arXiv subjects

Siddharth Karkare

Publications and source records attributed to Siddharth Karkare.

15 recordsLinked to original sources

arXiv2026

Photoemission from Semi-Infinite Crystals: First-Principles Scattering States and Quantitative Ag(111) Validation

Photoemission is an escape problem, yet first-principles calculations usually trap the electron in a periodic box. We present a parameter-free \emph{ab initio} framework that removes this artificial boundary by constructing open scattering states for semi-infinite crystal-vacuum interfaces from Wannier Hamiltonians and Green-function embedding. The method gives continuum-normalized time-reversed LEED final states with microscopic quasiparticle attenuation. For Ag(111), it predicts absolute quantum efficiency, vectorial photoemission, and mean transverse energy on the experimental scale.

cond-mat.mtrl-sci↗

arXiv2026

Beam Sources for 10 TeV Wakefield Collider

Due to its unique advantages, wakefield particle acceleration has been proposed as a promising pathway toward a 10 TeV collider. Several concepts, including Laser Wakefield Acceleration (LWFA), Plasma Wakefield Acceleration (PWFA), and Structure Wakefield Acceleration (SWFA), are being actively explored as potential approaches toward a 10 TeV collider. Each of these approaches requires particle sources (for the witness beam or for both drive and witness beams) with specific parameter sets to enable efficient wakefield acceleration. This work represents evaluation of existing and emerging particle generation technologies in the context of specific 10 TeV wakefield collider design requirements, with a particular focus on achievable brightness.

physics.acc-ph↗

arXiv2024

Harnessing Plasmonic Interference for Nanoscale Ultrafast Electron Sources

In this paper we demonstrate the use of plasmonic focusing in conjunction with non-linear photoemisison to develop geometrically flat nanoscale electron sources with less than 40 pm-rad root mean squared (rms) normalized transverse emittance. Circularly polarized light is incident on a gold Archimedean spiral structure to generate surface-plasmon-polaritons which interfere coherently at the center resulting in a 50 nm rms emisison area. Such a nanostructured flat surface enables simultaneous spatio-temporal confinement of emitted electrons at the nanometer and femtosecond level and can be used as an advanced electron source for high-repetition-rate ultrafast electron diffraction and microscopy experiments as well as next-generation of miniaturized particle accelerators.

physics.acc-ph↗

arXiv2022

Electron Sources for Accelerators

Electron sources are essential to an array of electron accelerator supporting research in high-energy physics and beyond. This report summarizes the "Snowmass 2021 Electron Source Workshop" which reviewed the current state-of-the art research and identified some possible research directions.

physics.acc-ph↗

arXiv2021

Monte Carlo Modeling of Spin-polarized Photoemission from p-doped GaAs Activated to Negative Electron Affinity

The anticorrelation between quantum efficiency (QE) and electron spin polarization (ESP) from a p-doped GaAs activated to negative electron affinity (NEA) is studied in detail using an ensemble Monte Carlo approach. The photoabsorption, momentum and spin relaxation during transport, and tunnelling of electrons through the surface potential barrier are modeled to identify fundamental mechanisms, which limit the efficiency of GaAs spin-polarized electron sources. In particular, we study the response of QE and ESP to various parameters such as the photoexcitation energy, doping density, and electron affinity level. Our modeling results for various transport and emission characteristics are in a good agreement with available experimental data. Our findings show that the behaviour of both QE and ESP at room temperature can be fully explained by the bulk relaxation mechanisms and the time which electrons spend in the material before being emitted.

physics.app-ph↗

arXiv2020

Ab initio many-body photoemission theory of transverse energy distribution of photoelectrons: PbTe(111) as a case study with experimental comparisons

This manuscript presents, to our knowledge, the first fully ab initio many-body photoemission framework to predict the transverse momentum distributions and the mean transverse energies (MTEs) of photoelectrons from single-crystal photocathodes. The need to develop such a theory stems from the lack of studies that provide complete understanding of the underlying fundamental processes governing the transverse momentum distribution of photoelectrons emitted from single crystals. For example, initial predictions based on density-functional theory calculations of effective electron masses suggested that the (111) surface of PbTe would produce very small MTEs ($\leq$ 15 meV), whereas our experiments yielded MTEs ten to twenty times larger than these predictions, and also exhibited a lower photoemission threshold than predicted. The ab initio framework presented in this manuscript correctly reproduces the magnitude of the MTEs from our measurements in PbTe(111) and also the observed photoemission below the predicted threshold. Our results show that photoexcitations into bulk-like states and coherent, many-body electron-photon-phonon scattering processes, both of which initial predictions ignored, indeed play important roles in photoemission from PbTe(111). Finally, from the lessons learned, we recommend a procedure for rapid computational screening of potential single-crystal photocathodes for applications in next-generation ultrafast electron diffraction and X-ray free-electron lasers, which will enable new, significant advances in condensed matter research.

cond-mat.mtrl-sci↗

arXiv2020

Ultracold electrons via Near-Threshold Photoemission from Single-Crystal Cu(100)

Achieving a low mean transverse energy or temperature of electrons emitted from the photocathode-based electron sources is critical to the development of next-generation and compact X-ray Free Electron Lasers and Ultrafast Electron Diffraction, Spectroscopy and Microscopy experiments. In this paper, we demonstrate a record low mean transverse energy of 5 meV from the cryo-cooled (100) surface of copper using near-threshold photoemission. Further, we also show that the electron energy spread obtained from such a surface is less than 11.5 meV, making it the smallest energy spread electron source known to date: more than an order of magnitude smaller than any existing photoemission, field emission or thermionic emission based electron source. Our measurements also shed light on the physics of electron emission and show how the energy spread at few meV scale energies is limited by both the temperature and the vacuum density of states.

physics.acc-ph↗

arXiv2018

Brightness of nonequilibrium photoemission in metallic photocathodes near threshold

The operation of photoemission electron sources with wavelengths near the photoemission threshold has been shown to dramatically decrease the minimum achievable photocathode emittance, but at the cost of significantly reduced quantum efficiency (QE). In this work, we show that for femtosecond laser and electron pulses, the increase in required laser intensities due to the low QE drives the photocathode electronic distribution far from static equilibrium. We adapt an existing dynamic model of the electron occupation under high intensity laser illumination to predict the time-dependent effects of the nonequilibrium electron distribution on the QE, mean transverse energy (MTE), and emission brightness of metal phtocathodes. We find that multiphoton photoemission dramatically alters the MTE as compared to thermal equilibrium models, causing the MTE to no longer be a monotonic function of photon excess energy.

physics.acc-ph↗

arXiv2016

A One-Step Model of Photoemission from Single Crystal Surfaces

In this paper, we present a 3-D one step photoemission model that can be used to calculate the quantum efficiency and momentum distributions of electrons photoemitted from ordered single crystal surfaces close to the photoemission threshold. Using Ag(111) as an example, we show that the model can not only calculate the quantum efficiency from the surface state accurately without using any ad hoc parameters, but also provides a theoretical quantitative explanation of the vectorial photoelectric effect. This model in conjunction with other band structure and wave function calculation techniques can be effectively used to screen single crystal photoemitters for use as electron sources for particle accelerator and ultrafast electron diffraction applications.

physics.acc-ph↗

arXiv2016

Near atomically smooth alkali antimonide photocathode thin films

Nano-roughness limits the emittance of electron beams that can be generated by high efficiency photocathodes, such as the thermally reacted alkali antimonide thin films. However there is an urgent need for photocathodes that can produce an order of magnitude or more lower emittance than present day systems in order to increase the transverse coherence width of the electron beam. In this paper we demonstrate a method for producing alkali antimonide cathodes with near atomic smoothness with high reproducibility.

physics.acc-ph↗

arXiv2015

Cold electron beams from cryo-cooled, alkali antimonide photocathodes

In this letter we report on the generation of cold electron beams using a Cs3Sb photocathode grown by co-deposition of Sb and Cs. By cooling the photocathode to 90 K we demonstrate a significant reduction in the mean transverse energy validating the long standing speculation that the lattice temperature contribution limits the mean transverse energy or thermal emittance near the photoemission threshold, opening new frontiers in generating ultra-bright beams. At 90 K, we achieve a record low thermal emittance of 0.2 $μ$m (rms) per mm of laser spot diameter from an ultrafast (sub-picosecond) photocathode with quantum efficiency greater than $7\times 10^{-5}$ using a visible laser wavelength of 690 nm.

physics.acc-ph↗

arXiv2013

Demonstration of Low Emittance in the Cornell Energy Recovery Linac Injector Prototype

We present a detailed study of the six-dimensional phase space of the electron beam produced by the Cornell Energy Recovery Linac Photoinjector, a high-brightness, high repetition rate (1.3 GHz) DC photoemission source designed to drive a hard x-ray energy recovery linac (ERL). A complete simulation model of the injector has been constructed, verified by measurement, and optimized. Both the horizontal and vertical 2D transverse phase spaces, as well as the time-resolved (sliced) horizontal phase space, were simulated and directly measured at the end of the injector for 19 pC and 77 pC bunches at roughly 8 MeV. These bunch charges were chosen because they correspond to 25 mA and 100 mA average current if operating at the full 1.3 GHz repetition rate. The resulting 90% normalized transverse emittances for 19 (77) pC/bunch were 0.23 +/- 0.02 (0.51 +/- 0.04) microns in the horizontal plane, and 0.14 +/- 0.01 (0.29 +/- 0.02) microns in the vertical plane, respectively. These emittances were measured with a corresponding bunch length of 2.1 +/- 0.1 (3.0 +/- 0.2) ps, respectively. In each case the rms momentum spread was determined to be on the order of 1e-3. Excellent overall agreement between measurement and simulation has been demonstrated. Using the emittances and bunch length measured at 19 pC/bunch, we estimate the electron beam quality in a 1.3 GHz, 5 GeV hard x-ray ERL to be at least a factor of 20 times better than that of existing storage rings when the rms energy spread of each device is considered. These results represent a milestone for the field of high-brightness, high-current photoinjectors.

physics.acc-ph↗

arXiv2011

Photocathode Behavior During High Current Running in the Cornell ERL Photoinjector

The Cornell University Energy Recovery Linac (ERL) photoinjector has recently demonstrated operation at 20 mA for approximately 8 hours, utilizing a multialkali photocathode deposited on a Si substrate. We describe the recipe for photocathode deposition, and will detail the parameters of the run. Post-run analysis of the photocathode indicates the presence of significant damage to the substrate, perhaps due to ion back-bombardment from the residual beamline gas. While the exact cause of the substrate damage remains unknown, we describe multiple surface characterization techniques (X-ray fluorescence spectroscopy, X-ray diffraction, atomic force and scanning electron microscopy) used to study the interesting morphological and crystallographic features of the photocathode surface after its use for high current beam production. Finally, we present a simple model of crystal damage due to ion back-bombardment, which agrees qualitatively with the distribution of damage on the substrate surface.

physics.acc-ph↗

arXiv2011

Thermal emittance measurements of a cesium potassium antimonide photocathode

Thermal emittance measurements of a CsK2Sb photocathode at several laser wavelengths are presented. The emittance is obtained with a solenoid scan technique using a high voltage dc photoemission gun. The thermal emittance is 0.56+/-0.03 mm-mrad/mm(rms) at 532 nm wavelength. The results are compared with a simple photoemission model and found to be in a good agreement.

physics.acc-ph↗

arXiv2011

Effect of nano-scale surface roughness on transverse energy spread from GaAs photocathodes

High quantum yield, low transverse energy spread and prompt response time make GaAs activated to negative electron affnity, an ideal candidate for a photocathode in high brightness photoinjectors. Even after decades of investigation, the exact mechanism of electron emission from GaAs is not well understood. We show that a nanoscale surface roughness can affect the transverse electron spread from GaAs by nearly an order of magnitude and explain the seemingly controversial experimental results obtained so far. This model can also explain the measured dependence of transverse energy spread on the wavelength of incident light.

physics.acc-ph↗