arXiv subjects

Soham Pal

Publications and source records attributed to Soham Pal.

At least 19 recordsLinked to original sources

arXiv2026

Ancilla mediated steady-state engineering in open quantum systems

Engineering the properties of a reservoir and its coupling to a quantum system is a powerful tool for simulating quantum thermodynamic processes and for generating otherwise inaccessible steady states. Yet tailoring both the reservoir and its coupling within a single platform remains challenging. Here we introduce a platform, in which an ancilla qubit mediates the coupling of a target system to a reservoir, providing independent control over the interaction form, coupling strength, and effective reservoir temperature. Our implementation uses the electron spin of a single nitrogen-vacancy center in diamond as the ancilla and a proximal $^{13}$C nuclear spin as the target. By alternating engineered unitary interactions with dissipative ancilla resets, we realize dynamics naturally described by a collision model, enabling straight-forward tracking of the work, heat, coherence, and entropy generated at every collision. We experimentally demonstrate conventional thermalization and also realize anti-thermalization: the stabilization of the target system in a temperature opposite to that of its reservoir. Finally, harnessing this steady-state engineering, we utilize the nuclear spin as a quantum battery, achieving a steady-state ergotropy exceeding $70\%$ of the theoretical maximum.

quant-ph↗

arXiv2026

Microkelvin resolution thermometry at the nanometre scale

Accurate temperature readings of transient events at the nanometer scale are challenging due to the low sensitivity of available sensors. Nanodiamonds containing nitrogen-vacancy (NV) centers have been used for nanoscale thermometry in complex environments, including inside living cells. However, their performance has been limited by short coherence times and low photon counts. In this work, we use isotopically-purified dual-NV nanodiamonds and a bespoke quantum sensing chip to showcase an order of magnitude improvement in temperature measurement sensitivity compared with previous reports. We demonstrate robust temperature measurements with an error of 682 $\mu$K, experimental sensitivities below 50 mK/$\surd \text{Hz}$ and a shot-noise limited sensitivity of 9.6 mK/$\surd \text{Hz}$. To confirm the utility of these high-performance nanothermometers, we quantify the temperature change induced by the thermometry measurement itself, specifically the optical excitation laser used to probe the NV spin state. In addition, we observe directly at the nanometre scale the transient heating caused by the exothermic mixing of dimethyl sulfoxide in water. Sub-millikelvin resolution and millikelvin sensitivity thermometry unlock the possibility of monitoring minute thermal fluctuations in living systems and assessing catalyst performance at the nanometre scale.

quant-ph↗

arXiv2025

Robust Spin Polarization by Adiabatic Dynamical Decoupling

High-fidelity multi-qubit initialization is vital for quantum simulation, quantum information processing (QIP), and quantum sensing. In diamond platforms, nuclear spin registers can be initialized through polarization transfer from a nearby electronic spin whose high gyromagnetic ratio enables efficient dynamical nuclear polarization (DNP). These hybrid systems are typically controlled using diabatic spin rotations, which require precise knowledge of all system parameters. Adiabatic DNP protocols on the other hand have less strict requirements and could enable robust and high fidelity spin transfer. However, due to the slow adiabatic sweeps and limited electron spin coherence times, this approach has remained inaccessible. Here, we demonstrate adiabatic pulsed nuclear spin polarization at room temperature in diamond. We achieve enhanced polarization efficiency, a broad resonance window, and improved tolerance to hyperfine coupling uncertainties relative to conventional diabatic pulsed protocols. We also show how this approach can benefit the initialization of spin clusters. These results set the scene for enhanced qubit initialization in solid state through adiabatic pulsed driving, with applications in solid-state quantum sensor and quantum memory technologies.

quant-ph↗

arXiv2024

Q-BiC: A biocompatible integrated chip for in vitro and in vivo spin-based quantum sensing

Optically addressable spin-based quantum sensors enable nanoscale measurements of temperature, magnetic field, pH, and other physical properties of a system. Advancing the sensors beyond proof-of-principle demonstrations in living cells and multicellular organisms towards reliable, damage-free quantum sensing poses three distinct technical challenges. First, spin-based quantum sensing requires optical accessibility and microwave delivery. Second, any microelectronics must be biocompatible and designed for imaging living specimens. Third, efficient microwave delivery and temperature control are essential to reduce unwanted heating and to maintain an optimal biological environment. Here, we present the Quantum Biosensing Chip (Q-BiC), which facilitates microfluidic-compatible microwave delivery and includes on-chip temperature control. We demonstrate the use of Q-BiC in conjunction with nanodiamonds containing nitrogen vacancy centers to perform optically detected magnetic resonance in living systems. We quantify the biocompatibility of microwave excitation required for optically detected magnetic resonance both in vitro in HeLa cells and in vivo in the nematode Caenorhabditis elegans for temperature measurements and determine the microwave-exposure range allowed before detrimental effects are observed. In addition, we show that nanoscale quantum thermometry can be performed in immobilised but non-anaesthetised adult nematodes with minimal stress. These results enable the use of spin-based quantum sensors without damaging the biological system under study, facilitating the investigation of the local thermodynamic and viscoelastic properties of intracellular processes.

quant-ph↗

arXiv2023

Magnetic moments of $A = 3$ nuclei with chiral effective field theory operators

Chiral effective field theory ($χ$EFT) provides a framework for obtaining internucleon interactions in a systematically improvable fashion from first principles, while also providing for the derivation of consistent electroweak current operators. In this work, we apply consistently derived interactions and currents towards calculating the magnetic dipole moments of the $A=3$ systems Triton and Helium-3. We focus here on LENPIC interactions obtained using semilocal coordinate-space (SCS) regularization. Starting from the momentum-space representation of the LENPIC $χ$EFT vector current, we derive the SCS-regularized magnetic dipole operator up through N2LO. We then carry out no-core shell model calculations for Triton and Helium-3 systems, using the SCS LENPIC interaction at N2LO in $χ$EFT, and evaluate the magnetic dipole moments obtained using the consistently derived one-nucleon and two-nucleon electromagnetic currents. As anticipated by prior results with $χ$EFT currents, the current corrections through N2LO provide improved, but not yet complete, agreement with experiment for the Triton and Helium-3 magnetic dipole moments.

nucl-th↗

arXiv2022

Solving hadron structures using the basis light-front quantization approach on quantum computers

Quantum computing has demonstrated the potential to revolutionize our understanding of nuclear, atomic, and molecular structure by obtaining forefront solutions in non-relativistic quantum many-body theory. In this work, we show that quantum computing can be used to solve for the structure of hadrons, governed by strongly-interacting relativistic quantum field theory. Following our previous work on light unflavored mesons as a relativistic bound-state problem within the nonperturbative Hamiltonian formalism, we present the numerical calculations on simulated quantum devices using the basis light-front quantization (BLFQ) approach. We implement and compare the variational quantum eigensolver (VQE) and the subspace-search variational quantum eigensolver (SSVQE) to find the low-lying mass spectrum of the light meson system and its corresponding light-front wave functions as quantum states from ideal simulators, noisy simulators, and IBM quantum computers. Based on obtained quantum states, we evaluate the meson decay constants and parton distribution functions directly on the quantum circuits. Our calculations on the quantum computers and simulators are in reasonable agreement with accurate numerical solutions solved on classical computers when noises are moderately small, and our overall results are comparable with the available experimental data.

quant-ph↗

arXiv2022

Calculations of $p(n,\gamma )d$ reaction in chiral effective field theory

We present a calculation of the radiative capture cross section $p(n,\gamma )d$ in the low-energy range, where the $M1$ reaction channel dominates. Employing the LENPIC nucleon-nucleon interaction up to the fifth order (N4LO) that is regularized by the semi-local coordinate space regulators, we obtain the initial and final state wave functions, and evaluate the phase shifts of the scattering state and deuteron properties. We derive the transition operator from the chiral effective field theory up to the next-to-next-to leading order (N2LO), where we also regularize the transition operator using regulators consistent with those of the interactions. We compute the capture cross sections and the results show a converging pattern with the chiral-order expansion of the nucleon-nucleon interaction, where the regulator dependence of the results is weak when higher-order nucleon-nucleon interactions are employed. We quantify the uncertainties of the cross-section results due to the chiral-order truncation. The chirally complete and consistent cross-section results are performed up to N2LO and they compare well with the experiments and other theoretical predictions.

nucl-th↗

arXiv2021

Tomographic entanglement indicators from NMR experiments

In recent years, the performance of different entanglement indicators obtained directly from tomograms has been assessed in continuous-variable and hybrid quantum systems. In this paper, we carry out this task in the case of spin systems. We compute the entanglement indicators from actual experimental data obtained from three liquid-state NMR experiments, and compare them with standard entanglement measures calculated from the corresponding density matrices, both experimentally reconstructed and numerically computed. The gross features of entanglement dynamics and spin squeezing properties are found to be reproduced by these entanglement indicators. However, the extent to which these indicators and spin squeezing track the entanglement during time evolution of the multipartite systems in the NMR experiments is very sensitive to the precise nature and strength of interactions as well as the manner in which the full system is partitioned into subsystems. We also use the IBM quantum computer to implement equivalent circuits that capture the dynamics of the multipartite system in one of the NMR experiments. We compute and compare the entanglement indicators obtained from the tomograms corresponding to the experimental execution and simulation of these equivalent circuits. This exercise shows that these indicators can estimate the degree of entanglement without necessitating detailed state reconstruction procedures, establishing the advantage of the tomographic approach.

quant-ph↗

arXiv2021

Stateful Detection of Model Extraction Attacks

Machine-Learning-as-a-Service providers expose machine learning (ML) models through application programming interfaces (APIs) to developers. Recent work has shown that attackers can exploit these APIs to extract good approximations of such ML models, by querying them with samples of their choosing. We propose VarDetect, a stateful monitor that tracks the distribution of queries made by users of such a service, to detect model extraction attacks. Harnessing the latent distributions learned by a modified variational autoencoder, VarDetect robustly separates three types of attacker samples from benign samples, and successfully raises an alarm for each. Further, with VarDetect deployed as an automated defense mechanism, the extracted substitute models are found to exhibit poor performance and transferability, as intended. Finally, we demonstrate that even adaptive attackers with prior knowledge of the deployment of VarDetect, are detected by it.

cs.LG↗

arXiv2021

Experimental localisation of quantum entanglement through monitored classical mediator

Quantum entanglement is a form of correlation between quantum particles that cannot be increased via local operations and classical communication. It has therefore been proposed that an increment of quantum entanglement between probes that are interacting solely via a mediator implies non-classicality of the mediator. Indeed, under certain assumptions regarding the initial state, entanglement gain between the probes indicates quantum coherence in the mediator. Going beyond such assumptions, there exist other initial states which produce entanglement between the probes via only local interactions with a classical mediator. In this process the initial entanglement between any probe and the rest of the system "flows through" the classical mediator and gets localised between the probes. Here we theoretically characterise maximal entanglement gain via classical mediator and experimentally demonstrate, using liquid-state NMR spectroscopy, the optimal growth of quantum correlations between two nuclear spin qubits interacting through a mediator qubit in a classical state. We additionally monitor, i.e., dephase, the mediator in order to emphasise its classical character. Our results indicate the necessity of verifying features of the initial state if entanglement gain between the probes is used as a figure of merit for witnessing non-classical mediator. Such methods were proposed to have exemplary applications in quantum optomechanics, quantum biology and quantum gravity.

quant-ph↗

arXiv2021

Observation of interaction induced blockade and local spin freezing in a NMR quantum simulator

We experimentally emulate interaction induced blockade and local spin freezing in two and three qubit Nuclear Magnetic Resonance (NMR) architecture. These phenomena are identical to the Rydberg blockade and Rydberg biased freezing. In Rydberg blockade, the simultaneous excitation of two or more atoms is blocked due to the level shift induced by the strong Van der Waal's interaction. In such a strong interaction regime, one can also observe Rydberg biased freezing, wherein the dynamics is confined to a subspace, with the help of multiple drives with unequal amplitudes. Here we drive NMR qubits with specific transition-selective radio waves, while intermittently characterizing the quantum states via quantum state tomography. This not only allows us to track the population dynamics, but also helps to probe quantum correlations, by means of quantum discord, evolving under blockade and freezing phenomena. While, our work constitutes the first experimental simulations of these phenomena in the NMR platform, it is also the first experimental demonstration of Rydberg biased freezing. Moreover, these studies open up interesting quantum control perspectives in exploiting the above phenomena for entanglement generation as well as subspace manipulations.

quant-ph↗

arXiv2019

Experimental study of the thermodynamic uncertainty relation

A cost-precision trade-off relationship, the so-called thermodynamic uncertainty relation (TUR), has been recently discovered in stochastic thermodynamics. It bounds certain thermodynamic observables in terms of the associated entropy production. In this work, we experimentally study the TUR in a two-qubit system using an NMR setup. Each qubit is prepared in an equilibrium state, but at different temperatures. The qubits are then coupled, allowing energy exchange (in the form of heat). Using the quantum state tomography technique we obtain the moments of heat exchange within a certain time interval and analyze the relative uncertainty of the energy exchange process. We find that generalized versions of the TUR, which are based on the fluctuation relation, are obeyed. However, the specialized TUR, a tighter bound that is valid under specific dynamics, is violated in certain regimes of operation, in excellent agreement with analytic results. Altogether, this experiment-theory study provides a deep understanding of heat exchange in quantum systems, revealing favorable noise-dissipation regimes of operation.

cond-mat.stat-mech↗

arXiv2019

A framework for the extraction of Deep Neural Networks by leveraging public data

Machine learning models trained on confidential datasets are increasingly being deployed for profit. Machine Learning as a Service (MLaaS) has made such models easily accessible to end-users. Prior work has developed model extraction attacks, in which an adversary extracts an approximation of MLaaS models by making black-box queries to it. However, none of these works is able to satisfy all the three essential criteria for practical model extraction: (1) the ability to work on deep learning models, (2) the non-requirement of domain knowledge and (3) the ability to work with a limited query budget. We design a model extraction framework that makes use of active learning and large public datasets to satisfy them. We demonstrate that it is possible to use this framework to steal deep classifiers trained on a variety of datasets from image and text domains. By querying a model via black-box access for its top prediction, our framework improves performance on an average over a uniform noise baseline by 4.70x for image tasks and 2.11x for text tasks respectively, while using only 30% (30,000 samples) of the public dataset at its disposal.

cs.LG↗

arXiv2018

Experimental verification of quantum heat exchange fluctuation relation

We experimentally verify the Jarzynski and Wöjcik quantum heat exchange fluctuation relation by implementing the interferometric technique in liquid-state Nuclear Magnetic Resonance setup and study the exchange heat statistics between two weakly coupled spin-1/2 quantum systems. In presence of uncorrelated initial state with individual spins prepared in local Gibbs thermal states at different temperatures, the exchange fluctuation symmetry is verified for arbitrary transient time. In contrast, when the initial preparation includes correlation, the fluctuation symmetry breaks down and further leads to an apparent spontaneous flow of heat from cold to hot. Our experimental approach is general and can be systematically extended to study heat statistics for more complex out-of-equilibrium many-body quantum systems.

cond-mat.stat-mech↗

arXiv2018

Effective operators in two-nucleon systems

Effective Hamiltonians and effective electroweak operators are calculated with the Okubo-Lee-Suzuki formalism for two-nucleon systems. Working within a harmonic oscillator basis, first without and then with a confining harmonic oscillator trap, we demonstrate the effects of renormalization on observables calculated for truncated basis spaces. We illustrate the renormalization effects for the root-mean-square point-proton radius, electric quadrupole moment, magnetic dipole moment, Gamow-Teller transition and neutrinoless double-beta decay operator using nucleon-nucleon interactions from chiral Effective Field Theory. Renormalization effects tend to be larger in the weaker traps and smaller basis spaces suggesting applications to heavier nuclei with transitions dominated by weakly-bound nucleons would be subject to more significant renormalization effects within achievable basis spaces.

nucl-th↗

arXiv2018

Temporal order in periodically driven spins in star-shaped clusters

We experimentally study the response of star-shaped clusters of initially unentangled $N=4$, 10 and 37 nuclear spin-$\frac{1}{2}$ moments to an inexact $π$-pulse sequence, and show that an Ising coupling between the centre and the satellite spins results in robust period-two magnetization oscillations. The period is stable against bath-effects but the amplitude decays with a time scale that depends on the inexactness of the pulse. Simulations reveal a semiclassical picture where the rigidity of the period is due to a randomizing effect of the Larmor precession under the magnetization of surrounding spins. The time scales with stable periodicity increase with net initial magnetization even in the presence of perturbations, indicating a robust temporal ordered phase for large systems with finite magnetization per spin.

cond-mat.stat-mech↗

arXiv2018

Ab Initio No Core Shell Model with Leadership-Class Supercomputers

Nuclear structure and reaction theory is undergoing a major renaissance with advances in many-body methods, strong interactions with greatly improved links to Quantum Chromodynamics (QCD), the advent of high performance computing, and improved computational algorithms. Predictive power, with well-quantified uncertainty, is emerging from non-perturbative approaches along with the potential for guiding experiments to new discoveries. We present an overview of some of our recent developments and discuss challenges that lie ahead. Our foci include: (1) strong interactions derived from chiral effective field theory; (2) advances in solving the large sparse matrix eigenvalue problem on leadership-class supercomputers; (3) selected observables in light nuclei with the JISP16 interaction; (4) effective electroweak operators consistent with the Hamiltonian; and, (5) discussion of A=48 system as an opportunity for the no-core approach with the reintroduction of the core.

nucl-th↗

arXiv2016

Hybrid scheme for factorization: Factoring 551 using a 3-qubit NMR quantum adiabatic processor

Quantum processors are potentially superior to their classical counterparts for many computational tasks including factorization. Circuit methods as well as adiabatic methods have already been proposed and implemented for finding the factors of a given composite number. The main challenge in scaling it to larger numbers is the unavailability of large number of qubits. Here we propose a hybrid scheme that involves both classical and quantum computation, which reduces the number of qubits required for factorization. The classical part involves setting up and partially simplifying a set of bit-wise factoring equations and the quantum part involves solving these coupled equations using a quantum adiabatic process. We demonstrate the hybrid scheme by factoring 551 using a three qubit NMR quantum register.

quant-ph↗