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Shengtao Jiang

Publications and source records attributed to Shengtao Jiang.

14 recordsLinked to original sources

Finite-temperature crossover from coherent magnons to energy superdiffusion in the PXP model

The PXP chain was recently shown to exhibit superdiffusive energy transport with Kardar-Parisi-Zhang-like scaling, $z\approx3/2$, joining a growing number of spin chains with this exponent. An understanding of how this anomalous hydrodynamics emerges from microscopics is, however, still lacking. In this work, we show that finite-temperature energy transport in this model provides a window into the emergence of superdiffusion. At finite temperature, the energy autocorrelation function exhibits a crossover from short-time coherent dynamics to long-time hydrodynamics. The short-time behavior is dominated by a single magnon band and can be understood analytically. In momentum space, this regime is characterized by spectral weight near $q=π$. The damping time $τ$, which separates the short-time magnon-dominated behavior from the late-time hydrodynamics, grows rapidly upon cooling, consistent with an activated form $τ(β)\sim βe^{Δβ}$ with a gap scale set by the magnon band. At longer times, the spectral weight transfers to $q=0$ and the running decay exponent drifts toward the superdiffusive value $z=3/2$. Finite-temperature energy transport therefore provides a bridge between microscopic magnon physics and late-time superdiffusion in the PXP model.

cond-mat.stat-mech

Competing states in the $S=1/2$ triangular-lattice $J_1$-$J_2$ Heisenberg model: a dynamical density-matrix renormalization group study

Previous studies of the $S=1/2$ triangular-lattice $J_1$--$J_2$ Heisenberg antiferromagnet have inferred the existence of a non-magnetic ground-state phase for an intermediate range of $J_2$, but disagree concerning whether it is a gapped $\mathbb{Z}_2$ quantum spin liquid (QSL), a gapless (Dirac) QSL, or a weakly symmetry-broken phase. Using an improved dynamical density-matrix renormalization group method, we investigate the relevant intermediate $J_2$ regime for cylinders with circumferences from 6 to 9. Depending on the initial state and boundary conditions, we find two {\it distinct} variational states. The higher energy state is consistent with a Dirac QSL. In the lower-energy state, both the static and dynamical properties are qualitatively similar to the magnetically ordered state at $J_2=0$, suggestive of either a weakly magnetically ordered non-QSL or a gapped QSL proximate to a continuous transition to such an ordered state.

cond-mat.str-el

Quantifying the Phase Diagram and Hamiltonian of $S=1/2$ Kagome Antiferromagnets: Bridging Theory and Experiment

Spin-$1/2$ kagome antiferromagnets are leading candidates for realizing quantum spin liquid (QSL) ground states. While QSL ground states are predicted for the pure Heisenberg model, understanding the robustness of the QSL to additional interactions that may be present in real materials is a forefront question in the field. Here we employ large-scale density-matrix renormalization group simulations to investigate the effects of next-nearest neighbor exchange couplings $J_2$ and Dzyaloshinskii-Moriya interactions $D$, which are relevant to understanding the prototypical kagome materials herbertsmithite and Zn-barlowite. By utilizing clusters as large as XC12 and extrapolating the results to the thermodynamic limit, we precisely delineate the scope of the QSL phase, which remains robust across an expanded parameter range of $J_2$ and $D$. Direct comparison of the simulated static and dynamic spin structure factors with inelastic neutron scattering reveals the parameter space of the Hamiltonians for herbertsmithite and Zn-barlowite, and, importantly, provides compelling evidence that both materials exist within the QSL phase. These results establish a powerful convergence of theory and experiment in this most elusive state of matter.

cond-mat.str-el

The Saga of $α$-RuCl$_3$: Parameters, Models, and Phase Diagrams

RuCl$_3$ was likely the first ever deliberately synthesized ruthenium compound, following the discovery of the $_{44}$Ru element in 1844. For a long time it was known as an oxidation catalyst, with its physical properties being discrepant and confusing, until a decade ago when its allotropic form $α$-RuCl$_3$ rose to exceptional prominence. This "re-discovery" of $α$-RuCl$_3$ has not only reshaped the hunt for a material manifestation of the Kitaev spin liquid, but it has opened the floodgates of theoretical and experimental research in the many unusual phases and excitations that the anisotropic-exchange magnets as a class of compounds have to offer. Given its importance for the field of Kitaev materials, it is astonishing that the low-energy spin model that describes this compound and its possible proximity to the much-desired spin-liquid state is still a subject of significant debate ten years later. In the present study, we argue that the existing key phenomenological observations put strong natural constraints on the effective microscopic spin model of $α$-RuCl$_3$, and specifically on its spin-orbit-induced anisotropic-exchange parameters that are responsible for the non-trivial physical properties of this material. These constraints allow one to focus on the relevant region of the multi-dimensional phase diagram of the $α$-RuCl$_3$ model, suggest an intuitive description of it via a different parametrization of the exchange matrix, offer a unifying view on the earlier assessments of its parameters, and bring closer together several approaches to the derivation of anisotropic-exchange models. We explore extended phase diagrams relevant to the $α$-RuCl$_3$ parameter space using quasi-classical, Luttinger-Tisza, exact diagonalization, and density-matrix renormalization group methods, demonstrating a remarkably c... (arxiv cutoff; for the rest, see the paper)

cond-mat.str-el

BaCo$_2$(AsO$_4$)$_2$: Strong Kitaev, After All

The inelastic neutron scattering results and their analysis unequivocally point to a dominant Kitaev interaction in the honeycomb-lattice cobaltate BaCo$_2$(AsO$_4$)$_2$. Our anisotropic-exchange model closely describes $all$ available neutron scattering data in the material's field-polarized phase. The density-matrix renormalization group results for our model are in close accord with the unusual double-zigzag magnetic order and the low in-plane saturation field of BaCo$_2$(AsO$_4$)$_2$.

cond-mat.str-el

Ground-State-Based Model Reduction with Unitary Circuits

We present a method to numerically obtain low-energy effective models based on a unitary transformation of the ground state. The algorithm finds a unitary circuit that transforms the ground state of the original model to a projected wavefunction with only the low-energy degrees of freedom. The effective model can then be derived using the unitary transformation encoded in the circuit. We test our method on the one-dimensional and two-dimensional square-lattice Hubbard model at half-filling, and obtain more accurate effective spin models than the standard perturbative approach.

cond-mat.str-el

Phase Diagram of the Easy-Axis Triangular-Lattice $J_1\!-\!J_2$ Model

The phase diagram of the $S\!=\!1/2$ easy-axis triangular-lattice $J_1\!-\!J_2$ model is investigated using the density-matrix renormalization group and analytical insights. We find a significant spin-liquid region extending from the Heisenberg limit and residing between the Y phase-known as the magnetic analogue of the "supersolid"-and collinear stripe phase. The order parameters of the supersolid are analyzed and an understanding of its lack of ferromagnetic moment is suggested.

cond-mat.str-el

Quantum Phases in the Honeycomb-Lattice $J_1$--$J_3$ Ferro-Antiferromagnetic Model

Using large-scale density-matrix renormalization group calculations and minimally augmented spin-wave theory, we demonstrate that the phase diagram of the quantum $S\!=\!\frac12$ $J_1$--$J_3$ ferro-antiferromagnetic model on the honeycomb lattice differs dramatically from the classical one. It hosts the double-zigzag and Ising-z phases as unexpected intermediaries between ferromagnetic and zigzag states that are also extended beyond their classical regions of stability. In broad agreement with quantum order-by-disorder arguments, these collinear phases replace the classical spiral state.

cond-mat.str-el

Density-matrix-renormalization-group-based downfolding of the three-band Hubbard model: the importance of density-assisted hopping

Typical Wannier-function downfolding starts with a mean-field or density functional set of bands to construct the Wannier functions. Here we carry out a controlled approach, using DMRG-computed natural orbital bands, to downfold the three-band Hubbard model to an effective single band model. A sharp drop-off in the natural orbital occupancy at the edge of the first band provides a clear justification for a single-band model. Constructing Wannier functions from the first band, we compute all possible two-particle terms and retain those with significant magnitude. The resulting single-band model includes two-site density-assisted hopping terms with $t_n \sim 0.6 t$. These terms lead to a reduction of the ratio $U/t_{\rm eff}$, and are important in capturing the doping-asymmetric carrier mobility, as well as in enhancing the pairing in a single-band model for the hole-doped cuprates.

cond-mat.str-el

Where is the Quantum Spin Nematic?

We provide strong evidence of the spin-nematic state in a paradigmatic ferro-antiferromagnetic $J_1$--$J_2$ model using analytical and density-matrix renormalization group methods. In zero field, the attraction of spin-flip pairs leads to a first-order transition and no nematic state, while pair-repulsion at larger $J_2$ stabilizes the nematic phase in a narrow region near the pair-condensation field. A devil's staircase of multi-pair condensates is conjectured for weak pair-attraction. A suppression of the spin-flip gap by many-body effects leads to an order-of-magnitude contraction of the nematic phase compared to naïve expectations. The proposed phase diagram should be broadly valid.

cond-mat.str-el

Pairing Properties of the $t$-$t'$-$t''$-$J$ model

We study the pairing properties of the two-dimensional $t$-$t'$-$t''$-$J$ model, where $t'$ and $t''$ are second and third neighbor hoppings, at a doping level $x\approx0.1$. Recent studies of the $t$-$t'$-$J$ model find strong pairing for $t'>0$, associated with electron doping, but an absence of pairing for $t'<0$ associated with hole doping. This is in contrast to the cuprates, where the highest transition temperatures appear for hole doping. Model parameterizations for the cuprates estimate a $t''$ comparable to $t'$, which, in principle, might fix this discrepancy. However, we find that it does not; we observe a suppression of pairing for the hole-doped system ($t'<0, t''>0$) while for the electron-doped system ($t'>0, t''<0$) $d$-wave pairing is robust. Extended hoppings appear to be insufficient to make the one-band $t$-$t'$-$J$ model capable of describing the pairing in the hole doped system.

cond-mat.supr-con

Transport in the emergent Bose liquid: Bad metal, strange metal, and weak insulator, all in one system

Non-saturating high-temperature resistivity ("bad metal"), T-linear low-temperature resistivity ("strange metal"), and a crossover to activation-free growth of the resistivity in the low-temperature limit ("weak insulator") are among the most exotic behaviors widely observed in many strongly correlated materials for decades that defy the standard Fermi liquid description of solids. Here we investigate these puzzling behaviors by computing temperature-dependent optical conductivity of an emergent Bose liquid and find that it reproduces all the unexplained features of the experiments, including a featureless continuum and a well-known mid-infrared peak. Amazingly and with physically intuitive mechanisms, the corresponding doping- and temperature-dependent resistivity displays the bad metal and strange metal simultaneously and sometimes weak insulating behaviors as well. The unification of all these non-Fermi liquid behaviors in a single model suggests that a new quantum state of matter, namely the emergent Bose liquid, will guide the development of the next generation of solid state physics.

cond-mat.str-el

Ground State Phase Diagram of the $t$-$t'$-$J$ model

We report results of large scale ground state density matrix renormalization group(DMRG) calculations on $t$-$t'$-$J$ cylinders with circumferences 6 and 8. We determine a rough phase diagram which appears to approximate the 2D system. While for many properties, positive and negative $t'$ values ($t'/t = \pm 0.2$) appear to correspond to electron and hole doped cuprate systems, respectively, the behavior of superconductivity itself shows an inconsistency between the model and the materials. The $t'<0$ (hole doped) region shows antiferromagnetism limited to very low doping, stripes more generally, and the familiar Fermi-surface of the hole doped cuprates. However, we find $t'<0$ strongly suppresses superconductivity. The $t'>0$ (electron doped) region shows the expected circular Fermi pocket of holes around the $(π,π)$ point and a broad low-doped region of coexisting antiferromagnetism and $d$-wave pairing with a strong triplet $p$ component at wave-vector $(π,π)$ induced by the antiferromagnetism and $d$-wave pairing. The pairing for the electron low-doped system with $t'>0$ is strong and unambiguous in the DMRG simulations. At larger doping another broad region with stripes in addition to weaker $d$-wave pairing and striped $p$-wave pairing appears. In a small doping region near $x=0.08$ for $t'\sim-0.2$, we find a new type of stripe involving unpaired holes located predominantly on chains spaced three lattice spacings apart. The undoped two-leg ladder regions in between mimic the short-ranged spin correlations seen in two-leg Heisenberg ladders.

cond-mat.str-el

Non-Fermi liquid scattering against an emergent Bose liquid: manifestations in the kink and other exotic quasiparticle behaviors in the normal-state cuprate superconductors

The normal state of cuprate superconductors exhibits many exotic behaviors qualitatively different from the Fermi liquid, the foundation of condensed matter physics. Here we demonstrate that non-Fermi liquid behaviors emerge naturally from scattering against an emergent Bose liquid. Particularly, we find a finite zero-energy scattering rate at low-temperature limit that grows linearly with respect to temperature, against clean fermions' generic non-dissipative characteristics. Surprisingly, three other seemingly unrelated experimental observations are also produced, including the well-studied "kink" in the quasi-particle dispersion, as well as the puzzling correspondences between the normal and superconducting state. Our findings provide a general route for fermionic systems to generate non-Fermi liquid behavior, and suggest strongly that by room temperature the doped holes in the cuprates have already formed an emergent Bose liquid of tightly bound pairs, whose low-temperature condensation gives unconventional superconductivity.

cond-mat.supr-con