arXiv subjects

Shumpei Uno

Publications and source records attributed to Shumpei Uno.

12 recordsLinked to original sources

arXiv2026

Auger Spectroscopy via Generative Quantum Eigensolver: A Quantum Approach to Molecular Excitations

Auger electron spectroscopy, a way of characterizing electronic structure through core-level decay processes, is widely used in materials characterization; however direct calculation from molecular geometry requires accurate treatment of many excited states, posing a challenge for classical methods. We present a hybrid quantum-classical workflow for calculating Auger spectra that combines the generative quantum eigensolver (GQE) for ground-state preparation, the quantum self-consistent equation-of-motion method for excited-state calculations, and the one-centre approximation for Auger transition rates. GQE uses a GPT-2 model to generate quantum circuits for ground-state optimization, allowing our workflow to benefit from HPC parallelization and GPU-acceleration for favourable scaling with system size. We demonstrate the validity of our workflow by calculating the Auger spectrum of water with the STO-3G basis set and demonstrating qualitative and quantitative agreement with spectra obtained using completely classical full configuration interaction calculations, from the computational literature, and from the experimental literature. We also find that for water, substituting the variational quantum eigensolver (VQE) for GQE results in near-identical spectra, but that the ground state estimator generated by GQE contains about half the total gate count as that generated by VQE.

quant-ph↗

arXiv2024

Adaptive measurement strategy for noisy quantum amplitude estimation with variational quantum circuits

In quantum computation, amplitude estimation is a fundamental subroutine that is utilized in various quantum algorithms. A general important task of such estimation problems is to characterize the estimation lower bound, which is referred to as quantum Cram\'er-Rao bound (QCRB), and to construct an optimal estimator that achieves QCRB. This paper studies the amplitude estimation in the presence of depolarizing noise with unknown intensity. The main difficulty in this problem is that the optimal measurement depends on both the unknown quantum state and the amplitude we aim to estimate. To deal with these issues, we utilize the variational quantum circuits to approximate the (unknown) optimal measurement basis combined with the 2-step adaptive estimation strategy which was proposed in the quantum estimation theory.We numerically show that the proposed method can nearly attain the QCRB.

quant-ph↗

arXiv2022

Generative model for learning quantum ensemble via optimal transport loss

Generative modeling is an unsupervised machine learning framework, that exhibits strong performance in various machine learning tasks. Recently we find several quantum version of generative model, some of which are even proven to have quantum advantage. However, those methods are not directly applicable to construct a generative model for learning a set of quantum states, i.e., ensemble. In this paper, we propose a quantum generative model that can learn quantum ensemble, in an unsupervised machine learning framework. The key idea is to introduce a new loss function calculated based on optimal transport loss, which have been widely used in classical machine learning due to its several good properties; e.g., no need to ensure the common support of two ensembles. We then give in-depth analysis on this measure, such as the scaling property of the approximation error. We also demonstrate the generative modeling with the application to quantum anomaly detection problem, that cannot be handled via existing methods. The proposed model paves the way for a wide application such as the health check of quantum devices and efficient initialization of quantum computation.

quant-ph↗

arXiv2022

Approximate amplitude encoding in shallow parameterized quantum circuits and its application to financial market indicator

Efficient methods for loading given classical data into quantum circuits are essential for various quantum algorithms. In this paper, we propose an algorithm called Approximate Amplitude Encoding that can effectively load all the components of a given real-valued data vector into the amplitude of quantum state, while the previous proposal can only load the absolute values of those components. The key of our algorithm is to variationally train a shallow parameterized quantum circuit, using the results of two types of measurement; the standard computational-basis measurement plus the measurement in the Hadamard-transformed basis, introduced in order to handle the sign of the data components. The variational algorithm changes the circuit parameters so as to minimize the sum of two costs corresponding to those two measurement basis, both of which are given by the efficiently-computable maximum mean discrepancy. We also consider the problem of constructing the singular value decomposition entropy via the stock market dataset to give a financial market indicator; a quantum algorithm (the variational singular value decomposition algorithm) is known to produce a solution faster than classical, which yet requires the sign-dependent amplitude encoding. We demonstrate, with an in-depth numerical analysis, that our algorithm realizes loading of time-series of real stock prices on quantum state with small approximation error, and thereby it enables constructing an indicator of the financial market based on the stock prices.

quant-ph↗

arXiv2022

Efficient quantum readout-error mitigation for sparse measurement outcomes of near-term quantum devices

The readout error on near-term quantum devices is one of the dominant noise factors, which can be mitigated by classical postprocessing called quantum readout error mitigation (QREM). The standard QREM applies the inverse of noise calibration matrix to the outcome probability distribution using exponential computational resources to the number of measured qubits. This becomes infeasible for the current quantum devices with tens of qubits or more. Here we propose two efficient QREM methods finishing in $O(ns^2)$ time for probability distributions of $n$ qubits and $s$ shots, which mainly aim at mitigating sparse probability distributions such that only a few states are dominant. We compare the proposed methods with several recent QREM methods in the following three cases: expectation values of the GHZ state, its fidelities, and the estimation error of maximum likelihood amplitude estimation (MLAE) algorithm with a modified Grover iterator. The two cases of the GHZ state are on real IBM quantum devices, while the third is with numerical simulation. Using the proposed method, the mitigation of the 65-qubit GHZ state takes only a few seconds, and we witness the fidelity of the 29-qubit GHZ state exceeding 0.5. The proposed methods also succeed in reducing the estimation error in the MLAE algorithm, outperforming the results by other QREM methods in general.

quant-ph↗

arXiv2022

Noisy quantum amplitude estimation without noise estimation

Many quantum algorithms contain an important subroutine, the quantum amplitude estimation. As the name implies, this is essentially the parameter estimation problem and thus can be handled via the established statistical estimation theory. However, this problem has an intrinsic difficulty that the system, i.e., the real quantum computing device, inevitably introduces unknown noise; the probability distribution model then has to incorporate many nuisance noise parameters, resulting that the construction of an optimal estimator becomes inefficient and difficult. For this problem, we apply the theory of nuisance parameters (more specifically, the parameter orthogonalization method) to precisely compute the maximum likelihood estimator for only the target amplitude parameter, by removing the other nuisance noise parameters. That is, we can estimate the amplitude parameter without estimating the noise parameters. We validate the parameter orthogonalization method in a numerical simulation and study the performance of the estimator in the experiment using a real superconducting quantum device.

quant-ph↗

arXiv2021

Efficient Construction of a Control Modular Adder on a Carry-Lookahead Adder Using Relative-phase Toffoli Gates

Control modular addition is a core arithmetic function, and we must consider the computational cost for actual quantum computers to realize efficient implementation. To achieve a low computational cost in a control modular adder, we focus on minimizing KQ, defined by the product of the number of qubits and the depth of the circuit. In this paper, we construct an efficient control modular adder with small KQ by using relative-phase Toffoli gates in two major types of quantum computers: Fault-Tolerant Quantum Computers (FTQ) on the Logical layer and Noisy Intermediate-Scale Quantum Computers (NISQ). We give a more efficient construction compared to Van Meter and Itoh's, based on a carry-lookahead adder. In FTQ, $T$ gates incur heavy cost due to distillation, which fabricates ancilla for running $T$ gates with high accuracy but consumes a lot of specially prepared ancilla qubits and a lot of time. Thus, we must reduce the number of $T$ gates. We propose a new control modular adder that uses only 20% of the number of $T$ gates of the original. Moreover, when we take distillation into consideration, we find that we minimize $\text{KQ}_{T}$ (the product of the number of qubits and $T$-depth) by running $Θ\left(n / \sqrt{\log n} \right)$ $T$ gates simultaneously. In NISQ, CNOT gates are the major error source. We propose a new control modular adder that uses only 35% of the number of CNOT gates of the original. Moreover, we show that the $\text{KQ}_{\text{CX}}$ (the product of the number of qubits and CNOT-depth) of our circuit is 38% of the original. Thus, we realize an efficient control modular adder, improving prospects for the efficient execution of arithmetic in quantum computers.

quant-ph↗

arXiv2021

The Present and Future of Discrete Logarithm Problems on Noisy Quantum Computers

The discrete logarithm problem (DLP) is the basis for several cryptographic primitives. Since Shor's work, it has been known that the DLP can be solved by combining a polynomial-size quantum circuit and a polynomial-time classical post-processing algorithm. Evaluating and predicting the instance size that quantum devices can solve is an emerging research topic. In this paper, we propose a quantitative measure based on the success probability of the post-processing algorithm to determine whether an experiment on a quantum device (or a classical simulator) succeeded. We also propose a procedure to modify bit strings observed from a Shor circuit to increase the success probability of a lattice-based post-processing algorithm. We report preliminary experiments conducted on IBM-Quantum quantum computers and near-future predictions based on noisy-device simulations. We conducted our experiments with the ibm_kawasaki device and discovered that the simplest circuit (7 qubits) from a 2-bit DLP instance achieves a sufficiently high success probability to proclaim the experiment successful. Experiments on another circuit from a slightly harder 2-bit DLP instance, on the other hand, did not succeed, and we determined that reducing the noise level by half is required to achieve a successful experiment. Finally, we give a near-term prediction based on required noise levels to solve some selected small DLP and integer factoring instances.

cs.CR↗

arXiv2021

Amplitude estimation via maximum likelihood on noisy quantum computer

Recently we find several candidates of quantum algorithms that may be implementable in near-term devices for estimating the amplitude of a given quantum state, which is a core sub- routine in various computing tasks such as the Monte Carlo methods. One of those algorithms is based on the maximum likelihood estimate with parallelized quantum circuits. In this paper, we extend this method so that it incorporates the realistic noise effect, and then give an experimental demonstration on a superconducting IBM Quantum device. The maximum likelihood estimator is constructed based on the model assuming the depolarization noise. We then formulate the problem as a two-parameters estimation problem with respect to the target amplitude parameter and the noise parameter. In particular we show that there exist anomalous target values, where the Fisher information matrix becomes degenerate and consequently the estimation error cannot be improved even by increasing the number of amplitude amplifications. The experimental demonstration shows that the proposed maximum likelihood estimator achieves quantum speedup in the number of queries, though the estimation error saturates due to the noise. This saturated value of estimation error is consistent to the theory, which implies the validity of the depolarization noise model and thereby enables us to predict the basic requirement on the hardware components (particularly the gate error) in quantum computers to realize the quantum speedup in the amplitude estimation task.

quant-ph↗

arXiv2021

Modified Grover operator for amplitude estimation

In this paper, we propose a quantum amplitude estimation method that uses a modified Grover operator and quadratically improves the estimation accuracy in the ideal case, as in the conventional one using the standard Grover operator. Under the depolarizing noise, the proposed method can outperform the conventional one in the sense that it can in principle achieve the ultimate estimation accuracy characterized by the quantum Fisher information in the limit of a large number of qubits, while the conventional one cannot achieve the same value of ultimate accuracy. In general this superiority requires a sophisticated adaptive measurement, but we numerically demonstrate that the proposed method can outperform the conventional one and approach to the ultimate accuracy, even with a simple non-adaptive measurement strategy.

quant-ph↗

arXiv2020

Analysis and synthesis of feature map for kernel-based quantum classifier

A method for analyzing the feature map for the kernel-based quantum classifier is developed; that is, we give a general formula for computing a lower bound of the exact training accuracy, which helps us to see whether the selected feature map is suitable for linearly separating the dataset. We show a proof of concept demonstration of this method for a class of 2-qubit classifier, with several 2-dimensional dataset. Also, a synthesis method, that combines different kernels to construct a better-performing feature map in a lager feature space, is presented.

quant-ph↗

arXiv2020

Amplitude estimation without phase estimation

This paper focuses on the quantum amplitude estimation algorithm, which is a core subroutine in quantum computation for various applications. The conventional approach for amplitude estimation is to use the phase estimation algorithm, which consists of many controlled amplification operations followed by a quantum Fourier transform. However, the whole procedure is hard to implement with current and near-term quantum computers. In this paper, we propose a quantum amplitude estimation algorithm without the use of expensive controlled operations; the key idea is to utilize the maximum likelihood estimation based on the combined measurement data produced from quantum circuits with different numbers of amplitude amplification operations. Numerical simulations we conducted demonstrate that our algorithm asymptotically achieves nearly the optimal quantum speedup with a reasonable circuit length.

quant-ph↗