arXiv subjects

Shubhankar Das

Publications and source records attributed to Shubhankar Das.

10 recordsLinked to original sources

arXiv2025

Revealing the Altermagnetism in Hematite via XMCD Imaging and Anomalous Hall Electrical Transport

Altermagnets are a class of magnetic materials that exhibit unconventional transport properties, such as an anomalous Hall effect, despite having compensated sublattice magnetic moments. In this study, we report fundamental experimental evidence of the altermagnetic nature of hematite ($α$-\ch{Fe2O3}), combining electrical transport with advanced XPEEM imaging with linear and circular dichroism contrast. Our measurements directly visualize the Néel vector's coupling to the crystal orientation, confirming hematite's altermagnetic order and its symmetry-driven transport behavior. Transport measurements reveal an anisotropic AHE with a pronounced crystal orientation dependence, including a sign inversion for specific Néel vector alignments. Supported by first-principles theoretical calculations, we explain how the interplay between collinear spin and crystal symmetry breaking drives the observed anomalous Hall effect. These findings establish hematite as an altermagnet, paving the way for experimental identification of altermagnetic materials and their integration into spintronic technologies.

cond-mat.mtrl-sci↗

arXiv2023

Magnetic properties of hematite revealed by an ab initio parameterized spin model

Hematite is a canted antiferromagnetic insulator, promising for applications in spintronics. Here, we present ab initio calculations of the tensorial exchange interactions of hematite and use them to understand its magnetic properties by parameterizing a semiclassical Heisenberg spin model. Using atomistic spin dynamics simulations, we calculate the equilibrium properties and phase transitions of hematite, most notably the Morin transition. The computed isotropic and Dzyaloshinskii--Moriya interactions result in a Néel temperature and weak ferromagnetic canting angle that are in good agreement with experimental measurements. Our simulations show how dipole-dipole interactions act in a delicate balance with first and higher-order on-site anisotropies to determine the material's magnetic phase. Comparison with spin-Hall magnetoresistance measurements on a hematite single-crystal reveals deviations of the critical behavior at low temperatures. Based on a mean-field model, we argue that these differences result from the quantum nature of the fluctuations that drive the phase transitions.

cond-mat.mtrl-sci↗

arXiv2021

Anisotropic long-range spin transport in canted antiferromagnetic orthoferrite YFeO$_3$

In antiferromagnets, the efficient propagation of spin-waves has until now only been observed in the insulating antiferromagnet hematite, where circularly (or a superposition of pairs of linearly) polarized spin-waves propagate over long distances. Here, we report long-distance spin-transport in the antiferromagnetic orthoferrite YFeO$_3$, where a different transport mechanism is enabled by the combined presence of the Dzyaloshinskii-Moriya interaction and externally applied fields. The magnon decay length is shown to exceed hundreds of nano-meters, in line with resonance measurements that highlight the low magnetic damping. We observe a strong anisotropy in the magnon decay lengths that we can attribute to the role of the magnon group velocity in the propagation of spin-waves in antiferromagnets. This unique mode of transport identified in YFeO$_3$ opens up the possibility of a large and technologically relevant class of materials, i.e., canted antiferromagnets, for long-distance spin transport.

cond-mat.str-el↗

arXiv2021

Damping in yttrium iron garnet film with an interface

We report strong damping enhancement in a 200 nm thick yttrium iron garnet (YIG) film due to spin inhomogeneity at the interface. The growth-induced thin interfacial gadolinium iron garnet (GdIG) layer antiferromagnetically (AFM) exchange couples with the rest of the YIG layer. The out-of-plane angular variation of ferromagnetic resonance (FMR) linewidth $ΔH$ reflects a large inhomogeneous distribution of effective magnetization $Δ4 πM_{eff}$ due to the presence of an exchange springlike moments arrangement in YIG. We probe the spin inhomogeneity at the YIG-GdIG interface by performing an in-plane angular variation of resonance field $H_{r}$, leading to a unidirectional feature. The large extrinsic $Δ4πM_{eff}$ contribution, apart from the inherent intrinsic Gilbert contribution, manifests enhanced precessional damping in YIG film.

cond-mat.mtrl-sci↗

arXiv2020

A four-state magnetic tunnel junction switchable with spin-orbit torques

We present a magnetic tunnel junction (MTJ) where its two ferromagnetic layers are in the form of a single ellipse (SE) and two-crossing ellipses (TCE). The MTJ exhibits four distinct resistance states corresponding to the four remanent states of the TCE structure. Flowing current in an underlying Ta layer generates in the adjacent TCE structure spin-orbit torques which induce field-free switching of the four-state MTJ between all its resistance states. The demonstrated four-state MTJ is an important step towards fabricating multi-level MTJs with numerous resistance states which could be important in various spintronics applications, such as multi-level magnetic random access or neuromorphic memory.

physics.app-ph↗

arXiv2020

Stabilization of exponential number of discrete remanent states with localized spin-orbit torques

Using bilayer films of $β$-Ta/Ni$_{0.8}$Fe$_{0.2}$, we fabricate structures consisting of two, three and four crossing ellipses which exhibit shape-induced bi-axial, tri-axial and quadro-axial magnetic anisotropy in the crossing area, respectively. Structures consisting of N crossing ellipses can be stabilized in 2N remanent states by applying (and removing) an external magnetic field. However, we show that with field-free spin-orbit torques induced by flowing currents in individual ellipses, the number of remanent states grows to 2$^\text{N}$. Furthermore, when the current flows between the edges of different ellipses the number of remanent states jumps to 2$^\text{2N}$, including states which exhibit a $π$-Néel domain wall in the overlap area. The very large number of accessible remanent magnetic states that are exhibited by the relatively simple magnetic structures paves the way for intriguing spintronics applications including memory devices.

cond-mat.mes-hall↗

arXiv2018

Kondo effect with tunable spin orbit interaction in LaTiO3/CeTiO3/SrTiO3 heterostructure

We have fabricated epitaxial films of CeTiO3 (CTO) on (001)oriented SrTiO3(STO) substrates, which exhibit highly insulating and diamagnetic properties. X-ray photoelectron spectroscopy (XPS) was to establish the 3+ valence state of the Ve and Ti ions. Furthermore, we also fabricated delta (CTO) doped LatiO3 (LTO)-STO thin films which exhibit variety of interesting properties including Kondo effect and spin orbit interaction (SOI) at low temperatures. SOI shows a non-monotonic behaviour as the thickness of the CTO layer is increased and is reflected in the value of the characteristic SOI field (B_SO) obtained from weak antilocalization fitting. The maximum value of B_SO is 1.00 T for delta layer thickness of 6 u.c. This non-monotonic behaviour of SOI is attributed to the strong screening of the confining potential at the interface. The thicker CTO film in addition to the increased dielectric constant of the STO substrate at low temperature leads to strong screening as a result of which the electrons confined at the interface are spread deeper into the STO bulk where it starts to populate the Ti d_xz_yz subbands; consequently the Fermi level crosses over from the d_xy to the d_xz_yz subbands. At the crossover region of d_xy - d_xz_yz where there is orbital mixing, SOI goes through a maximum.

cond-mat.str-el↗

arXiv2016

Signature of enhanced spin-orbit interaction in the magnetoresistance of LaTiO$_3$/SrTiO$_3$ interfaces on $δ$-doping

We present a study of modulation of spin-orbit interaction (SOI) at the interface of LaTiO$_3$/SrTiO$_3$ by $δ$-doping with an iso-structural ferromagnetic perovskite LaCoO$_3$. The sheet carrier density at the interface decreases exponentially with $δ$-doping thickness. We have explored that the spin-orbit scattering time ($τ_{so}$) can be decreased by nearly 3 orders of magnitude, whereas the inelastic scattering time ($τ_{i}$) remains almost constant with $δ$-doping thickness. We have also observed that the $τ_{i}$ varies almost inversely proportional to temperature and $τ_{so}$ remains insensitive to temperature, which suggest that the spin relaxation in these interfaces follows D'yakonov-Perel mechanism. The observed in-plane anisotropic magnetoresistance is attributed to the mixing of the spin up and spin down states of d-band at Fermi level due to SOI.

cond-mat.str-el↗

arXiv2014

Magnetothermopower of $δ$-doped LaTiO$_3$/SrTiO$_3$ interfaces in the Kondo regime

Measurements of magneto-thermopower (S(H, T)) of interfacial delta doped LaTiO$_3$/SrTiO$_3$ (LTO/STO) heterostructure by an iso-structural antiferromagnetic perovskite LaCrO$_3$ are reported. The thermoelectric power of the pure LTO/STO interface at 300 K is $\approx$ 118 $μ$V/K, but increases dramatically on $δ$-doping. The observed linear temperature dependence of S(T) over the temperature range 100 K to 300 K is in agreement with the theory of diffusion thermopower of a two-dimensional electron gas. The S(T) displays a distinct enhancement in the temperature range (T $<$ 100 K) where the sheet resistance shows a Kondo-type minimum. We attributed this maximum in S(T) to Kondo scattering of conduction electron by localized impurity spins at the interface. The suppression of S by a magnetic field, and the isotropic nature of the suppression in out-of-plane and in-plane field geometries further strengthen the Kondo model based interpretation of S(H, T).

cond-mat.str-el↗

arXiv2014

Enhanced spin-orbit interaction and Kondo scattering in $δ$-doped LaTiO$_3$/SrTiO$_3$ interfaces

We present a study of delta ($δ$) doping at LaTiO$_3$/SrTiO$_3$ (LTO/STO) interface with iso-structural antiferromagnetic perovskite LaCrO$_3$ (LCO) that dramatically alters the properties of the two dimensional electron gas (2-DEG) at the interface. The effects include a reduction in sheet-carrier density, prominence of the low temperature resistivity minimum, enhancement of weak antilocalization below 10 K and observation of a strong anisotropic magnetoresistance (MR). The positive and negative MR for out-of-plane and in-plane field respectively and the field and temperature dependencies of MR suggest Kondo scattering by localized Ti$^{3+}$ moments renormalized by spin-orbit interaction at T $<$ 10 K, with the increased $δ$-layer thickness. Electron energy loss spectroscopy and density functional calculations provide convincing evidence for blocking of electron transfer from LTO to STO by the $δ$-layer.

cond-mat.str-el↗