arXiv subjects

Sophie Collin

Publications and source records attributed to Sophie Collin.

17 recordsLinked to original sources

arXiv2026

3D tomographic imaging of skyrmionic cocoons using HERALDO

Uncovering the rich and intricate characteristics of three-dimensional (3D) magnetic textures is essential for functional materials such as magnetic multilayers, where the delicate balance of various magnetic interactions leads to complex 3D spin arrangements. Among these textures, skyrmionic cocoons-tubular 3D magnetic structures characterized by a closed magnetization surface wrapping around a core-have emerged as particularly intriguing. Stabilized by competing magnetic interactions, these textures reside within a fraction of the thickness of the magnetic material and exhibit a typical lateral size of approximately 100 nm. Here, we present a vector tomographic reconstruction of the 3D magnetization in aperiodic Pt/Co/Al chiral multilayers, where skyrmionic cocoons have been recently reported. Using soft X-ray Holography with Extended Reference by Autocorrelation Linear Differential Operator (HERALDO), we acquire tomographic projections of the magnetic configuration and reconstruct the full 3D magnetization vector field with a spatial resolution of approximately 30 nm, as determined by Fourier shell correlation (FSC). This resolution allows us to observe critical features of the cocoons, such as their vertical misalignment and their overall chirality. Our findings demonstrate that HERALDO-based vector tomography is a powerful approach for revealing the internal structure and vertical extent of these nanoscale magnetic textures, offering new experimental insights into their intrinsic behavior.

cond-mat.mtrl-sci↗

arXiv2024

Interfacial spin-orbitronic effects controlled with different oxidation levels at the Co|Al interface

Perpendicular magnetic anisotropy (PMA) and Dzyaloshinskii-Moriya interactions are key interactions in modern spintronics. These interactions are thought to be dominated by the oxidation of the Co|Al interface in the archetypal Platinum-Cobalt-Aluminum oxide system. Here, we observe a double sign change in the anisotropy and about threefold variation in interfacial chiral interaction, influenced not only by the oxidation, but also by the metallic Al thickness. Contrary to previous assumptions about negligible spin-orbit effects at light metal interfaces, we not only observe strong PMA with fully oxidized Al, decreasing and turning negative (in-plane) with less oxygen at the Co|Al interface, we also observe that the magnetic anisotropy reverts to positive (out-of-plane) values at fully metallic Co|Al interface. These findings suggest modification in Co d band via Co|Al orbital hybridization, an effect supported by X-ray absorption spectroscopy and ab initio theory calculations, highlighting the key impact of strain on interfacial mechanisms at fully metallic Co|Al interface.

cond-mat.mtrl-sci↗

arXiv2024

Control of the magnetic anisotropy in multi-repeat Pt/Co/Al heterostructures using magneto-ionic gating

Controlling magnetic properties through the application of an electric field is a significant challenge in modern nanomagnetism. In this study, we investigate the magneto-ionic control of magnetic anisotropy in the topmost Co layer in Ta/Pt/[Co/Al/Pt]$_n$/Co/Al/AlO$_\text{x}$ multilayer stacks comprising $n +1$ Co layers and its impact on the magnetic properties of the multilayers. We demonstrate that the perpendicular magnetic anisotropy can be reversibly quenched through gate-driven oxidation of the intermediary Al layer between Co and AlO$_\text{x}$, enabling dynamic control of the magnetic layers contributing to the out-of-plane remanence - varying between $n$ and $n +1$. For multilayer configurations with $n = 2$ and $n = 4$, we observe reversible and non-volatile additions of 1/3 and 1/5, respectively, to the anomalous Hall effect amplitude based on the applied gate voltage. Magnetic imaging reveals that the gate-induced spin-reorientation transition occurs through the propagation of a single 90$^{\circ}$ magnetic domain wall separating the perpendicular and in-plane anisotropy states. In the 5-repetition multilayer, the modification leads to a doubling of the period of the magnetic domains at remanence. These results demonstrate that the magneto-ionic control of the anisotropy of a single magnetic layer can be used to control the magnetic properties of coupled multilayer systems, extending beyond the gating effects on a single magnetic layer.

cond-mat.mtrl-sci↗

arXiv2023

Neuromorphic weighted sums with magnetic skyrmions

Integrating magnetic skyrmions into neuromorphic computing could help improve hardware efficiency and computational power. However, developing a scalable implementation of the weighted sum of neuron signals - a core operation in neural networks - has remained a challenge. Here, we show that weighted sum operations can be performed in a compact, biologically-inspired manner by using the non-volatile and particle-like characteristics of magnetic skyrmions that make them easily countable and summable. The skyrmions are electrically generated in numbers proportional to an input with an efficiency given by a non-volatile weight. The chiral particles are then directed using localized current injections to a location where their presence is quantified through non-perturbative electrical measurements. Our experimental demonstration, which currently has two inputs, can be scaled to accommodate multiple inputs and outputs using a crossbar array design, potentially nearing the energy efficiency observed in biological systems.

cs.ET↗

arXiv2023

Driving skyrmions in flow regime in synthetic ferrimagnets

Despite significant advances in the last decade regarding the room temperature stabilization of skyrmions or their current induced dynamics, the impact of local material inhomogeneities still remains an important issue that impedes to reach the regime of steady state motion of these spin textures. Here, we study the spin-torque driven motion of skyrmions in synthetic ferrimagnetic multilayers with the aim of achieving high mobility and reduced skyrmion Hall effect. We consider Pt|Co|Tb multilayers of various thicknesses with antiferromagnetic coupling between the Co and Tb magnetization. The increase of Tb thickness in the multilayers allows to reduce the total magnetic moment and increases the spin-orbit torques allowing to reach velocities up to 400 m.s-1 for skyrmions with diameters of about 160 nm. We demonstrate that due to reduced skyrmion Hall effect, combined with the edge repulsion of the magnetic track making the skyrmions moving along the track without any transverse deflection. Further, by comparing the field-induced domain wall motion and current-induced skyrmion motion, we demonstrate that the skyrmions at the largest current densities present all the characteristics of a dynamical flow regime.

cond-mat.mtrl-sci↗

arXiv2023

Field-free switching of perpendicular magnetization in an ultrathin epitaxial magnetic insulator

For energy efficient and fast magnetic memories, switching of perpendicular magnetization by the spin-orbit torque (SOT) appears as a very promising solution, even more using magnetic insulators that suppress electrical shunting. This SOT switching generally requires the assistance of an in-plane magnetic field to break the symmetry. Here, we present experiments demonstrating the field-free SOT switching of perpendicularly magnetized layers of the thulium iron garnet (Tm_{3}Fe_{5}O_{12}) magnetic insulator. The polarity of the switching loops, clockwise (CW) or counter-clockwise (CCW), is determined by the direction of the initial current pulses, in contrast with field-assisted switchings in which this polarity is controlled by the direction of the field. After an independent determination of Dzyaloshinskii-Moriya interaction (DMI), we relate the field free switching to the interplay of SOT and DMI and the polarity of the loops to the imprint of a Néel domain wall induced by the first pulse, in agreement with Kerr imaging. Our observation and interpretation of field-free electrical switching of a magnetic insulator is an important milestone for future low power spintronic devices.

physics.app-ph↗

arXiv2022

Densely packed skyrmions stabilized at zero magnetic field by indirect exchange coupling in multilayers

Room-temperature stabilization of skyrmions in magnetic multilayered systems is the result of a fine balance between different magnetic interactions namely symmetric and antisymmetric exchange, dipolar, perpendicular magnetic anisotropy as well as, in most cases, Zeeman through an applied external field. Such field-driven stabilization approach is not compatible with most of the anticipated skyrmion based applications, e.g. skyrmion memories, logic or neuromorphic computing which motivates a reduction or a cancellation of field requirements. Here we present a method to stabilize at room-temperature and zero-field, a densely packed skyrmion phase in ferromagnetic multilayers with moderate number of repetitions. To this aim, we finely tune the multilayer parameters to stabilize a dense skyrmion phase. Then, relying on the interlayer electronic coupling to an adjacent bias magnetic layer with strong perpendicular magnetic anisotropy and uniform magnetization, we demonstrate the stabilization of sub-60 nm diameter skyrmion at zero-field with adjustable skyrmion density.

cond-mat.mtrl-sci↗

arXiv2022

Characterization and modeling of spiking and bursting in experimental NbOx neuron

Hardware spiking neural networks hold the promise of realizing artificial intelligence with high energy efficiency. In this context, solid-state and scalable memristors can be used to mimic biological neuron characteristics. However, these devices show limited neuronal behaviors and have to be integrated in more complex circuits to implement the rich dynamics of biological neurons. Here we studied a NbOx memristor neuron that is capable of emulating numerous neuronal dynamics, including tonic spiking, stochastic spiking, leaky-integrate-and-fire features, spike latency, temporal integration. The device also exhibits phasic bursting, a property that has scarcely been observed and studied in solid-state nano-neurons. We show that we can reproduce and understand this particular response through simulations using non-linear dynamics. These results show that a single NbOx device is sufficient to emulate a collection of rich neuronal dynamics that paves a path forward for realizing scalable and energy-efficient neuromorphic computing paradigms.

physics.app-ph↗

arXiv2022

Three-dimensional skyrmionic cocoons in magnetic multilayers

Three-dimensional (3D) topological spin textures emerge as promising quasi-particles for encoding information in future spintronic devices. The third dimension provides more malleability regarding their magnetic properties as well as more flexibility for potential applications. However, the stabilization and characterization of such quasi-particles in easily implementable systems remain a work in progress. Here we observe a new type of 3D magnetic textures that we called skyrmionic cocoons that sits in the interior of magnetic thin films multilayers and possesses a characteristic ellipsoidal shape. Interestingly, these cocoons can coexist with more standard `tubular' skyrmions going through all the multilayer as evidenced by the existence of two very different contrasts in the MFM images recorded at room temperature. The presence of these novel skyrmionic textures as well as the understanding of their layer resolved chiral and topological properties have been investigated by micromagnetic simulations. In order to experimentally stabilize the combination of 3D skyrmion tubes and cocoons, we have elaborated metallic multilayers in which the magnetic properties, notably the anisotropy, of the magnetic films in the stacks is varied depending on their vertical position. Finally, in complement to the magnetic imaging, we also measure the magneto-resistive response of the multilayers as a function of the magnetic field, and succeed to fit its evolution using the 3D micromagnetic simulations as inputs for the magnetic configuration. The excellent agreement that is reached brings additional evidence of the presence of skyrmionic cocoons that hence can be electrically detected.

cond-mat.mes-hall↗

arXiv2021

Element-selective modulation of interfacial Dzyaloshinskii-Moriya interaction in Pt|Co|Metal based multilayers

Despite a decade of research, the precise mechanisms occurring at interfaces underlying the Dzyaloshinskii-Moriya interaction (DMI), and thus the possibility of fine-tuning it, are not yet fully identified. In this study, we investigate the origin of the interfacial DMI, aiming at disentangling how independent are the interfaces around the ferromagnetic layer, and what are their relative contributions to the effective DMI amplitude. For this purpose, we have grown and investigated a large variety of systems with a common structure Pt$|$Co$|M$ with $M =$ Ni, Pd, Ru, Al, Al$|$Ta and MoSi. We explore the correlation between the effective interfacial DMI, and different intrinsic properties of metals, namely atomic number, electronegativity and work function difference at the Co$|M$ interfaces. We find a linear relationship between interfacial DMI and the work function difference between the two elements, hence relating the nature of this behavior to the interfacial potential gradient at the metallic interfaces. The understanding of the DMI mechanism is of utmost importance since it opens up the possibility of precisely engineering the magnetic and hence the spintronic properties for future devices.

cond-mat.mtrl-sci↗

arXiv2021

Spin injection efficiency at metallic interfaces probed by THz emission spectroscopy

Terahertz (THz) spin-to-charge conversion has become an increasingly important process for THz pulse generation and as a tool to probe ultrafast spin interactions at magnetic interfaces. However, its relation to traditional, steady state, ferromagnetic resonance techniques is poorly understood. Here we investigate nanometric trilayers of Co/X/Pt (X=Ti, Au or Au0:85W0:15) as a function of the 'X' layer thickness, where THz emission generated by the inverse spin Hall effect is compared to the Gilbert damping of the ferromagnetic resonance. Through the insertion of the 'X' layer we show that the ultrafast spin current injected in the non-magnetic layer defines a direct spin conductance, whereas the Gilbert damping leads to an effective spin mixing-conductance of the trilayer. Importantly, we show that these two parameters are connected to each other and that spin-memory losses can be modeled via an effective Hamiltonian with Rashba fields. This work highlights that magneto-circuits concepts can be successfully extended to ultrafast spintronic devices, as well as enhancing the understanding of spin-to-charge conversion processes through the complementarity between ultrafast THz spectroscopy and steady state techniques.

cond-mat.mes-hall↗

arXiv2019

Transient magnetic domain wall AC dynamics by means of MOKE microscopy

The domain wall response under constant external magnetic fields reveals a complex behavior where sample disorder plays a key role. Furthermore, the response to alternating magnetic fields has only been explored in limited cases and analyzed in terms of the constant field solution. Here we unveil phenomena in the evolution of magnetic domain walls under the application of alternating magnetic fields within the creep regime, well beyond a small fuctuation limit of the domain wall position. Magnetic field pulses were applied in ultra-thin ferromagnetic films with perpendicular anisotropy, and the resulting domain wall evolution was characterized by polar magneto-optical Kerr effect microscopy. Whereas the DC characterization is well predicted by the elastic interface model, striking unexpected features are observed under the application of alternating square pulses: magneto-optical images show that after a transient number of cycles, domain walls evolve toward strongly distorted shapes concomitantly with a modification of domain area. The morphology of domain walls is characterized with a roughness exponent when possible and contrasted with alternative observables which result to be more suitable for the characterization of this transient evolution. The final stationary convergence as well as the underlying physics is discussed.

cond-mat.stat-mech↗

arXiv2018

Excess velocity of magnetic domain walls close to the depinning field

Magnetic field driven domain wall velocities in [Co/Ni] based multilayers thin films have been measured using polar magneto-optic Kerr effect microscopy. The low field results are shown to be consistent with the universal creep regime of domain wall motion, characterized by a stretched exponential growth of the velocity with the inverse of the applied field. Approaching the depinning field from below results in an unexpected excess velocity with respect to the creep law. We analyze these results using scaling theory to show that this speeding up of domain wall motion can be interpreted as due to the increase of the size of the deterministic relaxation close to the depinning transition. We propose a phenomenological model which allows to accurately fit the observed excess velocity and to obtain characteristic values for the depinning field $H_d$, the depinning temperature $T_d$, and the characteristic velocity scale $v_0$ for each sample.

cond-mat.dis-nn↗

arXiv2018

Hybrid chiral domain walls and skyrmions in magnetic multilayers

Noncollinear spin textures in ferromagnetic ultrathin films are currently the subject of renewed interest since the discovery of the interfacial Dzyaloshinskii-Moriya interaction (DMI). This antisymmetric exchange interaction selects a given chirality for the spin textures and allows stabilising configurations with nontrivial topology. Moreover, it has many crucial consequences on the dynamical properties of these topological structures, including chiral domain walls (DWs) and magnetic skyrmions. In the recent years the study of noncollinear spin textures has been extended from single ultrathin layers to magnetic multilayers with broken inversion symmetry. This extension of the structures in the vertical dimension allows very efficient current-induced motion and room-temperature stability for both Néel DWs and skyrmions. Here we show how in such multilayered systems the interlayer interactions can actually lead to more complex, hybrid chiral magnetisation arrangements. The described thickness-dependent reorientation of DWs is experimentally confirmed by studying demagnetised multilayers through circular dichroism in x-ray resonant magnetic scattering. We also demonstrate a simple yet reliable method for determining the magnitude of the DMI from static domains measurements even in the presence of these hybrid chiral structures, by taking into account the actual profile of the DWs. The advent of these novel hybrid chiral textures has far-reaching implications on how to stabilise and manipulate DWs as well as skymionic structures in magnetic multilayers.

cond-mat.mtrl-sci↗

arXiv2017

Electrical signature of individual magnetic skyrmions in multilayered systems

Magnetic skyrmions are topologically protected whirling spin textures that can be stabilized in magnetic materials in which a chiral interaction is present. Their limited size together with their robustness against the external perturbations promote them as the ultimate magnetic storage bit in a novel generation of memory and logic devices. Despite many examples of the signature of magnetic skyrmions in the electrical signal, only low temperature measurements, mainly in magnetic materials with B20 crystal structure, have demonstrated the skyrmions contribution to the electrical transport properties. Using the combination of Magnetic Force Microscopy (MFM) and Hall resistivity measurements, we demonstrate the electrical detection of sub-100 nm skyrmions in multilayered thin film at room temperature (RT). We furthermore analyse the room temperature Hall signal of a single skyrmion which contribution is mainly dominated by anomalous Hall effect.

cond-mat.mes-hall↗

arXiv2017

Room-temperature current-induced generation and motion of sub-100nm skyrmions

Magnetic skyrmions are nanoscale windings of the spin configuration that hold great promise for technology due to their topology-related properties and extremely reduced sizes. After the recent observation at room temperature of sub-100 nm skyrmions stabilized by interfacial chiral interaction in magnetic multilayers, several pending questions remain to be solved, notably about the means to nucleate individual compact skyrmions or the exact nature of their motion. In this study, a method leading to the formation of magnetic skyrmions in a micrometer-sized nanotrack using homogeneous current injection is evidenced. Spin-transfer-induced motion of these small electricalcurrent-generated skyrmions is then demonstrated and the role of the out-of-plane magnetic field in the stabilization of the moving skyrmions is also analysed. The results of these experimental observations of spin torque induced motion are compared to micromagnetic simulations reproducing a granular type, non-uniform magnetic multilayer, in order to address the particularly important role of the magnetic inhomogeneities on the current-induced motion of sub-100 nm skyrmions, for which the material grains size is comparable to the skyrmion diameter.

cond-mat.mes-hall↗

arXiv2014

Electron-Phonon Coupling on the NbSi Transition Edge Sensors

We have built an electron-phonon coupling model to describe the behavior of the NbxSi1-x transition edge sensor (TES) bolometers, fabricated by electron-beam coevaporation and photolithography techniques on a 2-inch silicon wafer. The resistance versus temperature curves of several sensors with different thickness are measured with different bias currents, ranging from 200 nA to 10 micro A, and the electron-phonon coupling coefficient and the electron-phonon thermal conductance are calculated herein. Our values are quite comparable with those in metallic TES samples of other groups using different measurement methods, while we are using the transition region of our TES sample to calculate the electron-phonon coupling interaction.

astro-ph.IM↗