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Sofia Pazzagli

Publications and source records attributed to Sofia Pazzagli.

4 recordsLinked to original sources

AlGaN/AlN heterostructures: an emerging platform for nonlinear integrated photonics

In the rapidly evolving area of integrated photonics, there is a growing need for materials that satisfy the particular requirements of increasingly complex and specialized devices and applications. Present photonic material platforms have made significant progress over the past years; however, each platform still faces specific material and performance challenges. We introduce a novel material for integrated photonics: Aluminum Gallium Nitride (AlGaN) on Aluminum Nitride (AlN) as a platform for developing reconfigurable and nonlinear on-chip optical systems. AlGaN combines compatibility with standard semiconductor fabrication technologies, high electro-optic modulation capabilities, and large nonlinear coefficients while providing a broad and low-loss spectral transmission range, making it a viable material for advanced photonic applications. In this work, we design and grow AlGaN/AlN heterostructures and integrate fundamental photonic building blocks into these chips. In particular, we fabricate edge couplers, low-loss waveguides, directional couplers, and tunable high-quality factor ring resonators to enable nonlinear light-matter interaction and quantum functionality. The comprehensive platform we present in this work paves the way for nonlinear photon-pair generation applications, on-chip nonlinear quantum frequency conversion, and fast electro-optic modulation for switching and routing classical and quantum light fields.

physics.optics

Narrow Line Width Quantum Emitters in an Electron-Beam-Shaped Polymer

Solid-state single photon sources (SPSs) with narrow line width play an important role in many leading quantum technologies. Within the wide range of SPSs studied to date, single fluorescent molecules hosted in organic crystals stand out as bright, photostable SPSs with a lifetime-limited optical resonance at cryogenic temperatures. Furthermore, recent results have demonstrated that photostability and narrow line widths are still observed from single molecules hosted in a nanocrystalline environment, which paves the way for their integration with photonic circuitry. Polymers offer a compatible matrix for embedding nanocrystals and provide a versatile yet low-cost approach for making nanophotonic structures on chip that guide light and enhance coupling to nanoscale emitters. Here, we present a deterministic nanostructuring technique based on electron-beam lithography for shaping polymers with embedded single molecules. Our approach provides a direct means of structuring the nanoscale environment of narrow line width emitters while preserving their emission properties.

physics.app-ph

Quantum optics with single molecules in a three-dimensional polymeric platform

The successful development of future photonic quantum technologies heavily depends on the possibility of realizing robust, reliable and, crucially, scalable nanophotonic devices. In integrated networks, quantum emitters can be deployed as single-photon sources or non-linear optical elements, provided their transition linewidth is broadened only by spontaneous emission. However, conventional fabrication approaches are hardly scalable, typically detrimental for the emitter coherence properties and bear limitations in terms of geometries and materials. Here we introduce an alternative platform, based on molecules embedded in polymeric photonic structures. Three-dimensional patterns are achieved via direct laser writing around selected molecular emitters, which preserve near-Fourier-limited fluorescence. By using an integrated polymeric design, record-high photon fluxes from a single cold molecule are reported. The proposed technology allows to conceive a novel class of quantum devices, including integrated multi-photon interferometers, arrays of indistinguishable single photon sources and hybrid electro-optical nanophotonic devices.

physics.app-ph

Photostable single-photon emission from self-assembled nanocrystals of polycyclic aromatic hydrocarbons

Quantum technologies could largely benefit from the control of quantum emitters in sub-micrometric size crystals. These are naturally prone to the integration in hybrid devices, including heterostructures and complex photonic devices. Currently available quantum emitters sculpted in nanocrystals suffer from spectral instability, preventing their use as single photon sources e.g., for most quantum optics operations. In this work we report on unprecedented performances of single-photon emission from organic nanocrystals (average size of hundreds \SI{}{\nano\meter}), made of anthracene (Ac) and doped with dibenzoterrylene (DBT) molecules. The source has hours-long photostability with respect to frequency and intensity, both at room and at cryogenic temperature. When cooled down to \SI{3}{K}, the 00-zero phonon line shows linewidth values (\SI{50}{MHz}) close to the lifetime-limit. Such optical properties in a nanocrystalline environment make the proposed organic nanocrystals a unique single-photon source for integrated photonic quantum technologies.

physics.app-ph