arXiv subjects

Simon L. Cornish

Publications and source records attributed to Simon L. Cornish.

At least 37 records · Page 2Linked to original sources

arXiv2022

A motorized rotation mount for fast and reproducible optical polarization control

We present a simple motorised rotation mount for a half-wave plate that can be used to rapidly change the polarization of light. We use the device to switch a high power laser beam between different optical dipole traps in an ultracold atom experiment. The device uses a stepper motor with a hollow shaft, which allows a beam to propagate along the axis of the motor shaft, minimising inertia and mechanical complexity. A simple machined adapter is used to mount the wave plate. We characterise the performance of the device, focusing on its capability to switch a beam between the output ports of a polarizing beamsplitter cube. We demonstrate a switching time of 15.9(3) ms, limited by the torque of the motor. The mount has a reaction time of 0.52(3) ms, and a rotational resolution of 0.45 degrees. The rotation is highly reproducible, with the stepper motor not missing a step in 2000 repeated tests over 11 hours.

physics.ins-det↗

arXiv2022

Preparation of $^{87}$Rb and $^{133}$Cs in the motional ground state of a single optical tweezer

We report simultaneous Raman sideband cooling of a single $^{87}$Rb atom and a single $^{133}$Cs atom held in separate optical tweezers at 814\,nm and 938\,nm, respectively. Starting from outside the Lamb-Dicke regime, after 45\,ms of cooling we measure probabilities to occupy the three-dimensional motional ground state of 0.86$^{+0.03}_{-0.04}$ for Rb and 0.95$^{+0.03}_{-0.04}$ for Cs. Our setup overlaps the Raman laser beams used to cool Rb and Cs, reducing hardware requirements by sharing equipment along the same beam path. The cooling protocol is scalable, and we demonstrate cooling of single Rb atoms in an array of four tweezers. After motional ground-state cooling, a 938\,nm tweezer is translated to overlap with a 814\,nm tweezer so that a single Rb and a single Cs atom can be transferred into a common 1064\,nm trap. By minimising the heating during the merging and transfer, we prepare the atoms in the relative motional ground state with an efficiency of 0.81$^{+0.08}_{-0.08}$. This is a crucial step towards the formation of single RbCs molecules confined in optical tweezer arrays.

physics.atom-ph↗

arXiv2022

Diatomic-py: A python module for calculating the rotational and hyperfine structure of $^1Σ$ molecules

We present a computer program to calculate the quantised rotational and hyperfine energy levels of $^{1}Σ$ diatomic molecules in the presence of dc electric, dc magnetic, and off-resonant optical fields. Our program is applicable to the bialkali molecules used in ongoing state-of-the-art experiments with ultracold molecular gases. We include functions for the calculation of space-fixed electric dipole moments, magnetic moments and transition dipole moments.

physics.comp-ph↗

arXiv2022

Observation of magnetic Feshbach resonances between Cs and ${}^{173}$Yb

We report the first observation of magnetic Feshbach resonances between ${}^{173}$Yb and $^{133}$Cs. In a mixture of Cs atoms prepared in the $(f=3, m_f=3)$ state and unpolarized fermionic ${}^{173}$Yb we observe resonant atom loss due to two sets of magnetic Feshbach resonances around 622~G and 702~G. Resonances for individual Yb nuclear spin components $m_{i,\mathrm{Yb}}$ are split by its interaction with the Cs electronic spin, which also provides the main coupling mechanism for the observed resonances. The observed splittings and relative resonance strengths are in good agreement with theoretical predictions from coupled-channel calculations.

physics.atom-ph↗

arXiv2021

Measurement of the tune-out wavelength for $^{133}$Cs at $880$ nm

We perform a measurement of the tune-out wavelength, $λ_{0}$, between the $D_{1}$, $6^2S_{1/2}\rightarrow6^2P_{1/2}$, and $D_{2}$, $6^2S_{1/2}\rightarrow6^2P_{3/2}$, transitions for $^{133}$Cs in the ground hyperfine state $(F=3, m_{F}=+3)$. At $λ_{0}$, the frequency-dependent scalar polarizability is zero leading to a zero scalar ac Stark shift. We measure the polarizability as a function of wavelength using Kapitza-Dirac scattering of a $^{133}$Cs Bose-Einstein condensate in a one-dimensional optical lattice, and determine the tune-out wavelength to be $λ_{0}=880.21790(40)_{\textrm{stat}}(8)_{\textrm{sys}}$ nm. From this measurement we determine the ratio of reduced matrix elements to be $\left|\left<{6P_{3/2}\| d\|6S_{1/2}}\right>\right|^{2}\left|\left<{6P_{1/2}\| d\|6S_{1/2}}\right>\right|^{2}=1.9808(2)$. This represents an improvement of a factor of 10 over previous results derived from excited-state lifetime measurements. We use the present measurement as a benchmark test of high-precision theory.

physics.atom-ph↗

arXiv2021

Molecule-molecule and atom-molecule collisions with ultracold RbCs molecules

Understanding ultracold collisions involving molecules is of fundamental importance for current experiments, where inelastic collisions typically limit the lifetime of molecular ensembles in optical traps. Here we present a broad study of optically trapped ultracold RbCs molecules in collisions with one another, in reactive collisions with Rb atoms, and in nonreactive collisions with Cs atoms. For experiments with RbCs alone, we show that by modulating the intensity of the optical trap, such that the molecules spend 75% of each modulation cycle in the dark, we partially suppress collisional loss of the molecules. This is evidence for optical excitation of molecule pairs mediated via sticky collisions. We find that the suppression is less effective for molecules not prepared in the spin-stretched hyperfine ground state. This may be due either to longer lifetimes for complexes or to laser-free decay pathways. For atom-molecule mixtures, RbCs+Rb and RbCs+Cs, we demonstrate that the rate of collisional loss of molecules scales linearly with the density of atoms. This indicates that, in both cases, the loss of molecules is rate-limited by two-body atom-molecule processes. For both mixtures, we measure loss rates that are below the thermally averaged universal limit.

physics.atom-ph↗

arXiv2021

Quantum Degenerate Mixtures of Cs and Yb

We report the production of quantum degenerate Bose-Bose mixtures of Cs and Yb with both attractive (Cs + $^{174}$Yb) and repulsive (Cs + $^{170}$Yb) interspecies interactions. Dual-species evaporation is performed in a bichromatic optical dipole trap that combines light at 1070 nm and 532 nm to enable control of the relative trap depths for Cs and Yb. Maintaining a trap which is shallower for Yb throughout the evaporation leads to highly efficient sympathetic cooling of Cs for both isotopic combinations at magnetic fields close to the Efimov minimum in the Cs three-body recombination rate at around 22 G. For Cs + $^{174}$Yb, we produce quantum mixtures with typical atom numbers of $N_\mathrm{Yb} \sim 5 \times 10^4$ and $N_\mathrm{Cs} \sim 5 \times 10^3$. We find that the attractive interspecies interaction (characterised by the scattering length $a_\mathrm{CsYb} = -75\,a_0$) is stabilised by the repulsive intraspecies interactions. For Cs + $^{170}$Yb, we produce quantum mixtures with typical atom numbers of $N_\mathrm{Yb} \sim 4 \times 10^4$, and $N_\mathrm{Cs} \sim 1 \times 10^4$. Here, the repulsive interspecies interaction ($a_\mathrm{CsYb} = 96\,a_0$) can overwhelm the intraspecies interactions, such that the mixture sits in a region of partial miscibility.

cond-mat.quant-gas↗

arXiv2021

Robust storage qubits in ultracold polar molecules

Quantum states with long-lived coherence are essential for quantum computation, simulation and metrology. The nuclear spin states of ultracold molecules prepared in the singlet rovibrational ground state are an excellent candidate for encoding and storing quantum information. However, it is important to understand all sources of decoherence for these qubits, and then eliminate them, in order to reach the longest possible coherence times. Here, we fully characterise the dominant mechanisms for decoherence of a storage qubit in an optically trapped ultracold gas of RbCs molecules using high-resolution Ramsey spectroscopy. Guided by a detailed understanding of the hyperfine structure of the molecule, we tune the magnetic field to where a pair of hyperfine states have the same magnetic moment. These states form a qubit, which is insensitive to variations in magnetic field. Our experiments reveal an unexpected differential tensor light shift between the states, caused by weak mixing of rotational states. We demonstrate how this light shift can be eliminated by setting the angle between the linearly polarised trap light and the applied magnetic field to a magic angle of $\arccos{(1/\sqrt{3})}\approx55^{\circ}$. This leads to a coherence time exceeding 6.9 s (90% confidence level). Our results unlock the potential of ultracold molecules as a platform for quantum computation.

cond-mat.quant-gas↗

arXiv2020

Dynamics of a degenerate Cs-Yb mixture with attractive interspecies interactions

We probe the collective dynamics of a quantum degenerate Bose-Bose mixture of Cs and $^{174}$Yb with attractive interspecies interactions. Specifically, we excite vertical center of mass oscillations of the Cs condensate, and observe significant damping for the Cs dipole mode, due to the rapid transfer of energy to the larger Yb component, and the ensuing acoustic dissipation. Numerical simulations based on coupled Gross-Pitaevskii equations provide excellent agreement, and additionally reveal the possibility of late-time revivals (beating) which are found to be highly sensitive to the Cs and Yb atom number combinations. By further tuning the interaction strength of Cs using a broad Feshbach resonance, we explore the stability of the degenerate mixture, and observe collapse of the Cs condensate mediated by the attractive Cs-Yb interaction when $a_{\mathrm{Cs}}<50 \, a_0$, well above the single-species collapse threshold, in good agreement with simulations.

cond-mat.quant-gas↗

arXiv2020

Coherent Manipulation of the Internal State of Ultracold $^{87}$Rb$^{133}$Cs Molecules with Multiple Microwave Fields

We explore coherent multi-photon processes in $^{87}$Rb$^{133}$Cs molecules using 3-level lambda and ladder configurations of rotational and hyperfine states, and discuss their relevance to future applications in quantum computation and quantum simulation. In the lambda configuration, we demonstrate the driving of population between two hyperfine levels of the rotational ground state via a two-photon Raman transition. Such pairs of states may be used in the future as a quantum memory, and we measure a Ramsey coherence time for a superposition of these states of 58(9) ms. In the ladder configuration, we show that we can generate and coherently populate microwave dressed states via the observation of an Autler-Townes doublet. We demonstrate that we can control the strength of this dressing by varying the intensity of the microwave coupling field. Finally, we perform spectroscopy of the rotational states of $^{87}$Rb$^{133}$Cs up to $N=6$, highlighting the potential of ultracold molecules for quantum simulation in synthetic dimensions. By fitting the measured transition frequencies we determine a new value of the centrifugal distortion coefficient $D_v=h\times207.3(2)~$Hz.

cond-mat.quant-gas↗

arXiv2020

Prospects of forming high-spin polar molecules from ultracold atoms

We have investigated Feshbach resonances in collisions of high-spin atoms such as Er and Dy with closed-shell atoms such as Sr and Yb, using coupled-channel scattering and bound-state calculations. We consider both low-anisotropy and high-anisotropy limits. In both regimes we find many resonances with a wide variety of widths. The wider resonances are suitable for tuning interatomic interactions, while some of the narrower resonances are highly suitable for magnetoassociation to form high-spin molecules. These molecules might be transferred to short-range states, where they would have large magnetic moments and electric dipole moments that can be induced with very low electric fields. The results offer the opportunity to study mixed quantum gases where one species is dipolar and the other is not, and open up important prospects for a new field of ultracold high-spin polar molecules.

physics.atom-ph↗

arXiv2020

Sticky collisions of ultracold RbCs molecules

Understanding and controlling collisions is crucial to the burgeoning field of ultracold molecules. All experiments so far have observed fast loss of molecules from the trap. However, the dominant mechanism for collisional loss is not well understood when there are no allowed 2-body loss processes. Here we experimentally investigate collisional losses of nonreactive ultracold RbCs molecules, and compare our findings with the sticky collision hypothesis that pairs of molecules form long-lived collision complexes. We demonstrate that loss of molecules occupying their rotational and hyperfine ground state is best described by second-order rate equations, consistent with the expectation for complex-mediated collisions, but that the rate is lower than the limit of universal loss. The loss is insensitive to magnetic field but increases for excited rotational states. We demonstrate that dipolar effects lead to significantly faster loss for an incoherent mixture of rotational states.

cond-mat.quant-gas↗

arXiv2020

Controlling the ac Stark effect of RbCs with dc electric and magnetic fields

We investigate the effects of static electric and magnetic fields on the differential ac Stark shifts for microwave transitions in ultracold bosonic $^{87}$Rb$^{133}$Cs molecules, for light of wavelength $λ= 1064~\mathrm{nm}$. Near this wavelength we observe unexpected two-photon transitions that may cause trap loss. We measure the ac Stark effect in external magnetic and electric fields, using microwave spectroscopy of the first rotational transition. We quantify the isotropic and anisotropic parts of the molecular polarizability at this wavelength. We demonstrate that a modest electric field can decouple the nuclear spins from the rotational angular momentum, greatly simplifying the ac Stark effect. We use this simplification to control the ac Stark shift using the polarization angle of the trapping laser.

physics.atom-ph↗

arXiv2020

A robust entangling gate for polar molecules using magnetic and microwave fields

Polar molecules are an emerging platform for quantum technologies based on their long-range electric dipole-dipole interactions, which open new possibilities for quantum information processing and the quantum simulation of strongly correlated systems. Here, we use magnetic and microwave fields to design a fast entangling gate with $>0.999$ fidelity and which is robust with respect to fluctuations in the trapping and control fields and to small thermal excitations. These results establish the feasibility to build a scalable quantum processor with a broad range of molecular species in optical-lattice and optical-tweezers setups.

quant-ph↗

arXiv2020

Loss of ultracold RbCs molecules via optical excitation of long-lived two-body collision complexes

We show that the lifetime of ultracold ground-state $^{87}$Rb$^{133}$Cs molecules in an optical trap is limited by fast optical excitation of long-lived two-body collision complexes. We partially suppress this loss mechanism by applying square-wave modulation to the trap intensity, such that the molecules spend 75% of each modulation cycle in the dark. By varying the modulation frequency, we show that the lifetime of the collision complex is $0.53\pm0.06$ ms in the dark. We find that the rate of optical excitation of the collision complex is $3^{+4}_{-2}\times10^{3}$ W$^{-1}$ cm$^2$ s$^{-1}$ for $λ= 1550$ nm, leading to a lifetime of <100 ns for typical trap intensities. These results explain the two-body loss observed in experiments on nonreactive bialkali molecules.

physics.atom-ph↗

arXiv2019

Splitting and recombination of bright-solitary-matter waves

Solitons are long-lived wavepackets that propagate without dispersion and exist in a wide range of one-dimensional (1D) nonlinear systems. A Bose-Einstein condensate trapped in a quasi-1D waveguide can support bright-solitary-matter waves (3D analogues of solitons) when interatomic interactions are sufficiently attractive that they cancel dispersion. Solitary-matter waves are excellent candidates for a new generation of highly sensitive interferometers, as their non-dispersive nature allows them to acquire phase shifts for longer times than conventional matter-waves interferometers. However, such an interferometer is yet to be realised experimentally. In this work, we demonstrate the splitting and recombination of a bright-solitary-matter wave on a narrow repulsive barrier, which brings together the fundamental components of an interferometer. We show that both interference-mediated recombination and classical velocity filtering effects are important, but for a sufficiently narrow barrier interference-mediated recombination can dominate. We reveal the extreme sensitivity of interference-mediated recombination to the experimental parameters, highlighting the potential of soliton interferometry.

cond-mat.quant-gas↗

arXiv2019

Magnetic Feshbach resonances in ultracold collisions between Cs and Yb atoms

We investigate magnetically tunable Feshbach resonances in ultracold collisions between ground-state Yb and Cs atoms, using coupled-channel calculations based on an interaction potential recently determined from photoassociation spectroscopy. We predict resonance positions and widths for all stable isotopes of Yb, together with resonance decay parameters where appropriate. The resonance patterns are richer and more complicated for fermionic Yb than for spin-zero isotopes, because there are additional level splittings and couplings due to scalar and tensorial Yb hyperfine interactions. We examine collisions involving Cs atoms in a variety of hyperfine states, and identify resonances that appear most promising for experimental observation and for magnetoassociation to form ultracold CsYb molecules.

physics.atom-ph↗

arXiv2018

Two-photon photoassociation spectroscopy of CsYb: ground-state interaction potential and interspecies scattering lengths

We perform two-photon photoassociation spectroscopy of the heteronuclear CsYb molecule to measure the binding energies of near-threshold vibrational levels of the $X~^{2}Σ_{1/2}^{+}$ molecular ground state. We report results for $^{133}$Cs$^{170}$Yb, $^{133}$Cs$^{173}$Yb and $^{133}$Cs$^{174}$Yb, in each case determining the energy of several vibrational levels including the least-bound state. We fit an interaction potential based on electronic structure calculations to the binding energies for all three isotopologs and find that the ground-state potential supports 77 vibrational levels. We use the fitted potential to predict the interspecies s-wave scattering lengths for all seven Cs+Yb isotopic mixtures.

physics.atom-ph↗