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Sophia E. Economou

Publications and source records attributed to Sophia E. Economou.

At least 127 records · Page 7Linked to original sources

Spin Coherence and Echo Modulation of the Silicon Vacancy in 4H-SiC at Room Temperature

The silicon vacancy in silicon carbide is a strong emergent candidate for applications in quantum information processing and sensing. We perform room temperature optically-detected magnetic resonance and spin echo measurements on an ensemble of vacancies and find the properties depend strongly on magnetic field. The spin echo decay time varies from less than 10 $μ$s at low fields to 80 $μ$s at 68 mT, and a strong field-dependent spin echo modulation is also observed. The modulation is attributed to the interaction with nuclear spins and is well-described by a theoretical model.

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Analytical approach to swift nonleaky entangling gates in superconducting qubits

We develop schemes for designing pulses that implement fast and precise entangling quantum gates in superconducting qubit systems despite the presence of nearby harmful transitions. Our approach is based on purposely involving the nearest harmful transition in the quantum evolution instead of trying to avoid it. Using analytical tools, we design simple microwave control fields that implement maximally entangling gates with fidelities exceeding 99% in times as low as 40 ns. We demonstrate our approach in a two-qubit circuit QED system by designing the two most important quantum entangling gates: a conditional-NOT gate and a conditional-Z gate. Our results constitute an important step toward overcoming the problem of spectral crowding, one of the primary challenges in controlling multi-qubit systems.

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Theory of dynamic nuclear polarization and feedback in quantum dots

An electron confined in a quantum dot interacts with its local nuclear spin environment through the hyperfine contact interaction. This interaction combined with external control and relaxation or measurement of the electron spin allows for the generation of dynamic nuclear polarization. The quantum nature of the nuclear bath, along with the interplay of coherent external fields and incoherent dynamics in these systems renders a wealth of intriguing phenomena seen in recent experiments such as electron Zeeman frequency focusing, hysteresis, and line dragging. We develop in detail a fully quantum, self-consistent theory that can be applied to such experiments and that moreover has predictive power. Our theory uses the operator sum representation formalism in order to incorporate the incoherent dynamics caused by the additional, Markovian bath, which in self-assembled dots is the vacuum field responsible for electron-hole optical recombination. The beauty of this formalism is that it reduces the complexity of the problem by encoding the joint dynamics of the external coherent and incoherent driving in an effective dynamical map that only acts on the electron spin subspace. This together with the separation of timescales in the problem allows for a tractable and analytically solvable formalism. The key role of entanglement between the electron spin and the nuclear spins in the formation of dynamic nuclear polarization naturally follows from our solution. We demonstrate the theory in detail for an optical pulsed experiment and present an in-depth discussion and physical explanation of our results.

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Excitation spectrum as a resource for efficient two-qubit entangling gates

Physical systems representing qubits typically have one or more accessible quantum states in addition to the two states that encode the qubit. We demonstrate that active involvement of such auxiliary states can be beneficial in constructing entangling two-qubit operations. We investigate the general case of two multi-state quantum systems coupled via a quantum resonator. The approach is illustrated with the examples of three systems: self-assembled InAs/GaAs quantum dots, NV-centers in diamond, and superconducting transmon qubits. Fidelities of the gate operations are calculated based on numerical simulations of each system.

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Two-qubit quantum gates for defect qubits in diamond and similar systems

We propose a fast, scalable all-optical design for arbitrary two-qubit operations for defect qubits in diamond (NV centers) and in silicon carbide, which are promising candidates for room temperature quantum computing. The interaction between qubits is carried out by microcavity photons. The approach uses constructive interference from higher energy excited states activated by optical control. In this approach the cavity mode remains off-resonance with the directly accessible optical transitions used for initialization and readout. All quantum operations are controlled by near-resonant narrow-bandwidth optical pulses. We perform full quantum numerical modeling of the proposed gates and show that high-fidelity operations can be obtained with realistic parameters.

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Strong Hyperfine-Induced Modulation of an Optically-Driven Hole Spin in an InAs Quantum Dot

Compared to electrons, holes in InAs quantum dots have a significantly weaker hyperfine interaction that leads to less dephasing from nuclear spins. Thus many recent studies have suggested that nuclear spins are unimportant for hole spin dynamics compared to electric field fluctuations. We show that the hole hyperfine interaction can have a strong effect on hole spin coherence measurements through a nuclear feedback effect. The nuclear polarization is generated through a unique process that is dependent on the anisotropy of the hole hyperfine interaction and the coherent precession of nuclear spins, giving rise to strong modulation at the nuclear precession frequency.

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Fast Two-Qubit Gates in Semiconductor Quantum Dots using a Photonic Microcavity

Implementations for quantum computing require fast single- and multi-qubit quantum gate operations. In the case of optically controlled quantum dot qubits theoretical designs for long-range two- or multi-qubit operations satisfying all the requirements in quantum computing are not yet available. We have developed a design for a fast, long-range two-qubit gate mediated by a photonic microcavity mode using excited states of the quantum dot-cavity system that addresses these needs. This design does not require identical qubits, it is compatible with available optically induced single qubit operations, and it advances opportunities for scalable architectures. We show that the gate fidelity can exceed 90% in experimentally accessible systems.

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Quantum control of a spin qubit coupled to a photonic crystal cavity

A key ingredient for a quantum network is an interface between stationary quantum bits and photons, which act as flying qubits for interactions and communication. Photonic crystal architectures are promising platforms for enhancing the coupling of light to solid state qubits. Quantum dots can be integrated into a photonic crystal, with optical transitions coupling to photons and spin states forming a long-lived quantum memory. Many researchers have now succeeded in coupling these emitters to photonic crystal cavities, but there have been no demonstrations of a functional spin qubit and quantum gates in this environment. Here we have developed a coupled cavity-quantum dot system in which the dot is controllably charged with a single electron. We perform the initialization, rotation and measurement of a single electron spin qubit using laser pulses and find that the cavity can significantly improve these processes.

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Scalable qubit architecture based on holes in quantum dot molecules

Spins confined in quantum dots are a leading candidate for solid-state quantum bits that can be coherently controlled by optical pulses. There are, however, many challenges to developing a scalable multibit information processing device based on spins in quantum dots, including the natural inhomogeneous distribution of quantum dot energy levels, the difficulty of creating all-optical spin manipulation protocols compatible with nondestructive readout, and the substantial electron-nuclear hyperfine interaction-induced decoherence. Here, we present a scalable qubit design and device architecture based on the spin states of single holes confined in a quantum dot molecule. The quantum dot molecule qubit enables a new strategy for optical coherent control with dramatically enhanced wavelength tunability. The use of hole spins allows the suppression of decoherence via hyperfine interactions and enables coherent spin rotations using Raman transitions mediated by a hole-spin-mixed optically excited state. Because the spin mixing is present only in the optically excited state, dephasing and decoherence are strongly suppressed in the ground states that define the qubits and nondestructive readout is possible. We present the qubit and device designs and analyze the wavelength tunability and fidelity of gate operations that can be implemented using this strategy. We then present experimental and theoretical progress toward implementing this design.

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High fidelity quantum gates via analytically solvable pulses

It is shown that a family of analytically solvable pulses can be used to obtain high fidelity quantum phase gates with surprising robustness against imperfections in the system or pulse parameters. Phase gates are important because they can implement the necessary operations for universal quantum computing. They are particularly suited for systems such as self-assembled quantum dots, trapped ions, and defects in solids, as these are typically manipulated by the transient excitation of a state outside the qubit subspace.

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Optical control of coherent interactions between quantum dot electron spins

Coherent interactions between spins in quantum dots are a key requirement for quantum gates. We have performed pump-probe experiments in which pulsed lasers emitting at different photon energies manipulate two distinct subsets of electron spins within an inhomogeneous InGaAs quantum dot ensemble. The spin dynamics are monitored through their precession about an external magnetic field. These measurements demonstrate spin precession phase shifts and modulations of the magnitude of one subset of oriented spins after optical orientation of the second subset. The observations are consistent with results from a model using a Heisenberg-like interaction with microeV-strength.

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Electron-nuclear dynamics in a quantum dot under non-unitary electron control

We introduce a method for solving the problem of an externally controlled electron spin in a quantum dot interacting with host nuclei via the hyperfine interaction. Our method accounts for generalized (non-unitary) evolution effected by external controls and the environment, such as coherent lasers combined with spontaneous emission. As a concrete example we develop the microscopic theory of the dynamics of nuclear-induced frequency focusing, as first measured in Science 317, 1896 (2007); we find that the nuclear relaxation rates are several orders of magnitude faster than those quoted in that work.

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Controlling the nuclear polarization in quantum dots using optical pulses with a modest bandwidth

We show that detuned optical pulse trains with a modest spectral width can polarize nuclear spins in InAs quantum dots. The pulse bandwidth is large enough to excite a coherent superposition of both electron spin eigenstates in these negatively charged dots but narrow enough to give partial spectral selectivity between the eigenstates. The coherent precession of electron spin states and periodic excitation focuses the nuclear spin distribution, producing a discrete set of precession modes. The spectral selectivity generates a net nuclear polarization, through a mechanism that relies on optical spin rotations rather than electron spin relaxation.

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Optically generated 2-dimensional photonic cluster state from coupled quantum dots

We propose a method to generate a two-dimensional cluster state of polarization encoded photonic qubits from two coupled quantum dot emitters. We combine the recent proposal [N. H. Lindner and T. Rudolph, Phys. Rev. Lett. 103, 113602 (2009)] for generating 1-dimensional cluster state strings from a single dot, with a new proposal for an optically induced conditional phase (CZ) gate between the two quantum dots. The entanglement between the two quantum dots translates to entanglement between the two photonic cluster state strings. Further inter-pair coupling of the quantum dots using cavities and waveguides can lead to a 2-dimensional cluster sheet. Detailed analysis of errors indicates that our proposal is feasible with current tech- nology. Crucially, the emitted photons need not have identical frequencies, and so there are no constraints on the resonance energies for the quantum dots, a standard problem for such sources.

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Ultrafast optical rotations of electron spins in quantum dots

Coherent manipulation of quantum bits (qubits) on time scales much shorter than the coherence time is a key prerequisite for quantum information processing. Electron spins in quantum dots (QDs) are particularly attractive for implementations of qubits. Efficient optical methods for initialization and readout of spins have been developed in recent years. Spin coherence times in the microsecond range have been demonstrated, so that spin control by picosecond optical pulses would be highly desirable. Then a large number of spin rotations could be performed while coherence is maintained. A major remaining challenge is demonstration of such rotations with high fidelity. Here we use an ensemble of QD electron spins focused into a small number of precession modes about a magnetic field by periodic optical pumping. We demonstrate ultrafast optical rotations of spins about arbitrary axes on a picosecond time scale using laser pulses as control fields.

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Control of the direction and rate of nuclear spin flips in InAs quantum dots using detuned optical pulse trains

We find that detuning an optical pulse train from electronic transitions in quantum dots controls the direction of nuclear spin flips. The optical pulse train generates electron spins that precess about an applied magnetic field, with a spin component parallel to the field only for detuned pulses. This component leads to asymmetry in the nuclear spin flips, providing a way to produce a stable and precise value of the nuclear spin polarization. This effect is observed using two-color, time-resolved Faraday rotation and ellipticity.

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Optical Spin Initialization and Non-Destructive Measurement in a Quantum Dot Molecule

The spin of an electron in a self-assembled InAs/GaAs quantum dot molecule is optically prepared and measured through the trion triplet states. A longitudinal magnetic field is used to tune two of the trion states into resonance, forming a superposition state through asymmetric spin exchange. As a result, spin-flip Raman transitions can be used for optical spin initialization, while separate trion states enable cycling transitions for non-destructive measurement. With two-laser transmission spectroscopy we demonstrate both operations simultaneously, something not previously accomplished in a single quantum dot.

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Optically induced spin gates in coupled quantum dots using the electron-hole exchange interaction

We propose a fast optically induced two-qubit \textsc{c-phase} gate between two resident spins in a pair of coupled quantum dots. An excited bound state which extends over the two dots provides an effective electron-electron exchange interaction. The gate is made possible by the electron-hole exchange interaction, which isolates a single transition in the system. When combined with appropriate single qubit rotations, this gate generates an entangled state of the two spins.

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