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Soong-Geun Je

Publications and source records attributed to Soong-Geun Je.

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Alternative understanding of the skyrmion Hall effect based on one-dimensional domain wall motion

A moving magnetic skyrmion exhibits transverse deflection. This so-called skyrmion Hall effect has been explained by the Thiele equation. Here, we provide an alternative interpretation of the skyrmion Hall effect based on the dynamics of domain walls enclosing the skyrmion. We relate the spin-torque-induced local rotation of the domain wall segments to the shift of the skyrmion core, explaining the skyrmion Hall effect at the micromagnetic level. Bases on our intuitive interpretation, we also show that the skyrmion Hall effect can be suppressed by combining the spin-transfer and spin-orbit torques, whereby removing the major obstacle to utilizing skyrmions in devices.

cond-mat.mes-hall

Targeted Writing and Deleting of Magnetic Skyrmions in Two-Terminal Nanowire Devices

Controllable writing and deleting of nanoscale magnetic skyrmions are key requirements for their use as information carriers for next-generation memory and computing technologies. While several schemes have been proposed, they require complex fabrication techniques or precisely tailored electrical inputs, which limits their long-term scalability. Here we demonstrate an alternative approach for writing and deleting skyrmions using conventional electrical pulses within a simple, two-terminal wire geometry. X-ray microscopy experiments and micromagnetic simulations establish the observed skyrmion creation and annihilation as arising from Joule heating and Oersted field effects of the current pulses, respectively. The unique characteristics of these writing and deleting schemes, such as spatial and temporal selectivity, together with the simplicity of the 2-terminal device architecture, provide a flexible and scalable route to the viable applications of skyrmions.

cond-mat.mtrl-sci

Unveiling the emergent traits of chiral spin textures in magnetic multilayers

Magnetic skyrmions are topologically wound nanoscale textures of spins whose ambient stability and electrical manipulation in multilayer films have led to an explosion of research activities. While past efforts focused predominantly on isolated skyrmions, recently ensembles of chiral spin textures, consisting of skyrmions and magnetic stripes, were shown to possess rich interactions with potential for device applications. However, several fundamental aspects of chiral spin texture phenomenology remain to be elucidated, including their domain wall structure, thermodynamic stability, and morphological transitions. Here we unveil the evolution of these textural characteristics on a tunable multilayer platform - wherein chiral interactions governing spin texture energetics can be widely varied - using a combination of full-field electron and soft X-ray microscopies with numerical simulations. With increasing chiral interactions, we demonstrate the emergence of Néel helicity, followed by a marked reduction in domain compressibility, and finally a transformation in the skyrmion formation mechanism. Together with an analytical model, these experiments establish a comprehensive microscopic framework for investigating and tailoring chiral spin texture character in multilayer films.

cond-mat.mes-hall

Topological charge analysis of dynamic process of transition to Néel-type skyrmion: role of domain wall skyrmions

Magnetic skyrmions are intriguing topological spin textures that promise future high-density spintronic devices. The creation of magnetic skyrmions has been understood based on the energetics of skyrmions, but the detailed dynamic process of the skyrmion creation remains unclear. Here topological evolution in conversion from uneven domains to Néel-skyrmions is investigated using micromagnetic simulations. We find that, rather than the overall topological charge, annihilation of novel topological defects, i.e., recently suggested domain wall skyrmions, dominantly govern the skyrmion creation process. Also, the topological charge evolution is interpreted in terms of the number and the combination of such topological defects.

cond-mat.mes-hall

Direct demonstration of topological stability of magnetic skyrmions via topology manipulation

Topological protection precludes a continuous deformation between topologically inequivalent configurations in a continuum. Motivated by this concept, magnetic skyrmions, topologically nontrivial spin textures, are expected to exhibit the topological stability, thereby offering a prospect as a nanometer-scale non-volatile information carrier. In real materials, however, atomic spins are configured as not continuous but discrete distribution, which raises a fundamental question if the topological stability is indeed preserved for real magnetic skyrmions. Answering this question necessitates a direct comparison between topologically nontrivial and trivial spin textures, but the direct comparison in one sample under the same magnetic fields has been challenging. Here we report how to selectively achieve either a skyrmion state or a topologically trivial bubble state in a single specimen and thereby show how robust the skyrmion structure is in comparison with the bubbles for the first time. We demonstrate that topologically nontrivial magnetic skyrmions show longer lifetimes than trivial bubble structures, evidencing the topological stability in a real discrete system. Our work corroborates the physical importance of the topology in the magnetic materials, which has hitherto been suggested by mathematical arguments, providing an important step towards ever-dense and more-stable magnetic devices.

cond-mat.mtrl-sci

Current-Driven Skyrmion Dynamics and Drive-Dependent Skyrmion Hall Effect in an Ultrathin Film

Magnetic skyrmions are chiral spin textures that hold great promise as nanoscale information carriers. Since their first observation at room temperature, progress has been made in their current-induced manipulation, with fast motion reported in stray-field-coupled multilayers. However, the complex spin textures with hybrid chiralities and large power dissipation in these multilayers limit their practical implementation and the fundamental understanding of their dynamics. Here, we report on the current-driven motion of Néel skyrmions with diameters in the 100-nm range in an ultrathin Pt/Co/MgO trilayer. We find that these skyrmions can be driven at a speed of 100 m/s and exhibit a drive-dependent skyrmion Hall effect, which is accounted for by the effect of pinning. Our experiments are well substantiated by an analytical model of the skyrmion dynamics as well as by micromagnetic simulations including material inhomogeneities. This good agreement is enabled by the simple skyrmion spin structure in our system and a thorough characterization of its static and dynamical properties.

cond-mat.mes-hall

Realization of Ordered Magnetic Skyrmions in Thin Films at Ambient Conditions

Magnetic skyrmions present interesting physics due to their topological nature and hold significant promise for future information technologies. A key barrier to realizing skyrmion devices has been stabilizing these spin structures under ambient conditions. In this manuscript, we exploit the tunable magnetic properties of amorphous Fe/Gd mulitlayers to realize skyrmion lattices which are stable over a large temperature and magnetic field parameter space, including room temperature and zero magnetic field. These hybrid skyrmions have both Bloch-type and Néel-type character and are stabilized by dipolar interactions rather than Dzyaloshinskii-Moriya interactions, which are typically considered required for the generation of skyrmions. Small angle neutron scattering (SANS) was used in combination with soft X-ray microscopy to provide a unique, multi-scale probe of the local and long-range order of these structures. These results identify a pathway to engineer controllable skyrmion phases in thin film geometries which are stable at ambient conditions.

cond-mat.mes-hall

Creation of Magnetic Skyrmion Bubble Lattices by Ultrafast Laser in Ultrathin Films

Magnetic skyrmions are topologically nontrivial spin textures which hold great promise as stable information carriers in spintronic devices at the nanoscale. One of the major challenges for developing novel skyrmion-based memory and logic devices is fast and controlled creation of magnetic skyrmions at ambient conditions. Here we demonstrate the single ultrafast (35-fs) laser pulse-induced generation of skyrmion bubbles and skyrmion bubble lattices from a ferromagnetic state in sputtered ultrathin magnetic films at room temperature. The skyrmion bubble density increases with the laser fluence in a controlled way, and it finally becomes saturated, forming disordered hexagonal lattices. Moreover, we present that the skyrmion bubble lattice configuration leads to enhanced topological stability as compared to isolated skyrmions, suggesting its promising use in data storage. Our findings shed light on the optical approach to the skyrmion bubble lattice in commonly accessible materials, paving the road toward the emerging skyrmion-based memory and synaptic devices.

cond-mat.mtrl-sci

Spin-orbit torque induced dipole skyrmion motion at room temperature

We demonstrate deterministic control of dipole-field-stabilized skyrmions by means of spin-orbit torques arising from heavy transition-metal seed layers. Experiments are performed on amorphous Fe/Gd multilayers that are patterned into wires and exhibit stripe domains and dipole skyrmions at room temperature. We show that while the domain walls and skyrmions are achiral on average due to lack of Dzyaloshinskii-Moriya interactions, the Néel-like closure domain walls at each surface are chiral and can couple to spin-orbit torques. The current-induced domain evolutions are reported for different magnetic phases, including disordered stripe domains, coexisting stripes and dipole skyrmions and a closed packed dipole skyrmion lattice. The magnetic textures exhibit motion under current excitations with a current density ~10^8 A/m2. By comparing the motion resulting from magnetic spin textures in Fe/Gd films with different heavy transition-metal interfaces, we confirm spin currents can be used to manipulate achiral dipole skyrmions via spin-orbit torques.

cond-mat.mtrl-sci

Thermal contribution to the spin-orbit torque in metallic/ferrimagnetic systems

We report a systematic study of current-induced perpendicular magnetization switching in W/Co$_{x}$Tb$_{1-x}$/Al thin films with strong perpendicular magnetic anisotropy. Various Co$_{x}$Tb$_{1-x}$ ferrimagnetic alloys with different magnetic compensation temperatures are presented. The systems are characterized using MOKE, SQUID and anomalous Hall resistance at different cryostat temperature ranging from 10 K to 350 K. The current-switching experiments are performed in the spin-orbit torque geometry where the current pulses are injected in plane and the magnetization reversal is detected by measuring the Hall resistance. The full reversal magnetization has been observed in all samples. Some experimental results could only be explained by the strong sample heating effect during the current pulses injection. We have found that, for a given composition $x$ and switching polarity, the devices always reach the same temperature $\textit{T}_{switch}(x)$ before switching independently of the cryostat temperature. $\textit{T}_{switch}$ seems to scale with the Curie temperature of the Co$_{x}$Tb$_{1-x}$ ferrimagnetic alloys. This explains the evolution of the critical current (and critical current density) as a function of the alloy concentration. Future application could take advantages of this heating effect which allows reducing the in-plane external field. Unexpected double magnetization switching has been observed when the heat generated by the current allows crosses the compensation temperature.

cond-mat.mtrl-sci

Magnetic Domain-Wall Tilting due to Domain-Wall Speed Asymmetry

Chiral magnetic materials provide a number of challenging issues such as the highly efficient domain wall (DW) and skyrmion motions driven by electric current, as of the operation principles of emerging spintronic devices. The DWs in the chiral materials exhibit asymmetric DW speed variation under application of in plane magnetic field. Here, we show that such DW speed asymmetry causes the DW tilting during the motion along wire structure. It has been known that the DW tilting can be induced by the direct Zeeman interaction of the DW magnetization under application of in plane magnetic field. However, our experimental observations manifests that there exists another dominant process with the DW speed asymmetry caused by either the Dzyaloshinskii Moriya interaction (DMI) or the chirality dependent DW speed variation. A theoretical model based on the DW geometry reveals that the DW tilting is initiated by the DW pinning at wire edges and then, the direction of the DW tilting is determined by the DW speed asymmetry, as confirmed by a numerical simulation. The present observation reveals the decisive role of the DW pinning with the DW speed asymmetry, which determines the DW geometry and consequently, the dynamics.

cond-mat.mtrl-sci

Magnetic skyrmions in confined geometries : effect of the magnetic field and the disorder

We report on the effect of the lateral confinement and a perpendicular magnetic field on isolated room-temperature magnetic skyrmions in sputtered Pt/Co/MgO nanotracks and nanodots. We show that the skyrmions size can be easily tuned by playing on the lateral dimensions of the nanostructures and by using external magnetic field amplitudes of a few mT, which allow to reach sub-100 nm diameters. Our XMCD-PEEM observations also highlight the important role of the pinning on the skyrmions size and stability under an out-of-plane magnetic field. Micromagnetic simulations reveal that the effect of local pinning can be well accounted for by considering the thin film grain structure with local anisotropy variations and reproduce well the dependence of the skyrmion diameter on the magnetic field and the geometry.

cond-mat.mes-hall

Chirality-induced Antisymmetry in Magnetic Domain-Wall Speed

In chiral magnetic materials, numerous intriguing phenomena such as built in chiral magnetic domain walls (DWs) and skyrmions are generated by the Dzyaloshinskii Moriya interaction (DMI). The DMI also results in asymmetric DW speed under in plane magnetic field, which provides a useful scheme to measure the DMI strengths. However, recent findings of additional asymmetries such as chiral damping have disenabled unambiguous DMI determination and the underlying mechanism of overall asymmetries becomes under debate. By extracting the DMI-induced symmetric contribution, here we experimentally investigated the nature of the additional asymmetry. The results revealed that the additional asymmetry has a truly antisymmetric nature with the typical behavior governed by the DW chirality. In addition, the antisymmetric contribution changes the DW speed more than 100 times, which cannot be solely explained by the chiral damping scenario. By calibrating such antisymmetric contributions, experimental inaccuracies can be largely removed, enabling again the DMI measurement scheme.

cond-mat.mtrl-sci

Drastic emergence of huge negative spin-transfer torque in atomically thin Co layers

Current-induced domain wall (DW) motion has drawn great attention in the last decades as the key operational principle of emerging magnetic memory devices. As the major driving force of the current-induced DW motion, the spin-orbit torque (SOT) on chiral DWs has been proposed and extensively studied nowadays. However, we demonstrate here that there exists another driving force, which is larger than the SOT in ultra-thin Co films. Moreover, the direction of the present force is found to be opposite to the prediction of the spin-transfer torque (STT), resulting in the DW motion along the current direction. The symmetry of the force and its peculiar dependence on the DW structure suggest that the present force is, most likely, attributed to considerable enhancement of the nonadiabatic STT with a negative spin polarization in atomically thin Co layers. These findings open a new pathway to enhance the overall spin torque efficiency-the critical parameter in emerging spintronic devices.

cond-mat.mtrl-sci

Skyrmion Motion Driven by Oscillating Magnetic Field

Magnetic skyrmion motion induced by an electric current has drawn much interest because of its application potential in next-generation magnetic memory devices. Recently, unidirectional skyrmion motion driven by an oscillating magnetic field was also demonstrated on large (20 micrometer) bubble domains with skyrmion topology. At smaller length scale which is more relevant to high-density memory devices, we here show by numerical simulation that a skyrmion of a few tens of nanometers could also be driven by high-frequency field oscillations but with the motion direction different from the tilted oscillating field direction. We found that high-frequency field for small size skyrmions could excite skyrmion resonant modes and that a combination of different modes would result in the final skyrmion motion with a helical trajectory. Because this helical motion depends on the frequency of the field, we can control both the speed and the direction of the skyrmion motion, which is a distinguishable characteristic compared with other methods.

cond-mat.mtrl-sci

Magnetic Bubblecade Memory

Unidirectional motion of magnetic domain walls is the key concept underlying next-generation domain-wall-mediated memory and logic devices. Such motion has been achieved either by injecting large electric currents into nanowires or by employing domain-wall tension induced by sophisticated structural modulation. Herein, we demonstrate a new scheme without any current injection or structural modulation. This scheme utilizes the recently discovered chiral domain walls, which exhibit asymmetry in their speed with respect to magnetic fields. Because of this asymmetry, an alternating magnetic field results in the coherent motion of the domain walls in one direction. Such coherent unidirectional motion is achieved even for an array of magnetic bubble domains, enabling the design of a new device prototype-magnetic bubblecade memory-with two-dimensional data-storage capability.

cond-mat.mtrl-sci

Asymmetric Magnetic Domain-Wall Motion by the Dzyaloshinskii-Moriya Interaction

We demonstrate here that ultrathin ferromagnetic Pt/Co/Pt films with perpendicular magnetic anisotropy exhibit a sizeable Dzyaloshinskii-Moriya interaction (DMI) effect. Such a DMI effect modifies the domain-wall (DW) energy density and consequently, results in an asymmetric DW expansion driven by an out-of-plane magnetic field under an in-plane magnetic field bias. From an analysis of the asymmetry, the DMI effect is estimated to be strong enough for the DW to remain in the Néel-type configuration in contrast to the general expectations of these materials. Our findings emphasize the critical role of the DMI effect on the DW dynamics as the underlying physics of the asymmetries that are often observed in spin-transfer-related phenomena.

cond-mat.mtrl-sci