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Sota Kitamura

Publications and source records attributed to Sota Kitamura.

32 records · Page 2Linked to original sources

Floquet engineering of electric polarization with two-frequency drive

Electric polarization is a geometric phenomenon in solids and has a close relationship to the symmetry of the system. Here we propose a mechanism to dynamically induce and manipulate electric polarization by using an external light field. Specifically, we show that application of bicircular lights (BCLs) control the rotational symmetry of the system and can generate electric polarization. To this end, we use Floquet theory to study a system subjected to a two-frequency drive. We derive an effective Hamiltonian with high frequency expansions, for which the electric polarization is computed with the Berry phase formula. We demonstrate the dynamical control of polarization for a one-dimensional SSH chain, a square lattice model, and a honeycomb lattice model.

cond-mat.mes-hall↗

Electric polarization and nonlinear optical effects in noncentrosymmetric magnets

We study electric polarization and nonlinear optical effects in spin systems with broken inversion symmetry. We apply strong coupling expansion to the underlying electronic Hamiltonians, and systematically derive expressions for electric polarization in spin systems that are represented in terms of spin operators. The magnon representation of the obtained electric polarization operator allows us to compute linear and nonlinear optical responses by the standard diagrammatic method. We apply our formalism to Heisenberg model with alternating coupling constants and $J_1$-$J_2$ model with inversion symmetry breaking. We demonstrate that these inversion broken spin systems support dc current flow upon magnon excitations which arises from the shift current mechanism.

cond-mat.str-el↗

Topological charge pumping in quasiperiodic systems characterized by Bott index

We study topological charge pumping in one-dimensional quasiperiodic systems. Since these systems lack periodicity, we cannot use the conventional approach based on the topological Chern number defined in the momentum space. Here, we develop a general formalism based on a real space picture using the so-called Bott index. We extend the Bott index that was previously used to characterize quantum Hall effects in quasiperiodic systems, and apply it to topological charge pumping in quasiperiodic systems. The Bott index allows us to systematically compute topological indices of charge pumping, regardless of the detail of quasiperiodic models. We apply this formalism to the Fibonacci-Rice-Mele model which we made from Fibonacci lattice, a well-known quasiperiodic system, and Rice-Mele model. We find that these quasiperiodic systems show topological charge pumping with a multi-level behavior due to the fractal nature of the Fibonacci lattice. Such multi-level pumping behaviors can be understood by a real space renormalization group analysis.

cond-mat.mes-hall↗

Current response of nonequilibrium steady states in Landau-Zener problem: Nonequilibrium Green's function approach

The carrier generation in insulators subjected to strong electric fields is characterized by the Landau-Zener formula for the tunneling probability with a nonperturbative exponent. Despite its long history with diverse applications and extensions, study of nonequilibrium steady states and associated current response in the presence of the generated carriers has been mainly limited to numerical simulations so far. Here, we develop a framework to calculate the nonequilibrium Green's function of generic insulating systems under a DC electric field, in the presence of a fermionic reservoir. Using asymptotic expansion techniques, we derive a semi-quantitative formula for the Green's function with nonperturbative contribution. This formalism enables us to calculate dissipative current response of the nonequilibrium steady state, which turns out to be not simply characterized by the intraband current proportional to the tunneling probability. We also apply the present formalism to noncentrosymmetric insulators, and propose nonreciprocal charge and spin transport peculiar to tunneling electrons.

cond-mat.str-el↗

Nonreciprocal Landau-Zener tunneling

Application of strong dc electric field to an insulator leads to quantum tunneling of electrons from the valence band to the conduction band, which is a famous nonlinear response known as Landau-Zener tunneling. One of the growing interests in recent studies of nonlinear responses is nonreciprocal phenomena where transport toward the left and the right differs. Here, we theoretically study Landau-Zener tunneling in noncentrosymmetric systems, i.e., the crystals without spatial inversion symmetry. A generalized Landau-Zener formula is derived taking into account the geometric nature of the wavefunctions. The obtained formula shows that nonreciprocal tunneling probability originates from the difference in the Berry connections of the Bloch wavefunctions across the band gap, i.e., shift vector. We also discuss application of our formula to tunneling in a one-dimensional model of a ferroelectrics.

cond-mat.mes-hall↗

Hidden kagome-lattice picture and origin of high conductivity in delafossite PtCoO$_2$

We study the electronic structure of delafossite PtCoO$_2$ to elucidate its extremely small resistivity and high mobility. The band exhibits steep dispersion near the Fermi level despite the fact that it is formed mainly by Pt $d$ orbitals that are typically localized. We propose a picture based on two hidden kagome-lattice-like electronic structure: one originating from Pt $s+p_x/p_y$ orbitals, and the other from Pt $d_{3z^2-r^2}+d_{xy}/d_{x^2-y^2}$ orbitals, each placed on the bonds of the triangular lattice. In particular, we find that the underlying Pt $s+p_x/p_y$ bands actually determine the steepness of the original dispersion, so that the large Fermi velocity can be attributed to the large width of the Pt $s+p_x/p_y$ band. More importantly, the kagome-like electronic structure gives rise to "orbital-momentum locking" on the Fermi surface, which reduces the electron scattering by impurities. We conclude that the combination of the large Fermi velocity and the orbital-momentum locking is likely to be the origin of the extremely small resistivity in PtCoO$_2$.

cond-mat.mtrl-sci↗

Spin Hall effect in 2D metallic delafossite PtCoO$_2$ and vicinity topology

The two-dimensional (2D) metal PtCoO$_2$ is renowned for the lowest room temperature resistivity among all oxides, close to that of the top two materials Ag and Cu. In addition, we theoretically predict a strong intrinsic spin Hall effect. This originates from six strongly-tilted Dirac cones that we find in the electronic structure near the Fermi surface, where a gap is opened by large spin-orbit coupling (SOC). This is underpinned by rich topological properties; in particular, the phenomenology of a mirror Chern metal is realized not exactly, but very accurately, on account of an approximate crystalline symmetry. We expect that such 'vicinity topology' to be a feature of relevance well beyond this material. Our Wilson loop analysis indicates further elaborate features such as fragile topology. These findings highlight PtCoO$_2$ as a promising material for spintronic applications as well as a platform to study the interplay of symmetry and topology.

cond-mat.mes-hall↗

Floquet Engineering of Quantum Materials

Floquet engineering, the control of quantum systems using periodic driving, is an old concept in condensed matter physics, dating back to ideas such as the inverse Faraday effect. There is a renewed interest in this concept owing to the rapid developments in laser and ultrafast spectroscopy techniques and discovery and understanding of various "quantum materials" hosting interesting exotic quantum properties. Here, starting from a nontechnical introduction with emphasis on the Floquet picture and effective Hamiltonians, we review the recent applications of Floquet engineering in ultrafast, nonlinear phenomena in the solid state. In particular, Floquet topological states, application to ultrafast spintronics, and to strongly correlated electron systems are overviewed.

cond-mat.str-el↗

Probing and controlling spin chirality in Mott insulators by circularly polarized laser

Scalar spin chirality, a three-body spin correlation that breaks time-reversal symmetry, is revealed to couple directly to circularly polarized laser. This is shown by the Floquet formalism for the periodically driven repulsive Hubbard model with a strong-coupling expansion. A systematic derivation of the effective low-energy Hamiltonian for a spin degree of freedom reveals that the coupling constant for scalar spin chirality can become significant for a situation in which the driving frequency and the on-site interaction are comparable. This implies that the scalar chirality can be induced by circularly polarized lights, or that it can be used conversely for probing the chirality in Mott insulators as a circular dichroism.

cond-mat.str-el↗

Emergent Weyl nodes and Fermi arcs in a Floquet Weyl semimetal

When a Dirac semimetal is subject to a circularly polarized laser, it is predicted that the Dirac cone splits into two Weyl nodes and a nonequilibrium transient state called the Floquet Weyl semimetal is realized. We focus on the previously unexplored low-frequency regime, where the upper and lower Dirac bands resonantly couple with each other through multi-photon processes, which is a realistic situation in solid state ultrafast pump-probe experiments. We find a series of new Weyl nodes emerging in pairs when the Floquet replica bands hybridize with each other. The nature of the Floquet Weyl semimetal with regard to the number, locations, and monopole charges of these Weyl nodes is highly tunable with the amplitude and frequency of the light. We derive an effective low energy theory using Brillouin-Wigner expansion and further regularize the theory on a cubic lattice. The monopole charges obtained from the low-energy Hamiltonian can be reconciled with the number of Fermi arcs on the lattice which we find numerically.

cond-mat.mes-hall↗

$η$-pairing superfluid in periodically-driven fermionic Hubbard model with strong attraction

We propose a novel possibility of dynamically changing the pairing of superconductors from $s$ wave to $η$ pairing (where the pairs condense at the Brillouin-zone corner momenta) by driving the system with ac fields. We consider a periodically-driven attractive Hubbard model in the strong-coupling regime, and show that the pair-hopping and pair-repulsion terms in the effective Hamiltonian in the Floquet formalism are drastically renormalized in different manners between the two terms, which can change the ground states from an $s$-wave superconductivity to an $η$-pairing superconductivity or a charge-ordered phase. While in isolated systems such as cold atoms a simple quench scheme would not realize the dynamical phase transition into $η$ pairing, we show that there are pathways that realize the dynamical transition, where the field amplitude is varied via a charge-ordered phase as an intermediate state.

cond-mat.quant-gas↗

Current-induced giant diamagnetism in the Mott insulator Ca2RuO4

Mott insulators have surprised us many times by hosting new and diverse quantum phenomena when the frozen electrons are perturbed by various stimuli. Superconductivity, metal-insulator transition, and colossal magnetoresistance induced by element substitution, pressure, and magnetic field are prominent examples. Here we report a novel phenomenon, namely giant diamagnetism, in the Mott insulator Ca2RuO4 induced by electric current. With application of 1 A/cm2 current, the strongest diamagnetism among all nonsuperconducting materials is induced as the system is tuned to a semimetallic state. The origin lies in the emergence of indirect Dirac cones in the many-body spectrum and associated monopole-like anomaly in the momentum dependent susceptibility. This record-breaking and switchable diamagnetism is a new class of non-equilibrium quantum phenomena on the verge of Mott insulating states.

cond-mat.str-el↗

Brillouin-Wigner theory for high-frequency expansion in periodically driven systems: Application to Floquet topological insulators

We construct a systematic high-frequency expansion for periodically driven quantum systems based on the Brillouin-Wigner (BW) perturbation theory, which generates an effective Hamiltonian on the projected zero-photon subspace in the Floquet theory, reproducing the quasienergies and eigenstates of the original Floquet Hamiltonian up to desired order in $1/ω$, with $ω$ being the frequency of the drive. The advantage of the BW method is that it is not only efficient in deriving higher-order terms, but even enables us to write down the whole infinite series expansion, as compared to the van Vleck degenerate perturbation theory. The expansion is also free from a spurious dependence on the driving phase, which has been an obstacle in the Floquet-Magnus expansion. We apply the BW expansion to various models of noninteracting electrons driven by circularly polarized light. As the amplitude of the light is increased, the system undergoes a series of Floquet topological-to-topological phase transitions, whose phase boundary in the high-frequency regime is well explained by the BW expansion. As the frequency is lowered, the high-frequency expansion breaks down at some point due to band touching with nonzero-photon sectors, where we find numerically even more intricate and richer Floquet topological phases spring out. We have then analyzed, with the Floquet dynamical mean-field theory, the effects of electron-electron interaction and energy dissipation. We have specifically revealed that phase transitions from Floquet-topological to Mott insulators emerge, where the phase boundaries can again be captured with the high-frequency expansion.

cond-mat.mes-hall↗

Interaction-Driven Topological Insulator in Fermionic Cold Atoms on an Optical Lattice: A Design with a Density Functional Formalism

We design an interaction-driven topological insulator for fermionic cold atoms in an optical lattice, that is, we pose the question of whether we can realize in a continuous space a spontaneous symmetry breaking induced by the inter-atom interaction into a topological Chern insulator. Such a state, sometimes called a "topological Mott insulator", has yet to be realized in solid-state systems, since this requires, in the tight-binding model, large offsite interactions on top of a small onsite interaction. Here we overcome the difficulty by introducing a spin-dependent potential, where a spin-selective occupation of fermions in $A$ and $B$ sublattices makes the onsite interaction Pauli-forbidden, while a sizeable inter-site interaction is achieved by a shallow optical potential with a large overlap between neighboring Wannier orbitals. This puts the system away from the tight-binding model, so that we adopt the density functional theory for cold-atoms, here extended to accommodate non-collinear spin structures emerging in the topological regime, to quantitatively demonstrate the phase transition to the topological Mott insulator.

cond-mat.quant-gas↗