arXiv subjects

Shu Nagata

Publications and source records attributed to Shu Nagata.

5 recordsLinked to original sources

arXiv2025

Universal coherent atom-molecule oscillations in the dynamics of the unitary Bose gas near a narrow Feshbach resonance

Quench experiments on a unitary Bose gas around a broad Feshbach resonance have led to the discovery of universal dynamics. This universality is manifested in the measured atomic momentum distributions where, asymptotically, a quasi-equilibrated metastable state is found in which both the momentum distribution and the time scales are determined by the particle density. In this paper we present counterpart studies but for the case of a very narrow Feshbach resonance of $^{133}$Cs atoms having a width of 8.3 mG. In dramatic contrast to the behavior reported earlier, a rapid quench of an atomic condensate to unitarity is observed to ultimately lead to coherent oscillations involving dynamically produced condensed and non-condensed molecules and atoms. The same characteristic frequency, determined by the Feshbach coupling, is observed in all types of particles. To understand these quench dynamics and how these different particle species are created, we develop a beyond Hartree-Fock-Bogoliubov dynamical framework including a new type of cross correlation between atoms and molecules. This leads to a quantitative consistency with the measured frequency. Our results, which can be applied to the general class of bosonic superfluids associated with narrow Feshbach resonances, establish a new paradigm for universal dynamics dominated by quantum many-body interactions.

cond-mat.quant-gas↗

arXiv2025

Observation of Phase Doubling and Entanglement in Coherent Matter-Wave Reactions

Chemical reactions in a statistical ensemble are conventionally regarded as incoherent processes driven by thermodynamics. In the quantum degenerate regime, where atoms and molecules form coherent matter waves, reactions are theoretically described by nonlinear mixing of matter-wave fields. In this scenario, we expect phase matching between reactants and products, analogous to the mixing of photonic fields in nonlinear optics. Here we report on the observation of phase coherent reaction dynamics of Bose-condensed atoms and molecules near a Feshbach resonance. Using matter-wave diffraction with optical lattices, we verify spatial coherence of both atoms and molecules and observe phase doubling when atomic waves combine into molecular waves, the matter-wave analogue of optical frequency doubling. The diffraction patterns further reveal two-atom entanglement generated during the reaction. Our observations establish phase coherence and entanglement generation as two essential features of "quantum many-body chemistry". Moreover, our work opens a pathway to control of reaction dynamics by manipulation of matter-wave phases.

cond-mat.quant-gas↗

arXiv2024

Stability and Dynamics of Atom-Molecule Superfluids Near a Narrow Feshbach Resonance

The recent observations of a stable molecular condensate emerging from a condensate of bosonic atoms and related "super-chemical" dynamics have raised an intriguing set of questions. Here we provide a microscopic understanding of this unexpected stability and dynamics in atom-molecule superfluids; we show one essential element behind these phenomena is an extremely narrow Feshbach resonance in $^{133}$Cs at 19.849G. Comparing theory and experiment we demonstrate how this narrow resonance enables the dynamical creation of a large closed-channel molecular fraction superfluid, appearing in the vicinity of unitarity. Theoretically the observed superchemistry (\textit{i.e.}, Bose enhanced reactions of atoms and molecules), is found to be assisted by the formation of Cooper-like pairs of bosonic atoms that have opposite momenta. Importantly, this narrow resonance opens the possibility to explore the quantum critical point of a molecular Bose superfluid and related phenomena which would not be possible near a more typically broad Feshbach resonance.

cond-mat.quant-gas↗

arXiv2024

Two dimensional arrays of Bose-Einstein condensates: interference and stochastic collapse dynamics

We demonstrate two-dimensional arrays of Bose-Einstein condensates (BECs) as a new experimental platform with parallel quantum simulation capability. A defect-free array of up to 49 BECs is formed by loading a single BEC with 50,000 atoms into 7*7 optical wells. Each BEC is prepared with independent phases, confirmed by matterwave interference. Based on BEC arrays, we realize fast determination of the phase boundary of BECs with attractive interactions. We also observe the stochastic collapse dynamics from the distribution of atom numbers in the array. We show that the collapse of a BEC can occur much faster than the averaged decay of an ensemble. The BEC arrays enable new forms of experiments to drastically increase the measurement throughput and to quantum simulate, say, large 2D Josephson-junction arrays.

cond-mat.quant-gas↗

arXiv2022

Many-body Chemical Reactions in a Quantum Degenerate Gas

Chemical reactions in the quantum degenerate regime are described by mixing of matterwave fields. Quantum coherence and bosonic enhancement are two unique features of many-body reactions involving bosonic reactants and products. Such collective reactions of chemicals, dubbed "super-chemistry", is an elusive goal in quantum chemistry research. Here we report the observation of coherent and collective reactive coupling between Bose condensed atoms and molecules near a Feshbach resonance. Starting from an atomic condensate, the reaction begins with a rapid formation of molecules, followed by oscillations of their populations in the equilibration process. Faster oscillations are observed in samples with higher densities, indicating bosonic enhancement. We present a quantum field model which describes the dynamics well and identifies three-body recombination as the dominant reaction process. Our findings exemplify the highly sought-after quantum many-body chemistry and offer a new paradigm for the control of quantum chemical reactions.

physics.atom-ph↗