arXiv subjects

Siegfried H. Glenzer

Publications and source records attributed to Siegfried H. Glenzer.

9 recordsLinked to original sources

arXiv2026

Continuous Laser-Driven α Source

Laser-driven proton-boron fusion offers a path for generation of $α$ particles on a compact scale. Conventional solid-target experiments, however, are fundamentally limited by target degradation and low shot-repetition capacity. Here, we demonstrate a continuous laser-driven $α$ particle source utilizing target-normal sheath acceleration from a continuously replenishable ultrathin water-leaf jet target. The proton beam interacts with a downstream boron nitride converter, driving the $^{11}\text{B}(p,α)^{8}\text{Be}$ reaction which yields three $α$ particles. The measurement was repeated across $18{,}000$ consecutive shots at a rate of $10\,\text{Hz}$. The outgoing $α$-particle yield and spectral fluence were measured and benchmarked against comprehensive particle-transport simulations. The numerical and experimental results reveal a pronounced flattening in the energy-differential $α$-particle spectrum escaping from the converter, driven by depth-dependent reaction yield and stopping power effects. The sustained stable $α$-particle production at high cumulative yields paves the way for applications in targeted particle therapy and laser-driven plasma-fusion research.

physics.plasm-ph↗

arXiv2026

Electronic Signature of Melting Onset in Polycrystalline Copper at Extreme Conditions

Ultrafast melting is fundamentally a structural transition of the ionic lattice, but this rearrangement also reshapes the electronic properties by changing the energy landscape and scattering mechanisms. Although the electrons react almost instantaneously, it is not a priori clear how much lattice disorder is required for a significant response. Here, we show that the onset of melting already produces a clear electronic signature in polycrystalline copper. Using single-shot terahertz time-domain spectroscopy on thin films excited over a wide range of laser fluences, we infer the transient conductivity during the first picoseconds after excitation. The data, supported by two-temperature molecular-dynamics simulations, show that before melting, electron transport is substantially limited by grain-boundary scattering and that melting strongly suppresses this channel. As melting begins at these interfaces, we observe a transient increase in the conductivity that directly marks the onset of the phase transition. More broadly, these results show that ionic and electronic relaxation stages are closely coupled in nonequilibrium laser-driven matter and that optical measurements can resolve distinct stages of melting.

cond-mat.mtrl-sci↗

arXiv2024

Speed of sound in methane under conditions of planetary interiors

We present direct observations of acoustic waves in warm dense matter. We analyze wave-number- and energy-resolved x-ray spectra taken from warm dense methane created by laser heating a cryogenic liquid jet. X-ray diffraction and inelastic free-electron scattering yield sample conditions of 0.3$\pm$0.1 eV and 0.8$\pm$0.1 g/cm$^3$, corresponding to a pressure of $\sim$13 GPa. Inelastic x-ray scattering was used to observe the collective oscillations of the ions. With a highly improved energy resolution of $\sim$50 meV, we could clearly distinguish the Brillouin peaks from the quasielastic Rayleigh feature. Data at different wave numbers were utilized to derive a sound speed of 5.9$\pm$0.5 km/s, marking a high-temperature data point for methane and demonstrating consistency with Birch's law in this parameter regime.

physics.plasm-ph↗

arXiv2023

X-ray Thomson scattering spectra from DFT-MD simulations based on a modified Chihara formula

We study state-of-the-art approaches for calculating x-ray Thomson scattering spectra from density functional theory molecular dynamics (DFT-MD) simulations based on a modified Chihara formula that expresses the inelastic contribution in terms of the dielectric function. We compare the electronic dynamic structure factor computed from the Mermin dielectric function using an ab initio electron-ion collision frequency to computations using a linear response time dependent density functional theory (LR-TDDFT) framework for hydrogen and beryllium and investigate the dispersion of free-free and bound-free contributions to the scattering signal. A separate treatment of these contributions in the Mermin dielectric function shows excellent agreement with LR-TDDFT results for ambient-density beryllium, but breaks down for highly compressed matter where the bound states become pressure ionized. LR-TDDFT is used to reanalyze x-ray Thomson scattering experiments on beryllium demonstrating strong deviations from the plasma conditions inferred with traditional analytic models at small scattering angles.

physics.plasm-ph↗

arXiv2022

On the control of electron heating for optimal laser radiation pressure ion acceleration

We study the onset of electron heating in intense laser-solid interactions and its impact on the spectral quality of radiation pressure accelerated ions in both hole boring and light sail regimes. Two- and three-dimensional particle-in-cell (PIC) simulations are performed over a wide range of laser and target parameters and reveal how the pulse duration, profile, polarization, and target surface stability control the electron heating, the dominant ion acceleration mechanisms, and the ion spectra. We find that the onset of strong electron heating is associated with the growth of the Rayleigh-Taylor-like instability at the front surface and must be controlled to produce high-quality ion beams, even when circularly polarized lasers are employed. We define a threshold condition for the maximum duration of the laser pulse that allows mitigation of electron heating and radiation pressure acceleration of narrow energy spread ion beams. The model is validated by three-dimensional PIC simulations, and the few experimental studies that reported low energy spread radiation pressure accelerated ion beams appear to meet the derived criteria. The understanding provided by our work will be important in guiding future experimental developments, for example for the ultrashort laser pulses becoming available at state-of-the-art laser facilities, for which we predict that proton beams with ~150 - 250 MeV, ~30% energy spread, and a total laser-to-proton conversion efficiency of ~20% can be produced.

physics.plasm-ph↗

arXiv2022

Radiation pressure acceleration of high-quality ion beams using ultrashort laser pulses

The generation of compact, high-energy ion beams is one of the most promising applications of intense laser-matter interactions, but the control of the beam spectral quality remains an outstanding challenge. We show that in radiation pressure acceleration of a thin solid target the onset of electron heating is determined by the growth of the Rayleigh-Taylor-like instability at the front surface and must be controlled to produce ion beams with high spectral quality in the light sail regime. The growth rate of the instability imposes an upper limit on the laser pulse duration and intensity to achieve high spectral beam quality and we demonstrate that under this optimal regime, the maximum peak ion beam energy per nucleon is independent of target density, composition, and laser energy (transverse spot size). Our predictions are validated by two- and three-dimensional particle-in-cell simulations, which indicate that for recent and upcoming experimental facilities using ultrashort ($\lesssim 25$ fs) laser pulses it is possible to produce $100 - 300$ MeV proton beams with $\sim 30\%$ energy spread and high laser-to-proton energy conversion efficiency.

physics.plasm-ph↗

arXiv2020

Structure retrieval in liquid-phase electron scattering

Electron scattering on liquid samples has been enabled recently by the development of ultrathin liquid sheet technologies. The data treatment of liquid-phase electron scattering has been mostly reliant on methodologies developed for gas electron diffraction, in which theoretical inputs and empirical fittings are often needed to account for the atomic form factor and remove the inelastic scattering background. The accuracy and impact of these theoretical and empirical inputs has not been benchmarked for liquid-phase electron scattering data. In this work, we present an alternative data treatment method that requires neither theoretical inputs nor empirical fittings. The merits of this new method are illustrated through the retrieval of real-space molecular structure from experimental electron scattering patterns of liquid water, carbon tetrachloride, chloroform, and dichloromethane.

physics.chem-ph↗

arXiv2020

Carbon ionization at Gbar pressures: an ab initio perspective on astrophysical high-density plasmas

A realistic description of partially-ionized matter in extreme thermodynamic states is critical to model the interior and evolution of the multiplicity of high-density astrophysical objects. Current predictions of its essential property, the ionization degree, rely widely on analytical approximations that have been challenged recently by a series of experiments. Here, we propose a novel ab initio approach to calculate the ionization degree directly from the dynamic electrical conductivity using the Thomas-Reiche-Kuhn sum rule. This Density Functional Theory framework captures genuinely the condensed matter nature and quantum effects typical for strongly-correlated plasmas. We demonstrate this new capability for carbon and hydrocarbon, which most notably serve as ablator materials in inertial confinement fusion experiments aiming at recreating stellar conditions. We find a significantly higher carbon ionization degree than predicted by commonly used models, yet validating the qualitative behavior of the average atom model Purgatorio. Additionally, we find the carbon ionization state to remain unchanged in the environment of fully-ionized hydrogen. Our results will not only serve as benchmark for traditional models, but more importantly provide an experimentally accessible quantity in the form of the electrical conductivity.

physics.plasm-ph↗

arXiv2014

Bent crystal spectrometer for both frequency and wavenumber resolved x-ray scattering at a seeded free-electron laser

We present a cylindrically curved GaAs x-ray spectrometer with energy resolution $ΔE/E = 1.1\cdot 10^{-4}$ and wave-number resolution of $Δk/k = 3\cdot 10^{-3}$, allowing plasmon scattering at the resolution limits of the Linac Coherent Light Source (LCLS) x-ray free-electron laser. It spans scattering wavenumbers of 3.6 to $5.2/$Å in 100 separate bins, with only 0.34\% wavenumber blurring. The dispersion of 0.418~eV/$13.5\,μ$m agrees with predictions within 1.3\%. The reflection homogeneity over the entire wavenumber range was measured and used to normalize the amplitude of scattering spectra. The proposed spectrometer is superior to a mosaic HAPG spectrometer when the energy resolution needs to be comparable to the LCLS seeded bandwidth of 1~eV and a significant range of wavenumbers must be covered in one exposure.

physics.plasm-ph↗