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Shu-Shen Li

Publications and source records attributed to Shu-Shen Li.

At least 55 records · Page 3Linked to original sources

Zinc-blende and wurtzite GaAs quantum dots in nanowires studied using hydrostatic pressure

We report both zinc-blende (ZB) and wurtzite (WZ) crystal phase self-assembled GaAs quantum dots (QDs) embedding in a single GaAs/AlGaAs core-shell nanowires (NWs). Optical transitions and single-photon characteristics of both kinds of QDs have been investigated by measuring photoluminescence (PL) and time-resolved PL spectra upon application of hydrostatic pressure. We find that the ZB QDs are of direct band gap transition with short recombination lifetime (~1 ns) and higher pressure coefficient (75-100 meV/GPa). On the contrary, the WZ QDs undergo a direct-to-pseudodirect bandgap transition as a result of quantum confinement effect, with remarkably longer exciton lifetime (4.5-74.5 ns) and smaller pressure coefficient (28-53 meV/GPa). These fundamentally physical properties are further examined by performing state-of-the-art atomistic pseudopotential calculations.

cond-mat.mes-hall↗

The classical nature of nuclear spin noise near clock transitions of Bi donors in silicon

Whether a quantum bath can be approximated as classical noise is a fundamental issue in central spin decoherence and also of practical importance in designing noise-resilient quantum control. Spin qubits based on bismuth donors in silicon have tunable interactions with nuclear spin baths and are first-order insensitive to magnetic noise at so-called clock-transitions (CTs). This system is therefore ideal for studying the quantum/classical nature of nuclear spin baths since the qubit-bath interaction strength determines the back-action on the baths and hence the adequacy of a classical noise model. We develop a Gaussian noise model with noise correlations determined by quantum calculations and compare the classical noise approximation to the full quantum bath theory. We experimentally test our model through dynamical decoupling sequence of up to 128 pulses, finding good agreement with simulations and measuring electron spin coherence times approaching one second - notably using natural silicon. Our theoretical and experimental study demonstrates that the noise from a nuclear spin bath is analogous to classical Gaussian noise if the back-action of the qubit on the bath is small compared to the internal bath dynamics, as is the case close to CTs. However, far from the CTs, the back-action of the central spin on the bath is such that the quantum model is required to accurately model spin decoherence.

quant-ph↗

Decoherence of a quantum system coupled to an XY spin chain: Role of the initial state of the spin chain

We study the decoherence of a coupled quantum system consisting of a central spin and its correlated environment described by a general $XY$ spin-chain model. We make it clear that the evolution of the coherence factor sensitively depends on the initial states of the environment spin-chain. Specially, the dynamical evolution of the coherence factor of the central spin is numerically and analytically investigated in both weak and strong coupling cases for different initial states including thermal equilibrium state. In both weak and strong coupling regimes, the decay of the coherence factor can be approximated by a Gaussian and in the strong coupling regime the coherence factor oscillate rapidly under a Gaussian envelope. The width of the Gaussian decay (envelope) has been studied in details and we explained the origin of the so-called universal regime.

quant-ph↗

Critical behavior of the energy gap and its relation with the Berry phase close to the excited state quantum phase transition in the Lipkin model

In our previous work [Phys. Rev. A \textbf{85}, 044102 (2012)], we have studied the Berry phase of the ground state and exited states in the Lipkin model. In this paper, using Hellmann-Feynman theorem, we derive the relation between the energy gap and the Berry phase close to the excited state quantum phase transition (ESQPT) in the Lipkin model. We find that the energy gap is linearly dependent upon the Berry phase close to the ESQPT. As a result, the critical behavior of the energy gap is similar to that of the Berry phase. In addition, we also perform a semiclassical qualitative analysis about the critical behavior of the energy gap.

cond-mat.str-el↗

Uncovering many-body correlations in nanoscale nuclear spin baths by central spin decoherence

Many-body correlations can yield key insights into the nature of interacting systems; however, detecting them is often very challenging in many-particle physics, especially in nanoscale systems. Here, taking a phosphorus donor electron spin in a natural-abundance 29Si nuclear spin bath as our model system, we discover both theoretically and experimentally that many-body correlations in nanoscale nuclear spin baths produce identifiable signatures in the decoherence of the central spin under multiple-pulse dynamical decoupling control. We find that when the number of decoupling -pulses is odd, central spin decoherence is primarily driven by second-order nuclear spin correlations (pairwise flip-flop processes). In contrast, when the number of -pulses is even, fourth-order nuclear spin correlations (diagonal interaction renormalized pairwise flip-flop processes) are principally responsible for the central spin decoherence. Many-body correlations of different orders can thus be selectively detected by central spin decoherence under different dynamical decoupling controls, providing a useful approach to probing many-body processes in nanoscale nuclear spin baths.

cond-mat.mes-hall↗

The Coexistence and Decoupling of Bulk and Edge States in Disordered Two-dimensional Topological Insulators

We investigate the scattering and localization properties of edge and bulk states in a disordered two-dimensional topological insulator when they coexist at the same fermi energy. Due to edge-bulk backscattering (which is not prohibited \emph{a priori} by topology or symmetry), Anderson disorder makes the edge and bulk states localized indistinguishably. Two methods are proposed to effectively decouple them and to restore robust transport. The first kind of decouple is from long range disorder, since edge and bulk states are well separated in $k$ space. The second one is from an edge gating, owing to the edge nature of edge states in real space. The latter can be used to electrically tune a system between an Anderson insulator and a topologically robust conductor, i.e., a realization of a topological transistor.

cond-mat.mes-hall↗

Valley polarization in graphene-silicene-graphene heterojunction

Considering the difference of energy bands in graphene and silicene, we put forward a new model of the graphene-silicene-graphene (GSG) heterojunction. In the GSG, we study the valley polarization properties in a zigzag nanoribbon in the presence of an external electric field. We find the energy range associated with the bulk gap of silicene has a valley polarization more than 95%. Under the protection of the topological edge states of the silicene, the valley polarization remains even the small non-magnetic disorder is introduced. These results have certain practical significance in applications for future valley valve.

cond-mat.mes-hall↗

Demonstrating nonlocality induced teleportation through Majorana bound states in a semiconductor nanowire

It was predicted by Tewari [Phys. Rev. Lett. {\bf 100}, 027001 (2008)] that a teleportationlike electron transfer phenomenon is one of the novel consequences of the existence of Majorana fermion, because of the inherently nonlocal nature. In this work we consider a concrete realization and measurement scheme for this interesting behavior, based on a setup consisting of a pair of quantum dots which are tunnel-coupled to a semiconductor nanowire and are jointly measured by two point-contact detectors. We analyze the teleportation dynamics in the presence of measurement backaction and discuss how the teleportation events can be identified from the current trajectories of strong response detectors.

cond-mat.mes-hall↗

Structural stability of lattice-matched heterovalent semiconductor superlattices

Lattice-matched heterovalent alloys and superlattices have some unique physical properties. For example, their band gap can change by a large amount without significant change in their lattice constants, thus they have great potential for optelectronic applications. Using first-principles total energy calculation and Monte Carlo simulation as well as lattice harmonic expansion, we systematically study the stability of the heterovalent superlattices. We show that the chemical trend of stability of lattice-matched heterovalent superlattices is significantly different from lattice-mismatched isovalent superlattices, because for lattice-mismatched isovalent superlattices the stability is mostly determined by strain, whereas for lattice-matched nonisovalent superlattices the interfacial energy depend not only on the bond energy but also on the Coulomb energy derived from donor- and acceptor-like wrong bonds. In the short-period heterovalent superlattices, the abrupt [111] interface has the lowest energy even though it is polar, whereas for the long-period heterovalent superlattices, the [110] interface has the lowest energy. On the contrary, [201] superlattices are usually the most stable for lattice-mismatched isovalent superlattices.

cond-mat.mtrl-sci↗

Electron Delocalization in Gate-Tunable Gapless Silicene

The application of a perpendicular electric field can drive silicene into a gapless state, characterized by two nearly fully spin-polarized Dirac cones owing to both relatively large spin-orbital interactions and inversion symmetry breaking. Here we argue that since inter-valley scattering from non-magnetic impurities is highly suppressed by time reversal symmetry, the physics should be effectively single-Dirac-cone like. Through numerical calculations, we demonstrate that there is no significant backscattering from a single impurity that is non-magnetic and unit-cell uniform, indicating a stable delocalized state. This conjecture is then further confirmed from a scaling of conductance for disordered systems using the same type of impurities.

cond-mat.mes-hall↗

Interplay between edge and bulk states in silicene nanoribbon

We investigate the interplay between the edge and bulk states, induced by the Rashba spin-orbit coupling, in a zigzag silicene nanoribbon in the presence of an external electric field. The interplay can be divided into two kinds, one is the interplay between the edge and bulk states with opposite velocities, and the other is that with the same velocity direction. The former can open small direct spin-dependent subgaps. A spin-polarized current can be generated in the nanoribbon as the Fermi energy is in the subgaps. While the later can give rise to the spin precession in the nanoribbon. Therefore, the zigzag silicene nanoribbon can be used as an efficient spin filter and spin modulation device.

cond-mat.mes-hall↗

Quantum spin Hall effect induced by electric field in silicene

We investigate the transport properties in a zigzag silicene nanoribbon in the presence of an external electric field. The staggered sublattice potential and two kinds of Rashba spin-orbit couplings can be induced by the external electric field due to the buckled structure of the silicene. A bulk gap is opened by the staggered potential and gapless edge states appear in the gap by tuning the two kinds of Rashba spin-orbit couplings properly. Furthermore, the gapless edge states are spin-filtered and are insensitive to the non-magnetic disorder. These results prove that the quantum spin Hall effect can be induced by an external electric field in silicene, which may have certain practical significance in applications for future spintronics device.

cond-mat.mes-hall↗

Theory of multiple magnetic scattering for quasiparticles on a gapless topological insulator surface

We develop a general low-energy multiple-scattering partial-wave theory for gapless topological insulator (TI) surfaces in the presence of magnetic impurities. As applications, we discuss the differential cross section (CS) $dΛ/dφ$, the total CS $Λ_{tot}$, the Hall component of resistivity $Ω$, and inverse momentum relaxation time $Γ_{M}$ for single- and two-centered magnetic scattering. We show that differing from the nonmagnetic impurity scattering, $s\mathtt{-}$wave approximation is not advisable and convergent in the present case. The symmetry of CS is reduced and the backscattering occurs and becomes stronger with increasing the effective magnetic moment $M$ of single magnetic impurity. We show a non-zero perpendicular resistivity component $Ω$, which may be useful for tuning the Hall voltage of the sample. Consistent with the analysis of $dΛ/dφ$, by comparing $Γ_{M}$ with $Λ_{tot}$, we can determine different weights of backscattering and forward scattering. Similar to CS, $Ω$ and $Γ_{M}$ also exhibit oscillating behavior for multiple magnetic scattering centers due to interference effect.

cond-mat.mes-hall↗

Spin-polarized current induced by a local exchange field in a silicene nanoribbon

A mechanism to generate a spin-polarized current in a two-terminal zigzag silicene nanoribbon is predicted. As a weak local exchange field that is parallel to the surface of silicene is applied on one of edges of the silicene nanoribbon, a gap is opened in the corresponding gapless edge states but another pair of gapless edge states with opposite spin are still protected by the time-reversal symmetry. Hence, a spin-polarized current can be induced in the gap opened by the local exchange field in this two-terminal system. What is important is that the spin-polarized current can be obtained even in the absence of Rashba spin-orbit coupling and in the case of the very weak exchange filed. That is to say, the mechanism to generate the spin-polarized currents can be easily realized experimentally.We also find that the spin-polarized current is insensitive to weak disorder.

cond-mat.mes-hall↗

Quasiparticle states and quantum interference induce by magnetic impurities on a two-dimensional topological superconductor

We theoretically study the effect of localized magnetic impurities on two-dimensional topological superconductor (TSC). We show that the local density of states (LDOS) can be tuned by the effective exchange field $m$, the chemical potential $μ$ of TSC, and the distance $Δr$ as well as relative spin angle $α$ between two impurities. The changes in $Δr$ between two impurities alter the interference and result in significant modifications to the bonding and antibonding states. Furthermore, the bound-state spin LDOS induced by single and double magnetic impurity scattering, the quantum corrals, and the quantum mirages are also discussed. Finally, we briefly compare the impurities in TSC with those in topological insulators.

cond-mat.supr-con↗

Pure spin current in a two-dimensional topological insulator

We predict a mechanism to generate a pure spin current in a two-dimensional topological insulator. As the magnetic impurities exist on one of edges of the two-dimensional topological insulator, a gap is opened in the corresponding gapless edge states but another pair of gapless edge states with opposite spin are still protected by the time-reversal symmetry. So the conductance plateaus with the half-integer values $e^2/h$ can be obtained in the gap induced by magnetic impurities, which means that the pure spin current can be induced in the sample. We also find that the pure spin current is insensitive to weak disorder. The mechanism to generate pure spin currents is generalized for two-dimensional topological insulators.

cond-mat.mes-hall↗

Probing crossover from analogous weak antilocalization to localization by an Aharonov-Bohm interferometer on topological insulator surface

We propose a scanning tunneling microscopy Aharonov-Bohm (AB) interferometer on the surface of a topological insulator (TI) to probe the crossover from analogous weak antilocalization (WAL) to weak localization (WL) phenomenon via the AB oscillations in spin-resolved local density of states (LDOS). Based on our analytical and numerical results, we show that with increasing the energy gap of TI surface states, the $Φ_{0}/2$=$hc/2e$ periodic AB oscillations in spin-resolved LDOS gradually transit into the $Φ_{0}$ periodic oscillations.

cond-mat.mes-hall↗

Adsorption and dissociation of H$_{2}$O monomer on ceria(111): Density functional theory calculations

The adsorption properties of isolated H$_{2}$O molecule on stoichiometric and reduced (with on-surface oxygen vacancy) ceria(1111) surfaces at low coverage are theoretically investigated by using density-functional-theory+\emph{U} calculations and \textit{ab initio} molecular dynamics simulations. We identify the most stable adsorption configurations on these two kinds of surfaces, which form two hydrogen bonds between the water molecule and the oxide surface. The electronic structures indicate that the hybridization of the molecular orbitals of water and surface-layer O-2\emph{p} states dominates the interactions between adsorbate and substrate. The barrier of 0.51 eV for water diffusion on the stoichiometric surface implies the inertia of water unless up to a high temperature of 600 K, which is confirmed by the molecular dynamics simulations. For the reduced surface, we find that the oxygen vacancy obviously enhances the interaction. Moreover, it is facilitated for water to dissociate into H and OH species with a hydroxyl surface formed, instead of oxidizing the reduced surface with the production of hydrogen gas. In addition, the molecular dynamics simulations at low temperature 100 K confirm the dissociation process.

cond-mat.mtrl-sci↗