arXiv subjects

Shinsuke Haze

Publications and source records attributed to Shinsuke Haze.

14 recordsLinked to original sources

arXiv2026

Observation of $\Pi$-symmetry ultralong-range Rydberg molecules

We observe weakly-bound $\Pi$-symmetry electronic states in the spectroscopy of $^{87}$Rb$(nP_{3/2})$+$^{87}$Rb($5S_{1/2}$) ultralong-range Rydberg molecules. We detect these molecules in Rydberg states having principal quantum number $13\le n \le 16$. Their $\Pi$-state character is unambiguously identified via their observed multiplet structure: the $2F+1$ magnetic sublevels of the ground-state rubidium atom separate, as in the Zeeman effect, because of the spin-spin coupling between the Rydberg and valence electrons. We find a rapid decrease in the molecular binding energy $\propto (n-\mu_{P_{3/2}})^{-11}$, where $\mu_{P_{3/2}}$ is the quantum defect, indicating that the low-$n$ regime of Rydberg states is ideally suited for studies of $\Pi$-symmetry molecules. Our observations are in good agreement with Green's function-based calculations for $14\le n\le 16$, with poorer agreement for $n=13$ hinting at the beginning of a breakdown of the Fermi pseudopotential approach at low $n$.

physics.atom-ph↗

arXiv2026

Precision probing of ionic-core transitions in alkaline-earth Rydberg atoms

We report precision spectroscopy of ionic-core transitions in alkaline-earth Rydberg atoms. We demonstrate high-resolution measurements of isotope shifts and hyperfine splitting of dipole transitions in ionic cores which have not been explored so far. A key element of this work is the reduction of the linewidth by more than two orders of magnitude enabled by dynamical control of Rydberg electron's orbit which significantly enhances the spectral resolution. Furthermore, to unambiguously identify the frequency shift, we directly compare core ion's spectrum with a signal from a single trapped ion serving as an ultimate frequency reference. This work provides an important foundation for quantum control of inner-core transitions, which offer an useful tool in manipulating Rydberg atom as well as a sensitive probe for electron-core interactions in atomic and molecular systems.

physics.atom-ph↗

arXiv2025

Steering reaction flux by coupling product channels

We demonstrate a method for controlling the outcome of an ultracold chemical few-body reaction by redirecting a tunable fraction of reaction flux from one selected product channel to another one. In the reaction, three ultracold atoms collide to form a diatomic molecule. This product molecule can be produced in various internal states, characterizing the different product channels of the reaction. Our scheme relies on the coupling between two such product channels at an avoided molecular energy level crossing in the presence of an external magnetic field. The degree of coupling can be set by the magnetic field strength and allows for a widely tunable flux control between the two channels. This scheme is quite general and also holds great promise for a large variety of chemical processes with diverse species, since molecular energy level crossings are ubiquitous in molecular systems and are often easily accessible by standard laboratory equipment.

physics.atom-ph↗

arXiv2024

Controlling few-body reaction pathways using a Feshbach resonance

Gaining control over chemical reactions on the quantum level is a central goal of the modern field of cold and ultracold chemistry. Here, we demonstrate a novel method to coherently steer reaction flux of a three-body recombination process across different product spin channels. For this, we employ a magnetically-tunable Feshbach resonance to admix, in a controlled way, a specific spin state to the reacting collision complex. This allows for the control of the reaction flux into the admixed spin channel, which can be used to significantly change the reaction products. Furthermore, we also investigate the influence of an Efimov resonance on the reaction dynamics. We find that while the Efimov resonance can be used to globally enhance three-body recombination, the relative flux between the reaction channels remains unchanged. Our control scheme is general and can be extended to other reaction processes. It also provides new opportunities in combination with other control schemes, such as quantum interference of reaction paths.

cond-mat.quant-gas↗

arXiv2022

Energy-scaling of the product state distribution for three-body recombination of ultracold atoms

Three-body recombination is a chemical reaction where the collision of three atoms leads to the formation of a diatomic molecule. In the ultracold regime it is expected that the production rate of a molecule generally decreases with its binding energy $E_b$, however, its precise dependence and the physics governing it have been left unclear so far. Here, we present a comprehensive experimental and theoretical study of the energy dependency for three-body recombination of ultracold Rb. For this, we determine production rates for molecules in a state-to-state resolved manner, with the binding energies $E_b$ ranging from 0.02 to 77 GHz$\times h$. We find that the formation rate approximately scales as $E_b^{-\alpha}$, where $\alpha$ is in the vicinity of 1. The formation rate typically varies only within a factor of two for different rotational angular momenta of the molecular product, apart from a possible centrifugal barrier suppression for low binding energies. In addition to numerical three-body calculations we present a perturbative model which reveals the physical origin of the energy scaling of the formation rate. Furthermore, we show that the scaling law potentially holds universally for a broad range of interaction potentials.

physics.atom-ph↗

arXiv2021

Spin-conservation propensity rule for three-body recombination of ultracold Rb atoms

We explore the physical origin and the general validity of a propensity rule for the conservation of the hyperfine spin state in three-body recombination. This rule was recently discovered for the special case of $^{87}$Rb with its nearly equal singlet and triplet scattering lengths. Here, we test the propensity rule for $^{85}$Rb for which the scattering properties are very different from $^{87}$Rb. The Rb$_2$ molecular product distribution is mapped out in a state-to-state fashion using REMPI detection schemes which fully cover all possible molecular spin states. Interestingly, for the experimentally investigated range of binding energies from zero to $\sim13\:\textrm{GHz}\times h$ we observe that the spin-conservation propensity rule also holds for $^{85}$Rb. From these observations and a theoretical analysis we derive an understanding for the conservation of the hyperfine spin state. We identify several criteria to judge whether the propensity rule will also hold for other elements and collision channels.

physics.atom-ph↗

arXiv2021

Long-range atom-ion Rydberg molecule: A novel molecular binding mechanism

We present a novel binding mechanism where a neutral Rydberg atom and an atomic ion form a molecular bound state at large internuclear distance. The binding mechanism is based on Stark shifts and level crossings which are induced in the Rydberg atom due to the electric field of the ion. At particular internuclear distances between Rydberg atom and ion, potential wells occur which can hold atom-ion molecular bound states. Apart from the binding mechanism we describe important properties of the long-range atom-ion Rydberg molecule, such as its lifetime and decay paths, its vibrational and rotational structure, and its large dipole moment. Furthermore, we discuss methods how to produce and detect it. The unusual properties of the long-range atom-ion Rydberg molecule give rise to interesting prospects for studies of wave packet dynamics in engineered potential energy landscapes.

physics.atom-ph↗

arXiv2020

Observation of spin-orbit-dependent electron scattering using long-range Rydberg molecules

We present experimental evidence for spin-orbit interaction of an electron as it scatters from a neutral atom. The scattering process takes place within a Rb$_2$ ultralong-range Rydberg molecule, consisting of a Rydberg atomic core, a Rydberg electron, and a ground state atom. The spin-orbit interaction leads to characteristic level splittings of vibrational molecular lines which we directly observe via photoassociation spectroscopy. We benefit from the fact that molecular states dominated by resonant $p$-wave interaction are particularly sensitive to the spin-orbit interaction. Our work paves the way for studying novel spin dynamics in ultralong-range Rydberg molecules. Furthermore, it shows that the molecular setup can serve as a microlaboratory to perform precise scattering experiments in the low-energy regime of a few meV.

cond-mat.quant-gas↗

arXiv2019

Stark spectroscopy of Rydberg atoms in an atom-ion hybrid trap

We report on Rydberg spectroscopy of ultracold atoms in an atom-ion hybrid trap for probing the electric fields in a mixture of atoms and ions. We obtain spectra which exhibit excitation gaps corresponding to avoided level crossings in the Stark map. From these measurements we can conclude that the ground state atoms experience electrical fields of up to 250 V/cm. There is, however, a difficulty in interpreting the results, because some data indicate that the electrical fields are produced by the ions while other data indicate that they stem from the Paul trap. We discuss possible scenarios for explaining the measured data, provide first measurements to check these scenarios, and propose methods to finally solve this puzzle.

physics.atom-ph↗

arXiv2018

Cooling dynamics of a single trapped ion via elastic collisions with small-mass atoms

We demonstrated sympathetic cooling of a single ion in a buffer gas of ultracold atoms with small mass. Efficient collisional cooling was realized by suppressing collision-induced heating. We attempt to explain the experimental results with a simple rate equation model and provide a quantitative discussion of the cooling efficiency per collision. The knowledge we obtained in this work is an important ingredient for advancing the technique of sympathetic cooling of ions with neutral atoms.

physics.atom-ph↗

arXiv2015

Charge-exchange collisions between ultracold fermionic lithium atoms and calcium ions

Charge exchange collisions between ultracold fermionic 6Li atoms and 40Ca+ ions are observed in the mK temperature range. The reaction product of the charge exchange collision is identified via mass spectrometry during which the motion of the ions is excited parametrically. The cross-sections of the charge exchange collisions between 6Li atoms in the ground state and 40Ca+ ions in the ground and metastable excited states are determined. Investigation of the inelastic collision characteristics in the atom-ion mixture is an important step toward ultracold chemistry based on ultracold atoms and ions.

physics.atom-ph↗

arXiv2013

Experimental realization of a quantum phase transition of polaritonic excitations

We report an experimental realization of the Jaynes-Cummings-Hubbard (JCH) model using the internal and radial phonon states of two trapped ions. An adiabatic transfer corresponding to a quantum phase transition from a localized insulator ground state to a delocalized superfluid (SF) ground state is demonstrated. The SF phase of polaritonic excitations characteristic of the interconnected Jaynes-Cummings (JC) system is experimentally explored, where a polaritonic excitation refers to a combination of an atomic excitation and a phonon interchanged via a JC coupling.

quant-ph↗

arXiv2013

Observation of elastic collisions between lithium atoms and calcium ions

We observed elastic collisions between laser-cooled fermionic lithium atoms and calcium ions at the energy range from 100 mK to 3 K. Lithium atoms in an optical-dipole trap were transported to the center of the ion trap using an optical tweezer technique, and a spatial overlap of the atoms and ions was realized in order to observe the atom-ion interactions. The elastic scattering rate was determined from the decay of atoms due to elastic collisions with ions. The collision-energy dependence of the elastic scattering cross-section was consistent with semi-classical collision theory.

physics.atom-ph↗

arXiv2011

Generation of a decoherence-free entangled state using a radio frequency dressed state

We propose the generation of entangled states with trapped calcium ions using a combination of an rf dressed state and a spin dependent force. Using this method, a decoherence-free entangled state of rf qubits can be directly generated and ideally its fidelity is close to unity. We demonstrate an rf entangled state with a fidelity of 0.68, which has a coherence time of more than 200 ms by virtue of the fact that it is an eigenstate with energy gaps between adjacent levels.Using the same technique, we also produce a qutrit-qutrit entangled state with a fidelity of 0.77, which exceeds the threshold value for separability of 2/3.

quant-ph↗