arXiv subjects

Shoukang Yang

Publications and source records attributed to Shoukang Yang.

4 recordsLinked to original sources

arXiv2026

Capture velocities for direct loading of heavy molecules into conveyor-belt magneto-optical traps

Conveyor-belt magneto-optical traps (CB-MOTs) use blue-detuned polarization-gradient forces to provide simultaneous cooling, confinement, and loading on type-II molecular transitions. Recent experiments with \baf{138} showed that this mechanism can directly load a slowed molecular beam with an efficiency exceeding that of a conventional red-detuned MOT. Here we use established optical-Bloch-equation force calculations and classical trajectory propagation to ask whether this direct-loading strategy should extend beyond the specific molecule used in the first demonstration. For \baf{138}, the calculation reproduces the experimentally observed trend that the CB-MOT capture velocity increases with laser intensity. We then apply the same framework to two closely related but experimentally distinct cases: \baf{137}, whose dense hyperfine structure complicates a conventional dual-frequency MOT, and \bah{138}, whose narrower linewidth and longer wavelength reduce the available radiative force. In both cases, the CB-MOT retains a broad region of nonzero capture velocity. These results identify the molecular conditions under which direct CB-MOT loading should remain effective and show that the dipole-force-dominated conveyor-belt mechanism provides a practical loading route for heavy laser-coolable molecules whose MOT performance is otherwise limited by photon recoil, scattering rate, or hyperfine complexity.

physics.atom-ph↗

arXiv2025

Optical pumping and laser slowing of a heavy molecule

Precision measurements of the electron's electric dipole moment (eEDM) are critical for testing fundamental symmetries in particle physics, and heavy polar molecules-such as barium monofluoride (BaF)-have emerged as promising candidates for advancing the sensitivity. However, the achievement of a 3D magneto-optical trap (MOT) required slowing BaF molecules to near-zero velocity by scattering over 10^4 photons per molecule, demanding a quasi-cycling transition with minimal leakage. We present a detailed study of the leakage channels, including higher vibrational and rotational states. By combining microwave remixing with optical pumping of rotational and vibrational dark states, we reduced the total leakage fraction to 10^-5. Using frequency-chirped laser slowing, we slowed a subset of buffer-gas-cooled BaF molecules from approximately 80 m/s to near-zero velocity, which is critical for efficient MOT loading. This work establishes the technical foundation for precision eEDM measurements using laser-cooled heavy molecules.

physics.atom-ph↗

arXiv2025

Blue-detuned Magneto-optical Trap of BaF molecules

We report the realization of a blue-detuned magneto-optical trap (BDM) of BaF molecules. The (1 + 1) type BDM and (1 + 2) type conveyor-belt MOT are explored. While the (1+1) BDM provides only weak trapping force, the conveyor-belt MOT significantly compresses the molecular cloud, achieving a radius of 320(20) {\mu}m, a temperature of 240(60) {\mu}K, and a peak density of 1.3{\times}10^7 cm^{-3}, representing a significant improvement over the red MOT. Interestingly, the conveyor-belt MOT of BaF exhibits a large capture velocity, and the loading efficiency from red MOT reaches near unity even without gray molasses. We confirm this by directly loading slowed molecules into the conveyor-belt MOT.

physics.atom-ph↗

arXiv2024

Three-dimensional Magneto-optical Trapping of Barium Monofluoride

As a heavy molecule, barium monofluoride (BaF) presents itself as a promising candidate for measuring permanent electric dipole moment. The precision of such measurements can be significantly enhanced by utilizing a cold molecular sample. Here we report the realization of three-dimensional magneto-optical trapping (MOT) of BaF molecules. Through the repumping of all the vibrational states up to $v=3$, and rotational states up to $N=3$, we effectively close the transition to a leakage level lower than $10^{-5}$. This approach enables molecules to scatter a sufficient number of photons required for laser cooling and trapping. By employing a technique that involves chirping the slowing laser frequency, BaF molecules are decelerated to near-zero velocity, resulting in the capture of approximately $3\times 10^3$ molecules in a dual-frequency MOT setup. Our findings represent a significant step towards the realization of ultracold BaF molecules and the conduct of precision measurements with cold molecules.

physics.atom-ph↗