arXiv subjects

Simone L. Portalupi

Publications and source records attributed to Simone L. Portalupi.

17 recordsLinked to original sources

arXiv2026

Planar metal-semiconductor Yagi-Uda type antennas for tunable narrow-linewidth quantum dot emitters

Tunable photonic architectures that improve the extraction efficiency of light from embedded epitaxial quantum dots across a wide spectral range are key enablers for developing bright sources of single and indistinguishable photons. In this study, we experimentally demonstrate planar multilayer antenna structures consisting of epitaxially grown AlGaAs and InGaAs membranes containing quantum dots sandwiched between metallic Au (or Ag) reflector and director layers together with Al$_2$O$_3$ spacer layers. We show that the linewidths and fine-structure splitting of the neutral exciton emission remain comparable to those measured in the corresponding unprocessed samples, demonstrating that the fabrication process preserves the optical quality of the emitters. In addition to broadband operation, we demonstrate that the planar architecture is compatible with electrical tuning via integrated diode structures, and strain tuning using piezoelectric actuators. In spite of limitations related to optical losses in the ultrathin metallic layers, the demonstrated fabrication simplicity, scalability, and compatibility with tunable quantum emitters establish planar antennas as a promising platform for solid-state quantum photonic devices.

physics.optics↗

arXiv2025

Asymmetric two-photon response of an incoherently driven quantum emitter

Quantum emitters promise to emit exactly one photon with high probability when pumped by a laser pulse. However, even in ideal systems, re-excitation during a laser pulse causes the consecutive emission of two photons, thus limiting the single-photon purity. Although the probability and properties of re-excitation are largely determined by the optical excitation method, until now only resonant driving has been studied. Here, we demonstrate qualitative differences in the process arising from phonon-assisted excitation -- a scheme standing out for its robustness and straightforward spectral suppression of scattered laser light while preserving highly indistinguishable emission. In contrast to previous studies under resonant driving, we measure not only the $g^{(2)}(0)$ as a function of pulse length but also resolve the distinct temporal and spectral shape of each of the photons, report an asymmetric two-photon spectrum and uncover correlations between the emission time and wavelength, which are unique to phonon-assisted pumping. On the fundamental side, we show how the spectrum stemming from re-excitation provides direct access to the Rabi frequency of an incoherently driven quantum dot. On the application side, we use the asymmetric spectral response to selectively suppress multiphoton noise from re-excitation, ensuring a high-single photon purity regardless of the laser pulse length and thus enhancing implementations across quantum cryptography and quantum computing.

quant-ph↗

arXiv2025

Initialization of Neutral and Charged Exciton Spin States in a Telecom-Emitting Quantum Dot

Photonic cluster states are highly entangled states that allow for photonic quantum computing and memory-less quantum repeaters. Their generation has been recently demonstrated using semiconductor quantum dots emitting at the 900 nm wavelength range. However, a similar demonstration at the communication-optimal telecom range has remained elusive. A key ingredient that is still missing is an appropriate optical excitation method. A central requirement of such a method is to allow an arbitrary spin initialization of quantum dot excitonic complexes. In this work, we report on developing such a method based on a quasi-resonant p-shell excitation for a telecom-C-band-emitting quantum dot. We show qubit writing of a neutral exciton and spin-preserving excitation of a negative trion. Using the Larmor precession of the negative trion under an externally applied magnetic field, we determine the in-plane g-factors of both the electron and the hole in the investigated quantum dot. In addition, we measure a lower bound on the hole coherence time, $T_{2}^{*}>6.4$ ns, boosting its candidacy as a sound photon entangler for more advanced quantum photonic schemes.

quant-ph↗

arXiv2024

Telecom wavelength quantum dots interfaced with silicon-nitride circuits via photonic wire bonding

Photonic integrated circuits find ubiquitous use in various technologies, from communication, to computing and sensing, and therefore play a crucial role in the quantum technology counterparts. Several systems are currently under investigation, each showing distinct advantages and drawbacks. For this reason, efforts are made to effectively combine different platforms in order to benefit from their respective strengths. In this work, 3D laser written photonic wire bonds are employed to interface triggered sources of quantum light, based on semiconductor quantum dots embedded into etched microlenses, with low-loss silicon-nitride photonics. Single photons at telecom wavelengths are generated by the In(Ga)As quantum dots which are then funneled into a silicon-nitride chip containing single-mode waveguides and beamsplitters. The second-order correlation function of g(2)(0) = 0.11+/-0.02, measured via the on-chip beamsplitter, clearly demonstrates the transfer of single photons into the silicon-nitride platform. The photonic wire bonds funnel on average 28.6+/-8.8% of the bare microlens emission (NA = 0.6) into the silicon-nitride-based photonic integrated circuit even at cryogenic temperatures. This opens the route for the effective future up-scaling of circuitry complexity based on the use of multiple different platforms.

physics.optics↗

arXiv2024

Investigation of Purcell enhancement of quantum dots emitting in the telecom O-band with an open fiber-cavity

Single-photon emitters integrated in optical micro-cavities are key elements in quantum communication applications. However, optimizing their emission properties and achieving efficient cavity coupling remain significant challenges. In this study, we investigate semiconductor quantum dots (QDs) emitting in the telecom O-band and integrate them in an open fiber-cavity. Such cavities offer spatial and spectral tunability and intrinsic fiber-coupling. The design promises high collection efficiency and enables the investigation of multiple emitters in heterogeneous samples. We observe a reduction of the decay times of several individual emitters by up to a factor of $2.46(2)$ due to the Purcell effect. We comprehensively analyze the current limitations of the system, including cavity and emitter properties, the impact of the observed regime where cavity and emitter linewidths are comparable, as well as the mechanical fluctuations of the cavity length. The results elucidate the path towards efficient telecom quantum light sources.

quant-ph↗

arXiv2024

High fidelity distribution of triggered polarization-entangled telecom photons via a 36km intra-city fiber network

Fiber-based distribution of triggered, entangled, single-photon pairs is a key requirement for the future development of terrestrial quantum networks. In this context, semiconductor quantum dots (QDs) are promising candidates for deterministic sources of on-demand polarization-entangled photon pairs. So far, the best QD polarization-entangled-pair sources emit in the near-infrared wavelength regime, where the transmission distance in deployed fibers is limited. Here, to be compatible with existing fiber network infrastructures, bi-directional polarization-conserving quantum frequency conversion (QFC) is employed to convert the QD emission from \unit[780]{nm} to telecom wavelengths. We show the preservation of polarization entanglement after QFC (fidelity to Bell state $F_{ϕ^+, conv}=0.972\pm0.003$) of the biexciton transition. As a step towards real-world applicability, high entanglement fidelities ($F_{ϕ^+, loop}=0.945\pm0.005$) after the propagation of one photon of the entangled pair along a \unit[35.8]{km} field installed standard single mode fiber link are reported. Furthermore, we successfully demonstrate a second polarization-conversing QFC step back to \unit[780]{nm} preserving entanglement ($F_{ϕ^+, back}=0.903\pm0.005$). This further prepares the way for interfacing quantum light to various quantum memories.

quant-ph↗

arXiv2023

Robust excitation of C-band quantum dots for quantum communication

Building a quantum internet requires efficient and reliable quantum hardware, from photonic sources to quantum repeaters and detectors, ideally operating at telecommunication wavelengths. Thanks to their high brightness and single-photon purity, quantum dot (QD) sources hold the promise to achieve high communication rates for quantum-secured network applications. Furthermore, it was recently shown that excitation schemes, such as longitudinal acoustic phonon-assisted (LA) pumping, provide security benefits by scrambling the coherence between the emitted photon-number states. In this work, we investigate further advantages of LA-pumped quantum dots with emission in the telecom C-band as a core hardware component of the quantum internet. We experimentally demonstrate how varying the pump energy and spectral detuning with respect to the excitonic transition can improve quantum-secured communication rates and provide stable emission statistics regardless of network-environment fluctuations. These findings have significant implications for general implementations of QD single-photon sources in practical quantum communication networks.

quant-ph↗

arXiv2023

Triggered telecom C-band single-photon source with high brightness, high indistinguishability and sub-GHz spectral linewidth

Long-range, terrestrial quantum networks will require high brightness single-photon sources emitting in the telecom C-band for maximum transmission rate. Many applications additionally demand triggered operation with high indistinguishability and narrow spectral linewidth. This would enable the efficient implementation of photonic gate operations and photon storage in quantum memories, as for instance required for a quantum repeater. Especially, semiconductor quantum dots (QDs) have shown these properties in the near-infrared regime. However, the simultaneous demonstration of all these properties in the telecom C-band has been elusive. Here, we present a coherently (incoherently) optically-pumped narrow-band (0.8 GHz) triggered single-photon source in the telecom C-band. The source shows simultaneously high single-photon purity with $g^{(2)}(0) = 0.026$ ($g^{(2)}(0) = 0.014$), high two-photon interference visibility of 0.508 (0.664) and high application-ready rates of 0.75 MHz (1.45 MHz) of polarized photons. The source is based on a QD coupled to a circular Bragg grating cavity combined with spectral filtering. Coherent (incoherent) operation is performed via the novel SUPER scheme (phonon-assisted excitation).

quant-ph↗

arXiv2023

Highly indistinguishable single photons from droplet-etched GaAs quantum dots integrated in single-mode waveguides and beamsplitters

The integration of on-demand quantum emitters into photonic integrated circuits (PICs) has drawn much of attention in recent years, as it promises a scalable implementation of quantum information schemes. A central property for several applications is the indistinguishability of the emitted photons. In this regard, GaAs quantum dots (QDs) obtained by droplet etching epitaxy show excellent performances with visibilities close to one for both individual and remote emitters. Therefore, the realization of these QDs into PICs is highly appealing. Here, we show the first implementation in this direction, realizing the key passive elements needed in PICs, i.e. single-mode waveguides (WGs) with integrated GaAs-QDs, which can be coherently controlled, as well as beamsplitters. We study both the statistical distribution of wavelength, linewidth and decay times of the excitonic line of multiple QDs, as well as the quantum optical properties of individual emitters under resonant excitation. Here, we achieve single-photon purities as high as $1-\text{g}^{(2)}(0)=0.929\pm0.009$ as well as two-photon interference visibilities of up to V$_{\text{TPI}}=0.939\pm0.004$ for two consecutively emitted photons.

quant-ph↗

arXiv2021

Optical Charge Injection and Full Coherent Control of Spin-Qubit in the Telecom C-band Emitting Quantum Dot

Solid-state quantum emitters with manipulable spin-qubits are promising platforms for quantum communication applications. Although such light-matter interfaces could be realized in many systems only a few allow for light emission in the telecom bands necessary for long-distance quantum networks. Here, we propose and implement a new optically active solid-state spin-qubit based on a hole confined in a single InAs/GaAs quantum dot grown on an InGaAs metamorphic buffer layer emitting photons in the C-band. We lift the hole spin-degeneracy using an external magnetic field and demonstrate hole injection, initialization, read-out and complete coherent control using picosecond optical pulses. These results showcase a new solid-state spin-qubit platform compatible with preexisting optical fibre networks.

cond-mat.mes-hall↗

arXiv2021

Bright Purcell enhanced single-photon source in the telecom O-band based on a quantum dot in a circular Bragg grating

The combination of semiconductor quantum dots (QDs) with photonic cavities is a promising way to realize non-classical light sources with state-of-the-art performances in terms of brightness, indistinguishability and repetition rate. In the present work we demonstrate the coupling of an InGaAs/GaAs QDs emitting in the telecom O-band to a circular Bragg grating cavity. We demonstrate a broadband geometric extraction efficiency enhancement by investigating two emission lines under above-band excitation, inside and detuned from the cavity mode, respectively. In the first case, a Purcell enhancement of 4 is attained. For the latter case, an end-to-end brightness of 1.4% with a brightness at the first lens of 23% is achieved. Using p-shell pumping, a combination of high count rate with pure single-photon emission (g(2)(0) = 0.01 in saturation) is achieved. Finally a good single-photon purity (g(2)(0) = 0.13) together with a high detector count rate of 191kcps is demonstrated for a temperature of up to 77K.

physics.optics↗

arXiv2020

Delaying two-photon Fock-states in a hot cesium vapor using on-demand generated single-photons from a semiconductor quantum dot

Single photons from solid-state quantum emitters are playing a crucial role in the development of photonic quantum technologies. Higher order states, such as N-photon Fock-states allow for applications e.g. in quantum-enhanced sensing. In this study, we utilize the dispersion of a hot cesium vapor at the D1 lines to realize a temporal delay for one and two-photon Fock-states as a result of the slow-light effect. Single photons are generated on-demand from an InGaAs quantum dot, while their quantum interference at a beam splitter is used to generate a two-photon Fockstate. We verify the successful propagation and temporal delay of both the one and two-photon Fock-states, while a significant delay (5x initial photon length) with simultaneous high transmission (~90 %) is achieved.

quant-ph↗

arXiv2019

Highly indistinguishable single photons from incoherently and coherently excited GaAs quantum dots

Semiconductor quantum dots are converging towards the demanding requirements of photonic quantum technologies. Among different systems, quantum dots with dimensions exceeding the free-exciton Bohr radius are appealing because of their high oscillator strengths. While this property has received much attention in the context of cavity quantum electrodynamics, little is known about the degree of indistinguishability of single photons consecutively emitted by such dots and on the proper excitation schemes to achieve high indistinguishability. A prominent example is represented by GaAs quantum dots obtained by local droplet etching, which recently outperformed other systems as triggered sources of entangled photon pairs. On these dots, we compare different single-photon excitation mechanisms, and we find (i) a "phonon bottleneck" and poor indistinguishability for conventional excitation via excited states and (ii) photon indistinguishablilities above 90% for both strictly resonant and for incoherent acoustic- and optical-phonon-assisted excitation. Among the excitation schemes, optical phonon-assisted excitation enables straightforward laser rejection without a compromise on the source brightness together with a high photon indistinguishability.

cond-mat.mes-hall↗

arXiv2018

Fully on-chip single-photon Hanbury-Brown and Twiss experiment on a monolithic semiconductor-superconductor platform

Photonic quantum technologies such as quantum cryptography, photonic quantum metrology, photonic quantum simulators and computers will largely benefit from highly scalable and small footprint quantum photonic circuits. To perform fully on-chip quantum photonic operations, three basic building blocks are required: single-photon sources, photonic circuits and single-photon detectors. Highly integrated quantum photonic chips on silicon and related platforms have been demonstrated incorporating only one or two of these basic building blocks. Previous implementations of all three components were mainly limited by laser stray light, making temporal filtering necessary or required complex manipulation to transfer all components onto one chip. So far, a monolithic, simultaneous implementation of all elements demonstrating single-photon operation remains elusive. Here, we present a fully-integrated Hanbury-Brown and Twiss setup on a micron-sized footprint, consisting of a GaAs waveguide embedding quantum dots as single-photon sources, a waveguide beamsplitter and two superconducting nanowire single-photon detectors. This enables a second-order correlation measurement at the single-photon level under both continuous-wave and pulsed resonant excitation.

physics.app-ph↗

arXiv2018

Two-photon interference in the telecom C-band after frequency conversion of photons from remote quantum emitters

Efficient fiber-based long-distance quantum communication via quantum repeaters relies on deterministic single-photon sources at telecom wavelengths, with the potential to exploit the existing world-wide infrastructures. For upscaling the experimental complexity in quantum networking, two-photon interference (TPI) of remote non-classical emitters in the low-loss telecom bands is of utmost importance. With respect to TPI of distinct emitters, several experiments have been conducted, e.g., using trapped atoms [Beugnon2006], ions [Maunz2007], NV-centers [Bernien2012, Sipahigil2012], SiV-centers [Sipahigil2014], organic molecules [Lettow2010] and semiconductor quantum dots (QDs) [Patel2010, Flagg2010, He2013b, Gold2014, Giesz2015, Thoma2017, Reindl2017, Zopf2017]; however, the spectral range was far from the highly desirable telecom C-band. Here, we report on TPI at 1550 nm between down-converted single photons from remote QDs [Michler2017Book], demonstrating quantum frequency conversion [Zaske2012, Ates2012, Kambs2016] as precise and stable mechanism to erase the frequency difference between independent emitters. On resonance, a TPI-visibility of (29+-3)% has been observed, being only limited by spectral diffusion processes of the individual QDs [Robinson2000, Kuhlmann2015]. Up to 2-km of additional fiber channel has been introduced in both or individual signal paths with no influence on TPI-visibility, proving negligible photon wave-packet distortion. The present experiment is conducted within a local fiber network covering several rooms between two floors of the building. Our studies pave the way to establish long-distance entanglement distribution between remote solid-state emitters including interfaces with various quantum hybrid systems [DeGreve2012,Maring2017,Bock2017,Maring2018].

quant-ph↗

arXiv2018

Overcoming correlation fluctuations in two-photon interference experiments with differently bright and independently blinking remote quantum emitters

As a fundamental building block for quantum computation and communication protocols, the correct verification of the two-photon interference (TPI) contrast between two independent quantum light sources is of utmost importance. Here, we experimentally demonstrate how frequently present blinking dynamics and changes in emitter brightness critically affect the Hong-Ou-Mandel-type (HOM) correlation histograms of remote TPI experiments measured via the commonly utilized setup configuration. We further exploit this qualitative and quantitative explanation of the observed correlation dynamics to establish an alternative interferometer configuration, which is overcoming the discussed temporal fluctuations, giving rise to an error-free determination of the remote TPI visibility. We prove full knowledge of the obtained correlation by reproducing the measured correlation statistics via Monte-Carlo simulations. As exemplary system, we make use of two pairs of remote semiconductor quantum dots, however, the same conclusions apply for TPI experiments with flying qubits from any kind of remote solid state quantum emitters.

cond-mat.mes-hall↗

arXiv2018

Tuning emission energy and fine structure splitting in quantum dots emitting in the telecom O-band

We report on optical investigations of MOVPE-grown InGaAs/GaAs quantum dots emitting at the telecom O-band that were integrated onto uniaxial piezoelectric actuators. This promising technique, which does not degrade the optical quality or performances of the quantum emitters, enables us to tune the quantum dot emission wavelengths and their fine-structure splitting. By spectrally analyzing the emitted light with respect to its polarization, we are able to demonstrate the cancelation of the fine structure splitting within the experimental resolution limit. This work represents an important step towards the high-yield generation of entangled photon pairs at telecommunication wavelength, together with the capability to precisely tune the emission to target wavelengths.

cond-mat.mes-hall↗