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Simon Josephy

Publications and source records attributed to Simon Josephy.

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Nanoscale magnetometry of a synthetic three-dimensional spin texture

Multilayered synthetic antiferromagnets (SAFs) are artificial three-dimensional (3D) architectures engineered to create novel, complex, and stable spin textures. Non-invasive and quantitative nanoscale magnetic imaging of the two-dimensional stray field profile at the sample surface is essential for understanding the fundamental properties of the spin-structure and being able to tailor them to achieve new functionalities. However, the deterministic detection of spin textures and their quantitative characterization at the nanoscale remain challenging. Here, we use nitrogen-vacancy scanning probe microscopy (NV-SPM) under ambient conditions to perform the first quantitative vector-field magnetometry measurements in the multilayered SAF [(Co/Pt)$_5$/Co/Ru]$_3$/(Co/Pt)$_6$. We investigate nanoscale static and dynamic properties of antiferromagnetic domains with boundaries hosting ``one-dimensional'' ferromagnetic stripes with ~ 100 nm of width and periodic modulation of the magnetization. By employing NV-SPM measurements in different imaging modes and involving NV-probes with various crystallographic orientations, we demonstrated distinct fingerprints emerging from GHz-range spin noise and constant stray fields on the order of several mT. This provides quantitative insights into the structure of domains and domain walls, as well as, into magnetic noise associated with thermal spin-waves. Our work opens up new opportunities for quantitative vector-field magnetometry of modern magnetic materials with tailored 3D spin textures and stray field profiles, and potentially novel spin-wave dispersions--in a quantitative and non-invasive manner, with exceptional magnetic sensitivity and nanometer scale spatial resolution.

cond-mat.mes-hall

Above-room-temperature ferromagnetism in large-area epitaxial Fe3GaTe2/graphene van der Waals heterostructures

Fe3GaTe2 (FGaT), a two-dimensional (2D) layered ferromagnetic metal, exhibits a high Curie temperature (TC) ~ 360 K along with strong perpendicular magnetic anisotropy (PMA), making it a promising material candidate for next-generation energy-efficient magnetic devices. However, the vast majority of studies on FGaT to date have been limited to millimeter-sized bulk crystals and exfoliated flakes, which are unsuitable for practical applications and integration into device processing. Also, its combination with other 2D materials to form van der Waals heterostructures has only been achieved by flake stacking. Consequently, the controlled large-scale growth of FGaT and related heterostructures remains largely unexplored. In this work, we demonstrate a breakthrough in the high-quality, large-scale growth of epitaxial FGaT thin films on single-crystalline graphene/SiC templates using molecular beam epitaxy. Structural characterization confirms the high crystalline quality of the continuous FGaT/graphene van der Waals heterostructures. Temperature-dependent magnetization and anomalous Hall measurements reveal robust PMA with an enhanced TC well above room temperature, reaching up to 400 K. Furthermore, X-ray absorption and X-ray magnetic circular dichroism spectra provide insight into the spin and orbital magnetic moment contributions, further validating the high TC and robust PMA. These findings are highly significant for the future development of high-performance spintronic devices based on 2D heterostructures, with potential applications in next-generation data storage, logic processing and quantum technologies.

cond-mat.mtrl-sci