arXiv subjects

Shuyao Qiu

Publications and source records attributed to Shuyao Qiu.

6 recordsLinked to original sources

arXiv2026

Real-Space Imaging of Guided Exciton Polaritons in Free-standing Monolayer WSe2

Monolayers of transition metal dichalcogenides (TMDCs), known for their strong excitonic states with high binding energies in the visible spectrum at room temperature, offer great potential for polariton-driven devices. While polariton guided modes in bulk TMDCs have been reported the real space experimental observation of 2D exciton-polariton guided modes in a monolayer remains challenging due to various mode cut-off conditions that arise as the TMDC layer becomes thinner, including cut-off frequency, mode confinement and boundary conditions. Here using scanning near-field optical microscopy (s-SNOM), we directly visualized the real-space propagation of these guided modes for the first time in an angstrom-thick, suspended monolayer of WSe2. Through numerical simulations we have also validated that the guided mode can only exist in a monolayer WSe2 when symmetric cladding conditions are closely applied. By tuning the excitation laser energy and analysing the guided mode distribution, we observed a pronounced back-bending dispersion around the A exciton, indicating strong light-matter interactions, and confirmed the existence of the fundamental TE0 exciton polariton (EP) propagation mode. The unique dispersion characteristics of these modes were further validated through theoretical modelling of the mode in free-standing monolayer WSe2. Our findings provide crucial experimental evidence of guided mode EPs in atomically thin TMDCs, opening new possibilities for nanoscale photonic applications.

physics.optics↗

arXiv2025

Counter-propagating Entangled Photon Pairs from a Monolayer

Non-phase-matched spontaneous parametric down-conversion (SPDC) in atomically thin materials provides new degrees of freedom and enhanced quantum information capacity compared to conventional phase-matched sources. These systems emerged as promising platforms for quantum computing, communication, and imaging, with the potential to support higher-order nonlinear processes. However, direct observation of photon-pair emission from a monolayer has remained experimentally challenging. In this work, we theoretically modeled SPDC emission across the full angular space from a monolayer GaSe film and experimentally validated the model through measurements of both co- and counter-propagating photon pairs. We demonstrated two-photon quantum correlations in the telecom C-band from the thinnest SPDC source reported to date. The spatially symmetric, broadband emission predicted by theory was confirmed experimentally. Furthermore, we observed high-fidelity Bell states in the counter-propagating configuration, marking the first realization of polarization-entangled photon pairs from a monolayer. Our results revealed the emission characteristics of SPDC in the deeply subwavelength, non-phase-matched regime, and introduced atomically thin, counterpropagating SPDC as a scalable and integrable platform for programmable quantum state generation, extendable via moiré superlattice engineering.

quant-ph↗

arXiv2025

Enhanced photon-pair generation from a van der Waals metasurface

Quantum photon pairs play a pivotal role in many quantum applications. Metasurfaces, two-dimensional arrays of nanostructures, have been studied intensively to enhance and control pair generation via spontaneous parametric downconversion (SPDC). Van der Waals (VdW) layered materials have emerged as promising candidates for nonlinear materials in quantum light sources, owing to their high nonlinear susceptibility and compatibility with on-chip integration. In this work, we present the first demonstration of SPDC from a metasurface composed of the VdW material 3R-MoS2. The nanoresonators support quasi-bound states in the continuum (qBIC) with a quality factor of up to 120, enhancing light-matter interactions. This design achieves a 20-fold increase in SPDC rate compared to an unstructured film and significantly higher brightness, resulting in enhanced quantum photon-pair generation. This work establishes a new approach for utilizing van der Waals metasurfaces in the generation of quantum photon pairs, opening avenues for advanced quantum applications.

physics.optics↗

arXiv2025

Giant Second Harmonic Generation from 3R-MoS$_2$ Metasurfaces

Metasurfaces have long served as a cornerstone technique to enhance nonlinear processes, enabling frequency conversion, efficient light manipulation and integrated photonic devices. However, traditional bulk materials often suffer from high absorption losses, hindering the second harmonic generation (SHG) efficiency. Here, we develop a novel approach exploiting quasi-bound state in continuum (qBIC) to achieve giant SHG efficiency in metasurfaces utilizing 3R-MoS$_2$, with high index, superior damage threshold and inherent nonlinearity. The high refractive index of 3R-MoS$_2$, facilitates the high-quality factor (Q) metasurfaces, leading to reduced radiation leakage and localized light confinement within qBIC resonances, with which a remarkable 2000-fold enhancement in SHG intensity has been experimentally demonstrated. Additionally, the twist angle between the lattice orientation and the metasurface unit geometry exhibits a 120$^\circ$ periodicity in its influence on SHG behaviour. By strategically designing to realize the qBIC and exciton dual resonances and optimized twist angle (30$^\circ$), SHG conversion efficiency was boosted to ~1%, which is around 2 orders of magnitude higher than those of the best metasurfaces on traditional bulk materials. This approach enables potential applications in various areas of nonlinear optics, including frequency conversion, light manipulation, integrated photonics, and quantum communications.

physics.app-ph↗

arXiv2025

Optical Visualization of Carrier Surfing in 2D Monolayers Driven by Surface Acoustic Waves

Charge carrier transport is pivotal in advancing nanoelectronics. Despite progress in exciton transport within ultra-thin semiconductors, the intertwined transport of free carriers and excitons presents challenges. Surface Acoustic Waves (SAWs) offer a compelling solution, enabling remote, real-time control of excitonic states at room temperature via surfing carriers in 2D materials, a relatively unexplored domain. SAWs create a versatile platform for tailoring excitonic states from microwave to optical frequencies. This study first demonstrates a simple route to visualize directional light transport and carriers drift driven by non-perfect Rayleigh-SAWs. We observed a maximum drift velocity of ~16.4 um/s for ionized carriers with SAW, significantly surpassing their natural movement in monolayers, though free electrons drift remains in the order of ~103 m/s. Enhanced exciton emission was achieved through standing SAWs, generating periodic oscillations. By combining traveling and standing wave portions, controllable, on-demand single-chip emission is feasible. Our findings open avenues for light manipulation, photonic circuits, and on-chip communications technologies.

physics.optics↗

arXiv2024

Nonlinear chiral metasurfaces based on structured van der Waals materials

Nonlinear chiral photonics explores nonlinear response of chiral structures, and it offers a pathway to novel optical functionalities not accessible through linear or achiral systems. Here we present the first application of nanostructured van der Waals materials to nonlinear chiral photonics. We demonstrate the three orders of magnitude enhancement of the third-harmonic generation from hBN metasurfaces driven by quasi-bound states in the continuum and accompanied by strong nonlinear circular dichroism at the resonances. This novel platform for chiral metaphotonics can be employed for achieving large circular dichroism combined with high-efficiency harmonic generation in a broad frequency range.

physics.optics↗