arXiv subjects

Simon Trebst

Publications and source records attributed to Simon Trebst.

At least 73 records · Page 4Linked to original sources

arXiv2019

Functional renormalization group for frustrated magnets with nondiagonal spin interactions

In the field of quantum magnetism, the advent of numerous spin-orbit assisted Mott insulating compounds, such as the family of Kitaev materials, has led to a growing interest in studying general spin models with non-diagonal interactions that do not retain the SU(2) invariance of the underlying spin degrees of freedom. However, the exchange frustration arising from these non-diagonal and often bond-directional interactions for two- and three-dimensional lattice geometries poses a serious challenge for numerical many-body simulation techniques. In this paper, we present an extended formulation of the pseudo-fermion functional renormalization group that is capable of capturing the physics of frustrated quantum magnets with generic (diagonal and off-diagonal) two-spin interaction terms. Based on a careful symmetry analysis of the underlying flow equations, we reveal that the computational complexity grows only moderately, as compared to models with only diagonal interaction terms. We apply the formalism to a kagome antiferromagnet which is augmented by general in-plane and out-of-plane Dzyaloshinskii-Moriya (DM) interactions, as argued to be present in the spin liquid candidate material herbertsmithite. We calculate the complete ground state phase diagram in the strength of in-plane and out-of-plane DM couplings, and discuss the extended stability of the spin liquid of the unperturbed kagome antiferromagnet in the presence of these couplings.

cond-mat.str-el↗

arXiv2019

Chiral spin liquids with crystalline $\mathbb{Z}_2$ gauge order in a three-dimensional Kitaev model

Chiral spin liquids (CSLs) are time-reversal symmetry breaking ground states of frustrated quantum magnets that show no long-range magnetic ordering, but instead exhibit topological order and fractional excitations. Their realization in simple and tractable microscopic models has, however, remained an open challenge for almost two decades until it was realized that Kitaev models on lattices with odd-length loops are natural hosts for such states, even in the absence of a time-reversal symmetry breaking magnetic field. Here we report on the formation of CSLs in a three-dimensional Kitaev model, which differ from their widely studied two-dimensional counterparts, namely, they exhibit a crystalline ordering of the $\mathbb{Z}_2$ gauge fluxes and thereby break some of the underlying lattice symmetries. We study the formation of these unconventional CSLs via extensive quantum Monte Carlo simulations and demonstrate that they are separated from the featureless paramagnet at high temperatures by a single first-order transition at which both time-reversal and lattice symmetries are simultaneously broken. Using variational approaches for the ground state, we explore the effect of varying the Kitaev couplings and find at least five distinct CSL phases, all of which possess crystalline ordering of the $\mathbb{Z}_2$ gauge fluxes. For some of these phases, the complementary itinerant Majorana fermions exhibit gapless band structures with topological features such as Weyl nodes or nodal lines in the bulk and Fermi arc or drumhead surface states.

cond-mat.str-el↗

arXiv2019

Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures

Twisting moiré heterostructures to the flatband regime allows for the formation of strongly correlated quantum states, since the dramatic reduction of the bandwidth can cause the residual electronic interactions to set the principal energy scale. An effective description for such correlated moiré heterostructures, derived in the strong-coupling limit at integer filling, generically leads to spin-valley Heisenberg models. Here we explore the emergence and stability of spin liquid behavior in an SU(2)$^{\mathrm{spin}}\otimes$SU(2)$^{\mathrm{valley}}$ Heisenberg model upon inclusion of Hund's-induced and longer-ranged exchange couplings, employing a pseudofermion functional renormalization group approach. We consider two lattice geometries, triangular and honeycomb (relevant to different moiré heterostructures), and find, for both cases, an extended parameter regime surrounding the SU(4) symmetric point where no long-range order occurs, indicating a stable realm of quantum spin liquid behavior. For large Hund's coupling, we identify the adjacent magnetic orders, with both antiferromagnetic and ferromagnetic ground states emerging in the separate spin and valley degrees of freedom. For both lattice geometries the inclusion of longer-ranged exchange couplings is found to have both stabilizing and destabilizing effects on the spin liquid regime depending on the sign of the additional couplings.

cond-mat.str-el↗

arXiv2019

Thermal Hall signatures of non-Kitaev spin liquids in honeycomb Kitaev materials

Motivated by the recent surge of field-driven phenomena discussed for Kitaev materials, in particular the experimental observation of a finite thermal Hall effect and theoretical proposals for the emergence of additional spin liquid phases beyond the conventional Kitaev spin liquid, we develop a theoretical understanding of the thermal Hall effect in honeycomb Kitaev materials in magnetic fields. Our focus is on gapless U(1) spin liquids with a spinon Fermi surface, which have been shown to arise as field-induced phases. We demonstrate that in the presence of symmetry-allowed, second-neighbor Dzyaloshinskii-Moriya interactions these spin liquids give rise to a finite, non-quantized, thermal Hall conductance in a magnetic field. The microscopic origin of this thermal Hall effect can be traced back to an interplay of Dzyaloshinskii-Moriya interaction and Zeeman coupling, which generates an internal U(1) gauge flux that twists the motion of the emergent spinons. We argue that such a non-quantized thermal Hall effect is a generic response in Kitaev models for a range of couplings.

cond-mat.str-el↗

arXiv2019

Cluster functional renormalization group and absence of a bilinear spin liquid in the $J_1$-$J_2$-Heisenberg model

The pseudofermion functional renormalization group (pf-FRG) has been put forward as a semi-analytical scheme that, for a given microscopic spin model, allows to discriminate whether the low-temperature states exhibit magnetic ordering or a tendency towards the formation of quantum spin liquids. However, the precise nature of the putative spin liquid ground state has remained hard to infer from the original (single-site) pf-FRG scheme. Here we introduce a cluster pf-FRG approach, which allows for a more stringent connection between a microscopic spin model and its low-temperature spin liquid ground states. In particular, it allows to calculate spatially structured fermion bilinear expectation values on spatial clusters, which are formed by splitting the original lattice into several sublattices, thereby allowing for the positive identification of a family of bilinear spin liquid states. As an application of this cluster pf-FRG approach, we consider the $J_1$-$J_2$ SU($N$)-Heisenberg model on a square lattice, which is a paradigmatic example for a frustrated quantum magnet exhibiting quantum spin liquid behavior for intermediate coupling strengths. In the well-established large-$N$ limit of this model, we show that our approach correctly captures the emergence of the $π$-flux spin liquid state at low temperatures. For small $N$, where the precise nature of the ground state remains controversial, we focus on the widely studied case of $N=2$, for which we determine the low-temperature phase diagram near the strongly-frustrated regime after implementing the fermion number constraint by the flowing Popov-Fedotov method. Our results suggest that the $J_1$-$J_2$-Heisenberg model does not support the formation of a fermion bilinear spin liquid state.

cond-mat.str-el↗

arXiv2019

Monte Carlo Studies of Quantum Critical Metals

Metallic quantum critical phenomena are believed to play a key role in many strongly correlated materials, including high temperature superconductors. Theoretically, the problem of quantum criticality in the presence of a Fermi surface has proven to be highly challenging. However, it has recently been realized that many models used to describe such systems are amenable to numerically exact solution by quantum Monte Carlo (QMC) techniques, without suffering from the fermion sign problem. In this article, we review the status of the understanding of metallic quantum criticality, and the recent progress made by QMC simulations. We focus on the cases of spin density wave and Ising nematic criticality. We describe the results obtained so far, and their implications for superconductivity, non-Fermi liquid behavior, and transport in the vicinity of metallic quantum critical points. Some of the outstanding puzzles and future directions are highlighted.

cond-mat.str-el↗

arXiv2019

Emergence of a Field-Driven U(1) Spin Liquid in the Kitaev Honeycomb Model

In the field of quantum magnetism, the exactly solvable Kitaev honeycomb model serves as a paradigm for the fractionalization of spin degrees of freedom and the formation of $\mathbb{Z}_2$ quantum spin liquids. An intense experimental search has led to the discovery of a number of spin-orbit entangled Mott insulators that realize its characteristic bond-directional interactions and, in the presence of magnetic fields, exhibit no indications of long-range order. Here, we map out the complete phase diagram of the Kitaev model in tilted magnetic fields and report the emergence of a distinct gapless quantum spin liquid at intermediate field strengths. Analyzing a number of static, dynamical, and finite temperature quantities using numerical exact diagonalization techniques, we find strong evidence that this phase exhibits gapless fermions coupled to a massless $U(1)$ gauge field. We discuss its stability in the presence of perturbations that naturally arise in spin-orbit entangled candidate materials.

cond-mat.str-el↗

arXiv2019

Symmetry-protected non-Fermi liquids, Kagome spin liquids, and the chiral Kondo lattice model

The theoretical description of non-Fermi liquids is among the most challenging questions in strongly correlated quantum matter. While there are many experimental candidates for such phases, few examples can be studied using controlled theoretical approaches. Here we introduce a novel conceptual perspective to analytically describe the non-Fermi liquid physics of gapless spin liquids arising in a family of two- and three-dimensional Kagome models. We first discuss a symmetry-protection mechanism that is responsible for the stability of the gapless phase. We then re-cast the two-dimensional Kagome spin model as a chiral Kondo lattice model that can be tackled analytically using what is in a sense a generalization of coupled-wire constructions. We provide extensive numerical evidence for a gapless spin liquid in the two-dimensional Kagome model and discuss generalizations to three dimensions.

cond-mat.str-el↗

arXiv2018

Probing transport in quantum many-fermion simulations via quantum loop topography

Quantum many-fermion systems give rise to diverse states of matter that often reveal themselves in distinctive transport properties. While some of these states can be captured by microscopic models accessible to numerical exact quantum Monte Carlo simulations, it nevertheless remains challenging to numerically access their transport properties. Here we demonstrate that quantum loop topography (QLT) can be used to directly probe transport by machine learning current-current correlations in imaginary time. We showcase this approach by studying the emergence of superconducting fluctuations in the negative-U Hubbard model and a spin-fermion model for a metallic quantum critical point. For both sign-free models, we find that the QLT approach detects a change in transport in very good agreement with their established phase diagrams. These proof-of-principle calculations combined with the numerical efficiency of the QLT approach point a way to identify hitherto elusive transport phenomena such as non-Fermi liquids using machine learning algorithms.

cond-mat.str-el↗

arXiv2018

Topological Mechanics from Supersymmetry

In topological mechanics, the identification of a mechanical system's rigidity matrix with an electronic tight-binding model allows to infer topological properties of the mechanical system, such as the occurrence of `floppy' boundary modes, from the associated electronic band structure. Here we introduce an approach to systematically construct topological mechanical systems by an exact supersymmetry (SUSY) that relates the bosonic (mechanical) and fermionic (e.g. electronic) degrees of freedom. As examples we discuss mechanical analogues of the Kitaev honeycomb model and of a second-order topological insulator with floppy corner modes. Our SUSY construction naturally defines hitherto unexplored topological invariants for bosonic (mechanical) systems, such as bosonic Wilson loop operators that are formulated in terms of a SUSY-related fermionic Berry curvature.

cond-mat.str-el↗

arXiv2018

Landau theory of multipolar orders in Pr(TM)$_2$X$_{20}$ Kondo materials

A series of Pr(TM)$_2$X$_{20}$ (with TM=Ti,V,Rh,Ir and X=Al,Zn) Kondo materials, containing non-Kramers Pr$^{3+}$ $4f^2$ moments on a diamond lattice, have been shown to exhibit intertwined orders such as quadrupolar order and superconductivity. Motivated by these experiments, we propose and study a Landau theory of multipolar order to capture the phase diagram and its field dependence. In zero magnetic field, we show that different quadrupolar states, or the coexistence of quadrupolar and octupolar orderings, may lead to ground states with multiple broken symmetries. Upon heating, such states may undergo two-step thermal transitions into the symmetric paramagnetic phase, with partial restoration of broken symmetries in the intervening phase. For nonzero magnetic field, we show the evolution of these thermal phase transitions strongly depends on the field direction, due to clock anisotropy terms in the free energy. Our findings shed substantial light on experimental results in the Pr(TM)$_2$Al$_{20}$ materials. We propose further experimental tests to distinguish purely quadrupolar orders from coexisting quadrupolar-octupolar orders.

cond-mat.str-el↗

arXiv2018

Majorana Corner Modes in a Second-Order Kitaev Spin Liquid

Higher-order topological insulators are distinguished by the existence of topologically protected modes with codimension two or higher. Here, we report the manifestation of a second-order topological insulator in a two dimensional frustrated quantum magnet, which exhibits topological corner modes. Our exactly-solvable model is a generalization of the Kitaev honeycomb model to the Shastry-Sutherland lattice that, besides a chiral spin liquid phase, exhibits a gapped spin liquid with Majorana corner modes, which are protected by two mirror symmetries. This second-order Kitaev spin liquid remains stable in the presence of thermal fluctuations and undergoes a finite-temperature phase transition evidenced in large-scale quantum Monte Carlo simulations.

cond-mat.str-el↗

arXiv2018

Topological semimetals and insulators in three-dimensional honeycomb materials

Semimetals, in which conduction and valence bands touch but do not form Fermi surfaces, have attracted considerable interest for their anomalous properties starting with the discovery of Dirac matter in graphene and other two-dimensional honeycomb materials. Here we introduce a family of three-dimensional honeycomb systems whose electronic band structures exhibit a variety of topological semimetals with Dirac nodal lines. We show that these nodal lines appear in varying numbers and mutual geometries, depending on the underlying lattice structure. They are stabilized, in most cases, by a combination of time-reversal and inversion symmetries and are accompanied by topologically protected "drumhead" surface states. In the bulk, these nodal line systems exhibit Landau level quantization and flat bands upon applying a magnetic field. In the presence of spin-orbit coupling, these topological semimetals are found to generically form (strong) topological insulators. This comprehensive classification of the electronic band structures of three-dimensional honeycomb systems might serve as guidance for future material synthesis.

cond-mat.str-el↗

arXiv2018

Quantum spin liquids in frustrated spin-1 diamond antiferromagnets

Motivated by the recent synthesis of the spin-1 A-site spinel NiRh$_{\text 2}$O$_{\text 4}$, we investigate the classical to quantum crossover of a frustrated $J_1$-$J_2$ Heisenberg model on the diamond lattice upon varying the spin length $S$. Applying a recently developed pseudospin functional renormalization group (pf-FRG) approach for arbitrary spin-$S$ magnets, we find that systems with $S \geq 3/2$ reside in the classical regime where the low-temperature physics is dominated by the formation of coplanar spirals and a thermal (order-by-disorder) transition. For smaller local moments $S$=1 or $S$=1/2 we find that the system evades a thermal ordering transition and forms a quantum spiral spin liquid where the fluctuations are restricted to characteristic momentum-space surfaces. For the tetragonal phase of NiRh$_{\text 2}$O$_{\text 4}$, a modified $J_1$-$J_2^-$-$J_2^\perp$ exchange model is found to favor a conventionally ordered Néel state (for arbitrary spin $S$) even in the presence of a strong local single-ion spin anisotropy and it requires additional sources of frustration to explain the experimentally observed absence of a thermal ordering transition.

cond-mat.str-el↗

arXiv2017

Functional renormalization group approach to SU(N) Heisenberg models: Real-space RG at arbitrary N

The pseudofermion functional renormalization group (pf-FRG) is one of the few numerical approaches that has been demonstrated to quantitatively determine the ordering tendencies of frustrated quantum magnets in two and three spatial dimensions. The approach, however, relies on a number of presumptions and approximations, in particular the choice of pseudofermion decomposition and the truncation of an infinite number of flow equations to a finite set. Here we generalize the pf-FRG approach to SU(N)-spin systems with arbitrary N and demonstrate that the scheme becomes exact in the large-N limit. Numerically solving the generalized real-space renormalization group equations for arbitrary N, we can make a stringent connection between the physically most significant case of SU(2)-spins and more accessible SU(N) models. In a case study of the square-lattice SU(N) Heisenberg antiferromagnet, we explicitly demonstrate that the generalized pf-FRG approach is capable of identifying the instability indicating the transition into a staggered flux spin liquid ground state in these models for large, but finite values of N. In a companion paper (arXiv:1711.02183) we formulate a momentum-space pf-FRG approach for SU(N) spin models that allows us to explicitly study the large-N limit and access the low-temperature spin liquid phase.

cond-mat.str-el↗

arXiv2017

Functional renormalization group approach to SU(N) Heisenberg models: Momentum-space RG for the large-N limit

In frustrated magnetism, making a stringent connection between microscopic spin models and macroscopic properties of spin liquids remains an important challenge. A recent step towards this goal has been the development of the pseudofermion functional renormalization group approach (pf-FRG) which, building on a fermionic parton construction, enables the numerical detection of the onset of spin liquid states as temperature is lowered. In this work, focusing on the SU(N) Heisenberg model at large N, we extend this approach in a way that allows us to directly enter the low-temperature spin liquid phase, and to probe its character. Our approach proceeds in momentum space, making it possible to keep the truncation minimalistic, while also avoiding the bias introduced by an explicit decoupling of the fermionic parton interactions into a given channel. We benchmark our findings against exact mean-field results in the large-N limit, and show that even without prior knowledge the pf-FRG approach identifies the correct mean-field decoupling channel. On a technical level, we introduce an alternative finite temperature regularization scheme that is necessitated to access the spin liquid ordered phase. In a companion paper arXiv:1711.02182 we present a different set of modifications of the pf-FRG scheme that allow us to study SU(N) Heisenberg models (using a real-space RG approach) for arbitrary values of N, albeit only up to the phase transition towards spin liquid physics.

cond-mat.str-el↗

arXiv2017

Two-stage multipolar ordering in Pr(TM)$_2$Al$_{20}$ Kondo materials

Among heavy fermion materials, there is a set of rare-earth intermetallics with non-Kramers Pr$^{3+}$ $4f^2$ moments which exhibit a rich phase diagram with intertwined quadrupolar orders, superconductivity, and non-Fermi liquid behavior. However, more subtle broken symmetries such as multipolar orders in these Kondo materials remain poorly studied. Here, we argue that multi-spin interactions between local moments beyond the conventional two-spin exchange must play an important role in Kondo materials near the ordered to heavy Fermi liquid transition. We show that this drives a plethora of phases with coexisting multipolar orders and multiple thermal phase transitions, providing a natural framework for interpreting experiments on the Pr(TM)$_2$Al$_{20}$ class of compounds.

cond-mat.str-el↗

arXiv2017

Quantum phase recognition via unsupervised machine learning

The application of state-of-the-art machine learning techniques to statistical physic problems has seen a surge of interest for their ability to discriminate phases of matter by extracting essential features in the many-body wavefunction or the ensemble of correlators sampled in Monte Carlo simulations. Here we introduce a gener- alization of supervised machine learning approaches that allows to accurately map out phase diagrams of inter- acting many-body systems without any prior knowledge, e.g. of their general topology or the number of distinct phases. To substantiate the versatility of this approach, which combines convolutional neural networks with quantum Monte Carlo sampling, we map out the phase diagrams of interacting boson and fermion models both at zero and finite temperatures and show that first-order, second-order, and Kosterlitz-Thouless phase transitions can all be identified. We explicitly demonstrate that our approach is capable of identifying the phase transition to non-trivial many-body phases such as superfluids or topologically ordered phases without supervision.

cond-mat.str-el↗