arXiv subjects

Shuichi Iwakiri

Publications and source records attributed to Shuichi Iwakiri.

14 recordsLinked to original sources

arXiv2026

Observation of universal thermopolarization effect in insulators

Heat-to-charge conversion has traditionally been realized via the Seebeck effect in conductors and pyroelectricity in polar insulators. Here, we demonstrate that temperature gradients generate electrical polarization, namely thermopolarization, in a wide range of insulators through a thermomechanical pathway. We identify a mechanism where thermal expansion under a temperature gradient produces strain gradients that induce polarization via the flexoelectric effect. Using a device with an on-chip heater, we detect the heat-induced polarization in crystalline, polymeric, and amorphous systems, including MgO, Al$_2$O$_3$, MnO, mica, PET, PEN, polyimide, and soda-lime glass. The magnitude of the response exhibits a robust scaling with the coefficient of thermal expansion, which is reproduced by finite-element simulations. Furthermore, we identify two routes to enhance the response: reducing the sample thickness and exploiting structural instabilities such as glass and antiferromagnetic phase transitions, where more than an order-of-magnitude enhancement is observed. These results establish a symmetry-independent route for heat-to-charge conversion in insulators and provide a device-compatible platform for electrically probing lattice responses, with potential for enhancement in nanoscale systems such as two-dimensional materials.

cond-mat.mtrl-sci↗

arXiv2026

On-chip detection of anisotropic thermopolarization in quartz

Temperature gradients are widely used to drive and probe transport phenomena in solids, forming the basis of heat-to-charge conversion processes. In typical experiments, local heating is introduced to generate a temperature gradient, and the resulting electrical response is detected by separate electrodes. Such measurements usually regard heating purely as a source of thermal excitation. Here, we show that heating inherently generates mechanical stress through thermal expansion, which in turn produces measurable electrical signals via electromechanical coupling. Using quartz as a model piezoelectric system, we demonstrate that heat can be converted to electrical currents via thermally generated stress. The on-chip device used in our experiment enables us to probe the anisotropy of the piezoelectric tensor through the thermally generated current, exhibiting twofold and threefold responses for X-cut and Z-cut crystals, respectively. We further show that the response can be detected in both current and voltage modes. These results reveal a thermomechanical pathway for heat-to-charge conversion and establish a general platform for electrically probing thermomechanical responses in insulating materials.

cond-mat.mtrl-sci↗

arXiv2023

Gate-defined superconducting channel in magic-angle twisted bilayer graphene

Magic-angle twisted bilayer graphene (MATBG) combines in one single material different phases like insulating, metallic and superconducting. These phases and their in-situ tunability make MATBG an important platform for the fabrication of superconducting devices. We realize a split gate-defined geometry which enables us to tune the width of a superconducting channel formed in MATBG. We observe a smooth transition from superconductivity to highly resistive transport by progressively reducing the channel width using the split gates or by reducing the density in the channel. Using the gate-defined constriction, we control the flow of the supercurrent, either guiding it through the constriction or throughout the whole device or even blocking its passage completely. This serves as a foundation for developing quantum constriction devices like superconducting quantum point contacts, quantum dots, and Cooper-pair boxes in MATBG.

cond-mat.mes-hall↗

arXiv2023

High mobility transport in isotopically-enriched $^{12}$C and $^{13}$C exfoliated graphene

Graphene quantum dots are promising candidates for qubits due to weak spin-orbit and hyperfine interactions. The hyperfine interaction, controllable via isotopic purification, could be the key to further improving the coherence. Here, we use isotopically enriched graphite crystals of both $^{12}$C and $^{13}$C grown by high-pressure-high-temperature method to exfoliate graphene layers. We fabricated Hall bar devices and performed quantum transport measurements, revealing mobilities exceeding $10^{5}$$\textrm{cm}^{2}/Vs$ and a long mean free path of microns, which are as high as natural graphene. Shubnikov-de Haas oscillations, quantum Hall effect up to the filling factor of one, and Brown-Zak oscillations due to the alignment of hBN and graphene are observed thanks to the high mobility. These results constitute a material platform for physics and engineering of isotopically-enriched graphene qubits.

cond-mat.mes-hall↗

arXiv2023

Tunable quantum interferometer for correlated moiré electrons

Magic-angle twisted bilayer graphene (MATBG) can host an intriguing variety of gate-tunable correlated states, including superconducting and correlated insulator states. Junction-based superconducting devices, such as Josephson junctions and SQUIDs, have been introduced recently and enable the exploration of the charge, spin, and orbital nature of superconductivity and the coherence of moiré electrons in MATBG. However, complementary fundamental coherence effects - in particular, the Little-Parks effect in a superconducting and the Aharonov-Bohm effect in a normal conducting ring - remained to be observed. Here, we report the observation of both these phenomena in a single gate-defined ring device where we can embed a superconducting or normal conducting ring in a correlated or band insulator. We directly observe the Little-Parks effect in the superconducting phase diagram as a function of density and magnetic field, confirming the effective charge of $2e$. By measuring the Aharonov-Bohm effect, we find that in our device, the coherence length of normal conducting moiré electrons exceeds a few microns at 50 mK. Surprisingly, we also identify a regime characterized by $h/e$-periodic oscillations but with superconductor-like nonlinear transport. Taken together, these experiments establish a novel device platform in MATBG, and more generally in tunable 2D materials, to unravel the nature of superconductivity and other correlated quantum states in these materials.

cond-mat.mes-hall↗

arXiv2023

Nonlinear response of 2DEG in the quantum Hall regime

Breaking of inversion symmetry leads to nonlinear and nonreciprocal electron transport, in which the voltage response does not invert with the reversal of the current direction. Many systems have incorporated inversion symmetry breaking into their band or crystal structures. In this work, we demonstrate that a conventional two-dimensional electron gas (2DEG) system with a back gate shows non-reciprocal behavior (with voltage proportional to current squared) in the quantum Hall regime, which depends on the out-of-plane magnetic field and contact configuration. The inversion symmetry is broken due to the presence of the back gate and magnetic field, and our phenomenological model provides a qualitative explanation of the experimental data. Our results suggest a universal mechanism that gives rise to non-reciprocal behavior in gated samples.

cond-mat.mes-hall↗

arXiv2022

Gate-defined electron interferometer in bilayer graphene

We present an electron interferometer defined purely by electrostatic gating in encapsulated bilayer graphene. This minimizes possible sample degradation introduced by conventional etching methods when preparing quantum devices. The device quality is demonstrated by observing Aharonov-Bohm (AB) oscillations with a period of h/e, h/2e, h/3e, and h/4e, witnessing a coherence length of many microns. The AB oscillations as well as the type of carriers (electrons or holes) are seamlessly tunable with gating. The coherence length longer than the ring perimeter and semiclassical trajectory of the carrier are established from the analysis of the temperature and magnetic field dependence of the oscillations. Our gate-defined ring geometry has the potential to evolve into a platform for exploring correlated quantum states such as superconductivity in interferometers in twisted bilayer graphene.

cond-mat.mes-hall↗

arXiv2022

A Tunable Monolithic SQUID in Twisted Bilayer Graphene

Magic-angle twisted bilayer graphene (MATBG) hosts a number of correlated states of matter that can be tuned by electrostatic doping. Superconductivity has drawn considerable attention and the mechanism behind it is a topic of active discussion. MATBG has been experimentally characterized by numerous transport and scanning-probe experiments. The material has also emerged as a versatile platform for superconducting electronics, as proven by the realization of monolithic Josephson junctions. However, even though phase-coherent phenomena have been measured, no control of the superconducting phase has been demonstrated so far. Here, we present a Superconducting Quantum Interference Device (SQUID) in MATBG, where the superconducting phase difference is controlled through the magnetic field. We observe magneto-oscillations of the critical current, demonstrating long-range coherence agreeing with an effective charge of 2e for the superconducting charge carriers. We tune to both asymmetric and symmetric SQUID configurations by electrostatically controlling the critical currents through the junctions. With this tunability, we study the inductances in the device, finding values of up to 2μH. Furthermore, we directly observe the current-phase relation of one of the Josephson junctions of the device. Our results show that superconducting devices in MATBG can be scaled up and used to reveal properties of the material. We expect this to foster a more systematic realization of devices of this type, increasing the accuracy with which microscopic characteristics of the material are extracted. We also envision more complex devices to emerge, such as phase-slip junctions or high kinetic inductance detectors.

cond-mat.mes-hall↗

arXiv2021

Negative correlation between the linear and the nonlinear conductance in magnetic tunnel junctions

The current-voltage ($IV$) characteristics beyond the linear response regime of magnetic tunnel junction (MTJ) is systematically investigated. We find a clear negative correlation between the two coefficients to characterize the linear ($I$$\propto$$V$) and the lowest-order nonlinear ($I$$\propto$$V^3$) currents, which holds regardless of the temperature and the thickness of the tunnel barrier. This observation cannot simply be explained by the standard tunneling model such as the Brinkman model, suggesting a mechanism intrinsic to MTJ. We propose a phenomenological model based on the Julliére model that attributes the observed negative correlation to the spin-flip tunneling assisted by a magnon. These results suggest a fundamental law between the linear and the nonlinear response of MTJ.

cond-mat.mes-hall↗

arXiv2021

Interplay of Friction and Structural Asymmetry in Non-Reciprocal Dynamics of a Rolling Prism

We investigate how the dynamics of a hexagonal prism rolling on a floor change with friction and structural asymmetry. It is shown that the asymmetry induces the non-reciprocal dynamics where the prism rolls only in one direction regardless of the direction of the initial velocity. While such behavior is primarily suppressed with increasing friction, we observe that there is a certain range of friction coefficient where the non-reciprocity is restored. This suggests that the friction not only diminishes the dynamics, but also assists it by exerting a torque to the prism.

physics.class-ph↗

arXiv2020

Multiple modes of a single spin torque oscillator under the non-linear region

A numerical investigation is conducted for a single spin-torque oscillator under the non-linear region. A large angle precession triggers the generation of multiple modes without any feedbacked circuits and/or magnetic couplings with neighboring oscillators. Our simulations show that a single eigenmode of a given spin-torque oscillator can trigger up to six discrete modes as the sideband modes. These findings will offer the new functionality to the STO for developing the spintronic logic circuits.

physics.app-ph↗

arXiv2020

Etching process of narrow wire and application to tunable-barrier electron pump

Single electron sources have been studied as a device to establish an electric current standard for 30 years and recently as an on-demand coherent source for Fermion quantum optics. In order to construct the single electron source on a GaAs/AlGaAs two-dimensional electron gas (2DEG), it is often necessary to fabricate a sub-micron wire by etching. We have established techniques to make the wire made of the fragile 2DEG by combining photolithography and electron beam lithography with one-step photoresist coating, which enables us to etch fine and coarse structures simultaneously. It has been demonstrated that a single electron source fabricated on the narrow wire pumps fixed number of electrons per one cycle with radio frequency. The fabrication technique improves the lithography process with lower risk to damage the 2DEG and is applicable to etching of other materials and dry etching.

cond-mat.mes-hall↗

arXiv2020

Generation of Multipeak Spectrum of Spin Torque Oscillator in Non-linear Regime

We investigate the spectral characteristics of spin torque oscillator (STO) excited by the spin Hall-induced spin current. We observe that the modest spin current injection triggers the conventional single peak oscillating behavior of STO. As the spin current is further increased to enter the non-linear regime, we find the transition of the spectrum from a single peak to multipeak structure whose frequency spacing is constant. This behavior can be primarily explained by the extremely broadened peak of the STO, which is accompanied by the frequency-dependent filtering by the transmission line. To explain the observation more quantitatively, we also discuss that the multipeak may reflect the characteristics of the intrinsic dynamics of STO in the non-linear regime.

cond-mat.mes-hall↗

arXiv2017

Dynamics of Pure Spin Current in High-frequency Quantum Regime

Pure spin current is a powerful tool for manipulating spintronic devices, and its dynamical behavior is an important issue. By using mesoscopic transport theory for electron tunneling induced by spin accumulation, we investigate the dynamics of the spin current in the high-frequency quantum regime, where the frequency is much larger than temperature and bias voltage. Besides the thermal noise, frequency-dependent finite noise emerges, signaling the spin current across the tunneling barrier. We also find that the autocorrelation of the spin current exhibits sinusoidal oscillation in time as a consequence of the Pauli exclusion principle even without any net charge current.

cond-mat.mes-hall↗