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Shula Chen

Publications and source records attributed to Shula Chen.

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Gate-Tunable Mid-Infrared Electroluminescence from Te/MoS2 p-n Heterojunctions

Mid-infrared (MIR) emitters are critical components in advanced photonic systems, driving progress in fields such as chemical sensing, environmental monitoring, medical diagnostics, thermal imaging and free-space communications. Conventional MIR emitters based on III-V heterostructures rely on complex epitaxial growth on rigid lattice-matched substrates and suffer from limited integration compatibility with CMOS or flexible platforms. The recent development of novel MIR emitters based on two-dimensional (2D) materials such as black phosphorus (BP) is more suitable for on-chip applications but faces challenges related to stability and emission efficiency. Based on the recently discovered highly efficient photoluminescence of Te, we demonstrate a gate-tunable midinfrared light-emitting diode based on a van der Waals heterojunction formed by multilayer transition metal dichalcogenide (TMD) MoS2 and tellurium (Te). The device emits polarized electroluminescence (EL) centered at 3.5 $\mu$m under forward bias at 25 K, and the EL persists up to 80 K with reduced intensity. Gate control of the MoS2 Fermi level modulates the band alignment and injection efficiency, enabling dynamic tuning of the EL intensity. The emission remains spectrally stable under varying bias and gating, indicating robust band-edge recombination. These results establish the Te/TMD heterostructure as a promising platform for integrated polarized mid-infrared optoelectronics.

cond-mat.mes-hall

Ultrafast carriers' separation imaging in WS2-WSe2 in plane heterojunction by transient reflectivity microscopy

Carrier transport in nanodevices plays a crucial role in determining their functionality. In the post-Moore era, the behavior of carriers near surface or interface domains the function of the whole devices. However, the femtosecond dynamics and nanometer-scale movement of carriers pose challenges for imaging their behavior. Techniques with high spatial-temporal resolution become imperative for tracking their intricate dynamics. In this study, we employed transient reflectivity microscopy to directly visualize the charge separation in the atomic interface of WS2-WSe2 in-plane heterojunctions. The carriers' drifting behavior was carefully tracked, enabling the extraction of drift velocities of 30 nm/ps and 10.6 nm/ps for electrons and holes. Additionally, the width of the depletion layer was determined to be 300 nm based on the carriers' moving trajectory. This work provides essential parameters for the potential effective utilization of these covalent in-plane heterojunctions,and demonstrates the success of transient optical imaging in unraveling the electrical behavior of nano devices, paving the way for a new avenue of electro-optical analysis.

cond-mat.mes-hall