arXiv subjects

Shunfa Liu

Publications and source records attributed to Shunfa Liu.

13 recordsLinked to original sources

arXiv2026

Structured Cavity Quantum Electrodynamics

A cavity quantum electrodynamics (cQED) system consisting of a confined single photon and a single quantum emitter serves as a fundamental block for quantum optics and photonic quantum technologies. The canonical optical mode employed in the conventional cavity quantum electrodynamics features a uniform polarization distribution, leading to the scalar light-matter interaction in most existing experiments. Despite the rapid progress in the generation of structured light with spatially varied polarizations, the structured light-matter interaction, especially at the single quanta level, is highly intriguing yet largely unexplored. Here, we present the structured light-matter interaction at the single-photon level in a semiconductor cavity quantum electrodynamics system. Four distinct structured cavity modes that are spectrally close to each other are constructed in a micropillar cavity. By spatially locating a single epitaxial quantum dot (QD) at the periphery of a semiconductor micropillar cavity and spectrally tuning the QD emission wavelength into the resonances of the structured cavity modes, cavity-enhanced single-photon emissions with spin-locked chiral orbital angular momentum (OAM) and engineerable spin-orbit entanglements are achieved within a single wavelength-scale device. Our work opens an unexplored paradigm of structured quantum light-matter interactions and may further advance chiral quantum optics and high-dimensional photonic quantum technology.

physics.optics↗

arXiv2026

High-performance Sources of Multidimensionally Engineered Quantum Light Based on Monolithic Microcavity-metalens Interfaces

The ultimate non-classic light sources for modern photonic quantum technology require on-demand generation of indistinguishable quantum light with high brightness and flexible engineering of quantum emission in multiple degrees of freedom. In this work, we present monolithic microcavity-metalens interfaces consisting of quantum-dot-micropillar single-photon sources and ultra-thin metalenses accurately aligned on opposite sides of an III-V compound semiconductor chip. The pronounced cavity quantum electrodynamics effect enabled by the micropillar cavity facilitates single-photon emission from quantum dots with simultaneous high degrees of single-photon purity, source brightness and photon indistinguishability while the multi-functional metalenses concurrently tailor quantum emission in multiple physical degrees of freedom including radiation divergence, emission directionality, polarization state and orbital angular momentum (OAM). Furthermore, high-fidelity polarization-OAM entanglement and single photons with local spin topologies are successfully generated in our integrated device. In particular, we demonstrate stable propagations of single-photon skrymions in atmospheric turbulence and reveal their topological advantages over the conventional structured quantum light. Our work advances the research fields of integrated quantum photonics and meta-optics, providing integrated high-dimensional quantum light sources for advanced photonic quantum science and technology.

physics.optics↗

arXiv2025

In-situ three-dimensional strain engineering of solid-state quantum emitters in photonic structures towards scalable quantum networks

Solid-state quantum emitters are pivotal for modern photonic quantum technology, yet their inherent spectral inhomogeneity imposes a critical challenge in pursuing scalable quantum network. Here, we develop a cryogenic-compatible strain-engineering platform based on a polydimethylsiloxane (PDMS) stamp that is not obviously working properly at cryogenic temperature. In-situ three-dimensional (3D) strain control is achieved for quantum dots (QDs) embedded in photonic nanostructures. The compliant PDMS enables independent tuning of emission energy and elimination of fine structure splitting (FSS) of single QDs, as demonstrated by a 7 meV spectral shift with a near-vanishing FSS in circular Bragg resonators and an unprecedented 15 meV tuning range in the micropillar. The PDMS-based 3D strain-engineering platform, compatible with diverse photonic structures at cryogenic temperature, provides a powerful and versatile tool for exploring fundamental strain-related physics and advancing integrated photonic quantum technology.

physics.optics↗

arXiv2023

Telecom band quantum dot technologies for long-distance quantum networks

A future quantum internet is expected to generate, distribute, store and process quantum bits (qubits) over the globe by linking different quantum nodes via quantum states of light. To facilitate the long-haul operations, quantum repeaters, the building blocks for a long-distance quantum network, have to be operated in the telecom wavelengths to take advantage of both the low-loss fiber network and the well-established technologies for optical communications. Semiconductors quantum dots (QDs) so far have exhibited exceptional performances as key elements, i.e., quantum light sources and spin-photon interfaces, for quantum repeaters, but only in the near-infrared (NIR) regime. Therefore, the development of high-performance telecom-band QD devices is highly desirable for a future solid-state quantum internet based on fiber networks. In this review, we present the physics and the technological developments towards epitaxial QD devices emitting at the telecom O- and C-bands for quantum networks by using advanced epitaxial growth for direct telecom emission, and quantum frequency conversion (QFC) for telecom-band down-conversion. We also discuss the challenges and opportunities in the future to realize telecom QD devices with improved performances and expanded functionalities by taking advantage of hybrid integrations.

quant-ph↗

arXiv2023

Super-resolved snapshot hyperspectral imaging of solid-state quantum emitters for high-throughput integrated quantum technologies

Solid-state quantum emitters coupled to integrated photonic nanostructures are quintessential for exploring fundamental phenomena in cavity quantum electrodynamics and widely employed in photonic quantum technologies such as non-classical light sources, quantum repeaters, and quantum transducers, etc. One of the most exciting promises from integrated quantum photonics is the potential of scalability that enables massive productions of miniaturized devices on a single chip. In reality, the yield of efficient and reproducible light-matter couplings is greatly hindered by the spectral and spatial mismatches between the single solid-state quantum emitters and confined or propagating optical modes supported by the photonic nanostructures, preventing the high-throughput realization of large-scale integrated quantum photonic circuits for more advanced quantum information processing tasks. In this work, we introduce the concept of hyperspectral imaging in quantum optics, for the first time, to address such a long-standing issue. By exploiting the extended mode with a unique dispersion in a 1D planar cavity, the spectral and spatial information of each individual quantum dot in an ensemble can be accurately and reliably extracted from a single wide-field photoluminescence image with super-resolutions. With the extracted quantum dot positions and emission wavelengths, surface-emitting quantum light sources and in-plane photonic circuits can be deterministically fabricated with a high-throughput by etching the 1D confined planar cavity into 3D confined micropillars and 2D confined waveguides. Further extension of this technique by employing an open planar cavity could be exploited for pursuing a variety of compact quantum photonic devices with expanded functionalities for large-scale integration. Our work is expected to change the landscape of integrated quantum photonic technology.

physics.optics↗

arXiv2023

Dynamic resonance fluorescence in solid-state cavity quantum electrodynamics

The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.

quant-ph↗

arXiv2023

Bright Semiconductor Single-Photon Sources Pumped by Heterogeneously Integrated Micropillar lasers with Electrical Injections

The emerging hybrid integrated quantum photonics combines advantages of different functional components into a single chip to meet the stringent requirements for quantum information processing. Despite the tremendous progress in hybrid integrations of III-V quantum emitters with silicon-based photonic circuits and superconducting single-photon detectors, on-chip optical excitations of quantum emitters via miniaturized lasers towards single-photon sources (SPSs) with low power consumptions, small device footprints and excellent coherence properties is highly desirable yet illusive. In this work, we present realizations of bright semiconductor singe-photon sources heterogeneously integrated with on-chip electrically-injected microlasers. Different from previous one-by-one transfer printing technique implemented in hybrid quantum dot (QD) photonic devices, multiple deterministically coupled QD-circular Bragg Grating (CBG) SPSs were integrated with electrically-injected micropillar lasers at one time via a potentially scalable transfer printing process assisted by the wide-field photoluminescence (PL) imaging technique. Optically pumped by electrically-injected microlasers, pure single photons are generated with a high-brightness of a count rate of 3.8 M/s and an extraction efficiency of 25.44%. Such a high-brightness is due to the enhancement by the cavity mode of the CBG, which is confirmed by a Purcell factor of 2.5. Our work provides a powerful tool for advancing hybrid integrated quantum photonics in general and boosts the developments for realizing highly-compact, energy-efficient and coherent SPSs in particular.

quant-ph↗

arXiv2021

Double-Pulse Generation of Indistinguishable Single Photons with Optically Controlled Polarization

Single-photon sources play a key role in photonic quantum technologies. Semiconductor quantum dots can emit indistinguishable single photons under resonant excitation. However, the resonance fluorescence technique typically requires cross-polarization filtering which causes a loss of the unpolarized quantum dot emission by 50%. To solve this problem, we demonstrate a method to generate indistinguishable single photons with optically controlled polarization by two laser pulses off-resonant with neutral exciton states. This scheme is realized by exciting the quantum dot to the biexciton state and subsequently driving the quantum dot to an exciton eigenstate. Combining with magnetic field, we demonstrated the generation of photons with optically controlled polarization (polarization degree of 101(2)%), laser-neutral exciton detuning up to 0.81 meV, high single-photon purity (99.6(1)%) and indistinguishability (85(4)%). Laser pulses can be blocked using polarization and spectral filtering. Our work makes an important step towards indistinguishable single-photon sources with near-unity collection efficiency.

quant-ph↗

arXiv2021

Tailoring solid-state single-photon sources with stimulated emissions

The coherent interaction of electromagnetic fields with solid-state two-level systems can yield deterministic quantum light sources for photonic quantum technologies. To date, the performance of semiconductor single-photon sources based on three-level systems is limited mainly due to a lack of high photon indistinguishability. Here, we tailor the cavity-enhanced spontaneous emission from a ladder-type three-level system in a single epitaxial quantum dot (QD) through stimulated emission. After populating the biexciton (XX) of the QD through two-photon resonant excitation (TPE), we use another laser pulse to selectively depopulate the XX state into an exciton (X) state with a predefined polarization. The stimulated XX-X emission modifies the X decay dynamics and yields improved polarized single-photon source characteristics such as a source brightness of 0.030(2), a single-photon purity of 0.998(1), and an indistinguishability of 0.926(4). Our method can be readily applied to existing QD single-photon sources and expands the capabilities of three-level systems for advanced quantum photonic functionalities.

physics.optics↗

arXiv2021

Nanoscale positioning approaches for integrating single epitaxial quantum emitters with photonic nanostructures

Deterministically integrating single solid-state quantum emitters with photonic nanostructures serves as a key enabling resource in the context of photonic quantum technology. Due to the random spatial location of many widely-used solid-state quantum emitters, a number of positoning approaches for locating the quantum emitters before nanofabrication have been explored in the last decade. Here, we review the working principles of several nanoscale positioning methods and the most recent progress in this field, covering techniques including atomic force microscopy, scanning electron microscopy, confocal microscopy with \textit{in situ} lithography, and wide-field fluorescence imaging. A selection of representative device demonstrations with high-performance is presented, including high-quality single-photon sources, bright entangled-photon pairs, strongly-coupled cavity QED systems, and other emerging applications. The challenges in applying positioning techniques to different material systems and opportunities for using these approaches for realizing large-scale quantum photonic devices are discussed.

physics.optics↗

arXiv2021

Dual-Resonance Enhanced Quantum Light-Matter Interactions In Deterministically Coupled Quantum-Dot-Micopillars

Optical microcavities have widely been employed to enhance either the optical excitation or the photon emission processes for boosting light matter interactions at nanoscale. When both the excitation and emission processes are simultaneously facilitated by the optical resonances provided by the microcavities, as referred to the dual-resonance condition in this article, the performances of many nanophotonic devices approach to the optima. In this work, we present versatile accessing of dual-resonance conditions in deterministically coupled quantum-dot(QD)-micopillars, which enables emission from exciton (X) - charged exciton (CX) transition with improved single-photon purity. In addition, the rarely observed up-converted single-photon emission process is achieved under dual-resonance condition. We further exploit the vectorial nature of the high-order cavity modes to significantly improve the excitation efficiency under the dual-resonance condition. The dual-resonance enhanced light-matter interactions in the quantum regime provides a viable path for developing integrated quantum photonic devices based on cavity quantum electrodynamics (QED) effect e.g., highly-efficient quantum light sources and quantum logical gates.

physics.optics↗

arXiv2020

A highly efficient integrated source of twisted single-photons

Photons with a helical phase front (twisted photons) can carry a discrete, in principle, unbounded amount of orbital angular momentum (OAM). Twisted single-photons have been demonstrated as a high-dimensional quantum system with information processing ability far beyond the widely used two-level qubits. To date, the generations of single-photons carrying OAM merely rely on the non-linear process in bulk crystals, e.g., spontaneous parametric down-conversion (SPDC), which unavoidably limits both the efficiency and the scalability of the source. Therefore, an on-demand OAM quantum light source on a semiconductor chip is yet illusive and highly desirable for integrated photonic quantum technologies. Here we demonstrate highly-efficient emission of twisted single-photons from solid-state quantum emitters embedded in a microring with angular gratings. The cavity QED effect allows the generations of single-photons and encoding OAM in the same nanostructure and therefore enables the realization of devices with very small footprints and great scalability. The OAM states of singe-photons are clearly identified via quantum interference of single-photons with themselves. Our device may boost the development of integrated quantum photonic devices with potential applications towards high-dimensional quantum information processing.

physics.optics↗

arXiv2019

Quantum Frequency Conversion of a Quantum Dot Single-Photon Source on a Nanophotonic Chip

Single self-assembled InAs/GaAs quantum dots are promising bright sources of indistinguishable photons for quantum information science. However, their distribution in emission wavelength, due to inhomogeneous broadening inherent to their growth, has limited the ability to create multiple identical sources. Quantum frequency conversion can overcome this issue, particularly if implemented using scalable chip-integrated technologies. Here, we report the first demonstration of quantum frequency conversion of a quantum dot single-photon source on a silicon nanophotonic chip. Single photons from a quantum dot in a micropillar cavity are shifted in wavelength with an on-chip conversion efficiency of approximately 12 %, limited by the linewidth of the quantum dot photons. The intensity autocorrelation function g(2)(tau) for the frequency-converted light is antibunched with g(2)(0) = 0.290 +/- 0.030, compared to the before-conversion value g(2)(0) = 0.080 +/- 0.003. We demonstrate the suitability of our frequency conversion interface as a resource for quantum dot sources by characterizing its effectiveness across a wide span of input wavelengths (840 nm to 980 nm), and its ability to achieve tunable wavelength shifts difficult to obtain by other approaches.

quant-ph↗