arXiv subjects

Shun Fujii

Publications and source records attributed to Shun Fujii.

At least 19 recordsLinked to original sources

arXiv2026

Motion-Tracking Terahertz Time-Domain Spectroscopy Enabled by Time-Programmable Frequency Combs for Moving-Object Sensing

Terahertz time-domain spectroscopy (THz-TDS) provides direct access to both spectral information and time-of-flight features, making it attractive for dynamic sensing. However, conventional high-speed THz-TDS methods typically rely on a fixed delay trajectory, limiting their ability to selectively acquire only the relevant temporal window while tracking target motion. Here, we demonstrate motion-tracking THz-TDS based on time-programmable frequency combs (TPFCs), in which the THz measurement window is actively locked to a moving time-domain waveform. By continuously modulating the phase-lock set point of one TPFC, we perform real-time apodized acquisition of a specific temporal window centered on the main THz peak at rates up to 308 Hz. Simultaneously, the residual peak position within the window is detected in real time and fed back to the other comb, enabling the measurement window to follow target displacements exceeding the original acquisition window. The feedback command together with the residual peak position further enables reconstruction of the relative target displacement. As a proof-of-concept demonstration, we use a moving gold mirror to simulate respiration- and heartbeat-related motion superimposed on a much larger displacement representing body motion, and successfully resolve the two vital-sign-related components from the measured displacement. This work extends arbitrary-delay control with TPFCs to THz-TDS and establishes a motion-compensated spectroscopy platform for simultaneous displacement tracking and THz waveform acquisition.

physics.optics↗

arXiv2026

Ultralong pump-probe movies of magnon and phonon dynamics from ultrafast generation to microsecond relaxation

The long lifetimes of magnons and phonons make them attractive for information-processing devices, highlighting the importance of visualizing their spatiotemporal dynamics from generation through relaxation. Ultrafast pump-probe spectroscopy is a powerful tool for investigating their early-stage dynamics after impulsive excitation; however, their long-lived nature makes it challenging to comprehensively track their evolution across all relevant time scales while maintaining sufficient temporal resolution. Here, we demonstrate spatiotemporal tracking of magnon and phonon dynamics over more than seven orders of magnitude in time, from 500 femtoseconds to 20 microseconds, using $4 \times 10^7$ sampled time points enabled by the highly precise time base of optical frequency combs. The resulting spatiotemporal movie, consisting of $4.5 \times 10^{5}$ frames, captures their generation, coherent motion, propagation, and relaxation, providing a powerful platform for exploring their full dynamical evolution.

physics.optics↗

arXiv2026

Transmission of signals in the 300 GHz band with a bit-error rate below ${10}^{-9}$ using a soliton comb

To address the increasing demand for ultra-high-capacity wireless communication, terahertz (THz) frequencies near 300 GHz are attracting attention as a new spectral frontier. This work presents the first experimental demonstration of error-free (BER $< 1\times10^{-9}$) 10 Gbps transmission in the 300 GHz band using a soliton microcomb generated in an integrated silicon nitride (SiN) microring resonator. While many previous microcomb-based THz demonstrations have focused on coherent modulation formats and operation near the forward-error-correction (FEC) limit, this work investigates a simple intensity-modulation/direct-detection (IM-DD) on-off keying (OOK) architecture suitable for low-complexity THz links and fiber-wireless integrated systems. Although the experiment was conducted in a short back-to-back waveguide configuration, the generated THz wave enabled stable low-BER transmission without FEC or advanced offline signal processing. Analysis of the error-free threshold power indicates the feasibility of free-space transmission over several tens of meters with high-gain antennas and THz-band amplifiers. These results demonstrate the feasibility of robust low-complexity THz photonic links based on soliton microcombs for short-range fiber-wireless integrated systems.

physics.optics↗

arXiv2026

Quantitative cavity-enhanced photothermal dynamics in TMDC-integrated ultrahigh-Q microcavities

We investigate photothermal effects in monolayer transition metal dichalcogenides (TMDCs) integrated with an ultrahigh-Q silica microcavity. Launching a continuous-wave laser into a cavity resonance enables controlled intracavity heating, allowing direct observation of excitonic photoluminescence (PL) modulation. A distinct redshift of the PL peak energy is observed as the pump wavelength is tuned across resonance. This behavior is quantitatively reproduced by a temperature-dependent bandgap model that combines the Varshni relation with the thermo-optic response of the microcavity, from which the local temperature rise can be estimated. We further find that PL collected through a fiber waveguide exhibits spectral and temporal characteristics markedly different from free-space emission, indicating selective coupling of the microcavity to specific excitonic channels. These results provide a quantitative framework for understanding photothermal effects in TMDC-microcavity hybrid systems and offer a versatile approach for all-optical control and probing of thermal states in integrated nanophotonic devices.

physics.optics↗

arXiv2026

Ultrafast acoustic modulation of second-harmonic generation in monolayer transition metal dichalcogenides

High-speed modulation and deterministic control of optical nonlinear processes in nanomaterials are essential for realizing future nanoscale optoelectronic devices. Applying strain is a ubiquitous and versatile approach to deform atomically thin materials, allowing direct modification of their electronic and optical properties. Yet, strain engineering of nonlinear processes has so far relied predominantly on static approaches, which inherently limit modulation speed, reproducibility, and device scalability. Here, we demonstrate ultrafast acoustic modulation of second-harmonic (SH) generation in monolayer transition metal dichalcogenides using surface acoustic waves (SAWs). By employing a fully phase-synchronized SH measurement combined with stroboscopic surface displacement detection, we directly visualize dynamic SH modulation at a frequency of 226 MHz. Moreover, theoretical modeling and determination of photoelastic coefficients enable quantitative extraction of the SAW-induced dynamic strain. Our results establish a direct link between acoustic fields and optical nonlinearities, providing a robust platform for dynamic strain engineering in two-dimensional nanophotonic devices.

physics.app-ph↗

arXiv2026

Toward nanophotonic platforms for solid-state $^{229}$Th nuclear clocks

While the $^{229}$Th nuclear isomer has recently been observed and laser-excited, converting optical nuclear manipulation into a chip-scale solid-state frequency standard remains an open challenge. Here, we present a nanophotonic platform to realize an all-solid-state nuclear clock based on the low-energy isomeric transition of $^{229}$Th embedded in high-$Q$ fluoride photonic resonators. By coupling ensembles of thorium nuclei to confined optical modes, we show that resonant field build-up in the cavity can substantially enhance the nuclear excitation rate, enabling optical interrogation at practical laser intensities. We model the nuclei-photon interaction dynamics and outline a technological roadmap toward addressing this challenge, including resonator fabrication in fluoride crystals, thorium implantation, nuclear excitation with integrated lasers, and on-chip detection of vacuum-ultraviolet photons. As an initial proof of concept, we implant a crystalline fluoride whispering-gallery-mode resonator with $^{229}$Th and assess the impact of implantation-induced damage on resonator performance. Our platform leverages recent advances in materials integration and nanophotonics to chart a realistic route toward compact and scalable nuclear frequency standards.

physics.optics↗

arXiv2025

Systematic dispersion engineering of crystalline microresonators for broadband and coherent frequency comb generation

Ultraprecision machining offers a powerful route to dispersion control in crystalline microresonators, allowing the design of waveguide geometries for tailoring the spectrum of microresonator frequency combs. By precisely designing the geometry, both group-velocity and higher-order dispersions can be engineered across a broad wavelength range. However, despite their promising features, such advantages have remained largely unexplored due to fabrication challenges. Here, we demonstrate that resonators shaped by ultrapecision machining exhibit high precision and strongly suppressed spatial mode interactions, facilitating the generation of smooth dissipative Kerr soliton combs and broadband frequency combs beyond the telecommunication C-band. These results underscore the effectiveness of precision geometry control for realizing coherent and broadband microcombs on crystalline photonic platforms.

physics.optics↗

arXiv2025

Centi-combs: Low-noise sub-GHz repetition-rate soliton frequency combs from crystalline resonators

We demonstrate low-noise Kerr soliton frequency combs with repetition rates below 1~GHz in ultrahigh-Q crystalline magnesium fluoride resonators. Single soliton states with repetition rates of 0.90 GHz, 1.19 GHz, 1.59 GHz, 2.48 GHz, and 4.10 GHz are observed with continuous-wave laser excitation. The near-GHz soliton repetition frequency exhibits a single-sideband phase noise of -137 dBc/Hz at a 100 kHz offset, surpassing state-of-the-art microwave generators. These ``centi-combs'' bridge the gap between conventional mode-locked lasers and microresonator frequency combs, providing a new route towards real-time sampling, optical-to-microwave synchronization, and hybrid optical clock networks in a compact form. This work expands the operational range of Kerr soliton microcombs from the terahertz to the sub-gigahertz domain, opening new frontiers for frequency comb technologies.

physics.optics↗

arXiv2025

Record-high-Q AMTIR-1 microresonators for mid- to long-wave infrared nonlinear photonics

AMTIR-1 chalcogenide glass has shown its potential for use in thermal imaging systems owing to its low refractive index, thermal resistance and high transparency across the infrared wavelength regime. Here we report a millimeter-scale high-Q whispering gallery mode microresonator made of AMTIR-1. The recorded Q-factor has reached $1.2\times10^7$ at 1550 nm, which is almost two-orders of magnitude higher than previously reported values. We characterize the thermal properties, where low thermal conductivity plays an important role in thermal resonance tuning. We further show that AMTIR-1 resonators support anomalous dispersion as well as a low absorption coefficient near the 7~\textmu m wavelength band, thus offering the possibility of providing suitable platforms for mid-infrared, long-wave infrared nonlinear optics including microresonator frequency comb generation.

physics.optics↗

arXiv2024

Architecture for coherent dual-comb spectroscopy and low-noise photonic microwave generation using mechanically actuated soliton microcombs

Dissipative Kerr soliton microcombs have inspired various intriguing applications such as spectroscopy, ranging, telecommunication, and high purity microwave generation. Mechanically actuated soliton microcombs provide enhanced controllability and flexibility for Kerr solitons, thus enabling technological progress to be made on such practical applications. Here, we present architectures for coherent dual-comb techniques and ultralow-noise microwave generation by exploiting the mechanical actuation of ultrahigh-Q crystalline microresonators. By unifying a pump laser, we demonstrate highly coherent dual-soliton combs using distinct resonators with slightly different repetition rates. We also report significant phase noise reduction achieved by directly generating Kerr solitons from a sub-Hz linewidth ultrastable laser. This study paves the way for further advancements in a wide variety of applications based on Kerr soliton microcombs.

physics.optics↗

arXiv2024

Scalable fabrication of erbium-doped high-Q silica microtoroid resonators via sol-gel coating

This study explores sol-gel methods for fabricating erbium-doped silica microtoroid resonators, addressing the limitations of conventional doping techniques and enhancing device scalability. We develop a reproducible sol-gel process that yields defect-free films for photonic applications, and detail common defects and troubleshooting strategies. Two fabrication methods are compared: traditional film deposition on substrates and the direct coating of prefabricated resonators. The latter enables the fabrication of larger resonator diameters (up to 450 {\mu}m) without buckling, while achieving a high-Q factor and a low lasing threshold of 350 {\mu}W. These erbium-doped resonators exhibit multi-mode laser oscillations at 1550 nm, revealing the sol-gel method's potential for realizing scalable, gain-doped photonic devices.

physics.optics↗

arXiv2024

Intrinsic process for upconversion photoluminescence via $K$-momentum phonon coupling in carbon nanotubes

We investigate the intrinsic microscopic mechanism of photon upconversion in air-suspended single-walled carbon nanotubes through photoluminescence and upconversion photoluminescence spectroscopy. Nearly linear excitation power dependence of upconversion photoluminescence intensity is observed, indicating a one-photon process as the underlying mechanism. In addition, we find a strongly anisotropic response to the excitation polarization which reflects the intrinsic nature of the upconversion process. In upconversion photoluminescence excitation spectra, three peaks are observed which are similar to photoluminescence sidebands of the $K$-momentum dark singlet exciton. The features in the upconversion photoluminescence excitation spectra are well reproduced by our second-order exciton-phonon interaction model, enabling the determination of phonon energies and relative amplitudes. The analysis reveals that the upconversion photoluminescence can be described as a reverse process of the sideband emission linked to the $K$-momentum phonon modes. The validity of our model is further reinforced by temperature-dependent upconversion photoluminescence excitation measurements reflecting variations in the phonon population. Our findings underscore the pivotal role of the resonant exciton-phonon coupling in pristine carbon nanotubes and presents potential for advanced optothermal technologies by engineering the excitation pathways.

cond-mat.mes-hall↗

arXiv2024

Hybrid silicon all-optical switching devices integrated with two-dimensional material

We propose and demonstrate hybrid all-optical switching devices that combine silicon nanocavities and two-dimensional semiconductor material. By exploiting the refractive index modulation caused by photo-induced carriers in the two-dimensional material instead of the silicon substrate, we overcome the switching performance limitation imposed by the substrate material. Air-mode photonic crystal nanobeam cavities capable of efficient interaction with two-dimensional materials are fabricated, and molybdenum ditelluride, a two-dimensional material with rapid carrier recombination, is transferred onto the cavities. The molybdenum ditelluride flake is excited by an optical pump pulse to shift the resonant wavelength of the cavity for switching operation. We have successfully achieved all-optical switching operations on the time scale of tens of picoseconds while requiring low switching energies of a few hundred femtojoules.

physics.optics↗

arXiv2023

Spatiotemporal visualization of a surface acoustic wave coupled to magnons across a submillimeter-long sample by pulsed laser interferometry

Surface acoustic waves (SAWs) coupled to magnons have attracted much attention because they allow for the long-range transport of magnetic information which cannot be achieved by magnon alone. We employed pulsed laser interferometry to visualize the entire spatiotemporal dynamics of a SAW that travels on a nickel (Ni) thin film and is coupled to magnons. It was possible to trace the coupling-induced amplitude reduction and phase shift that occurs as the SAW propagates over a distance of 0.4 mm. The observed changes are consistent with results obtained from conventional radio-frequency transmission measurements, which probe the total SAW absorption due to magnon--phonon coupling. This result verifies that our method can accurately capture the spatiotemporal dynamics of a SAW coupled to magnons across the entire length of the sample. Additionally, we validated our time-resolved profiles by comparing them with theoretical results that take the echo wave due to reflection into account. The impact of the echo wave is significant even when it has propagated over a distance on the order of millimeters. Our imaging results highlight the visualization of the long-range propagation of the SAW coupled to magnons and offer more information about the surface vibration profiles in such devices.

cond-mat.mtrl-sci↗

arXiv2023

Van der Waals functionalization of ultrahigh-Q silica microcavities for $\chi^{(2)}$-$\chi^{(3)}$ hybrid nonlinear photonics

Optical nonlinear processes are indispensable in a wide range of applications including ultrafast laser sources, microscopy, metrology, and quantum information technologies. Combinations of the diverse nonlinear processes should further lead to the development of unique functionalities, but simultaneous use of second- and third-order nonlinear processes is generally difficult. Second-order effects usually overwhelm the higher-order ones, except in centrosymmetric systems where the second-order susceptibility vanishes to allow the use of the third-order nonlinearity. Here we demonstrate a hybrid photonic platform whereby the balance between second- and third-order susceptibilities can be tuned flexibly. Ultrahigh-Q silica microcavities capable of generating third-order effects are functionalized by atomically thin tungsten diselenide, and we observe cavity-enhanced second-harmonic generation and sum-frequency generation with continuous-wave excitation at a power level of only a few hundred microwatts. Pump power dependence exhibits drastic increase and saturation of the second-harmonic light, originating from the dynamic phase-matching process. We show that the coexistence of second- and third-order nonlinearities in a single device can be achieved by carefully choosing the size and the location of the two-dimensional material. Our approach can be generalized to other types of cavities, unlocking the potential of hybrid systems with controlled nonlinear susceptibilities for novel applications.

physics.optics↗

arXiv2023

Exceptional point proximity-driven mode-locking in coupled microresonators

We show theoretically and numerically that mode-locking is feasible with a coupled-cavity system with gain and loss, notably, without any natural saturable absorber. We highlight that in the vicinity of the exceptional point, system $Q$ exhibits substantial modulation even with minor refractive index changes and a minimal Kerr effect contribution. Leveraging this unique behaviour, we propose an unprecedented approach wherein the lossy auxiliary cavity functions as an efficient artificial saturable absorber, thus facilitating mode-locking. This approach is not only novel, but also presents considerable advantages over conventional systems where both gain and saturable absorption are contained within a single microcavity. These benefits include reduced operational power and ease of post-adjustment, achievable through the manipulation of the coupling strength between the two microcavities.

physics.optics↗

arXiv2023

Mechanically actuated Kerr soliton microcombs

Mode-locked ultrashort pulse sources with a repetition rate of up to several tens of gigahertz greatly facilitate versatile photonic applications such as frequency synthesis, metrology, radar, and optical communications. Dissipative Kerr soliton microcombs provide an attractive solution as a broadband, high-repetition-rate compact laser system in this context. However, its operation usually requires sophisticated pump laser control to initiate and stabilize the soliton microcombs, particularly in millimeter-sized ultrahigh-Q whispering-gallery resonators. Here, we realize a mechanically actuated soliton microcomb oscillator with a microwave repetition rate of 15 GHz. This enables direct soliton initiation, long-term stabilization, and fine tuning, where the operation now lifts the prerequisite pump laser tunability that must be relaxed if the technology is to be widely used outside the laboratory environment. We reveal the prospects for using this method with a wide range of applications that would benefit from mechanical soliton actuation such as optical clocks, spectral extension, and dual-comb spectroscopy.

physics.optics↗

arXiv2023

A two-color dual-comb system for time-resolved measurements of ultrafast magnetization dynamics using triggerless asynchronous optical sampling

We report on an Er-doped fiber (EDF)-laser-based dual-comb system that allows us to perform triggerless asynchronous optical sampling (ASOPS) pump-probe measurements of ultrafast demagnetization and spin precession in magnetic materials. Because the oscillation frequencies of the two frequency-comb light sources are highly stabilized, the pulse-to-pulse timing jitter is sufficiently suppressed and data accumulation without any trigger signals is possible. To effectively induce spin precession in ferromagnetic thin films, the spectral bandwidth of the output of one of the EDF frequency comb sources is broadened by a highly nonlinear fiber and then amplified at a wavelength of about 1030 nm by a Yb-doped fiber amplifier. The output of the other frequency comb source is converted to about 775 nm by second harmonic generation. We used this system to observe the ultrafast demagnetization and spin precession dynamics on the picosecond and nanosecond time scales in a permalloy thin film. This time-domain spectroscopy system is promising for the rapid characterization of spin-wave generation and propagation dynamics in magnetic materials.

physics.app-ph↗