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Shihao Ru

Publications and source records attributed to Shihao Ru.

17 recordsLinked to original sources

All-Optical Wide-Field Magnetometry with Van Der Waals Quantum Sensor

Negatively charged boron vacancy ($V_B^-$) centers in hexagonal boron nitride ($h$-BN) have attracted wide-range interests owing to their van der Waals lattice and their potentials for $in$-$situ$ quantum sensing. Here we propose and experimentally demonstrate an all-optical strategy for wide-field magnetometry based on $V_B^-$ centers. This strategy exploits the magnetically sensitive ground-state level anti-crossing (GSLAC) of $V_B^-$ centers, which induces a strong electron spin transition between $m_S = 0$ and $m_S = -1$ states, enabling microwave-free magnetic field measurement. By monitoring the shift of GSLAC feature, the external magnetic field can be precisely determined. Using this technique, we demonstrate all-optical wide-field imaging of near-field DC magnetic field distribution from current-carrying circuits over an area of around 42 $\times$ 21 $\mu$m$^2$. An estimated photon shot-noise-limited sensitivity of 67.1 $\mu$T/$\sqrt{\text{Hz}}$ is achieved for a single pixel, which is an approximately threefold improvement over the ODMR method, along with a spatial resolution of about 1 $\mu$m per pixel. Our approach expands the applicability of $V_B^-$ centers in quantum sensing, paving the way for robust and convenient magnetometry under extreme conditions.

quant-ph

Electronic Phonons in a Moir\'e Electron Crystal

Collective quantum phenomena, such as the excitation of composite fermions1, spin waves2, and exciton condensation3,4, can emerge in strongly correlated systems like the fractional quantum Hall states5, spin liquids6, or excitonic insulators7. Two-dimensional (2D) moir\'e superlattices have emerged as a powerful platform for exploring such correlated phases and their associated collective excitations8,9. Specifically, electron crystals stabilized by longrange Coulomb interactions may host collective vibrational excitations emerging from electron correlations10, termed electronic phonons, which are fundamentally distinct from atomic lattice phonons. Despite theoretical prediction of their existence in moir\'e electron crystals11, direct experimental evidence has remained elusive. Here we report the observation of electronic phonons in the Mott insulating and stripe phases of a WS2/WSe2 moir\'e superlattice, achieved through light scattering measurements. The phonon energies, temperature and filling factor dependencies, along with theoretical modeling, corroborate their origin as collective vibrations of a correlated electron crystal. Polarization-resolved measurements further indicate rotational symmetry breaking in the Mott state. Notably, these electronic phonons exhibit strong tunability in energy, intensity, and polarization under external electric or magnetic fields, highlighting rich and controllable lattice dynamics of the electron crystal. These findings provide direct spectroscopic evidence for the electronic crystalline nature of correlated phases, opening avenues for probing and manipulating collective excitations in correlated electron systems.

cond-mat.str-el

Experimental demonstration of scalable quantum cryptographic conferencing

Quantum network enables a variety of quantum information processing tasks, where multi-user quantum communication is one of the important objectives. Quantum cryptographic conferencing serves as an essential solution to establish secure keys to realize secure multi-user communications. However, existing QCC implementations have been fundamentally limited by the low probability of multi-user coincidence detection to measure or construct the Greenberger-Horne-Zeilinger (GHZ) entangled state. In this work, we report the experimental realization of QCC eliminating the need for coincidence detection, where the GHZ state is constructed by correlating detection events occurring within the coherence time, thereby greatly enhancing the success probability of GHZ-state measurement. Meanwhile, to establish and maintain high-visibility GHZ measurement among three independent users, we developed a three-party phase compensation scheme combined with precise temporal and polarization alignment within a time-bin-phase encoding framework. Furthermore, we designed an efficient pairing strategy to simplify subsequent data processing and enhance processing efficiency. Based on these techniques, we successfully performed QCC experiments over total channel losses of 66.3 dB, corresponding to 331.5 km of commercial fiber (0.2 dB/km), achieving secure key rates of 5.4 bit/s, whereas previous QCC experiments have been limited to 100 km. The results surpass the multi-user repeaterless bound in quantum networks, establishing a new regime of scalable, multi-user quantum communication and paving the way for metropolitan quantum networks.

quant-ph

Room-Temperature Electrical Readout of Spin Defects in van der Waals Materials

Negatively charged boron vacancy ($\mathrm{V_B^-}$) in hexagonal boron nitride (hBN) is the most extensively studied room-temperature quantum spin system in two-dimensional (2D) materials. Nevertheless, the current effective readout of $\mathrm{V_B^-}$ spin states is carried out by systematically optical methods. This limits their exploitation in compact and miniaturized quantum devices, which would otherwise hold substantial promise to address quantum sensing and quantum information tasks. In this study, we demonstrated a photoelectric spin readout technique for $\mathrm{V_B^-}$ spins in hBN. The observed photocurrent signals stem from the spin-dependent ionization dynamics of boron vacancies, mediated by spin-dependent non-radiative transitions to a metastable state. We further extend this electrical detection technique to enable the readout of dynamical decoupling sequences, including the Carr-Purcell-Meiboom-Gill (CPMG) protocols, and of nuclear spins via electron-nuclear double resonance. These results provide a pathway toward on-chip integration and real-field exploitation of quantum functionalities based on 2D material platforms.

quant-ph

Observation of Ferromagnetic Phase in the Second Moir\'e Band of Twisted MoTe2

Flat bands and electron correlation in moir\'e lattices give rise to many exotic phases, including Mott insulators, superconductivity, and topological states. Within the first moir\'e band, integer and fractional quantum anomalous Hall effects have been observed in twisted bilayer MoTe2 (tMoTe2) at one hole doping and fractional doping per moir\'e unit cell, respectively. When the second moir\'e band is fully hole doped, quantum spin Hall insulator has also been reported in tMoTe2 at a certain twist angle. Exotic topological states together with ferromagnetic (FM) states in the high moir\'e band can potentially exist as well. In this study, we report the observation of a FM phase in the second moir\'e band in tMoTe2. The FM phase can be tuned by both the doping level and displacement field. At filling around 2.58 holes per moir\'e unit cell, the FM phase reaches a Curie temperature of 3.5 K. A large displacement field can suppress the FM phase, like the FM phase at the filling of -1. Our results demonstrate the realization of time-reversal symmetry-breaking states in the higher moir\'e bands in tMoTe2.

cond-mat.mes-hall

Robust Nuclear Spin Polarization via Ground-State Level Anti-Crossing of Boron Vacancy Defects in Hexagonal Boron Nitride

Nuclear spin polarization plays a crucial role in quantum information processing and quantum sensing. In this work, we demonstrate a robust and efficient method for nuclear spin polarization with boron vacancy ($\mathrm{V_B^-}$) defects in hexagonal boron nitride (h-BN) using ground-state level anti-crossing (GSLAC). We show that GSLAC-assisted nuclear polarization can be achieved with significantly lower laser power than excited-state level anti-crossing, making the process experimentally more viable. Furthermore, we have demonstrated direct optical readout of nuclear spins for $\mathrm{V_B^-}$ in h-BN. Our findings suggest that GSLAC is a promising technique for the precise control and manipulation of nuclear spins in $\mathrm{V_B^-}$ defects in h-BN.

quant-ph

Quantum metric-induced nonlinear transport in a topological antiferromagnet

The Berry curvature and quantum metric are the imaginary part and real part, respectively, of the quantum geometric tensor which characterizes the topology of quantum states. The former is known to generate a zoo of important discoveries such as quantum Hall effect and anomalous Hall effect (AHE), while the consequences of the quantum metric have rarely been probed by transport. In this work, we observed quantum metric induced nonlinear transport, including both nonlinear AHE and diode-like nonreciprocal longitudinal response, in thin films of a topological antiferromagnet, MnBi$_2$Te$_4$. Our observation reveals that the transverse and longitudinal nonlinear conductivities reverse signs when reversing the antiferromagnetic order, diminish above the N\'eel temperature, and are insensitive to disorder scattering, thus verifying their origin in the band structure topology. They also flip signs between electron and hole-doped regions, in agreement with theoretical calculations. Our work provides a pathway to probe the quantum metric through nonlinear transport and to design magnetic nonlinear devices.

cond-mat.mes-hall

Experimental demonstration of Quantum Overlapping Tomography

Quantum tomography is one of the major challenges of large-scale quantum information research due to the exponential time complexity. In this work, we develop and apply a Bayesian state estimation method to experimentally demonstrate quantum overlapping tomography [Phys. Rev. Lett. \textbf{124}, 100401 (2020)], a scheme intent on characterizing critical information of a many-body quantum system in logarithmic time complexity. By comparing the measurement results of full state tomography and overlapping tomography, we show that overlapping tomography gives accurate information of the system with much fewer state measurements than full state tomography.

quant-ph

Experimental implementation of Hardy-like quantum pigeonhole paradoxes

We present the general Hardy-like quantum pigeonhole paradoxes for \textit{n}-particle states, and find that each of such paradoxes can be simply associated to an un-colorable solution of a specific vertex-coloring problem induced from the projected-coloring graph (a kind of unconventional graph). Besides, as a special kind of Hardy's paradox, several kinds of Hardy-like quantum pigeonhole paradoxes can even give rise to higher success probability in demonstrating the conflict between quantum mechanics and local or noncontextual realism than the previous Hardy's paradoxes. Moreover, not only multi-qubit states, but high-dimensional states can exhibit the paradoxes. In contrast to only one type of contradiction presented in the original quantum pigeonhole paradox, two kinds of three-qubit projected-coloring graph states as the minimal illustration are discussed in our work, and an optical experiment to verify such stronger paradox is performed. This quantum paradox provides innovative thoughts and methods in exploring new types of stronger multi-party quantum nonlocality and may have potential applications in multi-party untrusted communications and device-independent random number generation.

quant-ph

Quantum interference of resonance fluorescence from Germanium-vacancy color centers in diamond

Resonance fluorescence from a quantum emitter is an ideal source to extract indistinguishable photons. By using the cross polarization to suppress the laser scattering, we observed resonance fluorescence from GeV color centers in diamond at cryogenic temperature. The Fourier-transform-limited linewidth emission with $T_2/2T_1\sim0.86$ allows for two-photon interference based on single GeV color center. Under pulsed excitation, the 24 ns separated photons exhibit a Hong-Ou-Mandel visibility of $0.604\pm0.022$, while the continuous-wave excitation leads to a coalescence time window of 1.05 radiative lifetime. Together with single-shot readout of spin states, it paves the way towards building a quantum network with GeV color centers in diamond.

quant-ph

Multiparameter simultaneous optimal estimation with an SU(2) coding unitary evolution

In a ubiquitous $SU(2)$ dynamics, achieving the simultaneous optimal estimation of multiple parameters is significant but difficult. Using quantum control to optimize this $SU(2)$ coding unitary evolution is one of solutions. We propose a method, characterized by the nested cross-products of the coefficient vector $\mathbf{X}$ of $SU(2)$ generators and its partial derivative $\partial_\ell \mathbf{X}$, to investigate the control-enhanced quantum multiparameter estimation. Our work reveals that quantum control is not always functional in improving the estimation precision, which depends on the characterization of an $SU(2)$ dynamics with respect to the objective parameter. This characterization is quantified by the angle $\alpha_\ell$ between $\mathbf{X}$ and $\partial_\ell \mathbf{X}$. For an $SU(2)$ dynamics featured by $\alpha_\ell=\pi/2$, the promotion of the estimation precision can get the most benefits from the controls. When $\alpha_\ell$ gradually closes to $0$ or $\pi$, the precision promotion contributed to by quantum control correspondingly becomes inconspicuous. Until a dynamics with $\alpha_\ell=0$ or $\pi$, quantum control completely loses its advantage. In addition, we find a set of conditions restricting the simultaneous optimal estimation of all the parameters, but fortunately, which can be removed by using a maximally entangled two-qubit state as the probe state and adding an ancillary channel into the configuration. Lastly, a spin-$1/2$ system is taken as an example to verify the above-mentioned conclusions. Our proposal sufficiently exhibits the hallmark of control-enhancement in fulfilling the multiparameter estimation mission, and it is applicable to an arbitrary $SU(2)$ parametrization process.

quant-ph

Excited-state optically detected magnetic resonance of spin defects in hexagonal boron nitride

Negatively charged boron vacancy (VB-) centers in hexagonal boron nitride (hBN) are promising spin defects in a van der Waals crystal. Understanding the spin properties of the excited state (ES) is critical for realizing dynamic nuclear polarization. Here, we report zero-field splitting in the ES of DES = 2160 MHz and an optically detected magnetic resonance (ODMR) contrast of 12% at cryogenic temperature. The ES has a g-factor similar to the ground state. The ES photodynamics is further elucidated by measuring the level anti-crossing of the VB- defects under varying external magnetic fields. In contrast to nitrogen vacancy (NV-) centers in diamond, the emission change caused by excited-state level anti-crossing (ESLAC) is more prominent at cryo-temperature than at room temperature. Our results provide important information for utilizing the spin defects of hBN in quantum technology.

cond-mat.mes-hall

Quantum state transfer between two photons with polarization and orbital angular momentum via quantum teleportation technology

Quantum teleportation is a useful quantum information technology to transmit quantum states between different degrees of freedom. We here report a quantum state transfer experiment in the linear optical system, transferring a single photon state in the polarization degree of freedom (DoF) to another photon in the orbital angular momentum (OAM) quantum state via a biphoton OAM entangled channel. Our experimental method is based on quantum teleportation technology. The differences between ours and the original teleportation scheme is that the transfer state is known in ours, and our method is for different particles with different DoFs while the original one is for different particles with same DoF. Besides, our present experiment is implemented with a high Bell-efficiency since each of the four hybrid-entangled Bell states can be discriminated. We use six states of poles of the Bloch sphere to test our experiment, and the fidelity of the quantum state transfer is $91.8\pm1.3\%$.

quant-ph

Experimental Demonstration of a Quantum Controlled-SWAP Gate with Multiple Degrees of Freedom of a Single Photon

Optimizing the physical realization of quantum gates is important to build a quantum computer. The controlled-SWAP gate, also named Fredkin gate, can be widely applicable in various quantum information processing schemes. In the present research, we propose and experimentally implement quantum Fredkin gate in a single-photon hybrid-degrees-of-freedom system. Polarization is used as the control qubit, and SWAP operation is achieved in a four-dimensional Hilbert space spanned by photonic orbital angular momentum. The effective conversion rate $\mathcal{P}$ of the quantum Fredkin gate in our experiment is $(95.4\pm 2.6)\%$. Besides, we find that a kind of Greenberger-Horne-Zeilinger-like states can be prepared by using our quantum Fredkin gate, and these nonseparale states can show its quantum contextual characteristic by the violation of Mermin inequality. Our experimental design and coding method are useful for quantum computing and quantum fundamental study in high-dimensional and hybrid coding quantum systems.

quant-ph

Realization of a deterministic quantum Toffoli gate with a single photon

Quantum controlled-logic gates, including controlled NOT gate and Toffoli gate, play critical roles in lots of quantum information processing schemes. We design and experimentally demonstrate deterministic Toffoli gate by utilizing orbital-angular-momentum and polarization degrees of freedom of a single photon. In addition, we generate Bell states by using the controlled NOT gate. The effective conversion rate of the Toffoli gate in our experiment is $(95.1\pm3.2)\%$. Furthermore, our experimental setup does not require any auxiliary photons and probabilistic post selections.

quant-ph

Verification of Kochen-Specker-type quantum contextuality with a single photon

Contextuality provides one of the fundamental characterizations of quantum phenomena, and can be used as a resource in lots of quantum information processing. In this paper, we summarize and derive some equivalent noncontextual inequalities from different noncontextual models of the proofs for Kochen-Specker theorem based on Greenberger-Horne-Zeilinger states. These noncontextual inequalities are equivalent up to some correlation items which hold both for noncontextual hidden variable theories and quantum mechanics. Therefore, using single-photon hyperentangled Greenberger-Horne-Zeilinger states encoded by spin, path and orbital angular momentum, we experimentally verify several state-dependent noncontextual models of the proofs for the Kochen-Specker theorem by testing an extreme simplest Mermin-like inequality.

quant-ph

Experimental Demonstration of Efficient High-dimensional Quantum Gates with Orbital Angular Momentum

Quantum gates are essential for the realization of quantum computer and have been implemented in various types of two-level systems. However, high-dimensional quantum gates are rarely investigated both theoretically and experimentally even that high-dimensional quantum systems exhibit remarkable advantages over two-level systems for some quantum information and quantum computing tasks. Here we experimentally demonstrate the four-dimensional X gate and its unique higher orders with the average conversion efficiency 93\%. All these gates are based on orbital-angular-momentum degree of freedom of single photons. Besides, a set of controlled quantum gates is implemented by use of polarization degree of freedom. Our work is an important step towards the goal of achieving arbitrary high-dimensional quantum circuit and paves a way for the implementation of high-dimensional quantum communication and computation.

quant-ph