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Si-Yu Li

Publications and source records attributed to Si-Yu Li.

At least 55 records · Page 3Linked to original sources

Tibet's Ali: A New Window to Detect the CMB Polarization

The Cosmic Microwave Background (CMB) Polarization plays an important role in current cosmological studies. CMB B-mode polarization is the most effective probe to primordial gravitational waves (PGWs) and a test of the inflation as well as other theories of the early universe such as bouncing and cyclic universe. So far, major ground-based CMB polarization experiments are located in the southern hemisphere.Recently, China has launched the Ali CMB Polarization Telescope (AliCPT) in Tibetan Plateau to measure CMB B mode polarization and detect the PGWs in northern hemisphere. AliCPT include two stages, the first one is to build a telescope at the 5250m site (AliCPT-1) and the second one is to have a more sensitive telescope at a higher altitude of about 6000m (AliCPT-2). In this paper, we report the atmospherical conditions, sky coverage and the current infrastructure associated with AliCPT. We analyzed the reanalysis data from MERRA-2 together with radiosonde data from the Ali Meteorological Service and found that the amount of water vapor has a heavy seasonal variation and October to March is the suitable observation time. We also found 95/150 GHz to be feasible for AliCPT-1 and higher frequencies to be possible for AliCPT-2. Then we analyzed the observable sky and the target fields, and showed that Ali provides us a unique opportunity to observe CMB with less foreground contamination in the northern hemisphere and is complementary to the existed southern CMB experiments. Together with the developed infrastructure, we point out that Ali opens a new window for CMB observation and will be one of the major sites in the world along with Antarctic and Atacama.

astro-ph.IM↗

The tunnelling spectra of quasi-free-standing graphene monolayer

With considering the great success of scanning tunnelling microscopy (STM) studies of graphene in the past few years, it is quite surprising to notice that there is still a fundamental contradiction about the reported tunnelling spectra of quasi-free-standing graphene monolayer. Many groups observed V-shape spectra with linearly vanishing density-of-state (DOS) at the Dirac point, whereas, the others reported spectra with a gap of 60 meV pinned to the Fermi level in the quasi-free-standing graphene monolayer. Here we systematically studied the two contradicted tunnelling spectra of the quasi-free-standing graphene monolayer on several different substrates and provided a consistent interpretation about the result. The gap in the spectra arises from the out-of-plane phonons in graphene, which mix the Dirac electrons at the Brillouin zone corners with the nearly free-electron states at the zone center. Our experiment indicated that interactions with substrates could effectively suppress effects of the out-of-plane phonons in graphene and enable us to detect only the DOS of the Dirac electrons in the spectra. We also show that it is possible to switch on and off the out-of-plane phonons of graphene at the nanoscale, i.e., the tunnelling spectra show switching between the two distinct features, through voltage pulses applied to the STM tip.

cond-mat.mtrl-sci↗

Scanning tunneling microscopy and spectroscopy of nanoscale twisted bilayer graphene

Nanoscale twisted bilayer graphene (TBG) is quite instable and will change its structure to Bernal (or AB-stacking) bilayer with a much lower energy. Therefore, the lack of nanoscale TBG makes its electronic properties not accessible in experiment up to now. In this work, a special confined TBG is obtained in the overlaid area of two continuous misoriented graphene sheets. The width of the confined region of the TBG changes gradually from about 22 nm to 0 nm. By using scanning tunnelling microscopy, we studied carefully the structure and the electronic properties of the nanoscale TBG. Our results indicate that the low-energy electronic properties, including twist-induced van Hove singularities (VHSs) and spatial modulation of local density-of-state, are strongly affected by the translational symmetry breaking of the nanoscale TBG. Whereas, the electronic properties above the energy of the VHSs are almost not influenced by the quantum confinement even when the width of the TBG is reduced to only a single moire spot.

cond-mat.mes-hall↗

Evidence of electron-electron interactions around Van Hove singularities of a graphene Moiré superlattice

A variety of new and interesting correlated states have been predicted in graphene monolayer doped to Van Hove singularities (VHSs) of its density-of-state (DOS). However, tuning the Fermi energy to reach a VHS of graphene by either gating or chemical doping is prohibitively difficult, owning to their large energy distance (3 eV). Therefore, these correlated states, which arise from effects of strong electron-electron interactions at the VHSs, have remained experimentally elusive. Here, we report experimental evidences of electron-electron interactions around the VHSs of a twisted bilayer graphene (TBG) through scanning tunneling microscopy measurements. By introducing a small twisted angle between two adjacent graphene sheets, we are able to generate low-energy VHSs arbitrarily approaching the Fermi energy. The split of the VHSs are observed and the symmetry breaking of electronic states around the VHSs are directly visualized. These results experimentally demonstrate the important effects of electron-electron interactions on electronic properties around the VHSs of the TBG, therefore providing motivation for further theoretical and experimental studies in graphene systems with considering many-body interactions.

cond-mat.mes-hall↗

Landau quantization of Dirac fermions in graphene and its multilayer

When electrons are confined in a two dimensional (2D) system, typical quantum mechanical phenomena such as Landau quantization can be detected. Graphene systems, including the single atomic layer and few-layer stacked crystals, are ideal 2D materials for studying a variety of quantum mechanical problems. In this article, we review the experimental progress in the unusual Landau quantized behaviors of Dirac fermions in monolayer and multilayer graphene by using scanning tunneling microscopy(STM) and scanning tunneling spectroscopy(STS). Through STS measurement of the strong magnetic fields, distinct Landau-level spectra and rich level splitting phenomena are observed in different graphene layers. These unique properties provide an effective method for identifying the number of layers, as well as the stacking orders, and investigating the fundamentally physical phenomena of graphene. Moreover, in the presence of a strain and charged defects, the Landau quantization of graphene can be significantly modified, leading to unusual spectroscopic and electronic properties.

cond-mat.mes-hall↗

Imaging the dynamics of individual hydrogen atom intercalated between two graphene sheets

The interlayer gallery between two adjacent sheets of van der Waals materials is expected to modify properties of atoms and molecules confined at the atomic interfaces. Here, we directly image individual hydrogen atom intercalated between two graphene sheets and investigate its dynamics by scanning tunnelling microscope (STM). The intercalated hydrogen atom is found to be remarkably different from atomic hydrogen chemisorbed on external surface of graphene. Our STM measurements, complemented by first-principles calculations, show that the hydrogen atom intercalated between two graphene sheets has dramatically reduced potential barriers for elementary migration steps. Especially, the confined atomic hydrogen dissociation energy from graphene is reduced to 0.34 eV, which is only about a third of a hydrogen atom chemisorbed on graphene. This offers a unique platform for direct imaging of the atomic dynamics of confined atoms. Our results suggest that the atomic interfaces of van der Waals materials may provide a confined environment to tune the interfacial chemical reactions.

cond-mat.mes-hall↗

Corrugation induced stacking solitons with topologically confined states in gapped bilayer graphene

Graphene, as an atomic-thick ultrasoft membrane, almost has no resistance against out-of-plane deformations and, therefore, it is always wrinkled to a certain degree. Recently, corrugated structures and their effects on the electronic properties of monolayer graphene have been studied extensively. However, similar experimental studies in bilayer graphene have yet to be reported. Here, we show that corrugations in bilayer graphene can generate incommensurate stacking solitons (domain walls) between commensurate Bernal-stacked domains. By using scanning tunneling microscopy, we microscopically study electronic structures of a corrugation-induced stacking soliton that separates two adjacent AB and BA stacked bilayer regions with a uniform interlayer potential difference. Both topological gapless edge states and quasi-localized gapped quantum-well-like states are observed in the nanoscale corrugation. Atomic resolution mapping of the topological edge states along the stacking soliton reveals the existence of intervalley scattering between them, which could explain recent experiments where the conductance along domain walls of gapped graphene bilayer is smaller than a quantized value 4e2 h.

cond-mat.mes-hall↗

Direct experimental evidence of pi magnetism of a single atomic vacancy in graphene

The pristine graphene is strongly diamagnetic. However, graphene with single carbon atom defects could exhibit paramagnetism with local magnetic moments ~ 1.5 per vacancy1-6. Theoretically, both the electrons and electrons of graphene contribute to the magnetic moment of the defects, and the pi magnetism is characterizing of two spin-split DOS (density-of-states) peaks close to the Dirac point1,6. Since its prediction, many experiments attempt to study this pi magnetism in graphene, whereas, only a notable resonance peak has been observed around the atomic defects6-9, leaving the pi magnetism experimentally so elusive. Here, we report direct experimental evidence of the pi magnetism by using scanning tunnelling microscope. We demonstrate that the localized state of the atomic defects is split into two DOS peaks with energy separations of several tens meV and the two spin-polarized states degenerate into a profound peak at positions with distance of ~ 1 nm away from the monovacancy. Strong magnetic fields further increase the energy separations of the two spin-polarized peaks and lead to a Zeeman-like splitting. The effective g-factors geff around the atomic defect is measured to be about 40. Such a giant enhancement of the g-factor is attributed to the strong spin polarization of electron density and large electron-electron interactions near the atomic vacancy.

cond-mat.mtrl-sci↗

Energy gaps of atomically precise armchair graphene nanoribbons

Graphene nanoribbons (GNRs) are one-dimensional (1D) structures that exhibit a rich variety of electronic properties1-17. Therefore, they are predicted to be the building blocks in next-generation nanoelectronic devices. Theoretically, it has been demonstrated that armchair GNRs can be divided into three families, i.e., Na = 3p, Na = 3p + 1, and Na = 3p + 2 (here Na is the number of dimer lines across the ribbon width and p is an integer), according to their electronic structures, and the energy gaps for the three families are quite different even with the same p1,3-6. However, a systematic experimental verification of this fundamental prediction is still lacking, owing to very limited atomic-level control of the width of the armchair GNRs investigated7,9,10,13,17. Here, we studied electronic structures of the armchair GNRs with atomically well-defined widths ranging from Na = 6 to Na = 26 by using scanning tunnelling microscope (STM). Our result demonstrated explicitly that all the studied armchair GNRs exhibit semiconducting gaps due to quantum confinement and, more importantly, the observed gaps as a function of Na are well grouped into the three categories, as predicted by density-functional theory calculations3. Such a result indicated that we can tune the electronic properties of the armchair GNRs dramatically by simply adding or cutting one carbon dimer line along the ribbon width.

cond-mat.mtrl-sci↗

Cosmic Reionization Study : Principle Component Analysis After Planck

The study of reionization history plays an important role in understanding the evolution of our universe. It is commonly believed that the intergalactic medium (IGM) in our universe are fully ionized today, however the reionizing process remains to be mysterious. A simple instantaneous reionization process is usually adopted in modern cosmology without direct observational evidence. However, the history of ionization fraction, $x_e(z)$ will influence cosmic microwave background (CMB) observables and constraints on optical depth $τ$. With the mocked future data sets based on featured reionization model, we find the bias on $τ$ introduced by instantaneous model can not be neglected. In this paper, we study the cosmic reionization history in a model independent way, the so called principle component analysis (PCA) method, and reconstruct $x_e (z)$ at different redshift $z$ with the data sets of Planck, WMAP 9 years temperature and polarization power spectra, combining with the baryon acoustic oscillation (BAO) from galaxy survey and type Ia supernovae (SN) Union 2.1 sample respectively. The results show that reconstructed $x_e(z)$ is consistent with instantaneous behavior, however, there exists slight deviation from this behavior at some epoch. With PCA method, after abandoning the noisy modes, we get stronger constraints, and the hints for featured $x_e(z)$ evolution could become a little more obvious.

astro-ph.CO↗

Creating and probing wide-bandgap nanoribbon-like structures in a continuous metallic graphene sheet

The light-like dispersion of graphene monolayer results in many novel electronic properties in it1, however, this gapless feature also limits the applications of graphene monolayer in digital electronics2. A rare working solution to generate a moderate bandgap in graphene monolayer is to cut it into one-dimensional (1D) nanometre-wide ribbons3-13. Here we show that a wide bandgap can be created in a unique 1D strained structure, i.e., graphene-nanoribbon-like (GNR-like) structure, of a continuous graphene sheet via strong interaction between graphene and the metal substrate, instead of cutting graphene monolayer. The GNR-like structures with width of only a few nanometers are observed in a continuous graphene sheet grown on Rh foil by using thermal strain engineering. Spatially-resolved scanning tunnelling spectroscopy revealed bandgap opening of a few hundreds meV in the GNR-like structure in an otherwise continuous metallic graphene sheet, directly demonstrating the realization of a metallic-semiconducting-metallic junction entirely in a graphene monolayer. We also show that it is possible to tailor the structure and electronic properties of the GNR-like structure by using scanning tunnelling microscope.

cond-mat.mes-hall↗

Experimental Observation of Surface States and Landau Levels Bending in Bilayer Graphene

We report on microscopic measurements of the low-energy electronic structures both at zigzag and armchair edges of bilayer graphene using scanning tunneling microscopy and spectroscopy (STM and STS). We have found that, both in the absence and in the presence of a magnetic field, an almost zero-energy peak in density of states was localized at zigzag edges, as expected for the surface states at zigzag edges of bilayer graphene. In the quantum Hall regime, we have observed clearly Landau levels bending away from the charge neutrality point near both the zigzag and armchair edges. Such a result is a direct evidence for the evolution of Landau levels into the quantum Hall edge states in graphene bilayers. Our experiment indicates that it is possible to explore rich quantum Hall physics in graphene systems using STM and STS.

cond-mat.mes-hall↗

Spatial variation of energy gap and Landau levels around gapped bilayer graphene domain walls

Bilayer graphene contains, compared to graphene monolayer, an additional graphene sheet and, therefore, extra degrees of freedom, making it a unique system for complex electronic states to emerge. Here, we show that there are two types of domain walls, i.e., coupling domain wall and potential domain wall, in gapped graphene bilayers, which make microscopic electronic properties of the bilayers varying spatially. The coupling domain wall separates two graphene bilayer regions with different interlayer coupling strengths and the potential domain wall is a boundary separating two adjacent regions with different chemical potentials between two layers. We present a microscopically study, using scanning tunnelling microscopy and spectroscopy, around the two types of domain walls. The well-defined domain walls allow us to spatially resolve the energy gap and Landau levels around them, which show novel behaviour beyond what is expected from current theoretical models. Our result indicates that the graphene bilayer may exhibit exotic electronic properties related to the microscopic symmetry of the two layers.

cond-mat.mtrl-sci↗

Detecting giant electron-hole asymmetry in graphene monolayer generated by strain and charged-defect scattering via Landau level spectroscopy

The electron-hole symmetry in graphene monolayer, which is analogous to the inherent symmetric structure between electrons and positrons of the Universe, plays a crucial role in the chirality and chiral tunnelling of massless Dirac fermions. Here we demonstrate that both strain and charged-defect scattering could break this symmetry dramatically in graphene monolayer. In our experiment, the Fermi velocities of electrons and holes are measured directly through Landau level spectroscopy. In strained graphene with lattice deformation and curvature, the and are measured as 1.2 x 106 m/s and 1.02 x106 m/s, respectively. This giant asymmetry originates from enhanced next-nearest-neighbor hopping in the strained region. Around positively charged-defect, we observe opposite electron-hole asymmetry, and the and are measured to be 0.86x 106 m/s and 1.14 x106 m/s, respectively. Such a large asymmetry is attributed to the fact that the massless Dirac fermions in graphene monolayer are scattered more strongly when they are attracted to the charged-defect than when they are repelled from it.

cond-mat.mtrl-sci↗

Observation of Valley-polarized Landau Levels in Strained Graphene

In strained graphene, lattice deformation can create pseudo-magnetic fields and result in zero-field Landau level-like quantization. In the presence of an external magnetic field, valley-polarized Landau levels are predicted to be observed because the pseudo-magnetic fields are of opposite directions in the K and K' valleys of graphene. Here, we present experimental spectroscopic measurements by scanning tunneling microscopy of strained graphene on Rh foil. We direct observed valley splitting of the Landau level induced by the coexistence of the pseudo-magnetic fields and external magnetic fields. The observed result paves the way to exploit novel electronic properties in graphene through the combination of the pseudo-magnetic fields and the external magnetic fields.

cond-mat.mes-hall↗

Primordial Gravitational Waves Measurements and Anisotropies of CMB Polarization Rotation

Searching for the signal of primordial gravitational waves in the B-modes (BB) power spectrum is one of the key scientific aims of the cosmic microwave background (CMB) polarization experiments. However, this could be easily contaminated by several foreground issues, such as the thermal dust emission. In this paper we study another mechanism, the cosmic birefringence, which can be introduced by a CPT-violating interaction between CMB photons and an external scalar field. Such kind of interaction could give rise to the rotation of the linear polarization state of CMB photons, and consequently induce the CMB BB power spectrum, which could mimic the signal of primordial gravitational waves at large scales. With the recent polarization data of BICEP2 and the joint analysis data of BICEP2/Keck Array and Planck, we perform a global fitting analysis on constraining the tensor-to-scalar ratio $r$ by considering the polarization rotation angle which can be separated into a background isotropic part and a small anisotropic part. Since the data of BICEP2 and Keck Array experiments have already been corrected by using the "self-calibration" method, here we mainly focus on the effects from the anisotropies of CMB polarization rotation angle. We find that including the anisotropies in the analysis could slightly weaken the constraints on $r$, when using current CMB polarization measurements. We also simulate the mock CMB data with the BICEP3-like sensitivity. Very interestingly, we find that if the effects of the anisotropic polarization rotation angle can not be taken into account properly in the analysis, the constraints on $r$ will be dramatically biased. This implies that we need to break the degeneracy between the anisotropies of the CMB polarization rotation angle and the CMB primordial tensor perturbations, in order to measure the signal of primordial gravitational waves accurately.

astro-ph.CO↗

Atomic resolution imaging of the two-component Dirac-Landau levels in a gapped graphene monolayer

The wavefunction of massless Dirac fermions is a two-component spinor. In graphene, a one-atom-thick film showing two-dimensional Dirac-like electronic excitations, the two-component representation reflects the amplitude of the electron wavefunction on the A and B sublattices. This unique property provides unprecedented opportunities to image the two components of massless Dirac fermions spatially. Here we report atomic resolution imaging of the two-component Dirac-Landau levels in a gapped graphene monolayer by scanning tunnelling microscopy and spectroscopy. A gap of about 20 meV, driven by inversion symmetry breaking by the substrate potential, is observed in the graphene on both SiC and graphite substrates. Such a gap splits the n = 0 Landau level (LL) into two levels, 0+ and 0-. We demonstrate that the amplitude of the wavefunction of the 0- LL is mainly at the A sites and that of the 0+ LL is mainly at the B sites of graphene, characterizing the internal structure of the spinor of the n = 0 LL. This provides direct evidence of the two-component nature of massless Dirac fermions.

cond-mat.mtrl-sci↗

Spatially resolving unconventional interface Landau quantization in a graphene monolayer-bilayer planar junction

Graphene hybrid planar structures consisting of two regions with different quantum Hall (QH) states exhibit unusual transport properties1-5, originating from chiral edge states equilibration at the interface of the two different regions6. Here we present a sub-nanometre-resolved scanning tunnelling microscopy (STM) and spectroscopy (STS) study of a monolayer-bilayer graphene planar junction in the QH regime. The atomically well-defined interface of such a junction allows us to spatially resolve the interface electronic properties. Around the interface, we detect Landau quantization of massless Dirac fermions, as expected in graphene monolayer, below the charge neutrality point Nc of the junction, whereas unexpectedly, only Landau quantization of massive Dirac fermions, as expected in graphene bilayer, is observed above the Nc. The observed unconventional interface Landau quantization arises from the fact that the quantum conductance across the interface is solely determined by the minimum filling factors (number of edge modes) in the graphene monolayer and bilayer regions of the junction6,7.

cond-mat.mes-hall↗