arXiv subjects

Shigeru Kasahara

Publications and source records attributed to Shigeru Kasahara.

At least 19 recordsLinked to original sources

arXiv2025

In-plane and interlayer magnetoresistance in FeSe

We report measurements of the in-plane and interlayer magnetoresistances of FeSe. The in-plane magnetoresistance $Δρ_{ab}/ρ_{ab}(0)$ for $B \parallel c$ is positive below $T_s$ and increases with decreasing temperature, exceeding 2.5 at $T$ = 10 K and $B$ = 14 T. The field-direction dependence indicates that the in-plane magnetoresistance is basically determined by the $c$-axis component of the magnetic field. The interlayer magnetoresistance $Δρ_{c}/ρ_{c}(0)$ is negative below $T_s$ but turns positive below $\sim$18 K, which is probably due to the contamination by the large in-plane magnetoresistance. The field-direction dependence of the interlayer magnetoresistance can approximately be described by a standard formula for quasi-two-dimensional electron systems except near $B \parallel ab$. The experimental magnetoresistance near $B \parallel ab$ is larger than the formula, which can be attributed to the so-called interlayer coherence peak. The large width of the peak indicates the correspondingly large interlayer transfer energy.

cond-mat.supr-con↗

arXiv2025

Quasiparticle interaction originating from Bogoliubov Fermi Surfaces under pressure in 18%-S substituted FeSe studied via NMR

S-substituted FeSe superconductors in the tetragonal phase display several unique features among iron-based superconductors, particularly the presence of zero-energy excitations in the superconducting (SC) state. The recent concept of Bogoliubov Fermi Surfaces (BFSs), a theoretical model describing ultranodal states, has attracted considerable interest. Nuclear magnetic resonance (NMR) studies on FeSe$_{1-x}$S$_x$ (x=0.18) have revealed an anomalous low-energy spin fluctuations deep in the SC state. The low-energy spin fluctuations are enhanced with decreasing temperature, supporting strong Bogoliubov quasiparticle interactions associated with BFSs. Here, we further investigate these correlation effects through $^{77}$Se-NMR measurements of FeSe$_{1-x}$S$_x$ (x=0.18) under pressures up to 2.0 GPa and temperatures down to ~100 mK. The results demonstrate that the anomalous enhancement is suppressed but persists under pressure, implying that quasiparticle interactions become weak by applying pressure. Furthermore, spin fluctuations in the normal state exhibit different temperature dependence from those deep in the SC state, suggesting that the nesting properties of normal electrons differ from those of Bogoliubov quasiparticles. These findings are consistent with the theoretical model of BFSs with C$_2$ symmetry and strengthen evidence for Bogoliubov quasiparticle interactions, providing insights into the unconventional pairing state of this system.

cond-mat.supr-con↗

arXiv2025

Field-free superconducting diode effect in layered superconductor FeSe

The superconducting diode effect (SDE), where zero-resistance states appear nonreciprocally during current injection, is receiving tremendous interest in both fundamental and applied physics because the SDE is a novel manifestation of symmetry breaking and enables the creation of a novel diode. In particular, magnetic-field-free SDEs have been extensively investigated because of their potential to serve as building blocks for superconducting circuit technology. In this letter, we report the field-free SDE in a layered superconductor, FeSe. Its underlying physics is clarified by systematic controlled experiments to be an interplay of a large thermoelectric response and geometrical asymmetry in FeSe. Our findings can pave a new avenue for the construction of novel material and device platforms utilizing SDEs.

cond-mat.mtrl-sci↗

arXiv2025

Development of microwave surface elastoresistivity measurement technique under tunable strain

By integrating a dielectric microwave resonator with a piezoelectric-based strain device, we develop an in situ strain-tunable microwave spectroscopy technique that enables contactless measurements of superconducting properties under strain. In the slightly overdoped iron-based superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$, we successfully observe a systematic strain dependence of the superconducting transition, manifested as changes in the quality factor and resonance frequency shifts. Both compressive and tensile anisotropic lattice distortions along the [110]${_{\rm T}}$ direction suppress superconductivity, consistent with standard transport measurements, highlighting the pivotal role of nematic fluctuations in the superconducting mechanism. Our strain-tunable cavity therefore serves as a powerful, contactless probe of fundamental superconducting material properties under strain and may also potentially facilitate the design of hybrid quantum systems with strain-controlled quantum degrees of freedom.

cond-mat.supr-con↗

arXiv2025

Apparent nonreciprocal transport in FeSe bulk crystals

We performed low-frequency ac first- and second-harmonic resistance measurements and dc $I-V$ measurements on bulk FeSe crystals in a temperature range between 1.8 and 150 K and in magnetic field up to 14 T. We observed considerable second-harmonic resistance, indicative of nonreciprocal charge transport, in some samples. By examining correlation between contact resistances and second-harmonic signals, we concluded that the second-harmonic resistance was not due to the genuine nonreciprocal transport effect but was caused by joule heating at a current contact through the thermoelectric effect. Our conclusion is consistent with a recent preprint (Nagata \textit{et al.}, arXiv:2409.01715), in which the authors reported a zero-field superconducting diode effect in devices fabricated with FeSe flakes and attributed it to the thermoelectric effect.

cond-mat.supr-con↗

arXiv2024

Transport evidence for twin-boundary pinning of superconducting vortices in FeSe

We provide bulk transport evidence for twin-boundary pinning of vortices in FeSe. We measure interlayer resistance in FeSe in magnetic fields and find that, as the field is rotated in the $ab$ plane, the flux-flow resistivity is suppressed when the field direction is parallel to twinning planes. The width of the associated dip in the resistance vs in-plane field direction curve varies as $T^{1/2}B^{-3/4}$, consistent with the creation of kinked vortices near the parallel field geometry.

cond-mat.supr-con↗

arXiv2023

Spin fluctuations from Bogoliubov Fermi surfaces in the superconducting state of S-substituted FeSe

The study of the iron-based superconductor, FeSe, has resulted in various topics, such as the interplay among superconductivity, nematicity, and magnetism, Bardeen-Cooper-Schrieffer Bose-Einstein-condensation (BCS-BEC) crossover, and Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconductivity. Recently, topologically protected nodal Fermi surfaces, referred to as Bogoliubov Fermi surfaces (BFSs), have garnered much attention. A theoretical model for the S-substituted FeSe system demonstrated that BFSs can manifest under the conditions of spin-orbit coupling, multi-band systems, and superconductivity with time-reversal symmetry breaking. Here we report the observation of spin fluctuations originating from BFSs in the superconducting (SC) state via $^{77}$Se-nuclear magnetic resonance measurements to 100 mK. In a heavily S-substituted FeSe, we found an anomalous enhancement of low-energy spin fluctuations deep in the SC state, which cannot be explained by an impurity effect. Such unusual behavior implies the presence of significant spin fluctuations of Bogoliubov quasiparticles, which are associated with possible nesting properties between BFSs.

cond-mat.supr-con↗

arXiv2022

Resistivity and Thermal Conductivity of an Organic Insulator beta'-EtMe3Sb[Pd(dmit)2]2

A finite residual linear term in the thermal conductivity at zero temperature in insulating magnets indicates the presence of gapless excitations of itinerant quasiparticles, which has been observed in some candidate materials of quantum spin liquids (QSLs). In the organic triangular insulator beta'-EtMe3Sb[Pd(dmit)2]2, a QSL candidate material, the low-temperature thermal conductivity depends on the cooling process and the finite residual term is observed only in samples with large thermal conductivity. Moreover, the cooling rate dependence is largely sample dependent. Here we find that, while the low-temperature thermal conductivity significantly depends on the cooling rate, the high-temperature resistivity is almost perfectly independent of the cooling rate. These results indicate that in the samples with the finite residual term, the mean free path of the quasiparticles that carry the heat at low temperatures is governed by disorders, whose characteristic length scale of the distribution is much longer than the electron mean free path that determines the high-temperature resistivity. This explains why recent X-ray diffraction and nuclear magnetic resonance measurements show no cooling rate dependence. Naturally, these measurements are unsuitable for detecting disorders of the length scale relevant for the thermal conductivity, just as they cannot determine the residual resistivity of metals. Present results indicate that very careful experiments are needed when discussing itinerant spin excitations in beta'-EtMe3Sb[Pd(dmit)2]2.

cond-mat.str-el↗

arXiv2021

Decoupled nematic and magnetic criticality in FeSe$_{1-x}$S$_{x}$

Electronic nematicity in correlated metals often occurs alongside another instability such as magnetism. As a result, the question remains whether nematicity alone can drive unconventional superconductivity or anomalous (quantum critical) transport in such systems. In FeSe, nematicity emerges in isolation, providing a unique opportunity to address this question. Studies to date, however, have proved inconclusive; while signatures of nematic criticality are observed upon sulfur substitution, they appear to be quenched under the application of pressure due to the emergent magnetism. Here, we study the temperature and pressure dependence of the low-temperature resistivity of FeSe$_{1-x}$S$_{x}$ crystals at $x$ values just beyond the nematic quantum critical point. Two distinct components to the resistivity are revealed; one whose magnitude falls with increasing pressure and one which grows upon approaching the magnetic state at higher pressures. These findings indicate that nematic and magnetic critical fluctuations in FeSe$_{1-x}$S$_{x}$ are completely decoupled, in marked contrast to other Fe-based superconductors, and that nematic fluctuations alone may be responsible for the transport signatures of quantum criticality found in FeSe$_{1-x}$S$_{x}$ at ambient pressure.

cond-mat.str-el↗

arXiv2020

Description of resonant inelastic x-ray scattering in correlated metals

To fully capitalize on the potential and versatility of resonant inelastic x-ray scattering (RIXS), it is essential to develop the capability to interpret different RIXS contributions through calculations, including the dependence on momentum transfer, from first-principles for correlated materials. Toward that objective, we present new methodology for calculating the full RIXS response of a correlated metal in an unbiased fashion. Through comparison of measurements and calculations that tune the incident photon energy over a wide portion of the Fe L$_3$ absorption resonance of the example material BaFe$_2$As$_2$, we show that the RIXS response in BaFe$_2$As$_2$ is dominated by the direct channel contribution, including the Raman-like response below threshold, which we explain as a consequence of the finite core-hole lifetime broadening. Calculations are initially performed within the first-principles Bethe-Salpeter framework, which we then significantly improve by convolution with an effective spectral function for the intermediate-state excitation. We construct this spectral function, also from first-principles, by employing the cumulant expansion of the Green's function and performing a real-time time dependent density functional theory calculation of the response of the electronic system to the perturbation of the intermediate-state excitation. Importantly, this allows us to evaluate the indirect RIXS response from first-principles, accounting for the full periodicity of the crystal structure and with dependence on the momentum transfer.

cond-mat.str-el↗

arXiv2019

Reciprocity between local moments and collective magnetic excitations in the phase diagram of BaFe$_2$(As$_{1-x}$P$_x$)$_2$

Unconventional superconductivity arises at the border between the strong coupling regime with local magnetic moments and the weak coupling regime with itinerant electrons, and stems from the physics of criticality that dissects the two. Unveiling the nature of the quasiparticles close to quantum criticality is fundamental to understand the phase diagram of quantum materials. Here, using resonant inelastic x-ray scattering (RIXS) and Fe-K$_β$ emission spectroscopy (XES), we visualize the coexistence and evolution of local magnetic moments and collective spin excitations across the superconducting dome in isovalently-doped BaFe$_2$(As$_{1-x}$P$_x$)$_2$ (0.00$\leq$x$\leq0.$52). Collective magnetic excitations resolved by RIXS are gradually hardened, whereas XES reveals a strong suppression of the local magnetic moment upon doping. This relationship is captured by an intermediate coupling theory, explicitly accounting for the partially localized and itinerant nature of the electrons in Fe pnictides. Finally, our work identifies a local-itinerant spin fluctuations channel through which the local moments transfer spin excitations to the particle-hole (paramagnons) continuum across the superconducting dome.

cond-mat.supr-con↗

arXiv2019

Universal relationship between low-energy antiferromagnetic fluctuations and superconductivity in BaFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$

To identify the key parameter for optimal superconductivity in iron pnictides, we measured the $^{31}$P-NMR relaxation rate on BaFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ ($x = 0.22$ and 0.28) under pressure and compared the effects of chemical substitution and physical pressure. For $x = 0.22$, structural and antiferromagnetic (AFM) transition temperatures both show minimal changes with pressure up to 2.4~GPa, whereas the superconducting transition temperature $T_{\rm c}$ increases to twice its former value. In contrast, for $x=0.28$ near the AFM quantum critical point (QCP), the structural phase transition is quickly suppressed by pressure and $T_{\rm c}$ reaches a maximum. The analysis of the temperature-dependent nuclear relaxation rate indicates that these contrasting behaviors can be quantitatively explained by a single curve of the $T_{\rm c}$ dome as a function of Weiss temperature $θ$, which measures the distance to the QCP. Moreover, the $T_{\rm c}$-$θ$ curve under pressure precisely coincides with that with chemical substitution, which is indicative of the existence of a universal relationship between low-energy AFM fluctuations and superconductivity on BaFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$.

cond-mat.supr-con↗

arXiv2019

Photo-induced Superconducting State with Long-lived Disproportionate Band Filling in FeSe

Photo-excitation is a very powerful way to instantaneously drive a material into a novel quantum state without any fabrication, and variable ultrafast techniques have been developed to observe how electron-, lattice-, and spin-degrees of freedom change. One of the most spectacular phenomena is photo-induced superconductivity, and it has been suggested in cuprates that the transition temperature Tc can be enhanced from original Tc with significant lattice modulations. Here we show another photo-induced high-Tc superconducting state in the iron-based superconductor FeSe with semi-metallic hole and electron bands. The transient electronic state in the entire Brillouin zone is directly observed by the time- and angle-resolved photoemission spectroscopy using extreme ultraviolet pulses obtained from high harmonic generation. Our results of dynamical behaviors on timescales from 50 fs to 800 ps consistently support the favorable superconducting state after photo-excitation well above Tc. This finding demonstrates that multiband iron-based superconductors emerge as an alternative candidate for photo-induced superconductors.

cond-mat.supr-con↗

arXiv2019

$^{77}$Se-NMR Study under Pressure on 12%-S Doped FeSe

The 12%-S doped FeSe system has a high Tc of 30 K at a pressure of 3.0 GPa. We have successfully investigated its microscopic properties for the first time via $^{77}$Se-NMR measurements under pressure. The antiferromagnetic (AFM) fluctuations at the optimal pressure (~3 GPa) exhibited unexpected suppression compared with the AFM fluctuations at ambient pressure, even though the optimal pressure is close to the phase boundary of the AFM phase induced at the high-pressure region. In addition, we revealed that the SC phase at an applied field of 6.02 T exhibited a remarkable double-dome structure in the pressure-temperature phase diagram, unlike the SC phase at zero field.

cond-mat.supr-con↗

arXiv2018

In Situ STM Observation of Nonmagnetic Impurity Effect in MBE-grown CeCoIn$_5$ Films

Local electronic effects in the vicinity of an impurity provide pivotal insight into the origin of unconventional superconductivity, especially when the materials are located on the edge of magnetic instability. In high-temperature cuprate superconductors, a strong suppression of superconductivity and appearance of low-energy bound states are clearly observed near nonmagnetic impurities. However, whether these features are common to other strongly correlated superconductors has not been established experimentally. Here, we report the {$in$} {$situ$} scanning tunneling microscopy observation of electronic structure around a nonmagnetic Zn impurity in heavy-fermion CeCo(In$_{1-x}$Zn$_x$)$_5$ films, which are epitaxially grown by the state-of-the-art molecular beam epitaxy technique. The films have very wide atomically flat terraces and Zn atoms residing on two different In sites are clearly resolved. Remarkably, no discernible change is observed for the superconducting gap at and around the Zn atoms. Moreover, the local density of states around Zn atoms shows little change inside the $c$-$f$ hybridization gap, which is consistent with calculations for a periodic Anderson model without local magnetic order. These results indicate that no nonsuperconducting region is induced around a Zn impurity and do not support the scenario of antiferromagnetic droplet formation suggested by indirect measurements in Cd-doped CeCoIn$_5$. These results also highlight a significant difference of the impurity effect between cuprates and CeCoIn$_5$, in both of which $d$-wave superconductivity arises from the non-Fermi liquid normal state near antiferromagnetic instabilities.

cond-mat.str-el↗

arXiv2017

Impact of Disorder on the Superconducting Phase Diagram in BaFe$_2$(As$_{1-x}$P$_x$)$_2$

In many classes of unconventional superconductors, the question of whether the superconductivity is enhanced by the quantum-critical fluctuations on the verge of an ordered phase remains elusive. One of the most direct ways of addressing this issue is to investigate how the superconducting dome traces a shift of the ordered phase. Here, we study how the phase diagram of the iron-based superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$ changes with disorder via electron irradiation, which keeps the carrier concentrations intact. With increasing disorder, we find that the magneto-structural transition is suppressed, indicating that the critical concentration is shifted to the lower side. Although the superconducting transition temperature $T_c$ is depressed at high concentrations ($x\gtrsim$0.28), it shows an initial increase at lower $x$. This implies that the superconducting dome tracks the shift of the antiferromagnetic phase, supporting the view of the crucial role played by quantum-critical fluctuations in enhancing superconductivity in this iron-based high-$T_c$ family.

cond-mat.supr-con↗

arXiv2016

Quasiparticle Excitations in the Superconducting State of FeSe Probed by Thermal Hall Conductivity in the Vicinity of the BCS-BEC Crossover

There is growing evidence that the superconducting semimetal FeSe ($T_c\sim8$ K) is in the crossover regime between weak-coupling Bardeen-Cooper-Schrieffer (BCS) and strong-coupling Bose-Einstein-condensate (BEC) limits. We report on longitudinal and transverse thermal conductivities, $κ_{xx}$ and $κ_{xy}$, respectively, in magnetic fields up to 20 T. The field dependences of $κ_{xx}$ and $κ_{xy}$ imply that a highly anisotropic small superconducting gap forms at the electron Fermi-surface pocket whereas a more isotropic and larger gap forms at the hole pocket. Below $\sim1.0$ K, both $κ_{xx}$ and $κ_{xy}$ exhibit distinct anomalies (kinks) at the upper critical field $H_{c2}$ and at a field $H^*$ slightly below $H_{c2}$. The analysis of the thermal Hall angle ($κ_{xy}/κ_{xx}$) indicates a change of the quasiparticle scattering rate at $H^*$. These results provide strong support to the previous suggestion that above $H^*$ a distinct field-induced superconducting phase emerges with an unprecedented large spin imbalance.

cond-mat.supr-con↗

arXiv2016

Magnetotransport study of the pressure-induced antiferromagnetic phase in FeSe

The resistivity $ρ$ and Hall resistivity $ρ_H$ are measured on FeSe at pressures up to $P$ = 28.3 kbar in magnetic fields up to $B$ = 14.5 T. The $ρ(B)$ and $ρ_H(B)$ curves are analyzed with multicarrier models to estimate the carrier density and mobility as a function of $P$ and temperature ($ T\leqslant$ 110 K). It is shown that the pressure-induced antiferromagnetic transition is accompanied by an abrupt reduction of the carrier density and scattering. This indicates that the electronic structure is reconstructed significantly by the antiferromagnetic order.

cond-mat.supr-con↗