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Shengyuan A. Yang

Publications and source records attributed to Shengyuan A. Yang.

At least 19 recordsLinked to original sources

Symmetry-protected triplet Weyl complexes

The Nielsen-Ninomiya theorem dictates that Weyl nodes must appear in pairs of opposite chirality to preserve global charge neutrality. However, in crystals, specific crystalline symmetries can stabilize multi-Weyl nodes, circumventing this pairwise constraint and enabling compensated Weyl complexes with mixed chiral charges. The minimal configuration of this type is a triplet Weyl complex (TWC), comprising exactly three Weyl nodes. Here, we systematically investigate the symmetry conditions required to realize TWCs. By screening all 1651 magnetic space groups (MSGs) in both spinless and spinful systems, we establish that: (i) Only TWCs with charge magnitudes of $\{1,1,2\}$ and $\{1,2,3\}$ are permitted; (ii) the $\{1,1,2\}$ configuration can be realized in 166 spinless MSGs and 70 spinful MSGs; and (iii) the $\{1,2,3\}$-TWCs, which has not been reported before, can occur in 10 MSGs for both spinless and spinful cases. We explicitly demonstrate the existence of $\{1,2,3\}$-TWC in a tight-binding model. Furthermore, we present the first electronic realization of $\{1,1,2\}$-TWC topological semimetal state in the chiral carbon allotrope DZQH-C$_{36}$, in which the three Weyl nodes form a collinear configuration, leading to a characteristic ``S''-shaped surface Fermi arc pattern. Our findings uncover novel topological states featuring mixed chiral charges and provide guidance for exploring their physics in concrete material systems.

cond-mat.mtrl-sci

Quantum Geometric Origin of Nonlinear Current Induced Orbital Magnetization

Electric generation of magnetization is a focus of condensed matter research, and has recently been advanced into the nonlinear regime. However, due to the nonlocal nature of orbital magnetism, how to properly formulate nonlinear current-induced orbital magnetization remains a fundamental challenge. Here, we develop the proper theory for this effect. This is based on the microscopic derivation of field-corrected orbital magnetic moment of a Bloch electron, a critical missing piece in the present theory. We show that the quantum geometric origin of this phenomenon lies in both the anomalous orbital polarizability and the Berry-connection polarizability, which often provide competing contributions. Combining our theory with first-principles calculations, we predict significant, experimentally accessible nonlinear orbital magnetization generated in strained bilayer graphene, monolayer 1T' $\mathrm{MoS_2}$ and $\mathrm{MoTe_2}$. Remarkably, nonlinear orbital magnetization can dominate over its spin counterpart in materials with topological band features, irrespective of the spin-orbit coupling strength.

cond-mat.mes-hall

Room-temperature ferroelectrically switchable quantum geometry in few-layer WTe2 for complementary in-memory computing

Quantum geometry, describing the inherent geometric structure of electron wavefunctions in momentum space, transcends the traditional charge degree of freedom and provides a novel physical basis for information encoding and processing. The key to such new computing paradigms is the non-volatile electrical programming of quantum geometric states at room temperature, which, however, has not been established. Here, we demonstrate ferroelectrically switchable quantum geometry in few-layer WTe2, which uniquely enables complementary convolutional processing. By employing the intrinsic coupling between ferroelectric polarization and quantum geometry in few-layer WTe2, we show that the second- and third-order nonlinear anomalous Hall effects (NLAHE) can be deterministically and electrically switched in a nonvolatile and correlated manner. The switching is robust at room temperature for ~104 cycles and retention of ~105 s. Furthermore, leveraging the opposite switching behaviors of second- and third-order NLAHE at room temperature, we demonstrate complementary in-memory computing and implement a hardware-level complementary convolution kernel. This kernel overcomes the inherent directional specificity of conventional convolutional networks and achieves a texture recognition accuracy of 98%, thereby illustrating a viable pathway towards physics-native computing through exploiting exotic physics in quantum materials.

cond-mat.mtrl-sci

Surface Originated Cross-Field Anomalous Transport in Magnetoelectric Multilayers

In material systems with slab geometry, the surface contribution to physical responses is commonly expected to diminish rapidly with increasing thickness, giving way to the bulk response. Here, we show that this conventional wisdom is violated in a class of gate-induced responses, including gate-induced orbital and spin magnetization as well as cross-field anomalous thermoelectric transport. We develop a general framework for these effects, which naturally decomposes the total response into surface- and bulk-contributions treated on equal footing. Remarkably, the volume-averaged surface contribution remains finite in the thick-slab limit and exhibits the same thickness scaling as the bulk term. Furthermore, the surface response originates from band geometric quantities distinct from those in the bulk, being constrained solely by surface symmetries. As a result, it can dominate the overall response when the bulk contribution is symmetry-forbidden. Taking MnBi$_2$Te$_4$ multilayers as an example, we predict a strong surface-dominated cross-field anomalous Nernst effect arising from surface Berry curvature, which is readily accessible to experimental detection. These findings reveal a previously overlooked significance of surface response and open a new direction in the study of surface quantum geometry.

cond-mat.mes-hall

Higher-order Weyl nodes driven by helical magnetic order in EuAgAs

Magnetic topological semimetals provide a fertile ground for exploring how long-range magnetic order can alter electronic band structures and generate novel quasiparticles such as Weyl fermions. Here, we investigate the coupled magnetic and electronic structure of single-crystalline EuAgAs, a hexagonal pnictide whose magnetic ground state has remained elusive. Using neutron diffraction and resonant elastic X-ray scattering, we identify an unusual magnetic ordering sequence with two successive phase transitions at $T_\mathrm{N1} = 12$ K and $T_\mathrm{N2} = 8$ K. We observe two slightly different magnetic propagation vectors, one associated with $T_\mathrm{N1}$ and the other with $T_\mathrm{N2}$. Spherical neutron polarimetry reveals that the magnetic structure is a transverse helix aligned along the $c$ axis with a period that is approximately twice the $c$ lattice parameter. First-principles calculations for the helical phase predict subtle band folding effects and the emergence of effective higher-order Weyl nodes. These topological features appear near the calculated Fermi energy $E_{\mathrm{F}}$ which, however, lies above the position of $E_{\mathrm{F}}$ obtained from angle-resolved photoemission spectroscopy so could not be probed in this study.

cond-mat.str-el

Equivariant Space Group and Hamiltonian for Collinear Magnetic Systems

Condensed matter physics increasingly focuses on exploiting the magnetic order parameter orientation n as a tuning knob for properties of collinear magnetic materials, but a general method for constructing effective Hamiltonians with explicit n-dependence has been lacking. Here, we develop a symmetry-based framework, built on the equivariant space group, for constructing such Hamiltonians, termed equivariant magnetic Hamiltonians (EMHs). The resulting EMH lives in a higher-dimensional k-n space and exhibits unconventional symmetry actions and topological features. Using a 1D ferromagnetic chain and a 3D antiferromagnet as examples, we demonstrate that explicit n-dependence in EMHs enables the study of magnetic-dynamics-driven topological pumping, including even-integer charge pumping and a second-Chern-number-induced quantized pumping of surface anomalous Hall conductivity. Beyond model systems, we incorporate the framework into first-principles calculations to construct ab-initio EMHs that accurately capture the n-dependent band structures of real materials. The approach can also be generalized to non-collinear magnetic systems. Our work establishes a general framework for constructing EMHs and for exploring the rich physics arising from magnetic anisotropy and magnetic dynamics.

cond-mat.mtrl-sci

Symplectic connection third-order Hall effect in a room-temperature ferromagnet

Third-order nonlinear Hall effects (THE) have recently attracted considerable experimental interest as powerful probes for quantum geometric properties in emergent quantum materials, encompassing quadrupole moments of quantum metric and Berry curvature. Here, we report a fundamentally new THE in room-temperature van der Waals ferromagnet Fe3GaTe2 from second-order Berry connection polarizability, which manifests a higher-order characterization of band geometry called symplectic connection. Our observations show that the third-order transverse response in Fe3GaTe2 is odd to magnetization, vanishes above the Curie temperature and remains independent of driving current directions. Scaling law analysis combined with first-principles calculations establishes this response as the symplectic-connection-induced THE. This discovery opens the door to probing high-order quantum geometric properties beyond Berry curvature and quantum metric through nonlinear transport, unveiling the potential of exploring nonlinear Hall phenomena in broad classes of magnets without breaking inversion symmetry. Moreover, the room-temperature manipulation of THE holds promises for device applications based on harnessing the quantum-geometric connection structure.

cond-mat.mes-hall

Nonlinear Magnetic Orbital Hall Effect Induced by Spin-Orbit Coupling

Electrical readout of 180$^\circ$ switching in strictly compensated collinear antiferromagnets remains a major challenge in antiferromagnetic spintronics. Electrical writing of perpendicularly magnetized ferromagnets by out-of-plane orbital torque remains an important challenge in orbitronics. In this work, we propose a second-order nonlinear magnetic orbital Hall effect in the source antiferromagnet as a simultaneous recipe for both difficulties. This orbitronics effect is induced by spin-orbit coupling and is odd in the N\'eel vector, thus is a unique effect that integrates both functionalities via electric control of the N\'eel vector in the source antiferromagnet. Our first-principles calculations in CuMnAs predict significant non-perturbative orbital effects from spin-orbit coupling, with a orbital Berry-curvature dipole mechanism. These findings unveil new possibilities opened by topological antiferromagnetic orbitronics.

cond-mat.mtrl-sci

Eccentricity valley Hall effect

Valleytronics harnesses the valley degree of freedom -- energy-degenerate extrema in the electronic band structure -- for information storage and processing. Valley Hall effect (VHE) is a cornerstone of valleytronics, enabling electric generation of pure valley currents. While extensively studied in systems with valleys located at time-reversal-breaking points, here, we shift the paradigm to valleytronic platforms with time-reversal-invariant valleys (TRIVs), revealing a novel phenomenon: eccentricity VHE. Unlike conventional VHE, the valley Hall angle for eccentricity VHE is an intrinsic geometric property, governed solely by the eccentricity of the valley Fermi surface, rendering it highly robust against variations in temperature or carrier density. Eccentricity VHE emerges universally across all 25 layer groups supporting TRIVs. We demonstrate these distinctive features in monolayer GeS$_{2}$ via first-principles calculations, predicting a significant valley Hall angle of 0.74. This effect can be detected through nonlocal transport measurements exhibiting characteristic scaling behavior, or, in certain cases, through valley-layer coupling. Our findings reveal a critical overlooked facet of valley Hall physics, transcend the established VHE paradigm, and significantly broadens the scope of valleytronics.

cond-mat.mes-hall

Nonperturbative Magnetic Orbital Hall Effect in Altermagnets

Recent studies on altermagnets have focused considerable attention on nonrelativistic effects that persist in the absence of spin-orbit coupling (SOC). As a result, the relative importance of various phenomena in altermagnets has commonly been judged by their dependence on SOC. Here, we challenge this common wisdom by uncovering the magnetic orbital Hall effect, which is nonperturbative in SOC strength. We establish the symmetry properties of this effect, demonstrating that it is strictly forbidden in conventional collinear antiferromagnets yet universally allowed in all ten spin-Laue classes of collinear altermagnets. Counterintuitively, although SOC-induced, it reaches giant magnitudes in altermagnets-comparable to or even exceeding the nonrelativistic spin Hall effect. Moreover, altermagnetic symmetry enables unconventional collinear-polarized orbital currents, allowing field-free manipulation of perpendicular magnetization. Our first-principles calculations predict strong room-temperature responses in the experimentally established altermagnets CrSb and FeSb2. These findings reveal the previously overlooked potential of altermagnetic orbitronics and broaden the horizons for altermagnets in high-performance magnetic memory applications.

cond-mat.mtrl-sci

Altermagnetism and its induced higher-order topology on the Lieb lattice

Altermagnetism (AM) has brought renewed attention to the Lieb lattice. Here, we broaden the scope of altermagnetic models on the Lieb lattice by using a general scheme based on spin clusters. We design various altermagnetic models with d- and g-wave on the Lieb lattice, and investigate its interplay with spin-orbit coupling. While the altermagnetic unit cell reconstructs the topological edge states in the strip geometry and leads to the emergence of Dirac points, the in-plane magnetic moments of AM can induce gaps at these points. In an open square geometry, corner modes emerge within these gaps, realizing higher-order topological states. We further verify that the induction of higher-order topology is applicable to all altermagnetic configurations constructed here on the Lieb lattice, and is most pronounced for AM by comparing with the other types of magnetism such as ferromagnetism and ferrimagnetism. Our results highlight the exotic properties of AM, and suggest its potential applications in engineering topological quantum states.

cond-mat.str-el

Anomalous shift in scattering from topological nodal-ring semimetals

An electron beam may experience an anomalous spatial shift during an interface scattering process. Here, we investigate this phenomenon for reflection from mirror-symmetry-protected nodal-ring semimetals, which are characterized by an integer topological charge $\chi_h$. We show that the shift is generally enhanced by the presence of nodal rings, and the ring's geometry can be inferred from the profile of shift vectors in the interface momentum plane. Importantly, the anomalous shift encodes the topological information of the ring, where the circulation of the shift vector field $\kappa_s$ over a semicircle is governed by the topological charge, with a simple relationship: $\kappa_s=-2\pi \chi_h$. Furthermore, we demonstrate that the shift and its circulation reflect distinct features of topological phase transitions of the charged rings. This study uncovers a novel physical signature of topological nodal rings and positions anomalous scattering shifts as a powerful tool for probing topological band structures.

cond-mat.mtrl-sci

Out-of-Plane Nonlinear Orbital Hall Torque

Despite recent advances in orbitronics, generating out-of-plane orbital torques essential for field-free deterministic switching of perpendicular magnetization remains a key challenge. Here, we propose a strategy to produce such unconventional torques across broad classes of materials, by leveraging the nonlinear orbital Hall effect. We demonstrate that this nonlinear orbital response is dramatically amplified by topological band degeneracies, where it overwhelmingly dominates the spin response even in systems with strong spin-orbit coupling. These features are confirmed via a quantitative investigation of representative topological metals RhSi, YPtBi, and PbTaSe$_2$, by combining our theory with first-principles calculations. The resulting orbital torques substantially surpass those from linear mechanisms reported thus far. These findings propel the research of orbital transport into the nonlinear regime, broaden the scope of orbital source materials, and establish a new pathway towards high-performance orbitronic devices.

cond-mat.mtrl-sci

Lorentz Skew Scattering Nonreciprocal Magneto-Transport

In materials with broken inversion symmetry, nonreciprocal magneto-transport (NRMT) manifests as a bilinear dependence of charge conductivity on applied electric (E) and magnetic (B) fields. This phenomenon is deeply rooted in symmetry and electronic quantum geometry, holding promise for novel rectification and detector technologies. Existing experimental studies generally attribute NRMT to Zeeman-driven mechanisms and exhibit quadratic scaling with conductivity. Here, we report a previously unknown NRMT microscopic mechanism - Lorentz skew scattering (LSK) - revealed through the discovery of an unprecedented quartic scaling law of NRMT as well as quantitative agreement between theory and experiment in BiTeBr. LSK emerges from the interplay of Lorentz force and skew scattering, bridging classical field effect to quantum scattering effect on the Fermi surface. We demonstrate that the LSK dominates NRMT in BiTeBr, and elucidate that this dominance over other possible contributions stems from high mobility and strong Rashba splitting. The finding of LSK mechanism is of unique importance because it unveils the leading NRMT effect in high-mobility systems and suggests a universal principle towards strong NRMT by enhancing electronic relaxation time in topological materials, rendering a new designing idea for low-dissipation rectifiers and high-performance quantum electronics.

cond-mat.mes-hall

Giant field-tunable nonlinear Hall effect by Lorentz skew scattering in a graphene moire superlattice

The nonlinear Hall effect (NHE) can enable rectification and energy harvesting, and its control by external fields, including gate, strain and magnetic field, has been pursued intensively. However, existing tuning pathways rely predominantly on fully quantum mechanical effects and are typically inefficient, resulting in weak NHE signals that limit further progress. In this work, we report the discovery of a distinct type of NHE in a graphene-hBN moire superlattice, which arises from a classical-quantum cooperative effect called Lorentz skew scattering (LSK), induced by a perpendicular magnetic field. This field-driven NHE exhibits a linear dependence on magnetic field and a pronounced unidirectional angular dependence. Remarkably, its magnitude reaches up to 32% of the linear Hall signal. We show that this giant, field-tunable NHE originating from LSK follows a unique quartic scaling law and produces a record-high nonlinear Hall conductivity (36000 {\mu}mV-1{\Omega}-1) near van Hove singularities of moire minibands, which is over an order of magnitude larger than all previously reported NHEs. Our findings establish an efficient, magnetic-field-driven route to giant Hall rectification in high-mobility materials, offering a broadly applicable paradigm for modulating the NHE beyond electrostatic gating.

cond-mat.mes-hall

Two-Dimensional Altermagnetic Iron Oxyhalides: Real Chern Topology and Valley-Spin-Lattice Coupling

Altermagnets, a novel class of collinear magnetic materials, exhibit unique spin-split band structures, yet topological insulating states in intrinsic altermagnetic systems are rare. Here, we identify monolayer Fe$_2X_2$O ($X$ = Cl, Br, I) as a new family of 2D altermagnetic real Chern insulators. These materials display robust $d$-wave altermagnetic ordering, semiconducting band gaps, and nontrivial real Chern numbers per spin channel, yielding spin-polarized topological corner modes. They also feature spin-polarized valleys with strong altermagnetism-valley-spin-lattice coupling, enabling valley-selective excitation via linear dichroism and strain-induced valley polarization. In multiferroic Fe$_2$Cl$_2$O, magnetism coexists with ferroelasticity, and an applied strain can switch the N\'eel vector. These findings position 2D iron oxyhalides as a promising platform for exploring altermagnetism and magnetic topological states for spintronics and valleytronics.

cond-mat.mtrl-sci

Projective crystal symmetry and topological phases

Quantum states naturally represent symmetry groups, though often in a projective sense. Intriguingly, the projective nature of crystalline symmetries has remained underexplored until very recently. A series of groundbreaking theoretical and experimental studies have now brought this to light, demonstrating that projective representations of crystal symmetries lead to remarkable consequences in condensed matter physics and various artificial crystals, particularly in their connection to topological phenomena. In this article, we explain the basic ideas and notions underpinning these recent developments and share our perspective on this emerging research area. We specifically highlight that the appearance of momentum-space nonsymmorphic symmetry is a unique feature of projective crystal symmetry representations. This, in turn, has the profound consequence of reducing the fundamental domain of momentum space to all possible flat compact manifolds, which include torus and Klein bottle in 2D and the ten platycosms in 3D, presenting a significantly richer landscape for topological structures than conventional settings. Finally, the ongoing efforts and promising future research directions are discussed.

cond-mat.mes-hall

Intrinsic nonlinear valley Nernst effect

We investigate the intrinsic nonlinear valley Nernst effect, which induces a transverse valley current via a second-order thermoelectric response to a longitudinal temperature gradient. The effect arises from the Berry connection polarizability dipole of valley electrons and is permissible in both inversion-symmetric and inversion-asymmetric materials. We demonstrate that the response tensor is connected to the intrinsic nonlinear valley Hall conductivity through a generalized Mott relation, with the two being directly proportional at low temperatures, scaled by the Lorenz number. We elucidate the symmetry constraints governing this effect and develop a theory for its nonlocal measurement, revealing a nonlocal second-harmonic signal with a distinct $\rho^2$ scaling. This signal comprises two scaling terms, with their ratio corresponding to the square of the thermopower normalized by the Lorenz number. Key characteristics are demonstrated using a tilted Dirac model and first-principles calculations on bilayer WTe$_2$. Possible extrinsic contributions and alternative experimental detection methods, e.g., by valley pumping and by nonreciprocal directional dichroism, are discussed. These findings underscore the significance of band quantum geometry on electron dynamics and establish a theoretical foundation for nonlinear valley caloritronics.

cond-mat.mes-hall