arXiv subjects

Shufeng Wang

Publications and source records attributed to Shufeng Wang.

9 recordsLinked to original sources

arXiv2026

Sub-50 Picosecond exceptionally Bright Perovskite Scintillation by Unlocking Giant Oscillator Strength

Ultrafast scintillators are indispensable for precise timing in high-energy physics and medical diagnostics. Fundamentally constrained by the trade-off between emission rate and light yield, conventional scintillators remain kinetically trapped in the sub-nanosecond regime, failing to break 50-picosecond limit. Here, we demonstrate a strategy to bypass this limitation by harnessing the coherent radiative acceleration in weakly confined CsPbCl3 perovskite nanocrystals to generate an ultrafast photon burst. This effect originates from the giant oscillator strength, which we unlock by suppressing exciton-phonon scattering at mild cryogenic temperatures. Consequently, our scintillator achieves an unprecedented dominant lifetime of 13.11 ps alongside a high light yield of 21,851 ph/MeV. The resulting prompt photon emission rate more than 100 times higher than that of state-of-the-art ultrafast scintillators. We validate this breakthrough in realistic detection scenarios, achieving a coincidence time resolution of 30.8 ps and accurately resolving 13.5 ps electron bunches and 16.6 ps single-shot gamma-ray pulses. Our findings establish a robust coherent framework for next-generation ultrafast scintillators, pushing extreme radiation diagnostics into the picosecond frontier.

cond-mat.mes-hall↗

arXiv2026

PRBench: End-to-end Paper Reproduction in Physics Research

AI agents powered by large language models exhibit strong reasoning and problem-solving capabilities, enabling them to assist scientific research tasks such as formula derivation and code generation. However, whether these agents can reliably perform end-to-end reproduction from real scientific papers remains an open question. We introduce PRBench, a benchmark of 30 expert-curated tasks spanning 11 subfields of physics. Each task requires an agent to comprehend the methodology of a published paper, implement the corresponding algorithms from scratch, and produce quantitative results matching the original publication. Agents are provided only with the task instruction and paper content, and operate in a sandboxed execution environment. All tasks are contributed by domain experts from over 20 research groups at the School of Physics, Peking University, each grounded in a real published paper and validated through end-to-end reproduction with verified ground-truth results and detailed scoring rubrics. Using an agentified assessment pipeline, we evaluate a set of coding agents on PRBench and analyze their capabilities across key dimensions of scientific reasoning and execution. The best-performing agent, OpenAI Codex powered by GPT-5.3-Codex, achieves a mean overall score of 34%. All agents exhibit a zero end-to-end callback success rate, with particularly poor performance in data accuracy and code correctness. We further identify systematic failure modes, including errors in formula implementation, inability to debug numerical simulations, and fabrication of output data. Overall, PRBench provides a rigorous benchmark for evaluating progress toward autonomous scientific research.

cs.CL↗

arXiv2026

WorkflowGen:an adaptive workflow generation mechanism driven by trajectory experience

Large language model (LLM) agents often suffer from high reasoning overhead, excessive token consumption, unstable execution, and inability to reuse past experiences in complex tasks like business queries, tool use, and workflow orchestration. Traditional methods generate workflows from scratch for every query, leading to high cost, slow response, and poor robustness. We propose WorkflowGen, an adaptive, trajectory experience-driven framework for automatic workflow generation that reduces token usage and improves efficiency and success rate. Early in execution, WorkflowGen captures full trajectories and extracts reusable knowledge at both node and workflow levels, including error fingerprints, optimal tool mappings, parameter schemas, execution paths, and exception-avoidance strategies. It then employs a closed-loop mechanism that performs lightweight generation only on variable nodes via trajectory rewriting, experience updating, and template induction. A three-tier adaptive routing strategy dynamically selects among direct reuse, rewriting-based generation, and full initialization based on semantic similarity to historical queries. Without large annotated datasets, we qualitatively compare WorkflowGen against real-time planning, static single trajectory, and basic in-context learning baselines. Our method reduces token consumption by over 40 percent compared to real-time planning, improves success rate by 20 percent on medium-similarity queries through proactive error avoidance and adaptive fallback, and enhances deployability via modular, traceable experiences and cross-scenario adaptability. WorkflowGen achieves a practical balance of efficiency, robustness, and interpretability, addressing key limitations of existing approaches.

cs.LG↗

arXiv2024

Hyper-sampling imaging

In our research, we have developed a novel mechanism that allows for a significant reduction in the smallest sampling unit of digital image sensors (DIS) to as small as 1/16th of a pixel, through measuring the intra-pixel quantum efficiency for the first time and recomputing the image. Employing our method, the physical sampling resolution of DIS can be enhanced by 16 times. The method has undergone rigorous testing in real-world imaging scenarios.

physics.optics↗

arXiv2022

Lateral quantum confinement regulates charge carrier transfer and biexciton interaction in CdSe/CdSeS core/crown nanoplatelets

Charge carrier dynamics essentially determine the performance of various optoelectronic applications of colloidal semiconductor nanocrystals. Among them, two-dimensional nanoplatelets provide new adjustment freedom for their unique core/crown heterostructure. Herein, we demonstrate that by fine-tuning the core size and the lateral quantum confinement, the charge carrier transfer rate from the crown to the core can be varied by one order of magnitude in CdSe/CdSeS core/alloy-crown nanoplatelets. In addition, the transfer can be affected by a carrier blocking mechanism, i.e., the filled carriers hinder further possible transfer. Furthermore, we found that the biexciton interaction is oppositely affected by quantum confinement and electron delocalization, resulting in a non-monotonic variation of the biexciton binding energy with the emission wavelength. This work provides new observations and insights into the charge carrier transfer dynamics and exciton interactions in colloidal nanoplatelets and will promote their further applications in lasing, display, sensing, etc.

cond-mat.mes-hall↗

arXiv2019

Temperature dependent threshold for amplified emission from hybrid lead perovskite films

The optical amplification emission of hybrid lead perovskite attracted great research interests. We systematically examined and compared temperature dependent optical amplification behavior of a series of organic-inorganic hybrid perovskite films of (MA/FA)Pb(Br/I)3. The optical amplification threshold of the films showed considerable exponential increase towards the temperature increasing. We figured out that the critical temperature for the four films presented a sequence of FA+I < MA+I < FA+Br < MA+Br. Our systematical study is crucial for in depth understanding the fundamental mechanism of amplified emission of hybrid perovskite materials.

physics.app-ph↗

arXiv2017

Revealing two heat-annealing related photoproduct systems and widely existed subgrain domains in organolead perovskite

For highly interested organolead perovskite based solar cells, the photoproducts are regarded as the co-existed exciton and free carriers. In this study, we carefully re-examined this conclusion with our recently developed density-resolved spectroscopic method. Heat-annealing related two photoproduct systems are observed. We found that the widely accepted model is only true for single crystal and freshly made films without heat-annealing. For those sufficiently heat-annealed films, another system presenting significant emissive exciton-carrier collision (ECC) is discovered. In addition, the appearing of ECC indicates the emerging of an internal morphology after heat annealing, which is assigned to a recently discussed twinning subgrain structure. We proved that such subgrain structures broadly exist in perovskite films. This finding could prove the morphological basis for high performance of perovskite working layers.

cond-mat.mtrl-sci↗

arXiv2016

Dynamical co-existence of excitons and free carriers in perovskite probed by density-resolved fluorescent spectroscopic method

Using transient fluorescent spectra at time-zero, we develop a density-resolved fluorescent spectroscopic method for investigating photoproducts in CH3NH3PbI3 perovskite and related photophysics. The density dependent dynamical co-existence of excitons and free carriers over a wide density range is experimentally observed for the first time. The exciton binding energy (EB) and the effective mass of electron-hole pair can be estimated based on such co-existence. No ionic polarization is found contributing to photophysical behavior. It also solves the conflict between the large experimentally measured EB and the small predicted values. The spectroscopic method also helps to detect the true free carrier density under continuous illumination without the interference of ionic conductivity. Our methods and results profoundly enrich the study and understanding of the photophysics in perovskite materials for photovoltaic applications.

cond-mat.mtrl-sci↗

arXiv2015

Direct Observation of Long Electron-Hole Diffusion Distance in CH3NH3PbI3 Perovskite Thin Film

In high performance perovskite based solar cells, CH3NH3PbI3 is the key material. We carried out a study on charge diffusion in spin-coated CH3NH3PbI3 perovskite thin film by transient fluorescent spectroscopy. A thickness-dependent fluorescent lifetime was found. By coating the film with an electron or hole transfer layer, [6,6]-phenyl-C61-butyric acid methyl ester (PCBM) or 2,2,7,7-tetrakis(N,N-di-p-methoxyphenylamine)-9,9-spirobifluorene (Spiro-OMeTAD) respectively, we observed the charge transfer directly through the fluorescence quenching. One-dimensional diffusion model was applied to obtain long charge diffusion distances in thick films, which is ~1.7 um for electrons and up to ~6.3 um for holes. Short diffusion distance of few hundreds of nanosecond was also observed in thin films. This thickness dependent charge diffusion explained the formerly reported short charge diffusion distance (~100 nm) in films and resolved its confliction to thick working layer (300-500 nm) in real devices. This study presents direct support to the high performance perovskite solar cells and will benefit the devices design.

physics.chem-ph↗