arXiv subjects

Simone Finizio

Publications and source records attributed to Simone Finizio.

At least 37 records · Page 2Linked to original sources

arXiv2024

Competing anisotropies in the chiral cubic magnet Co$_8$Zn$_8$Mn$_4$ unveiled by resonant x-ray magnetic scattering

The cubic $β$-Mn-type alloy Co$_8$Zn$_8$Mn$_4$ is a chiral helimagnet that exhibits a peculiar temperature-dependent behavior in the spiral pitch, which decreases from 130 nm at room temperature to 70 nm below 20 K. Notably, this shortening is also accompanied by a structural transition of the metastable skyrmion texture, transforming from a hexagonal lattice to a square lattice of elongated skyrmions. The underlying mechanism of these transformations remain unknown, with interactions potentially involved including temperature-dependent Dzyaloshinskii-Moriya interaction, magnetocrystalline anisotropy, and exchange anisotropy. Here, x-ray resonant magnetic small-angle scattering in vectorial magnetic fields was employed to investigate the temperature dependence of the anisotropic properties of the helical phase in Co$_8$Zn$_8$Mn$_4$. Our results reveal quantitatively that the magnitude of the anisotropic exchange interaction increases by a factor of 4 on cooling from room temperature to 20 K, leading to a 5% variation in the helical pitch within the (001) plane at 20 K. While anisotropic exchange interaction contributes to the shortening of the spiral pitch, its magnitude is insufficient to explain the variation in the spiral periodicity from room to low temperatures. Finally, we demonstrate that magnetocrystalline and exchange anisotropies compete, favoring different orientations of the helical vector in the ground state.

cond-mat.mes-hall↗

arXiv2024

Three-dimensional spin-wave dynamics, localization and interference in a synthetic antiferromagnet

Spin waves are collective perturbations in the orientation of the magnetic moments in magnetically ordered materials. Their rich phenomenology is intrinsically three-dimensional; however, the three-dimensional imaging of spin waves has so far not been possible. Here, we image the three-dimensional dynamics of spin waves excited in a synthetic antiferromagnet, with nanoscale spatial resolution and sub-ns temporal resolution, using time-resolved magnetic laminography. In this way, we map the distribution of the spin-wave modes throughout the volume of the structure, revealing unexpected depth-dependent profiles originating from the interlayer dipolar interaction. We experimentally demonstrate the existence of complex three-dimensional interference patterns and analyze them via micromagnetic modelling. We find that these patterns are generated by the superposition of spin waves with non-uniform amplitude profiles, and that their features can be controlled by tuning the composition and structure of the magnetic system. Our results open unforeseen possibilities for the study and manipulation of complex spin-wave modes within nanostructures and magnonic devices.

cond-mat.mes-hall↗

arXiv2023

Magneto-Acoustic Waves in antiferromagnetic CuMnAs excited by Surface Acoustic Waves

Magnetoelastic effects in antiferromagnetic CuMnAs are investigated by applying dynamic strain in the 0.01% range through surface acoustic waves in the GaAs substrate. The magnetic state of the CuMnAs/GaAs is characterized by a multitude of submicron-sized domains which we image by x-ray magnetic linear dichroism combined with photoemission electron microscopy. Within the explored strain range, CuMnAs shows magnetoelastic effects in the form of Néel vector waves with micrometer wavelength, which corresponds to an averaged overall spin-axis rotation up to 2.4 deg driven by the time-dependent strain from the surface acoustic wave. Measurements at different temperatures indicate a reduction of the wave amplitude when lowering the temperature. However, no domain wall motion has been detected on the nanosecond timescale

cond-mat.mes-hall↗

arXiv2023

Quantifying the Topology of Magnetic Skyrmions in three Dimensions

Magnetic skyrmions have so far been treated as two-dimensional spin structures characterized by a topological winding number describing the rotation of spins across the skyrmion. However, in real systems with a finite thickness of the material being larger than the magnetic exchange length, the skyrmion spin texture extends into the third dimension and cannot be assumed as homogeneous. Using soft x-ray laminography we reconstruct with about 20nm spatial (voxel) resolution the full three-dimensional spin texture of a skyrmion in an 800 nm diameter and 95 nm thin disk patterned into a trilayer [Ir/Co/Pt] thin film structure. A quantitative analysis finds that the evolution of the radial profile of the topological skyrmion number and the chirality is non-uniform across the thickness of the disk. Estimates of local micromagnetic energy densities suggest that the changes in topological profile are related to non-uniform competing energetic interactions. Theoretical calculations and micromagnetic simulations are consistent with the experimental findings. Our results provide the foundation for nanoscale magnetic metrology for future tailored spintronics devices using topology as a design parameter, and have the potential to reverse-engineer a spin Hamiltonian from macroscopic data, tying theory more closely to experiment.

cond-mat.mtrl-sci↗

arXiv2023

Spatially reconfigurable topological textures in freestanding antiferromagnetic nanomembranes

Antiferromagnets hosting real-space topological spin textures are promising platforms to model fundamental ultrafast phenomena and explore spintronics. However, to date, they have only been fabricated epitaxially on specific symmetry-matched crystalline substrates, to preserve their intrinsic magneto-crystalline order. This curtails their integration with dissimilar supports, markedly restricting the scope of fundamental and applied investigations. Here, we circumvent this limitation by designing detachable crystalline antiferromagnetic nanomembranes of $α$-Fe$_{2}$O$_{3}$, that can be transferred onto other desirable supports after growth. We develop transmission-based antiferromagnetic vector-mapping to show that these nanomembranes harbour rich topological phenomenology at room temperature. Moreover, we exploit their extreme flexibility to demonstrate three-dimensional reconfiguration of antiferromagnetic properties, driven locally via flexure-induced strains. This allows us to spatially design antiferromagnetic states outside their typical thermal stability window. Integration of such freestanding antiferromagnetic layers with flat or curved nanostructures could enable spin texture designs tailored by magnetoelastic-/geometric-effects in the quasi-static and dynamical regimes, opening new explorations into curvilinear antiferromagnetism and unconventional computing.

cond-mat.mtrl-sci↗

arXiv2022

Collective skyrmion motion under the influence of an additional interfacial spin-transfer torque

Here we study the effect of an additional interfacial spin-transfer torque, as well as the well established spin-orbit torque and bulk spin-transfer torque, on skyrmion collections - group of skyrmions dense enough that they are not isolated from on another - in ultrathin heavy metal / ferromagnetic multilayers, by comparing modelling with experimental results. Using a skyrmion collection with a range of skyrmion diameters and landscape disorder, we study the dependence of the skyrmion Hall angle on diameter and velocity, as well as the velocity as a function of diameter. We show the experimental results are in good agreement with modelling when including the interfacial spin-transfer torque, and cannot be reproduced by using the spin-orbit torque alone. We also show that for skyrmion collections the velocity is approximately independent of diameter, in marked contrast to the motion of isolated skyrmions, as the group of skyrmions move together at an average group velocity. Moreover, the calculated skyrmion velocities are comparable to those obtained in experiments when the interfacial spin-transfer torque in included, whilst modelling using the spin-orbit torque alone shows large discrepancies with the experimental data. Our results thus show the significance of the interfacial spin-transfer torque in ultrathin magnetic multilayers, which is of similar strength to the spin-orbit torque, and both significantly larger than the bulk spin-transfer torque. Due to the good agreement with experiments, we conclude that the interfacial spin-transfer torque should be included in numerical modelling for correct reproduction of experimental results.

cond-mat.mes-hall↗

arXiv2022

Domain wall motion at low current density in a synthetic antiferromagnet nanowire

The current-driven motion of magnetic domain walls (DWs) is the working principle of magnetic racetrack memories. In this type of spintronic technology, high current densities are used to propel DW motion in magnetic nanowires, causing significant wire heating. Synthetic antiferromagnets are known to show very fast DW motion at high current densities, but lower current densities around onset of motion have received less attention. Here we use scanning transmission x-ray microscopy to study the response of DWs in a SAF multilayer to currents. We observe that the DWs depin at $\sim 3 \times 10^{11}$~A/m$^2$ and move more quickly in response to 5~ns duration current pulses than in comparable conventional multilayers. The results suggest that DWs in SAF structures are superior to conventional Néel DWs for low energy consumption racetrack technologies.

cond-mat.mes-hall↗

arXiv2021

Optical excitation of electromagnons in hexaferrite

Understanding ultrafast magnetization dynamics on the microscopic level is of strong current interest due to the potential for applications in information storage. In recent years, the spin-lattice coupling has been recognized to be essential for ultrafast magnetization dynamics. Magnetoelectric multiferroics of type II possess intrinsic correlations among magnetic sublattices and electric polarization (P) through spin-lattice coupling, enabling fundamentally coupled dynamics between spins and lattice. Here we report on ultrafast magnetization dynamics in a room-temperature multiferroic hexaferrite possessing ferrimagnetic and antiferromagnetic sublattices, revealed by time-resolved resonant x-ray diffraction. A femtosecond above-bandgap excitation triggers a coherent magnon in which the two magnetic sublattices entangle and give rise to a transient modulation of P. A novel microscopic mechanism for triggering the coherent magnon in this ferrimagnetic insulator based on the spin-lattice coupling is proposed. Our finding opens up a novel but general pathway for ultrafast control of magnetism.

cond-mat.str-el↗

arXiv2021

Three-dimensional Resonant Magnetization Dynamics Unraveled by Time-Resolved Soft X-ray Laminography

The imaging of magneto-dynamical processes has been, so far, mostly a two-dimensional business, due to the constraints of the available experimental techniques. In this manuscript, building on the recent developments of soft X-ray magnetic laminography, we present an experimental setup where magneto-dynamical processes can be resolved in all three spatial dimensions and in time, with the possibility to freely tune the frequency of the dynamical process. We then employ this setup to investigate the three-dimensional dynamics of two resonant magneto-dynamical modes in a CoFeB microstructure occurring at different frequencies, namely the fundamental vortex gyration mode and a magnetic field-induced domain wall excitation mode. This new technique provides much needed capabilities for the experimental investigation of the magnetization dynamics of three-dimensional magnetic systems.

cond-mat.mes-hall↗

arXiv2021

Skyrmions in synthetic antiferromagnets and their nucleation via electrical current and ultrafast laser illumination

Magnetic skyrmions are topological spin textures that hold great promise as nanoscale information carriers in non-volatile memory and logic devices. While room-temperature magnetic skyrmions and their current-induced manipulation were recently demonstrated, the stray field resulting from their finite magnetization as well as their topological charge limit their minimum size and reliable motion in tracks. Antiferromagnetic (AF) skyrmions allow these limitations to be lifted owing to their vanishing magnetization and net zero topological charge, promising room-temperature, ultrasmall skyrmions, fast dynamics, and insensitivity to external magnetic fields. While room-temperature AF spin textures have been recently demonstrated, the observation and controlled nucleation of AF skyrmions operable at room temperature in industry-compatible synthetic antiferromagnetic (SAF) material systems is still lacking. Here we demonstrate that isolated skyrmions can be stabilized at zero field and room temperature in a fully compensated SAF. Using X-ray microscopy techniques, we are able to observe the skyrmions in the different SAF layers and demonstrate their antiparallel alignment. The results are substantiated by micromagnetic simulations and analytical models using experimental parameters, which confirm the chiral SAF skyrmion spin texture and allow the identification of the physical mechanisms that control the SAF skyrmion size and stability. We also demonstrate the local nucleation of SAF skyrmions via local current injection as well as ultrafast laser excitations at zero field. These results will enable the utilization of SAF skyrmions in skyrmion-based devices.

cond-mat.mtrl-sci↗

arXiv2021

Symmetry- and curvature effects on spin waves in vortex-state hexagonal nanotubes

Analytic and numerical studies on curved magnetic nano-objects predict numerous exciting effects that can be referred to as magneto-chiral effects, which do not originate from intrinsic Dzyaloshinskii-Moriya interaction or interface-induced anisotropies. In constrast, these chiral effects stem from isotropic exchange or dipole-dipole interaction, present in all magnetic materials, which acquire asymmetric contributions in case of curved geometry of the specimen. As a result, for example, the spin-wave dispersion in round magnetic nanotubes becomes asymmetric, namely spin waves of the same frequency propagating in opposite directions along the nanotube exhibit different wavelenghts. Here, using time-resolved scanning transmission X-ray microscopy experiments, standard micromagntic simulations and a dynamic-matrix approach, we show that the spin-wave spectrum undergoes additional drastic changes when transitioning from a continuous to a discrete rotational symmetry, i.e. from round to hexagonal nanotubes, which are much easier to fabricate. The polygonal shape introduces localization of the modes both to the sharp, highly curved corners and flat edges. Moreover, due to the discrete rotational symmetry, the degenerate nature of the modes with azimuthal wave vectors known from round tubes is partly lifted, resulting in singlet and duplet modes. For comparison with our experiments, we calculate the microwave absorption from the numerically obtained mode profiles which shows that a dedicated antenna design is paramount for magnonic applications in 3D nano-structures. To our knowledge these are the first experiments directly showing real space spin-wave propagation in 3D nano objects.

cond-mat.mes-hall↗

arXiv2021

Direct X-ray detection of the spin Hall effect in CuBi

The spin Hall effect and its inverse are important spin-charge conversion mechanisms. The direct spin Hall effect induces a surface spin accumulation from a transverse charge current due to spin orbit coupling even in non-magnetic conductors. However, most detection schemes involve additional interfaces, leading to large scattering in reported data. Here we perform interface free x-ray spectroscopy measurements at the Cu L_{3,2} absorption edges of highly Bi-doped Cu (Cu_{95}Bi_{5}). The detected X-ray magnetic circular dichroism (XMCD) signal corresponds to an induced magnetic moment of (2.7 +/- 0.5) x 10-12 μ_{B} A^{-1} cm^{2} per Cu atom averaged over the probing depth, which is of the same order as for Pt measured by magneto-optics. The results highlight the importance of interface free measurements to assess material parameters and the potential of CuBi for spin-charge conversion applications.

cond-mat.mtrl-sci↗

arXiv2021

Field- and current-driven magnetic domain-wall inverter and diode

We investigate the inversion process of magnetic domain walls (DWs) propagating through synthetic noncollinear magnetic textures, whereby an up/down DW can be transformed into a down/up DW and vice versa. We exploit the lateral coupling between out-of-plane and in-plane magnetic regions induced by the interfacial Dzyaloshinskii-Moriya interaction in Pt/Co/AlOx trilayers to realize both field-driven and current-driven magnetic DW inverters. The inverters consist of narrow in-plane magnetic regions embedded in out-of-plane DW racetracks. Magnetic imaging and micromagnetic simulations provide insight into the DW inversion mechanism, showing that DW inversion proceeds by annihilation of the incoming domain on one side of the in-plane region and nucleation of a reverse domain on the opposite side. By changing the shape of the in-plane magnetic region, we show that the DW inversion efficiency can be tuned by adjusting the ratio between the chiral coupling energy at the inverter boundary and the energy cost of nucleating a reverse domain. Finally, we realize an asymmetric DW inverter that has nonreciprocal inversion properties and demonstrate that such a device can operate as a DW diode. Our results provide input for the versatile manipulation of DWs in magnetic racetracks and the design of efficient DW devices for nonvolatile magnetic logic schemes.

cond-mat.mes-hall↗

arXiv2020

Experimental observation of the curvature-induced asymmetric spin-wave dispersion in hexagonal nanotubes

Theoretical and numerical studies on curved magnetic nano-objects predict numerous exciting effects that can be referred to as magneto-chiral effects, which do not originate from the intrinsic Dzyaloshinskii-Moriya interaction or surface-induced anisotropies. The origin of these chiral effects is the isotropic exchange or the dipole-dipole interaction present in all magnetic materials but renormalized by the curvature. Here, we demonstrate experimentally that curvature induced effects originating from the dipole-dipole interaction are directly observable by measuring spin-wave propagation in magnetic nanotubes with hexagonal cross section using time resolved scanning transmission X-ray microscopy. We show that the dispersion relation is asymmetric upon reversal of the wave vector when the propagation direction is perpendicular to the static magnetization. Therefore counter-propagating spin waves of the same frequency exhibit different wavelenghts. Hexagonal nanotubes have a complex dispersion, resulting from spin-wave modes localised to the flat facets or to the extremely curved regions between the facets. The dispersion relations obtained experimentally and from micromagnetic simulations are in good agreement. %The asymmetric spin-wave transport is present for all modes, promoting hexagonal nanotubes for magnonic applications. These results show that spin-wave transport is possible in 3D, and that the dipole-dipole induced magneto-chiral effects are significant.

cond-mat.mes-hall↗

arXiv2020

Néel-type skyrmions and their current-induced motion in van der Waals ferromagnet-based heterostructures

Since the discovery of ferromagnetic two-dimensional (2D) van der Waals (vdW) crystals, significant interest on such 2D magnets has emerged, inspired by their appealing properties and integration with other 2D family for unique heterostructures. In known 2D magnets, spin-orbit coupling (SOC) stabilizes perpendicular magnetic anisotropy (PMA). Such a strong SOC could also lift the chiral degeneracy, leading to the formation of topological magnetic textures such as skyrmions through the Dzyaloshinskii-Moriya interaction (DMI). Here, we report the experimental observation of Néel-type chiral magnetic skyrmions and their lattice (SkX) formation in a vdW ferromagnet Fe3GeTe2 (FGT). We demonstrate the ability to drive individual skyrmion by short current pulses along a vdW heterostructure, FGT/h-BN, as highly required for any skyrmion-based spintronic device. Using first principle calculations supported by experiments, we unveil the origin of DMI being the interfaces with oxides, which then allows us to engineer vdW heterostructures for desired chiral states. Our finding opens the door to topological spin textures in the 2D vdW magnet and their potential device application.

cond-mat.mtrl-sci↗

arXiv2020

Imaging three-dimensional nanoscale magnetization dynamics

The ability to experimentally map the three-dimensional structure and dynamics in bulk and patterned three-dimensional ferromagnets is essential both for understanding fundamental micromagnetic processes, as well as for investigating technologically-relevant micromagnets whose functions are connected to the presence and dynamics of fundamental micromagnetic structures, such as domain walls and vortices. Here, we demonstrate time-resolved magnetic laminography, a technique which offers access to the temporal evolution of a complex three-dimensional magnetic structure with nanoscale resolution. We image the dynamics of the complex three-dimensional magnetization state in a two-phase bulk magnet with a lateral spatial resolution of 50 nm, mapping the transition between domain wall precession and the dynamics of a uniform magnetic domain that is attributed to variations in the magnetization state across the phase boundary. The capability to probe three-dimensional magnetic structures with temporal resolution paves the way for the experimental investigation of novel functionalities arising from dynamic phenomena in bulk and three-dimensional patterned nanomagnets.

cond-mat.mes-hall↗

arXiv2019

Magnetic skyrmion artificial synapse for neuromorphic computing

Since the experimental discovery of magnetic skyrmions achieved one decade ago, there have been significant efforts to bring the virtual particles into all-electrical fully functional devices, inspired by their fascinating physical and topological properties suitable for future low-power electronics. Here, we experimentally demonstrate such a device: electrically-operating skyrmion-based artificial synaptic device designed for neuromorphic computing. We present that controlled current-induced creation, motion, detection and deletion of skyrmions in ferrimagnetic multilayers can be harnessed in a single device at room temperature to imitate the behaviors of biological synapses. Using simulations, we demonstrate that such skyrmion-based synapses could be used to perform neuromorphic pattern-recognition computing using handwritten recognition data set, reaching to the accuracy of ~89 percents, comparable to the software-based training accuracy of ~94 percents. Chip-level simulation then highlights the potential of skyrmion synapse compared to existing technologies. Our findings experimentally illustrate the basic concepts of skyrmion-based fully functional electronic devices while providing a new building block in the emerging field of spintronics-based bio-inspired computing.

physics.app-ph↗

arXiv2019

Nonreciprocal nano-optics with spin-waves in synthetic antiferromagnets

Integrated optically-inspired wave-based processing is envisioned to outperform digital architectures in specific tasks, such as image processing and speech recognition. In this view, spin-waves represent a promising route due to their nanoscale wavelength in the GHz frequency range and rich phenomenology. Here, we realize a versatile optically-inspired platform using spin-waves, demonstrating the wavefront engineering, focusing, and robust interference of spin-waves with nanoscale wavelength. In particular, we use magnonic nanoantennas based on tailored spin-textures for launching spatially shaped coherent wavefronts, diffraction-limited spin-wave beams, and generating robust multi-beam interference patterns, which spatially extend for several times the spin-wave wavelength. Furthermore, we show that intriguing features, such as resilience to back-reflection, naturally arise from the spin-wave nonreciprocity in synthetic antiferromagnets, preserving the high quality of the interference patterns from spurious counterpropagating modes. This work represents a fundamental step towards the realization of nanoscale optically-inspired devices based on spin-waves.

cond-mat.mes-hall↗