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Shuaishuai Sun

Publications and source records attributed to Shuaishuai Sun.

11 recordsLinked to original sources

Magnetic hopfions at room temperature

Hopfions are three-dimensional (3D) topological solitons predicted to exist in diverse magnetic systems, yet their practical utility has been largely restricted to cryogenic environments. Here, we overcome this temperature constraint by demonstrating stable magnetic hopfions in the chiral magnet Co8Zn8Mn4 at and above room temperature. Using a transmission electron microscope equipped for in situ optical excitation, we generate magnetic hopfions with femtosecond laser pulses. Long-term observations further reveal Brownian-like motion at room temperature and thermally activated collapse upon approaching the high-temperature regime. Together with micromagnetic simulations and homotopy group analysis, our experimental observations uncover the hopfion formation mechanism through the fusion of bimeron pairs. These findings establish room-temperature magnetic hopfions and provide a framework for their further studies under technologically relevant conditions.

cond-mat.mtrl-sci

A Dual-Bearing Magnetorheological Grease Clutch with Intention-Based Demagnetization for Wearable Haptic Feedback

This paper presents the design, modeling, and control of a dual-bearing magnetorheological grease (MRG) clutch for wearable haptic feedback. Compared with conventional MR fluid devices, the proposed clutch avoids leakage-related reliability degradation while achieving high torque density in a compact structure. To provide physical insight into the torque-generation mechanism, a physics-inspired interpretive model is introduced to capture the dominant relationship among excitation current, magnetic-field evolution in the bearing gaps, and clutch locking torque. To mitigate the undesirable ``sticky'' sensation caused by passive bidirectional braking, an intention-based control strategy with active demagnetization is further developed to enable smoother release during human--robot interaction. Experimental characterization shows that the proposed clutch achieves a maximum locking torque of 43.42\,N$\cdot$m at 1.3\,A and a torque-to-mass ratio of 96.5\,N$\cdot$m/kg. Bench tests, replay validation, teleoperation experiments, and user studies indicate that the proposed approach accelerates clutch release and improves perceived release transparency and contact-to-release smoothness, while maintaining effective multi-level kinesthetic rendering.

eess.SY

Anomalous charge density wave in a two-dimensional superatomic superconductor

The spatial modulation of electron density into a wave-like pattern, known as charge density wave (CDW), represents a fundamental quantum state that often coexists with superconductivity, quantum Hall states, axion insulating phases and etc. Conventional CDWs are mediated by longitudinal acoustic phonons, exhibit picometer-scale lattice distortions ($10^{-12}$--$10^{-11}$ m), and typically vanish approaching the atomic limit. Here, we report a series of anomalous CDW behaviors in the 2D superatomic superconductor Au$_6$Te$_{12}$Se$_8$. Remarkably, its CDW is governed by transverse phonons, accompanied by an extraordinarily high real-space displacement of $\sim 4$ Ångström. Furthermore, we observe an exotic dimensional response persisting up to micrometer-scale thickness, a regime where other materials are already considered as bulk. Through liquid helium-temperature transmission electron microscopy, ultrafast pump-probe spectroscopy and transport measurements, we demonstrate a dramatic enhancement of the CDW transition temperature ($T_{\text{CDW}}$) from $<2$ K in the bulk to 110 K in approaching the ``superatomic limit''. Our findings not only reveal novel facets of both CDW and superatomic materials, but the competition between this anomalous CDW and superconductivity opens avenues for exploring unconventional electron-phonon interactions.

cond-mat.supr-con

Electrically steered conduction topologies and period-doubling phase dynamics in VO2

The insulator-to-metal transition (IMT) in strongly correlated materials, such as vanadium dioxide (VO2), offers a transformative platform for next-generation adaptive electronics and neuromorphic computing. However, harnessing this non-equilibrium phase transition for deterministic device operation is fundamentally hindered by the inability to disentangle electric-field effects from Joule heating, owing to a lack of operando techniques capable of resolving phase dynamics at nanoscale spatial and sub-nanosecond temporal scales. Here, using a newly developed electrical-pulse-pump ultrafast transmission electron microscope (E-UTEM), we directly visualize the multi-scale electro-thermo-mechanical dynamics of the IMT in suspended VO2 devices. Our results reveal that electric-field-induced Poole-Frenkel (PF) emission, localized by patterned oxygen vacancies, plays a decisive role in redistributing the internal electric field to trigger a deterministic Mott transition. The extreme non-linearity of this PF effect enables the formation of dynamically reconfigurable connectivity topologies that bypass conventional thermal limits. Furthermore, we observe that the coupling of thermal and elastic energies governs a discrete domain evolution, characterized by step-wise and period-doubling configurational resets, which is a hallmark of non-equilibrium phase dynamics in constrained geometries. By integrating experimental imaging with phase-field simulations, we establish a comprehensive framework for the electrically-driven IMT and predict sub-100-ps switching kinetics. These findings provide a fundamental basis for the rational design of ultrafast, low-energy functional devices through nanoscale defect and strain engineering in correlated systems.

cond-mat.mtrl-sci

Development of a magnetorheological hand exoskeleton featuring a high force-to-power ratio for enhanced grip endurance

Hand exoskeletons have significant potential in labor-intensive fields by mitigating hand grip fatigue, enhancing hand strength, and preventing injuries. However, most of the traditional hand exoskeletons are driven by motors, whose output force is limited in the constrained installation conditions. Besides, they also come with the disadvantages of high power consumption, complex and bulky assistive systems, and high instability. In this work, we develop a novel hand exoskeleton integrated with innovative magnetorheological (MR) clutches that offers a high force-to-power ratio to improve grip endurance. The clutch features an enhanced structure design, a micro roller enhancing structure, which can significantly boost output forces. The experimental data demonstrate that, when it is supplied with 2 V, the clutch can deliver a peak holding force of 381.15 N-55 times that when no voltage is provided (7 N). In this scenario, it only consumes 1.38 W, yielding a force-to-power ratio of 256.75N/W, which is 2.35 times higher than the best-reported actuator used for hand exoskeletons. This capability enables the designed MRHE to provide approximately 419.79 N support force for gripping. The designed MR hand exoskeleton is highly integrated, comprising an exoskeleton frame, MR clutches, a control unit, and a battery. Evaluations through static grip endurance tests and dynamic carrying and lifting tests confirm that the MR hand exoskeleton can effectively reduce muscle fatigue, extend grip endurance, and minimize injuries. These findings highlight its strong potential for practical applications in repetitive tasks such as carrying and lifting in industrial settings.

cs.RO

Spectroscopic origin of giant anomalous Hall effect in an interwoven magnetic kagome metal

The discovery of a giant anomalous Hall effect (AHE) and its novel mechanism holds significant promise for advancing both fundamental research and practical applications. Magnetic kagome lattice materials are uniquely suited for studying the AHE due to their interplay between electronic structure, topology, and magnetism. However, the geometric frustration inherent in kagome lattices often limits the configuration and tunability of magnetic order. Here, we present a new design strategy for kagome-lattice materials with emergent magnetism, exemplified by the magnetic kagome metal TbTi$_3$Bi$_4$, which features interwoven magnetic Tb zigzag chains and non-magnetic Ti kagome bilayers. This material exhibits a record-high anomalous Hall conductivity (AHC) of 10$^5$ $Ω^{-1}$ cm$^{-1}$. Spectroscopy measurements reveal a large band folding gap observed via angle-resolved photoemission spectroscopy, coexisting spin-density-wave (SDW) order detected through spin-polarized scanning tunneling spectroscopy, and a spiral magnetic order with large magnetic moments identified by neutron diffraction. These findings highlight a strong electron-magnetic coupling between itinerant charges and ordered magnetic moments, offering a spectroscopic explanation for the giant AHC in TbTi$_3$Bi$_4$. This work establishes a pathway for innovative material design strategies, unlocking new possibilities for future exploration and applications in quantum and spintronic technologies.

cond-mat.str-el

Toward nonthermal control of excited quantum materials: framework and investigations by ultrafast electron scattering and imaging

Quantum material systems upon applying ultrashort laser pulses provide a rich platform to access excited material phases and their transformations that are not entirely like their equilibrium counterparts. The addressability and potential controls of metastable or long-trapped out-of-equilibrium phases have motivated interests both for the purposes of understanding the nonequilibrium physics and advancing the quantum technologies. Thus far, the dynamical spectroscopic probes eminently focus on microscopic electronic and phonon responses. For characterizing the long-range dynamics, such as order parameter fields and fluctuation effects, the ultrafast scattering probes offer direct sensitivity. Bridging the connections between the microscopic dynamics and macroscopic responses is central toward establishing the nonequilibrium physics behind the light-induced phases. Here, we present a path toward such understanding by cross-examining the structure factors associated with different dynamical states obtained from ultrafast electrons scattering, imaging, and modeling. We give the basic theoretical framework on describing the non-equilibrium scattering problems and briefly describe how such framework relates to the out-of-equilibrium phenomena. We give effective models outlining the emergences of nonthermal critical points, hidden phases, and non-equilibrium relaxational responses from vacuum-suspended rare-earth tritellurides, tantalum disulfides thin films, and vanadium dioxide nanocrystalline materials upon light excitations.

cond-mat.str-el

Improving positioning accuracy of the mobile laser scanning in GPS-denied environments: An experimental case study

The positioning accuracy of the mobile laser scanning (MLS) system can reach the level of centimeter under the conditions where GPS works normally. However, in GPS-denied environments this accuracy can be reduced to the decimeter or even the meter level because the observation mode errors and the boresight alignment errors of MLS cannot be calibrated or corrected by the GPS signal. To bridge this research gap, this paper proposes a novel technique that appropriately incorporates the robust weight total least squares (RWTLS) and the full information maximum likelihood optimal estimation (FIMLOE) to improve the positioning accuracy of the MLS system under GPS-denied environment. First of all, the coordinate transformation relationship and the observation parameters vector of MLS system are established. Secondly, the RWTLS algorithm is used to correct the 3D point observation model; then the uncertainty propagation parameter vector and the boresight alignment errors between the laser scanner frame and the IMU frame are calibrated by FIMLOE. Lastly, experimental investigation in indoor scenarios was performed to evaluate the effectiveness of the proposed method. The experimental results demonstrate that the proposed method is able to significantly improve the positioning accuracy of an MLS system in GPS-denied environments.

eess.SP

An Anomalous Circular Photogalvanic Effect in the Weyl Semimetal TaAs

Weyl semimetal (WSM) is expected to be an ideal spintronic material owing to its spin currents carried by the bulk and surface states with spin-momentum locking. A photocurrent generation in noncentrosymmetric WSM was also predicted owing to its broken inversion symmetry and linear energy dispersion which are unique to Weyl systems. In our recent measurements, the circular photogalvanic effect (CPGE) has been demonstrated in WSM of TaAs. The CPGE voltage is proportional to the helicity of the incident light and reverses its direction on changing the radiation helicity from left handed to right handed, a periodical oscillation therefore appears following with the alteration of optical polarization. We herein attribute the CPGE to the asymmetric optical excitation of the Weyl cone, which could result in an asymmetric distribution of photoexcited carriers in momentum space according to an optical spin selection rule.

cond-mat.str-el

Ultrafast transmission electron microscopy on dynamic process of a CDW transition in 1T-TaSe2

Four-dimensional ultrafast transmission electron microscopy (4D-UTEM) measurements reveal a rich variety of structural dynamic phenomena at a phase transition in the charge-density-wave (CDW) 1T-TaSe2. Through the photoexcitation, remarkable changes on both the CDW intensity and orientation are clearly observed associated with the transformation from a commensurate (C) into an incommensurate (IC) phase in a time-scale of about 3 ps. Moreover, the transient states show up a notable "structurally isosbestic point" at a wave vector of qiso where the C and IC phases yield their diffracting efficiencies in an equally ratio. This fact demonstrates that the crystal planes parallel to qiso adopts visibly common structural features in these two CDW phases. The second-order characters observed in this nonequilibrium phase transition have been also analyzed based on the time-resolved structural data.

cond-mat.str-el

Clocking the anisotropic lattice dynamics of multi-walled carbon nanotubes by four-dimensional ultrafast transmission electron microscopy

Recent advances in the four-dimensional ultrafast transmission electron microscope (4D-UTEM) with combined spatial and temporal resolutions have made it possible to directly visualize structural dynamics of materials at the atomic level. Herein, we report on our development on a 4D-UTEM which can be operated properly on either the photo-emission or the thermionic mode. We demonstrate its ability to obtain sequences of snapshots with high spatial and temporal resolutions in the study of lattice dynamics of the multi-walled carbon nanotubes (MWCNTs). This investigation provides an atomic level description of remarkable anisotropic lattice dynamics at the picosecond timescales. Moreover, our UTEM measurements clearly reveal that distinguishable lattice relaxations appear in intra-tubular sheets on an ultrafast timescale of a few picoseconds and after then an evident lattice expansion along the radical direction. These anisotropic behaviors in the MWCNTs are considered arising from the variety of chemical bonding, i.e. the weak van der Waals bonding between the tubular planes and the strong covalent sp2-hybridized bonds in the tubular sheets.

cond-mat.mes-hall