arXiv subjects

Shoumik Debnath

Publications and source records attributed to Shoumik Debnath.

7 recordsLinked to original sources

arXiv2026

Polarization-Selective Near-Perfect Absorption via Mie-Type Resonance in van der Waals Anisotropic ReS$_2$/$α$-MoO$_3$/Au Heterostructure

We investigate polarization-selective absorption in a visible-wavelength heterostructure consisting of a ReS$_2$ stripe grating, an $α$-MoO$_3$ spacer, and an Au back-reflector using finite-difference time-domain simulations. For an optimized geometry with a grating period of 500 nm, stripe width of 250 nm, and ReS$_2$ thickness of 80 nm, the structure exhibits near-unity absorption of 99.99\% at 650.5 nm under TE-polarized illumination. The resonant field is concentrated near the outer edges of the ReS$_2$ stripe, while absorption power density is localized in the same region, consistent with a localized edge mode. The absorption response depends strongly on polarization, producing a TE--TM resonance separation of 16.2 nm. Replacing either the biaxial ReS$_2$ layer or the anisotropic $α$-MoO$_3$ spacer with isotropic equivalents substantially modifies the spectral response and reduces the polarization-dependent wavelength separation. In addition, rotating the crystal orientation of the ReS$_2$/$α$-MoO$_3$ stack shifts both the resonance wavelength and peak absorption without changing the device geometry. The results show that the combination of anisotropic resonator and spacer layers provides an effective means of controlling resonant absorption and polarization selectivity in van der Waals photonic structures.

physics.optics↗

arXiv2026

An Integrated DFT-FDTD Design of Plasmon-Enhanced Lead-Free $CsSn$$_x$$Ge$$_{1-x}$$I$$_3$ Perovskite LEDs

CsSn$_x$Ge$_{1-x}$I$_3$ as lead-free perovskites are promising for next generation NIR emitting perovskite LEDs due to their tunable bandgaps and stability. However, they suffer from poor light extraction efficiency, and accurate composition-specific optical data for these materials remain scarce. This study presents a DFT-FDTD framework to optimize light extraction via compositional tuning and plasmonic enhancement. First, DFT calculations were performed to obtain composition-specific complex refractive index and extinction coefficient values for $x = 0, 0.25, 0.5, 0.75$, and $1$. Results show bandgap increased from 1.331 eV for CsSnI$_3$ to 1.927 eV for CsGeI$_3$ with increasing Ge content, while refractive index ranges from 2.2 to 2.6 across compositions. These optical constants were then used as inputs for FDTD simulations of a PeLED structure with optimized Au/SiO$_2$ core-shell nanorods for plasmonic enhancement. A 12.1-fold Purcell enhancement was achieved for CsSn$_{0.25}$Ge$_{0.75}$I$_3$, while light extraction efficiency reached 25% for CsSn$_{0.5}$Ge$_{0.5}$I$_3$. LEE enhancement of 36% was obtained for CsSnI$_3$, and spectral overlap between emitter and plasmon resonance reached 96% for Sn-rich compositions. Design guidelines indicate CsSn$_{0.5}$Ge$_{0.5}$I$_3$ offers optimal balance of extraction efficiency (25%), Purcell enhancement (5.3$\times$), spectral overlap (93%), and oxidation stability for wearable and flexible optoelectronic applications, while CsSn$_{0.25}$Ge$_{0.75}$I$_3$ is recommended for applications prioritizing spontaneous emission rate.

physics.optics↗

arXiv2026

Polarization-Multiplexed Spatial Differentiation and Filtering Driven by van der Waals Birefringence

We report that the biaxial birefringence of $\alpha$-MoO$_3$ can activate two spectrally distinct quasi-bound states in the continuum (quasi-BICs) within a single symmetric TiO$_2$ nanobar-pair metasurface, with each resonance governed by a different crystallographic axis pair of the van der Waals crystal. With a full 60\,nm $\alpha$-MoO$_3$ gap fill, a TE resonance at 883.9\,nm ($Q=92$, Fano $q=0.090$) and a TM resonance at 923.2\,nm ($Q=31$, Fano $q=0.393$) are obtained. The Q ratio follows the inverse-square permittivity contrast, $Q\propto(\Delta\varepsilon)^{-2}$, calibrated across both polarization channels. Oblique-incidence sweeps show that the TE channel acts as a dual-null spatial highpass filter with a broadband stopband ($|H|<0.13$ for $|k_x|\leq0.63\,\mu$m$^{-1}$, $T_\mathrm{bg}=0.962$), while the TM channel transfers as $|H|\propto|k_x|$ ($R^2=0.94$), consistent with first-order spatial differentiation. Both operations are verified on a USAF~1951 resolution chart processed in a simulated 4$f$ framework. Channel selection is purely by input polarization angle with no structural modification.

physics.optics↗

arXiv2026

van der Waals Crystal Anisotropy Controls Dual-Channel Refractive Index Sensing in a TiO$_{2}$/$\alpha$-MoO$_{3}$ Nanobar Metasurface

Filling the gap of a TiO$_2$ nanobar-pair metasurface with $\alpha$-MoO$_3$, a biaxial orthorhombic crystal, produces two high-$Q$ Fano resonances with asymmetric quality factors: $Q_{\mathrm{TE}}=87$ at 863.3 nm and $Q_{\mathrm{TM}}=31$ at 960.1 nm, separated by 97 nm. The same device with amorphous or crystalline Sb$_2$S$_3$, both isotropic, yields comparable quality factors in both channels, confirming that the $Q$-ratio asymmetry originates in the biaxial crystal symmetry of $\alpha$-MoO$_3$ rather than the index magnitude of the fill. The two inequivalent permittivity contrasts of the orthorhombic lattice ($\Delta\varepsilon_{\beta\gamma}=0.983$ for TE, $\Delta\varepsilon_{\alpha\gamma}=2.420$ for TM) place each channel at a different point on the $Q\propto(\Delta\varepsilon)^{-2}$ scaling curve, consistent with quasi-BIC mode character. The TE channel delivers sensitivity $S=155.3$ nm RIU$^{-1}$, figure of merit 15.71 RIU$^{-1}$, and limit of detection $6.44\times10^{-5}$ RIU. TM delivers $S=139.1$ nm RIU$^{-1}$, figure of merit 4.44 RIU$^{-1}$, and limit of detection $7.19\times10^{-5}$ RIU. Simultaneous readout produces a polarization fingerprint with isotropic slope 0.896, deviations from which encode analyte optical anisotropy.

physics.optics↗

arXiv2026

Single-Device VOC Fingerprinting via Polarization-Selective Anisotropic BeS-Clad Silicon Microring Resonator

A silicon microring resonator with an anisotropic beryllium sulfide (BeS) cladding is proposed for polarization-selective detection of exhaled-breath volatile organic compound biomarkers. The anisotropic dielectric response of BeS enables the transverse-electric (TE) and transverse-magnetic (TM) modes to probe orthogonal components of the cladding permittivity tensor, generating two independent optical observables from a single device. Five clinically relevant biomarkers are investigated: acetone, isoprene, 4-hydroxyhexenal, 2-propenal, and benzene. First-principles optical constants are incorporated into three-dimensional finite-difference time-domain simulations to evaluate the sensing response. The TE mode exhibits a uniform resonance shift of 0.263 nm across all analytes and serves as a concentration reference channel, while the TM mode produces analyte-specific shifts ranging from 0.200 to 0.426 nm. A unique TM amplitude inversion is observed for benzene, enabling additional discrimination. The resulting dual-polarization response forms a two-dimensional optical fingerprint that distinguishes all five biomarkers without requiring a sensor array or multiple functionalized resonators. The device achieves quality factors of 4520 and 3151 for the TE and TM modes, respectively, with sensitivities up to 6.5 nm/RIU, figures of merit up to 14.9 RIU^-1, and detection limits as low as 1.5 mRIU. Cross-sensitivity analysis further shows that CO2 and H2O produce negative TM resonance shifts, separating interferents from target biomarkers in the fingerprint plane. The proposed platform demonstrates a compact route toward array-free photonic breath analysis using intrinsic cladding anisotropy.

physics.optics↗

arXiv2026

Inverse Design Validated Optimization of Lead-Free Cs$_3$Cu$_2$Cl$_5$ Visible-Light Microring Resonators Using a Coupled DFT-FDTD Framework

Microring resonators (MRRs) are indispensable for wavelength filtering, sensing, and on-chip signal routing in photonic integrated circuits, yet visible-wavelength implementations using environmentally benign materials remain scarce. We report a numerical design study of add-drop MRRs employing Cs$_3$Cu$_2$Cl$_5$, a lead-free all-inorganic halide with favorable optical properties in the visible spectral range. Wavelength-resolved refractive index (n) and extinction coefficient (k) of Cs$_3$Cu$_2$Cl$_5$, calculated using density functional theory (DFT), are used as direct inputs to three-dimensional finite-difference time-domain (FDTD) simulations. Independent parametric sweeps are performed over ring waveguide width (500-900 nm), coupling gap (150-300 nm), and bend radius (5-20 um). At the balanced operating point of 600 nm ring width, 200 nm gap, and 10 um radius, the device achieves a loaded quality factor Q approx 5386, a free spectral range of 11.3 nm, a drop-port extinction ratio of 32.2 dB, and a finesse of 95.8. The coupling-gap sweep reveals the full transition from over-coupled through critically coupled to under-coupled operation, with the critical point occurring near 200 nm. A pronounced bending-loss threshold is observed between 5 and 10 um, below which all performance metrics degrade rapidly. These results provide the first systematic geometry-performance map for Cs$_3$Cu$_2$Cl$_5$ based microring resonators. Cross-platform validation using Tidy3D reproduces the spectral characteristics of the optimized device, and inverse design of the bus coupling region yields an additional 3 percent improvement in drop-port power transfer.

physics.optics↗

arXiv2026

Composition-Dependent Plasmon-Enhanced Emission in Lead-Free Cs$_3$Cu$_2$X$_5$ Halides: A DFT--FDTD Study

Lead-free Cs$_3$Cu$_2$X$_5$ (X = Cl, Br, I) halides exhibit high photoluminescence quantum yields and excellent ambient stability, yet light-emitting devices based on these materials remain limited by poor optical outcoupling. In this work, we develop an integrated density functional theory (DFT) and finite-difference time-domain (FDTD) framework to establish quantitative links between halide composition, wavelength-dependent optical constants, and plasmonic enhancement. First-principles calculations are used to obtain composition-specific refractive index (n) and extinction coefficient (k) spectra, which are directly implemented into three-dimensional FDTD simulations of a complete PeLED stack incorporating Ag/SiO$_2$ core--shell nanostructures. Among the investigated compositions, Cs$_3$Cu$_2$Cl$_5$ demonstrates the strongest plasmonic response, achieving a 4.4$\times$ Purcell enhancement and 30\% light extraction efficiency (LEE) using optimized nanorods. The superior performance originates from its lower refractive index, which reduces dielectric screening and improves near-field coupling. Cs$_3$Cu$_2$Br$_5$ exhibits the highest spectral overlap ($J_{\mathrm{cos}} = 0.955$) but yields moderate extraction (26%) due to increased optical confinement. Cs$_3$Cu$_2$I$_5$ requires a nanosphere geometry and shows limited enhancement, with LEE restricted to 10%. Distance-ependent analysis reveals composition-specific optimal emitter--plasmon separations, ranging from 8--12 nm for Cs$_3$Cu$_2$Br$_5$ to approximately 15 nm for Cs$_3$Cu$_2$Cl$_5$. These results provide composition-dependent design guidelines for plasmon-enhanced lead-free PeLEDs and highlight the critical role of accurate optical constants in predictive device optimization.

physics.optics↗