arXiv subjects

Siyu Fan

Publications and source records attributed to Siyu Fan.

3 recordsLinked to original sources

arXiv2026

Evidence for Three-component Interlayer Coherent Exciton Condensation

Increasing the number of internal components in a quantum many-body system can host collective orders inaccessible to simpler settings. Quantum Hall bilayers provide a canonical realization of interlayer exciton condensation, yet extending such coherence across three independently addressable electronic fluids has remained elusive. Here we report evidence for three-component interlayer coherent exciton condensation in triple-layer graphene system. Using Rydberg excitons in an adjacent WSe2 monolayer as a layer-sensitive optical probe, we resolve interaction-induced incompressibility at zeroth-Landau-level crossings for all three pairwise layer combinations, establishing top-middle, middle-bottom and top-bottom exciton condensate channels within the same device. Independent control of displacement field and interlayer bias continuously tunes these pairwise states towards a regime where Landau levels from all three layers approach simultaneous degeneracy. At their convergence, incompressibility persists while the exciton energy and spectral weight evolve smoothly between the pairwise limits, suggesting coherent participation of all three layers in a single three-component state. More broadly, the ability to independently control layer potentials and engineer interlayer interactions establishes multilayer graphene as a programmable synthetic dimension for exploring higher-component quantum Hall order and simulating strongly correlated quantum matter.

cond-mat.mes-hall↗

arXiv2026

Supermoir\'e Chern mosaic in helical trilayer WSe2

Helically twisted multilayers offer access to moir\'e physics beyond the single-superlattice paradigm, yet their correlated and topological transport properties remain largely unexplored in semiconductor moir\'e materials. Here we report magnetotransport measurements of helical trilayer WSe2, in which two coupled moir\'e patterns relax into a supermoir\'e landscape composed of inequivalent local topological domains with distinct electronic structures and unequal spatial areas. By electrostatic tuning, we identify a trilayer-hybridized regime where interactions and real-space reconstruction combine to generate a plethora of magnetic and topological states absent in the twisted bilayers. At moir\'e filling factor $\nu$ = -1, we observe a ferromagnetic insulating state that is robust against magnetic field and accompanied by a non-quantized anomalous Hall response ~-4 kOhms. This behaviour is consistent with a time-reversal-symmetry-breaking supermoir\'e Chern mosaic, in which the Hall response arises from the non-cancelling contributions of local domains with opposite Chern character arranged by the relaxed structure. Under strong magnetic fields, a symmetry-broken Chern insulating state (C = 1) emerges near $\nu$ = -2/3, displaying a much larger positive Hall response together with strongly enhanced longitudinal resistance, suggestive of field-reconstructed topological minibands and domain-boundary scattering. These results establish relaxed supermoir\'e semiconductor trilayers as a platform for spatially organized magnetism and topology beyond the bilayer limit.

cond-mat.str-el↗

arXiv2026

Destructive interference of second harmonic generation in AA stacked MoTe$_2$/WSe$_2$

The stacking configuration of two-dimensional materials critically governs their optical and electronic responses. Monolayer transition-metal dichalcogenides (TMDC) lack inversion symmetry and exhibit exciton-enhanced second-harmonic generation (SHG). In TMDC bilayers, 60{\deg} (0{\deg}) stacking is conventionally expected to suppress (enhance) SHG owing to destructive (constructive) interference of the layer-resolved nonlinear polarizations. Here, we report an unconventional destructive SHG interference in nearly 0{\deg}-stacked (AA-stacked) MoTe2/WSe2 heterobilayers using two independent probes: atomic-resolution imaging and stacking-sensitive exciton hybridization measurements. Supported by ab initio GW and Bethe-Salpeter equation calculations, we show that distinct two-photon resonances associated with the WSe2 C exciton and the MoTe2 D exciton generate a nearly $\pi$ phase difference ($\Delta\phi$) in their second-order nonlinear susceptibilities $\chi^{(2)}$, leading to the anomalous destructive interference. We further demonstrate that in small-angle twisted MoTe2/WSe2, the SHG polarization state is governed by the interplay between twist angle $\alpha$ and phase difference $\Delta\phi$, and can be mapped onto trajectories on the Poincar\'e sphere. At excitation energies satisfying $\Delta\phi$ + 3$\alpha$ = 180{\deg}, the SHG output becomes nearly circularly polarized (ellipticity ~ 0.91) and undergoes an abrupt 90{\deg} azimuthal rotation, corresponding to a geometric polarization singularity in the parameter space. Our findings open new routes for exciton-resonance engineered nonlinear photonics and stacking-resolved optical functionality in moir\'e materials.

cond-mat.mes-hall↗