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Shouvik Sur

Publications and source records attributed to Shouvik Sur.

At least 19 recordsLinked to original sources

Quantum Fisher information of magnetic quantum phase transition on Kondo lattice

Strange metals exemplify highly collective quantum many-body systems that call for new means of characterization, and there is considerable potential for quantum information approaches contributing to the cause. We investigate multipartite entanglement across the quantum phase transition of a Kondo lattice model using the quantum Fisher information (QFI). We show that the QFI associated with the spin components transverse to the order parameter characterizes the destruction of heavy quasiparticles in the Kondo-destroyed magnetic-ordered phase. The physical origin of this observation is elucidated through an analysis of the antiferromagnetic Heisenberg model. We propose to test the results in terms of both unpolarized and polarized inelastic neutron scattering measurements in the ordered part of the heavy fermion phase diagram. Our findings illustrate how different operators of a many-body system can be employed to not only witness multipartite entanglement in different sectors and but also elucidate the overall physics across different parts of the phase diagram.

cond-mat.str-el

Nonperturbative Nonlinear Hall Effect in Nonequilibrium Steady States

The nonlinear Hall effect in quantum materials has attracted broad interest, yet most existing studies focus on the weak-field, perturbative regime. Here we develop a nonperturbative approach based on nonequilibrium steady-state Green's functions for dc-field-driven lattice systems, with dissipation and interactions incorporated through self-energies beyond the constant relaxation-time approximation and interband transitions treated alongside their intraband counterparts. Applied to a two-band semimetal model, our approach provides direct access to the strong-field Hall response beyond the nonperturbative crossover where the edge of the nonequilibrium distribution reaches Berry-curvature hot spots, a regime in which constant relaxation-time estimates and Berry curvature dipole calculations become unreliable. We further demonstrate that interaction and electron-phonon self-energies within dynamical mean-field theory can substantially change the Hall signal. Our framework enables quantitative simulations of nonequilibrium nonlinear Hall phenomena and provides guidance for strong-field transport experiments.

cond-mat.str-el

Dual-use quantum hardware for quantum resource generation and energy storage

Efficient generation of quantum resources is a central objective of modern quantum technological platforms. Independently, quantum batteries have emerged as nanoscale devices that utilize collective quantum effects to store energy with a charging advantage over classical strategies. Here, we show a direct connection between these two pursuits: protocols for fast generation of resourceful quantum states can simultaneously charge a quantum battery with a collective advantage, and conversely, a quantum battery protocol with a charging advantage rapidly produces resource-rich states. Using this connection, we propose an integrated hardware protocol on superconducting circuits in which each experimental run can interchangeably accomplish either quantum battery charging, or quantum sensing through generation of metrologically useful states. Our results establish that quantum resources and stored energy are distinct yet simultaneously-producible quantities within the same dynamics. This opens the door to polymorphic quantum architectures that dynamically switch between sensing and energy-storage functions, thereby producing additional functionalities without extra hardware cost.

quant-ph

Perturbative Kondo destruction and global phase diagram of heavy fermion metals

Strange metals represent a foundational problem in quantum condensed matter physics, and heavy fermion systems provide a canonical setting to advance a general understanding. The concept of a Kondo destruction quantum critical point is widely invoked to describe the competition of the Kondo effect and the local-moment magnetism. Here, we develop a unified field-theoretic approach, analyzing this competition from a rare approach that is anchored by the magnetically ordered side. Our analysis reveals, for the first time within a renormalization group framework, a quantum critical point across which the Kondo effect goes from being destroyed to dominating. Our findings elucidate not only the Kondo destruction quantum criticality but also an accompanying global phase diagram of heavy fermion metals.

cond-mat.str-el

Amplified response of cavity-coupled quantum-critical systems

A quantum critical point develops when matter undergoes a continuous transformation between distinct ground states at absolute zero. It hosts pronounced quantum fluctuations, which render the system highly susceptible to external perturbations. While light-matter coupling has rapidly moved forward as a means to probe and control quantum materials, the capacity of quantum critical fluctuations in the photon-mediated responses has been largely unexplored. Here we advance the notion that directly coupling a quantum critical mode to a quantized cavity field dramatically facilitates the realization of the elusive superradiant phase transition in equilibrium, circumventing at once the key obstacles that have prevented its attainment in spite of decades of pursuit. The superradiant phase transition develops far below the ultrastrong regime of light-matter couplings, and the transition is accompanied by the hybrid system showing strongly enhanced intrinsic squeezing and amplified quantum Fisher information. We also identify candidate cavity quantum materials platforms for validating the proposed effect. Our findings suggest a general principle by which quantum criticality amplifies the response to cavity photons. They also demonstrate that cavity coupling accesses the elevated quantum entanglement of the underlying matter at quantum criticality, thereby pointing to a pathway towards realizing the potential of highly collective quantum materials to expand the capacities of quantum information science.

cond-mat.str-el

Suppression of shot noise at a Kondo destruction quantum critical point

Strange metal behavior has been observed in an expanding list of quantum materials, with heavy fermion metals serving as a prototype setting. Among the intriguing questions is the nature of charge carriers; there is an increasing recognition that the quasiparticles are lost, as captured by Kondo destruction quantum criticality. Among the recent experimental advances is the measurement of shot noise in a heavy-fermion strange metal. We are thus motivated to study current fluctuations by advancing a minimal Bose-Fermi Kondo lattice model, which admits a well-defined large-$N$ limit. Showing that the model in equilibrium captures the essential physics of Kondo destruction, we proceed to derive quantum kinetic equations and compute shot noise to the leading nontrivial order in $1/N$. Our results reveal a strong suppression of the shot noise at the Kondo destruction quantum critical point, thereby providing the understanding of the striking experiment. Broader implications of our results are discussed.

cond-mat.str-el

Nonlinear thermal and thermoelectric transport from quantum geometry

Quantum geometry may enable the development of quantum phases ranging from superconductivity to correlated topological states. One powerful probe of quantum geometry is the nonlinear Hall response which detects Berry curvature dipole in systems with time-reversal invariance and broken inversion symmetry. With broken time-reversal symmetry, this response is also associated with quantum metric dipole. Here we investigate nonlinear thermal and thermoelectric responses, which provide a wealth of new information about quantum geometry. In particular, we uncover a web of connections between these quantities that parallel the standard Wiedemann-Franz and Mott relations. Implications for the studies of a variety of topological systems, including Weyl-Kondo semimetals and Bernal bilayer graphene, are discussed.

cond-mat.mes-hall

Correlated flat-band physics in a bilayer kagome metal based on compact molecular orbitals

Flat bands, when located close to the Fermi energy, can considerably enhance the influence of electron correlations on the low energy physics in kagome and other frustrated-lattice metals. A major challenge in describing the interaction effects in such bulk materials is that the flat band is often intermixed with a large number of other bands. Here we show that the recently introduced notion of compact molecular orbitals (CMOs) enable a path forward in describing the dominant effect of the Coulomb interactions in spite of the complexity of the bandstructure. Our materials-based analysis allows for the understanding of the scanning-tunneling-microscopy experiment [J. C. Souza et al., preprint (2024)] of the bilayer kagome metal Ni$_3$In in terms of the CMO notion. From the resulting CMO, an effective Anderson lattice model can be set up. This CMO-based approach enables the calculation of correlation effects that is difficult to do based on the atomic orbitals. Furthermore, it suggests an enriched phase diagram for the strange metal physics of the kagome metal, which can be tested by future experiments. We discuss the implications of our results for the general correlation physics of flat band systems and beyond.

cond-mat.str-el

Correlated Hopf insulators

Hopf insulators represent an exceptional class of topological matter unanticipated by the periodic table of topological invariants. These systems point to the existence of previously unexplored states of matter with unconventional topology. In this work, we take a step toward exploring this direction by investigating correlation-driven instabilities of Hopf insulators. Organizing our analysis around the topological quantum critical point that separates the Hopf insulating phase from a trivial insulator, we demonstrate the emergence of unconventional Weyl semimetallic and topological insulating states. Notably, the Weyl semimetal supports non-reciprocal superconductivity and a Bogoliubov-Fermi surface, potentially providing a novel framework for realizing the superconducting diode effect. Finally, we highlight the interconnectedness of the effective descriptions of correlated Hopf insulators, two-dimensional quadratic band-touching semimetals, and Luttinger semimetals.

cond-mat.str-el

Fully nonequilibrium Hall response from Berry curvature

In topological materials, Berry curvature leads to intrinsic Hall responses. Focusing on time-reversal symmetric systems with broken inversion symmetry, a spontaneoous (zero magnetic field) Hall effect is expected to develop under an applied electric field. Motivated by recent developments in Weyl-Kondo semimetals, here we advance a fully nonequilibrium (FNE) Hall response due to the Berry curvature. In particular, we show that, while the spontaneous Hall current is quadratic in the previously described regime of weak electric field, due to the contribution from the dipole moment of the Berry curvature, the FNE Hall response for non-perturbative electric fields is not controlled by the Berry curvature dipole. Remarkably, the FNE Hall response resembles what happens in systems that break the microscopic time-reversal symmetry. We illustrate the universality of these results by comparing them with their counterparts in systems with any higher-multipole of the Berry curvature. The implications of our results for the understanding of strongly correlated topological semimetals are discussed.

cond-mat.mes-hall

Cubic Dirac Semimetals: General Theory and Application to Rare-Earth Magnets

Rare-earth magnets with parent cubic symmetry exhibit unique topological properties. However, the origin of these behaviors remains presently unclear. Here, we develop minimal models for Dirac semimetals (DSMs) with accidental band crossings and higher-order topology in cubic systems, incorporating candidate magnetic order to analyze bulk, surface, and hinge state characteristics. In certain cubic-symmetric DSMs, we identify an effective Z2 chiral symmetry which significantly impacts surface and hinge-localized states. Our results highlight distinct features in surface state dispersions, Fermi arcs, polarization dependence, and band splitting that correlate with photoemission data in rare-earth monopnictides. We also suggest candidate materials and experimental tests for further validation. These findings advance our understanding of surface states in rare-earth magnets with parent cubic symmetries and illuminate the role of DSM physics in these systems.

cond-mat.str-el

Superconductivity in twisted WSe$_2$ from topology-induced quantum fluctuations

Recently, superconductivity has been observed in twisted WSe$_2$ moir\'{e} structures (Xia et al., Nature 2024; Guo et al., Nature 2025). Its transition temperature is high, reaching a few percent of the Fermi temperature scale. Here, we advance a mechanism for superconductivity based on the notion that electronic topology enables quantum fluctuations in a suitable regime of intermediate correlations. In this regime, the Coulomb interaction requires that an active topological flat band and nearby wider bands are considered together. Compact molecular orbitals arise, which give rise to quantum fluctuations through topology-dictated hybridization with the other molecular orbitals. The hybridization competes with the active flat band's natural tendency towards static electronic ordering, thereby weakening the latter; we link this effect with certain salient observations by experiments. Furthermore, the competition yields a quantum critical regime where quasiparticles are lost. The corresponding quantum critical fluctuations drive superconductivity. Broader implications and new connections among correlated materials platforms are discussed.

cond-mat.str-el

Shot noise in coupled electron-boson systems

The nature of charge carriers in strange metals has become a topic of intense current investigation. Recent shot noise measurements in the quantum critical heavy fermion metal YbRh$_2$Si$_2$ revealed a suppression of the Fano factor that cannot be understood from electron-phonon scattering or strong electron correlations in a Fermi liquid, indicating loss of quasiparticles. The experiment motivates the consideration of shot noise in a variety of theoretical models in which quasiparticles may be lost. Here we study shot noise in systems with co-existing itinerant electrons and dispersive bosons, going beyond the regime where the bosons are on their own in thermal equilibrium. We construct the Boltzmann-Langevin equations for the coupled system, and show that adequate electron-boson couplings restore the Fano factor to its Fermi liquid value. Our findings point to the beyond-Landau form of quantum criticality as underlying the suppressed shot noise of strange metals in heavy fermion metals and beyond.

cond-mat.str-el

Electron correlations in the kagome flat band metal $\rm CsCr_3Sb_5$

Kagome metals offer a unique platform for investigating robust electron-correlation effects because of their lattice geometry, flat bands and multi-orbital nature. In the cases with active flat bands, recent theoretical studies have pointed to a rich phase diagram that contains not only electronic orders but also quantum criticality. Very recently, $\rm CsCr_3Sb_5$ has emerged as a strong candidate for exploring such new physics. Here, using effective tight-binding models obtained from ab initio calculations, we study the effects of electronic correlations and symmetries on the electronic structure of $\rm CsCr_3 Sb_5$. The effective tight-binding model and Fermi surface comprise multiple Cr-$d$ orbitals and Sb-$p$ orbitals. The introduction of Hubbard-Kanamori interactions leads to orbital-selective band renormalization dominated by the $d_{xz}$ band, concurrently producing emergent flat bands very close to the Fermi level. Our analysis sets the stage for further investigations into the electronic properties of $\rm CsCr_3Sb_5$, including electronic orders, quantum criticality and unconventional superconductivity, which promise to shed much new light into the electronic materials with frustrated lattices and bring about new connections with the correlation physics of a variety of strongly correlated systems.

cond-mat.str-el

Particle-hole asymmetric phases in doped twisted bilayer graphene

Despite much theoretical work, developing a comprehensive ab initio model for twisted bilayer graphene (TBG) has proven challenging due to the inherent trade-off between accurately describing the band structure and incorporating the interactions within the Hamiltonian, particularly given the topological obstruction -- so-called fragile topology -- to the description of the model in terms of localized symmetric Wannier functions within the flat band manifold. Here, we circumvent this obstruction by using an extended 8-orbital model, for which localized Wannier orbitals have been formulated by Carr et al. [1]. We constructed an extended multi-orbital Hubbard model, and performed Hartree-Fock (HF) calculations to explore its phase diagram across commensurate fillings from -3 to 3. We found several nearly-degenerate insulating states at charge neutrality, all of which exhibit orbital orders. Crucially, TBG near magic angle is known to be particle-hole asymmetric, which is naturally captured by the single-particle band structure of our model and is reflected in the distinction between the symmetry broken states obtained at electron and hole dopings away from the charge neutral point. At filling -1 and +2, quantum anomalous hall states are obtained, while for the rest of the integer fillings away from charge neutrality, we found the system to realize metallic states with various orbital, valley and spin orderings. We also observed that most of the Hartree--Fock ground states exhibit a generalized valley Hund's-like rule, resulting in valley polarization. Importantly, we show that the incorporation of the intra-valley and inter-valley exchange interactions is crucial to properly stabilize the ordered symmetry-broken states. In agreement with experiments, we find significant particle-hole asymmetry, which underscores the importance of using particle-hole asymmetric models.

cond-mat.str-el

Topological Diagnosis of Strongly Correlated Electron Systems

The intersection of electronic topology and strong correlations offers a rich platform to discover exotic quantum phases of matter and unusual materials. An overarching challenge that impedes the discovery is how to diagnose topology in strongly correlated settings, as exemplified by Mott insulators. Here, we develop a general framework to address this outstanding question and illustrate its power in the case of Mott insulators. The concept of Green's function Berry curvature -- which is frequency dependent -- is introduced. We apply this notion in a system that contains symmetry-protected nodes in its noninteracting bandstructure; strong correlations drive the system into a Mott insulating state, creating contours in frequency-momentum space where the Green's function vanishes. The Green's function Berry flux of such zeros is found to be quantized, and is as such direct probe of the system's topology. Our framework allows for a comprehensive search of strongly correlated topological materials with Green's function topology.

cond-mat.str-el

Electronic properties, correlated topology and Green's function zeros

There is extensive current interest about electronic topology in correlated settings. In strongly correlated systems, contours of Green's function zeros may develop in frequency-momentum space, and their role in correlated topology has increasingly been recognized. However, whether and how the zeros contribute to electronic properties is a matter of uncertainty. Here we address the issue in an exactly solvable model for Mott insulator. We show that the Green's function zeros contribute to several physically measurable correlation functions, in a way that does not run into inconsistencies. In particular, the physical properties remain robust to chemical potential variations up to the Mott gap as it should be based on general considerations. Our work sets the stage for further understandings on the rich interplay among topology, symmetry and strong correlations.

cond-mat.str-el

Metallic quantum criticality enabled by flat bands in a kagome lattice

Strange metals arise in a variety of platforms for strongly correlated electrons, ranging from the cuprates, heavy fermions to flat band systems. Motivated by recent experiments in kagome metals, we study a Hubbard model on a kagome lattice whose noninteracting limit contains flat bands. A Kondo lattice description is constructed, in which the correlation effects are captured by symmetry preserving and exponentially localized molecular orbitals. These compact molecular orbitals represent the local degrees of freedom that emerge from topological flat bands. We identify a quantum critical point at which quasiparticles are lost and strange metallicity emerges. Our theoretical work opens up a new route for realizing beyond-Landau quantum criticality, as well as the associated strange metallicity and emergent quantum phases.

cond-mat.str-el