SearcharxivSearch

arXiv subjects

Sofiane Merkouche

Publications and source records attributed to Sofiane Merkouche.

8 recordsLinked to original sources

Gaussian versus non-Gaussian filtering of phase-insensitive nonclassicality

Measures of quantum properties are essential to understanding the fundamental differences between quantum and classical systems as well as quantifying resources for quantum technologies. Here two broad classes of bosonic phase-space functions, which are filtered versions of the Glauber-Sudarshan $P$ function, are compared with regard to their ability to uncover nonclassical effects of light through their negativities. Gaussian filtering of the $P$ function yields the family of $s$-parametrized quasiprobabilities, while more powerful regularized nonclassicality quasiprobabilities are obtained by non-Gaussian filtering. A method is proposed to directly sample such phase-space functions for the restricted case of phase-independent quantum states from balanced homodyne measurements. This overcomes difficulties of previous approaches that manually append uniformly distributed optical phases to the measured quadrature data. We experimentally demonstrate this technique for heralded single- and two-photon states using balanced homodyne detection with varying efficiency. The $s$-parametrized quasiprobabilities, which can be directly sampled, are non-negative for detection efficiencies below 0.5. By contrast, we show that significant negativities of non-Gaussian filtered quasiprobabilities uncover nonclassical effects even for low efficiencies.

quant-ph

Spectrally-resolved four-photon interference of time-frequency entangled photons

Pairs of photons entangled in their time-frequency degree of freedom are of great interest in quantum optics research and applications, due to their relative ease of generation and their high capacity for encoding information. Here we analyze, both theoretically and experimentally, the behavior of phase-insensitive spectrally-resolved interferences arising from two pairs of time-frequency entangled photons. At its core, this is a multimode entanglement swapping experiment, whereby a spectrally resolved joint measurement on the idler photons from both pairs results in projecting the signal photons onto a Bell state whose form depends on the measurement outcome. Our analysis is a thorough exploration of what can be achieved using time-frequency entanglement and spectrally-resolved Bell-state measurements.

quant-ph

A positive operator-valued measure for two-photon detection via sum-frequency generation

Spontaneous parametric down conversion (PDC), in the perturbative limit, can be considered as a probabilistic splitting of one input photon into two output photons. Conversely, sum-frequency generation (SFG) implements the reverse process of combining two input photons into one. Here we show that a single-photon projective measurement in the temporal-mode basis of the output photon of a two-photon SFG process effects a generalized measurement on the input two-photon state. We describe the positive-operator-valued measure (POVM) associated with such a measurement, and show that its elements are proportional to the two-photon states produced by the time-reversed PDC process. Such a detection acts as a joint measurement on two photons, and is thus an important component of many quantum information processing protocols relying on photonic entanglement. Using the retrodictive approach, we analyze the properties of the two-photon POVM that are relevant for quantum protocols exploiting two-photon states and measurements.

quant-ph

Quantifying the enhancement of two-photon absorption due to spectral-temporal entanglement

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency correlations. We present a quantum-theoretic derivation of entangled TPA (ETPA) and calculate an upper bound on the amount of quantum enhancement that is possible in such systems. The derived bounds indicate that in order to observe ETPA the experiments would need to operate at a combination of significantly higher rates of EPP illumination, molecular concentrations, and conventional TPA cross sections than are achieved in typical experiments.

quant-ph

Heralding multiple photonic pulsed Bell-pairs via frequency-resolved entanglement swapping

Entanglement is a unique property of quantum systems and an essential resource for many quantum technologies. The ability to transfer or swap entanglement between systems is an important protocol in quantum information science. Entanglement between photons forms the basis of distributed quantum networks and the demonstration of photonic entanglement swapping is essential for their realization. Here an experiment demonstrating entanglement swapping from two independent multimode time-frequency entangled sources is presented, resulting in multiple heralded temporal-mode Bell states. Entanglement in the heralded states is verified by measuring conditional anti-correlated joint spectra as well as quantum beating in two-photon interference. Our proof-of-concept experiment is able to distinguish up to five orthogonal Bell pairs within the same setup, limited in principle only by the entanglement of the sources.

quant-ph

Experimental feasibility of molecular two-photon absorption with isolated time-frequency-entangled photon pairs

Entangled photon pairs have been promised to deliver a substantial quantum advantage for two-photon absorption spectroscopy. However, recent work has challenged the previously reported magnitude of quantum enhancement in two-photon absorption. Here, we present an experimental comparison of sum-frequency generation and molecular absorption, each driven by isolated photon pairs. We establish an upper bound on the enhancement for entangled-two-photon absorption in Rhodamine-6G, which lies well below previously reported values.

quant-ph

Two-photon absorption of time-frequency-entangled photon pairs by molecules: the roles of photon-number correlations and spectral correlations

While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in practical quantum-enhanced molecular spectroscopy requires close examination. This paper presents a detailed theoretical study of quantum-enhanced TPA by both photon-number correlations and spectral correlations, including an account of the deleterious effects of dispersion. While such correlations in EPP created by spontaneous parametric down conversion can increase the TPA rate significantly in the regime of extremely low optical flux, we find that for typical molecules in solution this regime corresponds to such low TPA event rates as to be unobservable in practice. Our results support the usefulness of EPP spectroscopy in atomic or other narrow-linewidth systems, while questioning the efficacy of such approaches for broadband systems including molecules in solution.

quant-ph

Two-color Bell states heralded via entanglement swapping

We report on an experiment demonstrating entanglement swapping of time-frequency entangled photons. We perform a frequency-resolved Bell-state measurement on the idler photons from two independent entangled photon pairs, which projects the signal photons onto a two-color Bell state. We verify entanglement in this heralded state using two-photon interference and observing quantum beating without the use of filters, indicating the presence of two-color entanglement. Our method could lend itself to use as a highly-tunable source of frequency-bin entangled single photons.

quant-ph