arXiv subjects

Shyam Raj Karullithodi

Publications and source records attributed to Shyam Raj Karullithodi.

3 recordsLinked to original sources

arXiv2026

Giant Exfoliation Induced Magnetic Coercivity in Fe$_3$GaTe$_2$

Permanent magnets with strong anisotropy and high coercivity underpin modern information and energy technologies, yet rare-earth-free alternatives remain limited. Here, we show that thickness engineering via mechanical exfoliation induces hard magnetic behavior in the van der Waals ferromagnet Fe$_3$GaTe$_2$. Bulk crystals exhibit Curie temperatures above 350 K but negligible room-temperature coercivity. When thinned below 100 nm, the coercive field is dramatically enhanced, reaching nearly 1 T at room temperature for in-plane fields which is comparable to values of conventional hard magnets. Micromagnetic analysis reveals a crossover in magnetization reversal from domain-mediated processes in bulk samples to quasi-coherent rotation in thin flakes, driven by increased effective anisotropy and suppressed domain formation. This thickness-dependent transition enables tuning of magnetic hardness without chemical modification. Combined with high saturation magnetization and robust room-temperature performance, Fe$_3$GaTe$_2$ emerges as a promising rare-earth-free material for spintronic applications. Its layered structure further allows integration into van der Waals heterostructures, where large in-plane coercivity can stabilize magnetic states against perturbations and interlayer coupling, offering potential for high-density nonvolatile memory and domain-wall-based devices.

cond-mat.mtrl-sci↗

arXiv2026

Topological Hall Effect in Antiferromagnetic Co doped Fe$_3$GaTe$_2$

Fe$_3$GaTe$_2$ is van der Waals (vdW) ferromagnet with a Curie temperature $T_C$ ranging from 350 K to 380 K, followed upon cooling by a ferrimagnetic transition near room temperature. Substituting Fe with Co was previously reported to induce antiferromagnetism (AFM) at a Co fraction dependent Neel temperature $T_N$. In this work, we confirm the overall phase diagram of the Fe$_{3-x}$Co$_x$GaTe$_2$ series as a function of $x$ and temperature via magnetization and electrical transport measurements. For $x \simeq 0.6$ the Hall effect is observed to mimic the magnetization as the AF ground state is suppressed by the external magnetic field via a metamagnetic transition, thus displaying an anomalous Hall response. At low temperatures, we also observe a pronounced topological Hall signal peaking at $μ_0H$ = 4 T, or within the metamagnetic transition region of fields. This observation points to the presence of magnetic field-induced chiral spin textures, such as skyrmions upon approaching magnetization saturation. Magnetic force microscopy (MFM) reveals the emergence of nearly circular magnetic domains, with diameters on the order of 100 to 200 nm, within the antiferromagnetic phase. A detailed analysis of the MFM images indicates that the topological Hall effect is closely linked to the field-induced stabilization of magnetic domain structures, likely exhibiting chiral textures. This observation suggests the possible formation of skyrmions already in the AFM phase, i.e., AFM skyrmions, that evolve into ferromagnetic (FM) ones upon increasing the magnetic field. Consequently, Co-doped Fe$_3$GaTe$_2$ might provide a platform to investigate the transformation of skyrmions, initially coupled antiferromagnetically into ferromagnetic skyrmions, and to explore its impact on the topological and skyrmion Hall effects.

cond-mat.mes-hall↗

arXiv2025

Type-II Weyl nodes, flat bands, and evidence for a topological Hall-effect in the new ferromagnet FeCr$_3$Te$_6$

The interplay between linearly dispersing or Dirac-like, and flat electronic bands, for instance, in the kagome ferromagnets, has attracted attention due to a possible interplay between topology and electronic correlations. Here, we report the synthesis, structural, electrical, and magnetic properties of a single-crystalline ferromagnetic compound, namely Fe$_{1/3}$CrTe$_2$ or FeCr$_3$Te$_6$, which crystallizes in the $P\bar{3}m1$ space group instead of the $I2/m$ previously reported for FeCr$_2$Te$_4$. Electronic band structure calculations reveal type-II Dirac nodes and relatively flat bands near the Fermi level ($\varepsilon_F$). This compound shows onset Curie temperature $T_{\text{c}}\simeq 120$ K, followed by an additional ferromagnetic transition near $T_{\text{c2}} \sim 92.5 $ K. Below $T_{\text{c}}$, FeCr$_3$Te$_6$ displays a pronounced anomalous Hall effect, as well as sizable coercive fields that exceed $μ_0H = 1$~T at low $T$s. However, a scaling analysis indicates that the anomalous Hall effect results from a significant intrinsic contribution, as expected from the calculations, but also from the extrinsic mechanism, i.e., scattering. The extrinsic contribution probably results from occupational disorder at the 1b Fe-site within the van der Waals gap of the CrTe$_2$ host. We also observe evidence for a topological Hall component superimposed onto the overall Hall response, suggesting the presence of chiral spin textures akin to skyrmions in this centrosymmetric system. Their possible presence will require experimental confirmation.

cond-mat.other↗