport phenomena in Weyl semimetals with distinct band dispersion.

cond-mat.mtrl-sci