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Siddhartha Lal

Publications and source records attributed to Siddhartha Lal.

At least 19 recordsLinked to original sources

Tracking Entanglement Transfer: Emergence of Thermodynamics from Quantum Information

We study entanglement transfer in a minimal model of two qubits that are coupled with one another through an antiferromagnetic Heisenberg exchange ($\tilde{J}$), and where one of them is additionally coupled to a fermionic environment through another antiferromagnetic Heisenberg exchange ($J_{K}$). By tuning the coupling ratio $J_{K}/\tilde{J}$, the system undergoes a quantum phase transition at $T=0$, accompanied by a redistribution of entanglement from the $d'-d$ qubit-subsystem to the environment. Remarkably, the resulting physics exhibits properties that bear analogy with a quantum-information theoretic perspective of the physics of black hole thermodynamics. Carefully selected bipartite and tripartite mutual information measures displays behaviour analogous to the dynamical evolution of black hole entropy, Hawking entropy, and the Page curve expected during the process of evaporation. An effective temperature scale is obtained from the variation of the ground state energy with respect to changes in the bipartite mutual information between the subsystem and the bath. A steady growth of this temperature with the coupling ratio resembles that of the Hawking temperature with the inverse mass of the black hole. Concomitantly, the emergence of non-Fermi liquid behaviour observed near the quantum critical point and in the strong-coupling phase resembles strange-metal-like physics expected near the event horizon from a holographic duality perspective. Our results establish the minimal model as a platform for studying entanglement transfer and information scrambling within a fully unitary quantum framework, and offer new insights into a resolution of the black hole information paradox.

quant-ph

Ultrafast Critical Slowing of Spin Dynamics and Emergent Nonequilibrium Fano Interference in Fe3GeTe2

Fe$_3$GeTe$_2$ is a prototypical metallic van der Waals ferromagnet with itinerant magnetism and a highly tunable Curie temperature, yet how electronic excitations couple to spin and lattice degrees of freedom across its magnetic transition remains largely unexplored. Here, we use two-color pump-probe reflectivity to investigate the coupled electronic, spin, and lattice dynamics. The time-resolved reflectivity exhibits a tri-exponential relaxation, in which the intermediate component shows an anomaly near the Curie temperature due to enhanced interlayer spin-lattice interactions, while the slowest component displays pronounced critical slowing down with an exponent of ~ 0.3, revealing non-universal relaxation dynamics associated with intralayer spin correlations. Furthermore, we observe an emergent nonequilibrium A1g phonon Fano asymmetry that is suppressed in the ferromagnetic phase but anomalously enhanced in the paramagnetic regime, driven by thermally activated anharmonic decay pathways that bridge the kinematic gap to a hot electronic continuum. The pronounced enhancement of the acoustic strain pulse amplitude near T$_c$ further evidences robust magnetoelastic coupling. Overall, our results reveal how magnetic order governs the interplay among critical spin dynamics, electronic continuum excitations, and lattice response in metallic van der Waals ferromagnets

cond-mat.mtrl-sci

Kondo breakdown as an entanglement transition driven by continuous measurement

We study the breakdown of Kondo screening by a local magnetic field from the perspective of a measurement-driven entanglement transition in a monitored quantum system. Here, the Kondo coupling leads to the growth in entanglement of an impurity spin with it's fermionic environment, while the local field plays the role of a continuous observer. Using a non-perturbative Unitary Renormalization Group (URG) approach, we derive coupled renormalization-group flow equations for the Kondo exchange and the local field, and obtain a field-dependent RG phase diagram. The RG flows separate a low-energy Kondo-screened phase, where the impurity is absorbed into the Fermi sea and forms an entangled singlet with the conduction bath, from a polarized local-moment phase in which screening is frustrated and impurity-bath entanglement is suppressed. We identify the fixed-point Hamiltonians governing the two phases and the critical regime, and relate the transition to the emergence of a novel non-Fermi liquid. Various impurity signatures such as the spectral function and thermalisation of impurity observables are used to characterise this entanglement transition. These results offer insight into the interplay of decoherence and measurement in governing the dynamics of a prototypical quantum system.

cond-mat.str-el

Ultrafast Dynamics of Spin-Orbit Entangled Excitons Coupled to Magnetic Ordering in van der Waals Antiferromagnet NiPS3

Spin-orbit entangled excitons (SOEE) in two-dimensional (2D) antiferromagnets provide direct access to explore unconventional many body interactions in correlated electron systems. In this work, we carry out a detailed investigation using non-degenerate isotropic and anisotropic pump-probe reflection spectroscopy to probe the ultrafast dynamics of SOEE and their coupling to spin fluctuations in NiPS3. Transient reflectivity data reveals acoustic phonon oscillations at ~ 27 GHz, along with two distinct relaxation timescales: fast (1-9 ps) and slower components (1-4 ns) associated with SOEE coherence and spin reordering, respectively. Both timescales exhibit pronounced temperature dependence near the exciton dissociation (TED = 120 K) and Neel (TN = 155 K) temperatures. The SOEE coherence shortens from ~ 8-9 ps at T < TED to ~ 3 ps at T > TED with a finite tail persisting beyond TN. The spin reordering time grows near 120 K, and shows critical slowing down around TN. Pump fluence studies further corroborate their spin origin. Our findings uncover the direct interplay between the excitonic and spin degrees of freedom across ultrafast and longer timescales, offering new opportunities to probe and engineer emergent many-body interactions in 2D antiferromagnets.

cond-mat.other

Mott Criticality as the Confinement Transition of a Pseudogap-Mott Metal

The phenomenon of Mott insulation involves the localization of itinerant electrons due to strong local repulsion. Upon doping, a pseudogap (PG) phase emerges - marked by selective gapping of the Fermi surface without conventional symmetry breaking in spin or charge channels. A key challenge is understanding how quasiparticle breakdown in the Fermi liquid gives rise to this enigmatic state, and how it connects to both the Mott insulating and superconducting phases. Here, we develop a renormalization-based construction of strongly correlated lattice models that captures the emergence of the pseudogap phase and its transition to a Mott insulator. Applying a many-body tiling scheme to the fixed-point impurity model uncovers a lattice model with electron interactions and Kondo physics. At half-filling, the interplay between Kondo screening and bath charge fluctuations in the impurity model leads to Fermi liquid breakdown. This reveals a pseudogap phase characterized by a non-Fermi liquid (the Mott metal) residing on nodal arcs, gapped antinodal regions of the Fermi surface, and an anomalous scaling of the electronic scattering rate with frequency. The eventual confinement of holon-doublon excitations of this exotic metal obtains a continuous transition into the Mott insulator. Our results identify the pseudogap as a distinct long-range entangled quantum phase, and offer a new route to Mott criticality beyond the paradigm of local quantum criticality.

cond-mat.str-el

The Physics of Quantum 2.0: Challenges in understanding Quantum Matter

Almost a century on from the culmination of the first revolution in quantum physics, we are poised for another. Even as we engage in the creation of impactful quantum technologies, it is imperative for us to face the challenges in understanding the phenomenology of various emergent forms of quantum matter. This will involve building on decades of progress in quantum condensed matter physics, and going beyond the well-established Ginzburg-Landau-Wilson paradigm for quantum matter. We outline and discuss several outstanding challenges, including the need to explore and identify the organisational principles that can guide the development of theories, key experimental phenomenologies that continue to confound, and the formulation of methods that enable progress. These efforts will enable the prediction of new quantum materials whose properties facilitate the creation of next generation technologies.

cond-mat.str-el

Backbone Mediated Electrical Transport in a Double-Stranded DNA

In the field of DNA nanotechnology, it is common wisdom that charge transport occurs through the π stacked bases of double-stranded DNA. However, recent experimental findings by Zhuravel et. al. [Nat. Nanotech. 15, 836 (2020)] suggest that electronic transport happens through the backbone channels instead of π-π interaction of the nitrogen bases. These new experimental insights call for a detail investigation. In keeping with this, we examine charge transport properties of three characteristic double-stranded DNA sequences (periodic GC, periodic AT and random ATGC sequences) within a tight-binding framework where backbones form the main conduction channels. Using techniques based on the Green function method, we inspect the single-particle density of states and localization properties of DNA in the presence of discontinuities (nicks) along the backbone channels. We also investigate the effect of these nicks on current-voltage response using the Landauer - Buttiker formalism for a two-terminal geometry where the source electrode is attached to one backbone strand and the drain to the other. We observe that the periodic DNA sequence of GC bases is metallic in nature, while the periodic AT sequence and the random ATGC sequence are insulating. Further, the effects of nicks on the transport properties of the periodic GC sequence is interesting: while a single nick on the upper backbone does not affect electronic transport, the addition of a second nick on the lower backbone causes the current to vanish altogether. This is found to be robust against changes in the positions of the nicks, as well as the alternation of the source and drain electrodes.

cond-mat.mes-hall

Tomonaga-Luttinger liquid and quantum criticality in spin-1/2 antiferromagnetic Heisenberg chain C14H18CuN4O10 via Wilson ratio

The ground state of a one-dimensional spin-1/2 uniform antiferromagnetic Heisenberg chain (AfHc) is a Tomonaga-Luttinger liquid which is quantum-critical with respect to applied magnetic fields upto a saturation field Hs beyond which it transforms to a fully polarised state. Wilson ratio has been predicted to be a good indicator for demarcating these phases [Phys. Rev. B 96, 220401 (2017)]. From detailed temperature and magnetic field dependent magnetisation, magnetic susceptibility and specific heat measurements in a metalorganic complex and comparisons with field theory and quantum transfer matrix method calculations, the complex was found to be a very good realisation of a spin-1/2 AfHc. Wilson ratio obtained from experimentally obtained magnetic susceptibility and magnetic contribution of specific heat values was used to map the magnetic phase diagram of the uniform spin-1/2 AfHc over large regions of phase space demarcating Tomonaga-Luttinger liquid, saturation field quantum critical, and fully polarised states. Luttinger parameter and spinon velocity were found to match very well with the values predicted from conformal field theory.

cond-mat.str-el

Holographic entanglement renormalisation for fermionic quantum matter

We demonstrate the emergence of a holographic dimension in a system of 2D non-interacting Dirac fermions placed on a torus, by studying the scaling of multipartite entanglement measures under a sequence of renormalisation group (RG) transformations applied in momentum space. Geometric measures defined in this emergent space can be related to the RG beta function of the spectral gap, hence establishing a holographic connection between the spatial geometry of the emergent spatial dimension and the entanglement properties of the boundary quantum theory. We prove, analytically, that changing the boundedness of the holographic space involves a topological transition accompanied by a critical Fermi surface in the boundary theory. We go on to show that this results in the formation of a quantum wormhole geometry that connects the UV and the IR of the emergent dimension. The additional conformal symmetry at the transition also supports a relation between the emergent metric and the stress-energy tensor. In the presence of an Aharonov-Bohm flux, the entanglement gains a geometry-independent piece which is shown to be topological, sensitive to changes in boundary conditions, and related to the Luttinger volume of the system. Upon the insertion of a strong transverse magnetic field, we show that the Luttinger volume is linked to the Chern number of the occupied single-particle Landau levels.

cond-mat.str-el

Determining the purity of single-helical proteins from electronic specific heat measurements

We present a theoretical investigation of the electronic specific heat (ESH) at constant volume (Cv) of single-helical proteins modeled within the tight-binding (TB) framework. We study the effects of helical symmetry, long-range hopping, environment and biological defects on thermal properties. We employ a general TB model to incorporate all parameters relevant to the helical structure of the protein. In order to provide additional insights into our results for the ESH, we also study the electronic density of states for various disorder strengths. We observe that the variation of the specific heat with disorder is very different in low and high temperature regimes, though the variation of ESH with temperature possesses a universal pattern upon varying disorder strengths related to environmental effects. Lastly, we propose an interesting application of the ESH spectra of proteins. We show that by studying the ESH of single-helical proteins, one can distinguish a defective sample from a pure one. This observation can serve as the basis of a screening technique that can be applied prior to a whole genome testing, thereby saving valuable time & resources.

cond-mat.mes-hall

Probing of magnetic dimensional crossover in CrSiTe$_{3}$ through picosecond strain pulses

Elucidating the emergence of long-range magnetic ordering from its precursor short-range magnetic ordering (SRMO) in two-dimensional van der Waals materials holds profound implications for fundamental research and technological advancements. However, directly observing the intricate stages of this magnetic dimensional crossover (MDC) remains a significant experimental challenge. While magneto-elastic coupling offers a promising avenue, detecting the minute lattice response to SRMO proves challenging. Recent investigations utilizing second harmonic generation have unveiled a two-step MDC in a van der Waals ferromagnetic insulator. However, an unambiguous detection of MDC through the time-resolved techniques remains elusive. To meet this goal, we have executed an alternative approach by employing picosecond acoustic strain pulses generated by femtosecond lasers to probe the various stages of MDC through the magneto-elastic coupling for the first time. By analyzing the shape of the strain pulse in both the time and frequency domains as a function of temperature, we clearly demonstrate the detection of the subtle influence of spin fluctuations on the lattice. Additionally, the ultrafast carrier dynamics also show signatures of MDC. Our measurements pave the way towards characterizing magnetic materials in time-resolved experiments that are crucial in designing a new generation of spin-based optoelectronic devices.

cond-mat.mtrl-sci

Universal entanglement signatures of quantum liquids as a guide to fermionic criticality

An outstanding challenge involves understanding the many-particle entanglement of liquid states of quantum matter that arise in systems of interacting electrons. The Fermi liquid (FL) in $D$ spatial dimensions shows a violation of the area-law in real-space entanglement entropy of a subsystem (of length $L$), $S_{EE} \sim L^{D-1}\ln L$, widely believed to be a hallmark signature of the ground state of a gapless quantum critical system of interacting fermions. In this work, we apply a $T=0$ renormalisation group approach to a prototype of the FL in momentum (or, $k$)-space, unveiling thereby the RG relevant quantum fluctuations (due to forward and tangential scattering) from which long-range entanglement arises. A similar analysis of non-Fermi liquids such as the 2D marginal Fermi liquid (MFL) and the 1D Tomonaga-Luttinger liquid (TLL) reveals a universal logarithmic violation of the area-law in gapless electronic liquids for a subsystem defined within a $k$-space window (of size $Λ$) proximate to the Fermi surface, with a proportionality constant that depends on the nature of the underlying Fermi surface. We extend this analysis to the gapped quantum liquids emergent from the destabilisation of the Fermi surface by quantum fluctuations arising from backscattering processes. Indeed, we find that the $k$-space entanglement signatures of gapped quantum liquids appear to be governed by the nature of the Fermi surface (e.g., nested or not) from which they emerge, as well as the nature of their parent gapless metallic liquid (e.g., FL, MFL etc.). This is confirmed by our finding an enhanced entanglement entropy for the nodal MFL present at the quantum critical point recently discovered in the 2D Hubbard model at optimal hole-doping. Our work thus paves the way for an entanglement based classification of quantum liquids emergent from the criticality of interacting fermionic matter.

cond-mat.str-el

Kondo frustration via charge fluctuations: a route to Mott localisation

We propose a minimal effective impurity model that captures the phenomenology of the Mott-Hubbard metal-insulator transition (MIT) of the half-filled Hubbard model on the Bethe lattice in infinite dimensions as observed by dynamical mean field theory (DMFT). This involves extending the standard Anderson impurity model Hamiltonian to include an explicit Kondo coupling $J$, as well as a local on-site correlation $U_b$ on the conduction bath site connected directly to the impurity. For the case of attractive local bath correlations ($U_{b}<0$), the extended Anderson impurity model (e-SIAM) sheds new light on several aspects of the DMFT phase diagram. For example, the $T=0$ metal-to-insulator quantum phase transition (QPT) is preceded by an excited state quantum phase transition (ESQPT) where the local moment eigenstates are emergent in the low-lying spectrum. Long-ranged fluctuations are observed near both the QPT and ESQPT, suggesting that they are the origin of the quantum critical scaling observed recently at high temperatures in DMFT simulations. The $T=0$ gapless excitations at the QCP display particle-hole interconversion processes, and exhibit power-law behaviour in self-energies and two-particle correlations. These are signatures of non-Fermi liquid behaviour that emerge from the partial breakdown of the Kondo screening.

cond-mat.str-el

Frustration shapes multi-channel Kondo physics: a star graph perspective

We study the overscreened multi-channel Kondo (MCK) model using the recently developed unitary renormalization group (URG) technique. Our results display the importance of ground state degeneracy in explaining various important properties like the breakdown of screening and the presence of local non-Fermi liquids. The impurity susceptibility of the intermediate coupling fixed point Hamiltonian in the zero-bandwidth (or star graph) limit shows a power-law divergence at low temperature, signalling its critical nature. Despite the absence of inter-channel coupling in the MCK fixed point Hamiltonian, the study of mutual information between any two channels shows non-zero correlation between them. A spectral flow analysis of the star graph reveals that the degenerate ground state manifold possesses topological quantum numbers. The low energy effective Hamiltonian obtained upon adding a finite non-zero conduction bath dispersion to the star graph Hamiltonian for both the two and three-channel cases displays the presence of local non-Fermi liquids arising from inter-channel quantum fluctuations. Discontinuous behaviour is observed in several measures of ground state entanglement, signalling the underlying orthogonality catastrophe associated with the degenerate ground state manifold. We extend our results to underscreened and perfectly screened MCK models through duality arguments. A study of channel anisotropy under renormalisation flow reveals a series of quantum phase transitions due to the change in ground state degeneracy. Our work thus presents a template for the study of how a degenerate ground state manifold arising from symmetry and duality properties in a multichannel quantum impurity model can lead to novel multicritical phases at intermediate coupling.

cond-mat.str-el

Graph Polynomial for Colored Embedded Graphs: A Topological Approach

We study finite graphs embedded in oriented surfaces by associating a polynomial to it. The tools used in developing a theory of such graph polynomials are algebraic topological while the polynomial itself is inspired from ideas arising in physics. We also analyze a variant of these polynomials for colored embedded graphs. This is used to describe the change in the polynomial under basic graph theoretic operations. We conclude with several applications of this polynomial including detection of certain classes of graphs and the connection of this polynomial with topological entanglement entropy.

math.CO

Unveiling the Kondo cloud: unitary RG study of the Kondo model

We analyze the single-channel Kondo model using the recently developed unitary renormalization group (URG) method, and obtain a comprehensive understanding of the Kondo screening cloud. The fixed-point low-energy Hamiltonian enables the computation of a plethora of thermodynamic quantities (specific heat, susceptibility, Wilson ratio, etc.) as well as spectral functions, all of which are found to be in excellent agreement with known results. By integrating out the impurity, we obtain an effective Hamiltonian for the excitations of the electrons comprising the Kondo cloud. This is found to contain both k-space number-diagonal (Fermi liquid) as well off-diagonal four-fermion scattering terms. Our conclusions are reinforced by a URG study of the two-particle entanglement and many-body correlations among members of the Kondo cloud and impurity. The entanglement between the impurity and a cloud electron, as well as between any two cloud electrons, is found to increase under flow towards the singlet ground state at the strong-coupling fixed point. Both the number-diagonal and off-diagonal correlations within the conduction cloud are also found to increase as the impurity is screened under the flow, and the latter are found to be responsible for the macroscopic entanglement of the Kondo-singlet ground state. The unitary RG flow enables an analytic computation of the phase shifts suffered by the conduction electrons at the strong-coupling fixed point. This reveals an orthogonality catastrophe between the local moment and strong-coupling ground states, and is related to a change in the Luttinger volume of the conduction bath. Our results offer fresh insight on the nature of the emergent many-particle entanglement within the Kondo cloud, and pave the way for further investigations in more exotic contexts such as the fixed point of the over-screened multi-channel Kondo problem.

cond-mat.str-el

Unveiling topological order through multipartite entanglement

It is well known that the topological entanglement entropy ($S_{topo}$) of a topologically ordered ground state in 2 spatial dimensions can be captured efficiently by measuring the tripartite quantum information ($I^{3}$) of a specific annular arrangement of three subsystems. However, the nature of the general N-partite information ($I^{N}$) and quantum correlation of a topologically ordered ground state remains unknown. In this work, we study such $I^N$ measure and its nontrivial dependence on the arrangement of $N$ subsystems. For the collection of subsystems (CSS) forming a closed annular structure, the $I^{N}$ measure ($N\geq 3$) is a topological invariant equal to the product of $S_{topo}$ and the Euler characteristic of the CSS embedded on a planar manifold, $|I^{N}|=χS_{topo}$. Importantly, we establish that $I^{N}$ is robust against several deformations of the annular CSS, such as the addition of holes within individual subsystems and handles between nearest-neighbour subsystems. For a general CSS with multiple holes ($n_{h}>1$), we find that the sum of the distinct, multipartite informations measured on the annular CSS around those holes is given by the product of $S_{topo}$, $χ$ and $n_{h}$, $\sum^{n_{h}}_{μ_{i}=1}|I^{N_{μ_{i}}}_{μ_{i}}| = n_{h}χS_{topo}$. The $N^{th}$ order irreducible quantum correlations for an annular CSS of $N$ subsystems is also found to be bounded from above by $|I^{N}|$, which shows the presence of correlations among subsystems arranged in the form of closed loops of all sizes. Our results offer important insight into the nature of the many-particle entanglement and correlations within a topologically ordered state of matter.

quant-ph

Holographic entanglement renormalisation of topological order in a quantum liquid

We introduce a novel momentum space entanglement renormalization group (MERG) scheme for the topologically ordered (T.O.) ground state of the 2D Hubbard model on a square lattice (\cite{anirbanmotti,anirbanmott2}) using a unitary quantum circuit comprised of non-local unitary gates. At each MERG step, the unitary quantum circuit disentangles a set of electronic states, thereby transforming the tensor network representation of the many-particle state. By representing the non-local unitary gate as a product of two-qubit disentangler gates, we provide an entanglement holographic mapping (EHM) representation for MERG. Using entanglement based measures from quantum information theory and complex network theory, we study the emergence of topological order in the bulk of the EHM. The MERG reveals distinct holographic entanglement features for the normal metallic, topologically ordered insulating quantum liquid and Neél antiferromagnetic symmetry-broken ground states of the 2D Hubbard model at half-filling found in Ref.\cite{anirbanmotti}. An MERG analysis of the quantum critical point of the hole-doped 2D Hubbard model found in Ref.\cite{anirbanmott2} reveals the evolution of the many-particle entanglement of the quantum liquid ground state with hole-doping, as well as how the collapse of Mottness is responsible for the emergence of d-wave superconductivity. We perform an information theoretic analysis of the EHM network, demonstrating that the information bottleneck principle is responsible for the distillation of entanglement features in the heirarchical structure of the EHM network. As a result, we construct a deep neural network (DNN) architecture based on our EHM network, and employ it for predicting the onset of topological order. We also demonstrate that the DNN is capable of distinguishing between the topologically ordered and gapless normal metallic phases.

cond-mat.str-el